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Peng-Hui Chen

Publications and source records attributed to Peng-Hui Chen.

At least 19 recordsLinked to original sources

Synthesis mechanism of superheavy element 120: a dinuclear system model approach with microscopic inputs

The dinuclear system model incorporates several essential input physical quantities, including nuclear mass, fission barrier, shell correction energy, level density parameter, and shell damping factor, etc., which are derived from diverse nuclear structure models. To achieve theoretical consistency, we try to generate these essential input physical quantities from the finite-temperature covariant density functional theory using PC-PK1 energy density functional, with pairing correlations treated via the BCS approach. With microscopically determined input parameters, the dinuclear system model can successfully reproduce experimental results for: (i) cold fusion reaction systems ($^{48}$Ca + $^{204,206-208}$Pb $\rightarrow$ $^{252,254-256}$No$^*$), and (ii) hot fusion reaction systems ($^{48}$Ca + $^{239,240,242,244}$Pu $\rightarrow$ $^{287,288,290,292}$Fl$^*$). Furthermore, we perform calculations for the fusion reactions $^{50}$Ti+$^{249}$Cf, $^{51}$V+$^{249}$Bk, $^{54}$Cr+$^{248}$Cm, and $^{55}$Mn+$^{243}$Am, targeting the synthesis of element 120. It is found that the maximum synthesis cross section for these four reactions are 48.20 fb, 12.33 fb, 5.25 fb, 0.47 fb corresponding to $^{50}$Ti($^{249}$Cf,4n)$^{295}$120 at $E^*_{\rm CN}$ = 41 MeV, $^{51}$V($^{249}$Bk,3n)$^{297}$120 at $E^*_{\rm CN}$ = 34 MeV, $^{54}$Cr($^{248}$Cm,3n)$^{299}$120 at $E^*_{\rm CN}$ = 32 MeV, $^{55}$Mn($^{243}$Am,5n)$^{293}$120 at $E^*_{\rm CN}$ = 53 MeV, respectively.

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Systematic investigation on the superheavy nucleus formation in the reactions of $^{48}$Ca, $^{50}$Ti, $^{51}$V and $^{54}$Cr on actinide nuclei

The synthesis of superheavy elements strongly relies on the competition of the quasifission and fusion fission dynamics in the fusion-evaporation reactions. The systematics on the formation of superheavy nuclei in the $^{48}$Ca, $^{50}$Ti, $^{51}$V and $^{54}$Cr induced fusion reactions on actinide nuclei $^{232}$Th, $^{231}$Pa, $^{238}$U, $^{237}$Np, $^{242,244}$Pu, $^{243}$Am, $^{245,248}$Cm, $^{249}$Bk, $^{249}$Cf has been thoroughly investigated with the dinuclear system model by including the cluster transfer and coupling to the dynamical evolution of the quadrupole deformation parameters. The uncertainties of the fusion-evaporation excitation functions with the mass models of FRDM2012, KTUY05, LDM1966, SkyHFB, WS4 are investigated and compared with the available experimental data from Dubna, GSI, Berkeley and RIKEN. The production cross sections, optimal evaporation channels and beam energies in the synthesis of superheavy elements Z = 119 and 120 were predicted and compared for the different mass models in the reactions of $^{50}\mathrm{Ti} + ^{249}\mathrm{Bk}$, $^{51}\mathrm{V} + ^{248}\mathrm{Cm}$, $^{54}\mathrm{Cr} + ^{243}\mathrm{Am}$, $^{50}\mathrm{Ti} + ^{249}\mathrm{Cf}$, $^{51}\mathrm{V} + ^{249}\mathrm{Bk}$, $^{54}\mathrm{Cr} + ^{248}\mathrm{Cm}$, respectively.

