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Pengcheng Dai

Publications and source records attributed to Pengcheng Dai.

At least 19 recordsLinked to original sources

Crystal electric field excitations and an effective-spin-$1/2$ ground doublet in the hyperkagome magnet Yb$_3$Sc$_2$Ga$_3$O$_{12}$

We use inelastic neutron scattering (INS) to determine the crystal electric field (CEF) excitations of Yb$^{3+}$ in the rare-earth hyperkagome magnet Yb$_3$Sc$_2$Ga$_3$O$_{12}$. Three nearly dispersionless magnetic excitations are observed near 58, 68, and 74~meV, corresponding to transitions from the ground-state Kramers doublet to the three excited doublets of the $J=7/2$ multiplet. A Stevens-operator analysis constrained by the local $222$ ($D_2$) symmetry reproduces the excitation energies and spectral weights and yields an Ising-type ground-state $g$ tensor. The first excited doublet lies approximately 58~meV above the ground state, establishing a well-isolated effective $J_{\mathrm{eff}}=1/2$ degree of freedom over the low-temperature regime relevant to collective magnetism. Notably, the directly measured CEF spectrum substantially revises the level scheme previously inferred from bulk measurements, while preserving the essential low-energy pseudospin description. Two independent fitting protocols give consistent excitation energies, ground-doublet wave functions, and $g$ tensors, despite the nonuniqueness of the individual CEF parameters. The resulting single-ion model also reproduces the characteristic susceptibility, magnetization, and field evolution of the Schottky anomaly in specific heat. These results establish the microscopic single-ion basis needed to construct an effective exchange Hamiltonian and to interpret future measurements of low-energy collective excitations in Yb$_3$Sc$_2$Ga$_3$O$_{12}$.

cond-mat.str-el

Spin nematic liquid crystal and scalar spin chirality in tetragonal lattice YbMnBi$_2$

A spin nematic order, analogous to the nematic liquid crystal, characterizes the spontaneous breaking of spin-space rotational symmetry while preserving time-reversal ($T$) symmetry. In contrast, scalar spin chirality (SSC), a composite three-spin order, breaks $T$ symmetry and is known to induce an anomalous Hall effect (AHE). Although a spin nematic phase has been suggested in frustrated magnets and the square-lattice iridate, how it might affect magnetotransport properties is unknown. Here we use polarized neutron scattering to show that tetragonal $A$MnBi$_2$ ($A$ = Ca, Yb) is a strictly $c$-axis-aligned collinear antiferromagnet (C-type), with $T_N \approx 270$ K and 290 K, respectively. On cooling from 450 K to $T_N$, low-energy spin excitations in YbMnBi$_2$ spontaneously change from isotropic to anisotropic in spin space within the tetragonal plane, forming a dynamic spin nematic phase around 400 K due to heavy Yb-induced spin-orbit coupling, before gapping out below $T_N$. Similar measurements on CaMnBi$_2$ reveal isotropic paramagnetic scattering without a spin nematic phase above $T_N$. Under an in-plane magnetic field, the Yb$^{3+}$ moments may interact with the dynamic spin nematic phase to induce nonzero SSC, giving rise to AHE and an anomalous Nernst effect (ANE) in YbMnBi$_2$ that are absent in CaMnBi$_2$ above $T_N$. A symmetry-based Ginzburg-Landau analysis shows that coupling terms between the nematic order and SSC are allowed under an external magnetic field, which could explain the rapid increase of AHE with field in YbMnBi$_2$. Our results provide compelling evidence for dynamic SSC-induced AHE and ANE in the paramagnetic phase of a compensated collinear antiferromagnet, opening a new avenue for the physics of composite spin orders and room-temperature spintronics without magnetic order.

cond-mat.str-el

$d$-spacing distributions as a probe of nematoelastic response in iron-based superconductors