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Exploring the nuclear momentum anisotropy based on intermediate-energy heavy-ion collisions

We simulate ultra-central collisions of prolate uranium-uranium nuclei at intermediate energies using the isospin-dependent Boltzmann-Uehling-Uhlenbeck model to investigate the impact of momentum anisotropy on spatial geometric effects. By defining the quadrupole deformation parameter in momentum space $\beta_\text{p}$, we establish an ellipsoidal Fermi surface, aligning its rotational symmetry axis with the one in coordinate space. It is found that oblate momentum density enhances elliptic flow $v_2$, while prolate momentum density has the opposite effect, particularly pronounced in the outer, high transverse momentum $p_\text{t}$ region. Momentum anisotropy also causes differences in the initial momentum mean projection along the beam direction, with larger projections producing more pion mesons. Additionally, significant effects on mean square elliptic flow are observed in non-polarized collisions. We further examine the relationship between the $v_2$-$p_\text{t}$ slope and $\beta_\text{p}$, eliminating systematic errors through the two-system ratio. These findings provide important references for experimentalists in heavy-ion collisions and valuable feedback to theorists regarding nuclear structure.

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Production cross sections of superheavy elements: insights from the dinuclear system model with high-quality microscopic nuclear masses

To accurately predict the synthesis cross-sections of superheavy elements, identifying the optimal projectile-target combinations and the evaporation channels at specific collision energies, we have attempted to utilize high-quality microscopic nuclear masses (HQMNM) within the dinuclear system (DNS) model, which are obtained by fitting experimental data with the Skyrme energy density functional theory (DFT), as published in Phys. Lett. B 851 (2024) 138578. The atomic nuclear mass serves as a crucial input for the DNS model, as the Q-values and separation energies it generates directly influence the calculated fusion and survival probabilities. Our calculations have reproduced the experimental data for hot fusion and have been compared with results based on the finite-range droplet model (FRDM12) mass calculations. Compared to the FRDM12 mass results, we have found that the HQMNM provides a better fit to the experimental outcomes. For the specific reaction of \(^{48}\rm{Ca} + ^{243}\rm{Am} \rightarrow ^{291}\rm{Mc}^*\), we have conducted a detailed calculation of capture, fusion, and survival based on the HQMNM model and compared these with calculations based on other mass models. Based on these findings, we have systematically calculated available projectile target combinations for the synthesis of elements 119 and 120, and identified the optimal combinations. We provided the synthesis cross-sections, collision energies, and evaporation channels, offering a reference for conducting experiments on the synthesis of superheavy elements.

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Exploring the potential of synthesizing unknown superheavy isotopes via cold-fusion reactions based on the dinuclear system model

To assess the potential of cold-fusion for synthesizing superheavy nuclei (SHN) with proton numbers 104-113, we systematically calculated 145 naturally occurring projectile-target combinations within the DNS model. Reactions predominantly show maximum cross-sections in the 1n to 2n channels, peaking near the Coulomb barrier with a sum of barrier and Q-value within 30 MeV. The maximum cross-section occurs below the Bass barrier, suggesting either the Bass model's limitation or significant deformation reducing the effective Coulomb barrier. Our calculations align well with experimental data, revealing that more neutron-rich projectiles slightly enhance fusion, though the effect is minor. For fixed targets (Pb, Bi), evaporation residue cross-sections decrease linearly with increasing projectile proton number, attributed to reduced fusion probability and lower fission barriers in heavier SHN. The touching potential $V_{\rm in}$ shows a linear trend with the product of projectile-target proton numbers, with neutron-rich systems exhibiting lower $V_{\rm in}$. Some reactions with $V_{\rm in} < V_{\rm S}$ may involve nucleon transfer before capture. Based on the DNS model, we identified optimal combinations and collision energies for synthesizing SHN with significant cross-sections. Collectively, our findings indicate that cold fusion is a promising avenue for creating proton-rich SHN around the drip line in the Z=104-113 region, offering distinct advantages over alternative mechanisms.

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Assessing the Impact of Nuclear Mass Models on the Prediction of Synthesis Cross Sections for Superheavy Elements

Within the framework of the dinuclear system model, this study delves into the impact of various nuclear mass models on evaluating the fusion probability of superheavy nuclei. Nuclear mass models, as crucial inputs to the DNS model, exhibit slight variations in binding energy, quadrupole deformation, and extrapolation ability; these subtle differences can significantly influence the model's outcomes. Specifically, the study finds that nuclear mass plays a pivotal role in determining fusion probability, and Q-value. By numerically solving a set of master equations, the study examines how binding energies from different mass models affect the fusion probability of colliding nuclei, taking the example of $^{48}$Ca + $^{243}$Am $\rightarrow$ $^{291}$Mc. A careful analysis of the potential energy surface (PES) reveals that the inner fusion barriers lead to variations in fusion probabilities. Importantly, the study demonstrates that the synthesis cross sections of superheavy nuclei calculated using different nuclear mass models align well with experimental data, falling within an error range of one order of magnitude. This finding underscores the reliability of our model predictions. Looking ahead, the study utilizes five distinct nuclear mass models to predict the synthesis cross sections of superheavy elements 119 and 120, along with their associated uncertainties. These predictions offer valuable insights into the feasibility of synthesizing these elusive elements and pave the way for future experimental explorations.

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Impact of quadrupole deformation on intermediate-energy heavy-ion collisions

This study employs the isospin-dependent Boltzmann-Uehling-Uhlenbeck model to simulate intermediate-energy heavy-ion collisions between prolate nuclei $^{24}$Mg. The emphasis is on investigating the influence of centrality and orientation in several collision scenarios. The final-state particle multiplicities and anisotropic flows are primarily determined by the eccentricity and the area of the initial overlap. This not only provides feedback on the collision systems, but also, to some extent, provides a means to explore the fine structure inside deformed nuclei. Additionally, non-polarized collisions have been further discussed. These results contribute to the understanding of the geometric effects in nuclear reactions, and aid in the exploration of other information on reaction systems, such as the equation of state and nuclear high-momentum tail.

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Production cross-sections of new superheavy elements with Z = 119-120 in fusion-evaporation reactions

We have calculated production cross sections of new superheavy elements with atomic number Z=119,120 in the fusion-evaporation reactions of $^{48}$Ca+$^{252}$Es, $^{48}$Ca+$^{257}$Fm, $^{49}$Sc+$^{252}$Es, $^{49}$Sc+$^{251}$Cf, $^{50}$Ti+$^{247}$Bk, $^{50}$Ti+$^{251}$Cf, $^{51}$V+$^{247}$Cm, $^{51}$V+$^{247}$Cf, $^{54}$Cr+$^{243}$Am, $^{54}$Cr+$^{247}$Cm, $^{56}$Mn+$^{244}$Pu, $^{56}$Mn+$^{243}$Am, $^{60}$Fe+$^{237}$Np, $^{60}$Fe+$^{244}$Pu, $^{61}$Co+$^{238}$U, $^{61}$Co+$^{237}$Np, $^{64}$Ni+$^{231}$Pa, $^{64}$Ni+$^{238}$U, $^{65}$Cu+$^{232}$Th, $^{65}$Cu+$^{231}$Pa, and $^{68}$Zn+$^{232}$Th within the dinuclear system model systematically. The inner fusion barriers have been extracted from the driving potential or potential energy surface which could be used to predict the relative fusion probability roughly. The influence of mass asymmetry of the colliding partners on the production of new superheavy elements (SHE) has been investigated systematically. It is found that fusion probability increase along with the increasing mass asymmetry of colliding systems. The Ti-induced reactions have the largest cross-sections of the new SHE. The dependence of production cross-sections of new superheavy elements on the isospin of projectile nuclei has been discussed. The new SHE of $^{289-295}$119 has been predicted as the synthesis cross sections around serval picobarns in the $^{46,48,50,52}$Ti-induced reactions. Production cross-section of the element of $^{295}$120 has been evaluated as large as 1 picobarn in the reactions $^{46}$Ti ($^{251}$Cf, 2n) $^{295}$120 at $E^*$ = 26 MeV. The optimal projectile-target combinations and beam energies for producing new SHE with atomic number Z=119-120 are proposed for the forthcoming experiments.