Electronic nematicity in iron-based superconductors (FeSCs) couples bilinearly to orthorhombic strain, allowing nematic correlations to appear in the lattice response. Here we use neutron Larmor diffraction to measure the temperature-dependent distribution of relative $d$ spacings in electron-doped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, hole-doped Ba$_{0.83}$K$_{0.17}$Fe$_2$As$_2$, FeSe, and Fe$_{1.07}$Te. In Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ crystals without intentionally applied uniaxial stress, the in-plane distribution width, $\varepsilon_{\rm FWHM}$, increases on cooling in the tetragonal phase and can be described phenomenologically by a Curie--Weiss-like form. The fitted scale $T^*$ decreases with Co doping and evolves similarly to the nematic phase diagram inferred from elastoresistance, although the two experiments probe different response functions. Related broadening in Ba$_{0.83}$K$_{0.17}$Fe$_2$As$_2$ and FeSe supports extending this interpretation beyond electron-doped BaFe$_2$As$_2$. By contrast, Fe$_{1.07}$Te shows no extended Curie--Weiss-like regime without applied stress, whereas uniaxial pressure produces a strongly anisotropic broadening that can contain contributions from both the field-biased lattice response and inhomogeneous loading. A mean-field model with bilinear nematoelastic coupling and spatially varying symmetry-breaking stress explains the Curie--Weiss-like broadening in terms of the renormalized orthorhombic compliance. Neutron Larmor diffraction therefore provides a bulk-sensitive probe of nematic-related lattice broadening that complements electronic and elastic measurements.

cond-mat.supr-con

Nanoscale Imaging of Strain-Controlled Altermagnetic Domains in {\alpha}-MnTe

Altermagnets combine compensated magnetic order with momentum-dependent spin splitting, offering a route to spintronic functionality without the stray fields of conventional ferromagnets. Mechanical strain provides a promising means of controlling their N\'eel order, yet the microscopic pathway by which strain reorganizes an altermagnetic texture remains unresolved. Here, we combine scanning nitrogen-vacancy magnetometry with a piezo-driven uniaxial strain cell to directly image the strain-driven evolution of magnetic domains in bulk {\alpha}-MnTe at room temperature. By applying uniaxial stress along the nearest-neighbor Mn-Mn bond direction, we find that compressive strain reorganizes the magnetic texture through domain coalescence, increasing the size of the largest connected domain while reducing the domain-wall density. On sweeping toward tensile strain direction, however, the domain network follows a distinct trajectory from that observed during the compressive sweep. Instead, the large connected regions fragment into a new metastable configuration, producing pronounced hysteresis in the maximum domain size and stray-field distribution. These results identify domain connectivity and topology as key carriers of strain-induced magnetic memory. Our work reveals domain coalescence and hysteretic fragmentation as the microscopic pathway of strain control in {\alpha}-MnTe and establishes a route toward strain-programmable altermagnetic textures and reconfigurable spintronic devices.

cond-mat.mtrl-sci

Scalable Policy Optimization for Networked Multi-Agent Reinforcement Learning with Continuous State-Action Spaces

We develop the Continuous Distributed Coupled Policy Gradient (CDCPG) algorithm for cooperative reinforcement learning in networked Markov decision processes with continuous state and action spaces. Each agent maintains a local actor over a bounded graph neighborhood, and a localized least-squares temporal-difference critic evaluates a truncated action-value function through a spectral random-feature representation of the local transition kernel. The analysis makes four contributions. First, the truncated action-value function is constructed as a conditional expectation over the neighborhood, yielding a well-posed localized Bellman theory that removes the continuation-kernel mismatch of naive truncation arguments. Second, we expose a dimensional obstruction to temporal-difference stability for normalized random features and prove an unconditional excitation bound that reduces stability to a symmetric persistence-of-excitation condition, monitorable through an online matrix-concentration certificate. Third, under exponential spatial decay of agent interactions, the excitation condition, and smoothness of the objective, CDCPG drives an averaged per-agent stationarity measure to within any excess $\epsilon$ of an explicitly characterized approximation floor using $\widetilde{\mathcal{O}}(\epsilon^{-2})$ shared-oracle samples, and the excess dependence matches the smooth nonconvex first-order rate; per-agent computation and communication are governed by the neighborhood size rather than the network size. Fourth, an adaptive-locality rule selects the radius that balances truncation and graph-decay residuals against the target accuracy. Experiments on a networked linear-quadratic benchmark corroborate the locality and feature-dimension predictions.