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Prediction for the synthesis cross sections of new moscovium isotopes in fusion-evaporation reactions

In the framework of the dinuclear system model, the synthesis mechanism of the superheavy nuclides with atomic number $Z=112, 114, 115$ in the reactions of projectiles $^{40,48}$Ca bombarding on targets $^{238}$U, $^{242}$Pu, and $^{243}$Am at a wide incident energies (excitation energy from 0-100 MeV) have been investigated systematically. Based on the available experimental excitation functions, the dependence of calculated synthesis cross sections on collision orientations has been studied thoroughly. The TKEs of these collisions with the fixed collision orientation show its orientation dependence which can be used to predict the tendency of kinetic energy diffusion. The TKEs are dependent on incident energies which have been discussed. The method of Coulomb barrier distribution function has been applied in our calculations which could treat all of the collision orientations from the tip-tip to side-side approximately. The calculations of excitation functions of $^{48}$Ca + $^{238}$U, $^{48}$Ca + $^{242}$Pu, and $^{48}$Ca + $^{243}$Am have a nice agreement with the available experimental data. The isospin effect of projectiles on production cross sections of moscovium isotopes and the influence of entrance channel effect on the synthesis cross sections of superheavy nuclei have been discussed. The synthesis cross section of new moscovium isotopes $^{278-286}$Mc have been predicted as large as hundreds pb, in the fusion-evaporation reactions of $^{35,37}$Cl + $^{248}$Cf, $^{38,40}$Ar + $^{247}$Bk, $^{39,41}$K + $^{247}$Cm, $^{40,42,44,46}$Ca + $^{238}$Am, $^{45}$Sc + $^{242}$Pu, and $^{46,48,50}$Ti + $^{243}$Np, $^{51}$V + $^{238}$U at the excitation energy interval of 0-100 MeV.

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A local-density-approximation description of high-momentum tails in isospin asymmetric nuclei

We adapt the local density approximation to add the high-momentum tails (HMTs) to finite nuclei's Slater-determinant momentum distributions. The HMTs are extracted by the extended Brueckner-Hartree-Fock (EBHF) method or by the lowest order cluster approximation. With a correction factor being added to EBHF, it is sufficiently in agreement with the experimental benchmark, i.e., the high-momentum $N/Z$ ratios approximately equal to $1$, and the low-momentum $N/Z$ ratios approximately equal to $N/Z$ of the systems. It is also found that the tensor force makes the nucleon-nucleon correlations appear more easily on the nuclear surface region and the percentage of high-momentum ($p > 300$ MeV/c) nucleons, around $17\%$--$18\%$, independent of isospin asymmetry.

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Production of neutron-rich actinide nuclides in isobaric collisions via multinucleon transfer reactions

We have calculated the multinucleon transfer reactions of $^{208}$Os, $^{208}$Pt, $^{208}$Hg, $^{208}$Pb,$^{208}$Po, $^{208}$Rn, $^{208}$Ra,$^{132,136}$Xe bombarding on $^{232}$Th and $^{248}$Cm at Coulomb barrier energies within the dinuclear system model, systematically. The results are in good agreement with the available experimental data. Coulomb effect and shell effect on production of actinides in these reactions have been investigated thoroughly. Potential energy surface and total kinetic energy mass distributions in the reactions $^{208}$Hg, $^{208}$Pb and$^{208}$Po colliding on $^{248}$Cm and $^{232}$Th are calculated and analyzed, respectively. It is found that PES and TKE spectra manifest the fragment formation mechanism in the multinucleon transfer reactions. The isospin effect and shell effect are shown in PES and TKE. Production cross-sections of multinucleon transfer products are highly dependent on the isobar projectiles with mass number $A=208$. The isobar projectiles with larger N/Z ratios are favorable for creating the neutron-rich target-like fragments. The isobar projectiles with larger charge number induced products tend to shift to proton-rich region. Coulomb potential coupled to shell effect is shown in production cross-sections of actinide isotopes. Based on the radioactive projectiles induced reactions, we have predicted massive new actinide isotopes around nuclear drip lines, even could access the superheavy nuclei region.

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Rare Isotope Formation in Complete Fusion and Multinucleon Transfer Reactions in Collisions of 48Ca +248Cm around Coulomb Barrier Energies

Within the framework of the dinuclear system model, the reaction mechanisms for synthesizing target-like isotopes from Bk to compound nuclei Lv are thoroughly investigated in complete and incomplete fusion reaction of $^{48}$Ca +$^{248}$Cm around Coulomb barrier energies. Production cross-section of $^{292,293}$Lv as a function of excitation energy in fusion-evaporation reactions and target-like isotopic yields in multinucleon transfer reactions are evaluated, in which a statistical approach is used to describe the decay process of excited nuclei. The available experimental data can be reproduced well with the model reasonably. The products of all possible formed isotopes in the dynamical pre-equilibrium process for collision partners at incident energy $E_{\rm lab}$ = 5.5 MeV/nucleon are exported, systematically. It is found that the quasi-fission fragments are dominant in the yields. The optimal pathway from the target to compound nuclei shows up along the valley of potential surface energy. The effective impact parameter of two colliding partners leading to compound nuclei is selected from head-on collision to semi-central collision with $L$ = 52 $\rm \hbar$. The timescale boundary between complete fusion and multinucleon transfer reactions is about 5.7$\times 10^{-21}$ s with effective impact parameters. Synthesis cross-section of unknown neutron-rich actinides from Bk to Rf have been predicted around several nanobarns.

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Systematics on production of superheavy nuclei $Z = 119-122$ in fusion-evaporation reactions

The fusion dynamics on the formation of superheavy nuclei is investigated thoroughly within the dinuclear system model. The Monte Carlo approach is implemented into the nucleon transfer process for including all possible orientations, at which the dinuclear system is assumed to be formed at the touching configuration of dinuclear fragments. The production cross sections of superheavy nuclei Cn, Fl, Lv, Ts and Og are calculated and compared with the available data from Dubna. The evaporation residue excitation functions in the channels of pure neutrons and charged particles are analyzed systematically. The combinations with $^{44}$Sc, $^{48,50}$Ti, $^{49,51}$V, $^{52,54}$Cr, $^{58,62}$Fe and $^{62,64}$Ni bombarding the actinide nuclides $^{238}$U, $^{244}$Pu, $^{248}$Cm, $^{247,249}$Bk, $^{249,251}$Cf, $^{252}$Es and $^{243}$Am are calculated for producing the superheavy elements with Z=119-122. It is found that the production cross sections sensitively depend on the neutron richness of reaction system. The structure of evaporation residue excitation function is related to the neutron separation energy and fission barrier of compound nucleus.

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Production mechanism of neutron-deficient actinide isotopes in complete fusion reactions and multinucleon transfer reactions

Within the dinuclear system model, unknown neutron-deficient isotopes Np, Pu, Am, Cm, Bk, Cf, Es, Fm are investigated in $^{40}$Ca, $^{36,40}$Ar, $^{32}$S, $^{28}$Si,$^{24}$Mg induced fusion-evaporation reactions and multinucleon transfer reactions with radioactive beams $^{59}$Cu,$^{69}$As,$^{90}$Nb,$^{91}$Tc, $^{94}$Rh, $^{105,110}$Sn, $^{118}$Xe induced with $^{238}$U near Coulomb barrier energies. The production cross sections of compound nuclei in the fusion-evaporation reactions and fragments yields in the multinucleon transfer reactions are calculated within the model. A statistical approach is used to evaluate the survival probability of excited nuclei via the both reaction mechanisms. A dynamical deformation is implemented into the model in the dissipation process. It is found that charge particle channels (alpha and proton) dominate in the decay process of proton-rich nuclides and the fusion-evaporation reactions are favorable to produce the new neutron-deficient actinide isotopes. The total kinetic energies and angular spectra of primary fragments are strongly dependent on colliding orientations.