cs.MA

Field-induced first order transitions and phase coexistence in the Kitaev quantum spin liquid candidate BaCo2(AsO4)2

BaCo2(AsO4)2 (BCAO) is an insulating Kitaev quantum spin liquid candidate with a rich low-temperature phase diagram. Below 5 K, it exhibits double-zigzag magnetic order. Upon application of an in-plane magnetic field, the magnetic structure first transforms into an up-up-down (UUD) state near 0.12 T and then enters a fully spin-polarized ferromagnetic (FM) state near 0.5 T. In the narrow field regime close to the polarized phase, a finite residual thermal conductivity has been reported, suggesting a possible field-induced quantum spin liquid phase. Using neutron scattering, we show that the field-induced double-zigzag-to-UUD transition near 0.15 T is accompanied by the emergence of a cluster of localized UUD spin excitations that coexist with conventional spin waves. Upon further increasing field, BCAO undergoes a first-order UUD-to-FM transition with coexistence of UUD and FM phases, accompanied by a sharp response in the spin Seebeck coefficient. These results do not support a quantum spin liquid scenario near the UUD-to-FM critical field. Instead, modeling indicates that the broad excitations arise from bound spin-flip pairs, while a low-lying dispersive branch near the FM phase boundary carries the same sign of magnetization as the FM order. These excitations naturally account for the observed sign of the spin Seebeck response and are likely relevant to the thermal conductivity near the critical field.

cond-mat.str-el

Iron-Based Superconductors: A Decade of Materials, Magnetism, and Mechanisms

Since its discovery in 2008, iron-based superconductors (FeSCs) have become a central platform for exploring high-temperature superconductivity in multiband, electron-correlated materials. This review focuses on major developments over the past decade or so, emphasizing experimental advances, pairing mechanisms, and emerging applications. Structural tuning through chemical substitution, pressure, and epitaxial growth enables precise control of the electronic, magnetic, and superconducting ground states, thereby revealing their interplay. In particular, the electronic nematic phase and stripe-type antiferromagnetic order-often coexisting or competing-are central to understanding the phase diagrams. Spin waves in magnetically ordered parent compounds and spin excitations (fluctuations) in doped superconductors are extensively characterized by inelastic neutron scattering. While high-energy spin excitations in doped superconductors retain substantial spectral weight across a wide energy range reminiscent of spin waves in their undoped parents, the low-energy response reveals a collective spin excitation termed "resonance" coupled to superconductivity. The momentum structure of superconductivity-induced resonance provides strong evidence for sign-changing pairing in many FeSCs, while disorder effects, orbital-fluctuation scenarios, quasiparticle damping, and compound-dependent gap structures indicate that $s_{\pm}$, $s_{++}$, nodal $s$, $d$-wave, and multicomponent states must be discussed in a material-specific framework. Advances in thin-film growth, intercalation chemistry, and interface engineering-particularly in FeSe-based systems-have enabled enhanced $T_{c}$ and novel device geometries. With high upper critical fields, moderate anisotropy, and improving current densities, FeSCs continue to drive both fundamental insight and technological applications in superconductivity.

cond-mat.supr-con

Phonons and magnetism of kagome FeGe probed by nuclear resonant scattering

Kagome FeGe hosts a $2\times2\times2$ charge-density wave (CDW) that strongly interplays with antiferromagnetic order. Here, we report $^{57}$Fe nuclear resonant scattering measurement to study FeGe across its long-range CDW and incommensurate magnetic transitions. Upon entering the CDW state, hardening of acoustic phonons and optical phonons around 22~meV, 27~meV, and 31~meV are observed in the Fe partial phonon density of states, which can be qualitatively captured by first-principle calculations. Upon entering the incommensurate magnetic phase, neither the phonon density of states nor the hyperfine interaction parameters change significantly, although a subtle feature associated with the incommensurate magnetic order or slow fluctuations is detected in the time-domain M\"{o}ssbauer spectra. These findings show that the CDW in kagome FeGe significantly modifies its lattice dynamics and magnetism, evidencing an intertwined nature of the spin, charge, and lattice degrees of freedom.