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To reach neutron-rich heavy and superheavy nuclei by multinucleon transfer reactions with radioactive isotopes

The dynamical mechanism of multinucleon transfer (MNT) reactions has been investigated within the dinuclear system (DNS) model, in which the sequential nucleon transfer is described by solving a set of microscopically derived master equations. Production cross sections, total kinetic energy spectra, angular distribution of formed fragments in the reactions of $^{124,132}$Sn+ $^{238}$U/$^{248}$Cm near Coulomb barrier energies are thoroughly analyzed. It is found that the total kinetic energies of primary fragments are dissipated from the relative motion energy and rotational energy of the two colliding nuclei. The fragments are formed in the forward angle domain. The energy dependence of the angular spectra is different between projectile-like and target-like fragments. Isospin equilibrium is governed under the potential energy surface. The production cross sections of neutron-rich isotopes are enhanced around the shell closure.

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Isospin effect in peripheral heavy-ion collisions at Fermi energies

Within the framework of the Lanzhou quantum molecular dynamics (LQMD) transport model, the isospin effect in peripheral heavy-ion collisions has been investigated thoroughly. A coalescence approach is used for recognizing the primary fragments formed in nucleus-nucleus collisions. The secondary decay process of the fragments is described by the statistical code, GEMINI. Production mechanism and isospin effect of the projectile-like and target-like fragments are analyzed with the combined approach. It is found that the isospin migration from the high-isospin density to the low-density matter takes place in the neutron-rich nuclear reactions, i.e., $^{48}$Ca+$^{208}$Pb, $^{86}$Kr+$^{48}$Ca/$^{208}$Pb/$^{124}$Sn, $^{136}$Xe+$^{208}$Pb, $^{124}$Sn+$^{124}$Sn and $^{136}$Xe+$^{136}$Xe. A hard symmetry energy is available for creating the neutron-rich fragments, in particular in the medium-mass region. The isospin effect of the neutron to proton (n/p) ratio of the complex fragments is reduced once including the secondary decay process. However, a soft symmetry energy enhances the n/p ratio of the light particles, in particular at the kinetic energies above 15 MeV/nucleon.

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Multinucleon transfer dynamics in heavy-ion collisions near Coulomb barrier energies

The multinucleon transfer reactions near barrier energies has been investigated with a multistep model based on the dinuclear system (DNS) concept, in which the capture of two colliding nuclei, the transfer dynamics and the de-excitation process of primary fragments are described by the analytical formula, the diffusion theory and the statistical model, respectively. The nucleon transfer takes place after forming the DNS and is coupled to the dissipation of relative motion energy and angular momentum by solving a set of microscopically derived master equations within the potential energy surface. Specific reactions of $^{40,48}$Ca+$^{124}$Sn, $^{40}$Ca ($^{40}$Ar, $^{58}$Ni)+$^{232}$Th, $^{40}$Ca ($^{58}$Ni)+$^{238}$U and $^{40,48}$Ca ($^{58}$Ni) +$^{248}$Cm near barrier energies are investigated. It is found that the fragments are produced by the multinucleon transfer reactions with the maximal yields along the $β$-stability line. The isospin relaxation is particularly significant in the process of fragment formation. The incident energy dependence of heavy target-like fragments in the reaction of $^{58}$Ni+$^{248}$Cm is analyzed thoroughly.

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Production of proton-rich nuclei around Z=84-90 in fusion-evaporation reactions

Within the framework of the dinuclear system model, production cross sections of proton-rich nuclei with charged numbers of Z=84-90 are investigated systematically. Possible combinations with the $^{28}$Si, $^{32}$S, $^{40}$Ar bombarding the target nuclides $^{165}$Ho, $^{169}$Tm, $^{170-174}$Yb, $^{175,176}$Lu, $^{174,176-180}$Hf and $^{181}$Ta are analyzed thoroughly. The optimal excitation energies and evaporation channels are proposed to produce the proton-rich nuclei. The systems are feasible to be constructed in experiments. It is found that the neutron shell closure of N=126 is of importance during the evaporation of neutrons. The experimental excitation functions in the $^{40}$Ar induced reactions can be nicely reproduced. The charged particle evaporation is comparable with neutrons in cooling the excited proton-rich nuclei, in particular for the channels with $α$ and proton evaporation. The production cross section increases with the mass asymmetry of colliding systems because of the decrease of the inner fusion barrier. The channels with pure neutron evaporation depend on the isotopic targets. But it is different for the channels with charged particles and more sensitive to the odd-even effect.

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