cond-mat.str-el

Atomic-Scale Observation of Symmetry Breaking in Altermagnetic MnTe

The recent discovery of altermagnetism has sparked growing interest in compensated magnetic systems as promising platforms for highly scalable spintronics. Altermagnetism is a distinct magnetic order where opposite spin sublattices are connected by rotation, yielding zero net magnetization but momentum-dependent spin splitting. To date, experimental verification of altermagnetic order has been achieved predominantly through bulk-sensitive techniques, including spin-dependent electronic spectra and transport responses. However, direct atomic-scale evidence that explicitly correlates crystal symmetry, local structural distortions, and magnetic ordering has remained unexplored. Here, we report the direct atomic-scale observation of coexisting polar distortions and altermagnetic order in MnTe, combining atomic resolution scanning transmission electron microscopy (STEM) imaging with electron magnetic chiral dichroism (EMCD) measurements. We reveal that MnTe is not an ideal uniform P63/mmc g-wave altermagnet at the atomic scale. Instead, it hosts ubiquitous inversion-symmetry-breaking distortions that lower the spin-space-group (SSG) symmetry, admits d-wave altermagnetic components, and in lower-symmetry regimes, even allow s-wave spin splitting (net magnetization). The coexistence of ferroelectric signatures and altermagnetic order establishes local lattice symmetry in MnTe as a control knob for altermagnetic spin splitting, spin current generation, and multiferroic memory applications.

cond-mat.mtrl-sci

Distributed Zeroth-Order Policy Gradient for Networked Multi-agent Reinforcement Learning from Human Feedback

We study a networked multi-agent reinforcement learning (NMARL) problem with human feedback in an infinite-horizon setting, where agents interact over an underlying network with localized state dependencies and aim to collaboratively maximize the average discounted return. Existing approaches with preference feedback are primarily developed for single-agent settings and rely on centralized training, which limits their scalability and applicability to large-scale networked multi-agent systems. To address this, we introduce a novel human feedback mechanism based on spatiotemporally truncated trajectories, defined as $H$-horizon trajectory pairs aggregated over each agent's $\kappa$-hop neighborhood. Building on this, we develop a distributed zeroth-order policy gradient algorithm, where each agent estimates its local policy gradient using human preference feedback generated from both the current joint policy and a perturbed joint policy drawn from zero-mean Gaussian distribution. Specifically, the algorithm is fully distributed, as the feedback received by each agent depends solely on the state-action information within its $\kappa$-hop neighborhood and does not require explicit reward signals or centralized control. We further rigorously establish that the proposed algorithm converges to an $\epsilon$-stationary point with polynomial sample complexity. Finally, simulation results in a stochastic GridWorld environment and a predator-prey environment further demonstrate that the effectiveness and scalability of the proposed algorithm in achieving collaborative optimization based solely on human preference feedback.

cs.MA

Winding feature and thermal evolution of the Dirac magnons in CrI$_3$

Two-dimensional honeycomb lattice ferromagnet chromium tri-iodide (CrI$_3$) has attracted tremendous interest because it retains ferromagnetism down to the monolayer limit and hosts intriguing topological magnons. As a prototypical van der Waals magnet, CrI$_3$ provides an ideal platform for exploring the interplay between reduced dimensionality, magnetic order, and nontrivial spin excitations. Here, using inelastic neutron scattering together with improved sample quality, we uncover the magnon winding feature around the $K$-point of the hexagonal Brillouin zone, a key signature of Dirac magnons. In addition, we find that the magnon energy follows a $T^2$-renormalization behavior at elevated temperatures, consistent with magnon-magnon interactions. These results provide previously missing information on the magnon spectrum of CrI$_3$ and further consolidate the topological nature of its spin excitations.

cond-mat.mtrl-sci

Structural Phase Separation Couples to Charge-Density-Wave Formation in Kagome Metal FeGe

The intertwining of charge, spin, and lattice degrees of freedom underlies the emergent properties of correlated materials. A recent prominent example is the kagome metal FeGe, which hosts coexisting charge density wave (CDW) and antiferromagnetic orders, accompanied by a lattice distortion associated with partial Ge-Ge dimerization. Using temperature-dependent high-resolution X-ray diffraction measurements, we observed a robust splitting of the lattice reflection into two coexisting peaks with distinct lattice constants at the CDW transition temperature TCDW, providing direct evidence for a first-order structural phase transition that is absent in samples with suppressed CDW order. Furthermore, the long-range CDW order was found to be only commensurate with lattice structures with the compressed out-of-plane lattice constant. The Landau free energy analysis shows that strong lattice-charge coupling is a key factor in stabilizing long-range CDW order. Our work clarifies the critical role of structural transformation in the CDW formation and opens opportunities for strain control of electronic phases in FeGe.

cond-mat.mtrl-sci

Fermi surface of Kagome metal CsCr$_3$Sb$_5$ observed by laser photoemission microscopy

We investigated the Fermi surface (FS) in the paramagnetic state of Kagome metal CsCr$_3$Sb$_5$ by employing a laser photoemission microscopy. We found a circular FS and two hexagonal FSs around the Brillouin zone (BZ) center. Polarization-dependent measurements further enable us to detect small FS pockets at the BZ boundary. According to the density functional theory calculations, the orbital characters of the FSs were determined from their shape and orientations. We found that the size of the FS is strongly modified for the d$_{xz}$ orbital, suggesting the orbital-dependent correlation effect. These results provide an electronic basis for exploring the interplay of antiferromagnetic/charge density wave order and possible unconventional superconductivity in this compound.

cond-mat.str-el

Uniaxial strain tuned magnetism of the altermagnet candidate h-FeS

Altermagnets are collinear magnetic materials with 'alter'nating local crystalline environments, characterized by joint spin and crystalline symmetries that enable ferromagnetic-like transport properties but with vanishing net magnetization. Hexagonal FeS (h-FeS) is a recently identified altermagnet candidate that shows a spontaneous anomalous Hall effect (AHE) accompanied by a tiny net magnetization. Here, we show that both the spontaneous AHE and magnetization can be effectively suppressed by an in-plane compressive strain. Since neutron diffraction measurements show that the applied uniaxial strain only modifies the in-plane domain population but does not affect the in-plane magnetic structure, the major effect of the applied strain is to tune the small $c$-axis ferromagnetic moment. Our results demonstrate a strong correlation between the tiny net magnetization and the spontaneous AHE in h-FeS, and show that uniaxial strain provides an effective knob to tune both properties in this altermagnet candidate for spintronic applications.

cond-mat.mtrl-sci

Quasi-one-dimensional spin excitations in the iron pnictide NaFe$_{0.53}$Cu$_{0.47}$As

Spectroscopic measurements in model one-dimensional (1D) correlated systems offer insights for understanding their two-dimensional counterparts, which include the cuprate and iron pnictide/chalcogenide superconductors. A major challenge is the identification of such correlated systems with dominantly 1D physics. In this work, inelastic neutron scattering measurements on NaFe$_{0.53}$Cu$_{0.47}$As single crystal directly reveal quasi-1D spin excitations, resulting from atomic order that lead to magnetic Fe and nonmagnetic Cu chains. The dominant exchange interaction is antiferromagnetic along the chain ($SJ_{\rm \parallel}\approx90.1(3)$~meV), whereas the inter-chain couplings are much weaker ($SJ_{\rm \perp}\approx-2.4(1)$~meV and $SJ_{\rm c}\approx0.15(5)$~meV). The quasi-1D spin excitations in NaFe$_{0.53}$Cu$_{0.47}$As stem from both the N\'eel and stripe vectors, with N\'eel excitations sensitive to Fe impurities on the Cu site. The spin excitations in quasi-1D NaFe$_{0.53}$Cu$_{0.47}$As and quasi-2D FeSe exhibit a striking resemblance, suggesting a common origin for their coexistent stripe and N\'eel excitations. Our findings demonstrate magnetic dilution in NaFeAs leads to dimension reduction of its magnetic degree of freedom, presenting a strategy for discovering low-dimensional quantum materials.

cond-mat.str-el

Spectroscopic Demarcation of Emergent Photons and Spinons in a Dipolar-Octupolar Quantum Spin Liquid

The identification of fractionalized excitations in quantum spin liquids (QSLs) remains a central challenge in condensed matter physics. In dipolar-octupolar (DO) pyrochlores, such as $\text{Ce}_2\text{Zr}_2\text{O}_7$, the candidate $\pi$-flux quantum spin ice (QSI) state is predicted to host both gapless emergent photons and a continuum of spinons. However, resolving these modes at zero field is complicated by their spectral overlap and the presence of nonmagnetic scattering near zero energy. Here, we report neutron scattering experiments on $\text{Ce}_2\text{Zr}_2\text{O}_7$ under a magnetic field along the $[1,1,1]$ direction. In contrast to previous unpolarized studies at zero-field that relied on high-temperature subtraction, we use a same-temperature high-field subtraction protocol to isolate the photon mode. Leveraging the selective coupling of the magnetic field to the dipolar degrees of freedom, we demonstrate the spectroscopic demarcation of these excitations. We observe that weak fields ($\approx 0.15$ T) suppress the low-energy photon weight while leaving the high-energy spinon continuum robust, albeit hardened. Our results, supported by gauge mean-field theory and exact diagonalization calculations, provide strong evidence for the $\pi$-flux QSI state and introduce a powerful field-tuning protocol for investigating DO-QSLs.

cond-mat.str-el

Magnetic field-induced momentum-dependent symmetry breaking in a kagome superconductor

When multiple degrees of freedom share similar energy scales in quantum materials, intertwined electronic orders, which exhibit broken symmetries, are often strongly coupled. Recent studies on kagome superconductors such as CsV$_3$Sb$_5$ report rotational and time-reversal symmetry breaking linked to a charge density wave. Here, we observe a momentum-selective response of the electronic structure of CsV$_3$Sb$_5$ to an external magnetic field. By performing angle-resolved photoemission spectroscopy in a tuneable magnetic field, we demonstrate that the response of the electronic structure is compatible with piezomagnetism along with strong orbital selectivity. Our results show that the origin of the time-reversal symmetry breaking is associated with the vanadium Van Hove singularities at the onset of the charge density wave order. We also demonstrate the presence of fluctuations beyond the charge ordering temperature. Our results reveal that magnetic fields can be used as tuning knobs for disentangling intertwined orders in the momentum space for quantum materials.

cond-mat.str-el

Distributed scalable coupled policy algorithm for networked multi-agent reinforcement learning

This paper studies networked multi-agent reinforcement learning (NMARL) with interdependent rewards and coupled policies. In this setting, each agent's reward depends on its own state-action pair as well as those of its direct neighbors, and each agent's policy is parameterized by its local parameters together with those of its $\kappa_{p}$-hop neighbors, with $\kappa_{p}\geq 1$ denoting the coupled radius. The objective of the agents is to collaboratively optimize their policies to maximize the discounted average cumulative reward. To address the challenge of interdependent policies in collaborative optimization, we introduce a novel concept termed the neighbors' averaged $Q$-function and derive a new expression for the coupled policy gradient. Based on these theoretical foundations, we develop a distributed scalable coupled policy (DSCP) algorithm, where each agent relies only on the state-action pairs of its $\kappa_{p}$-hop neighbors and the rewards of its $(\kappa_{p}+1)$-hop neighbors. Specially, in the DSCP algorithm, we employ a geometric 2-horizon sampling method that does not require storing a full $Q$-table to obtain an unbiased estimate of the coupled policy gradient. Moreover, each agent interacts exclusively with its direct neighbors to obtain accurate policy parameters, while maintaining local estimates of other agents' parameters to execute its local policy and collect samples for optimization. These estimates and policy parameters are updated via a push-sum protocol, enabling distributed coordination of policy updates across the network. We prove that the joint policy produced by the proposed algorithm converges to a first-order stationary point of the objective function. Finally, the effectiveness of DSCP algorithm is demonstrated through simulations in a robot path planning environment, showing clear improvement over state-of-the-art methods.

cs.MA