arXiv subjects

Pepijn W. H. Pinkse

Publications and source records attributed to Pepijn W. H. Pinkse.

35 records · Page 2Linked to original sources

arXiv2014

Nanophotonic hybridization of narrow atomic cesium resonances and photonic stop gaps of opaline nanostructures

We study a hybrid system consisting of a narrowband atomic optical resonance and the long-range periodic order of an opaline photonic nanostructure. To this end, we have infiltrated atomic cesium vapor in a thin silica opal photonic crystal. With increasing temperature, the frequencies of the opal's reflectivity peaks shift down by >20% due to chemical reduction of the silica. Simultaneously, the photonic bands and gaps shift relative to the fixed near-infrared cesium D1 transitions. As a result the narrow atomic resonances with high finesse (f/df=8E5) dramatically change shape from a usual dispersive shape at the blue edge of a stop gap, to an inverted dispersion lineshape at the red edge of a stop gap. The lineshape, amplitude, and off-resonance reflectivity are well modeled with a transfer-matrix model that includes the dispersion and absorption of Cs hyperfine transitions and the chemically-reduced opal. An ensemble of atoms in a photonic crystal is an intriguing hybrid system that features narrow defect-like resonances with a strong dispersion, with potential applications in slow light, sensing and optical memory.

physics.optics↗

arXiv2014

Programmable multiport optical circuits in opaque scattering materials

We propose and experimentally verify a method to program the effective transmission matrix of general multiport linear optical circuits in random multiple-scattering materials by phase modulation of incident wavefronts. We demonstrate the power of our method by programming linear optical circuits in white paint layers with 2 inputs and 2 outputs, and 2 inputs and 3 outputs. Using interferometric techniques we verify our ability to program any desired phase relation between the outputs. The method works in a deterministic manner and can be directly applied to existing wavefront-shaping setups without the need of measuring a transmission matrix or to rely on sensitive interference measurements.

physics.optics↗

arXiv2014

Quantum-Secure Authentication with a Classical Key

Authentication provides the trust people need to engage in transactions. The advent of physical keys that are impossible to copy promises to revolutionize this field. Up to now, such keys have been verified by classical challenge-response protocols. Such protocols are in general susceptible to emulation attacks. Here we demonstrate Quantum-Secure Authentication ("QSA") of an unclonable classical physical key in a way that is inherently secure by virtue of quantum-physical principles. Our quantum-secure authentication operates in the limit of a large number of channels, represented by the more than thousand degrees of freedom of an optical wavefront shaped with a spatial light modulator. This allows us to reach quantum security with weak coherent pulses of light containing dozens of photons, too few for an adversary to determine their complex spatial shapes, thereby rigorously preventing emulation.

quant-ph↗

arXiv2013

Characterization of a Quantum Light Source Based on Spontaneous Parametric Down-Conversion

We have built a quantum light source capable of producing different types of quantum states. The quantum light source is based on entangled state preparation in the process of spontaneous parametric down-conversion. The single-photon detection rate of eight-hundred thousand per second demonstrates that we have created a bright state-of-the-art quantum light source. As a part of the characterization we measured two-photon quantum interference in a Hong-Ou-Mandel interferometer.

physics.optics↗

arXiv2012

Controlling single-photon Fock-state propagation through opaque scattering materials

The control of light scattering is essential in many quantum optical experiments. Wavefront shaping is a technique used for ultimate control over wave propagation in multiple-scattering materials by adaptive manipulation of incident waves. We control the propagation of single-photon Fock states in opaque scattering materials by phase modulation of the incident wavefront. We enhance the probability that a single photon arrives in a target output mode with a factor 10. Our proof-of-principle experiment shows that wavefront shaping can be applied to non-classical light, with prospective applications in quantum communication and quantum cryptography.

physics.optics↗

arXiv2012

Observation of squeezed light from one atom excited with two photons

Single quantum emitters like atoms are well-known as non-classical light sources which can produce photons one by one at given times, with reduced intensity noise. However, the light field emitted by a single atom can exhibit much richer dynamics. A prominent example is the predicted ability for a single atom to produce quadrature-squeezed light, with sub-shot-noise amplitude or phase fluctuations. It has long been foreseen, though, that such squeezing would be "at least an order of magnitude more difficult" to observe than the emission of single photons. Squeezed beams have been generated using macroscopic and mesoscopic media down to a few tens of atoms, but despite experimental efforts, single-atom squeezing has so far escaped observation. Here we generate squeezed light with a single atom in a high-finesse optical resonator. The strong coupling of the atom to the cavity field induces a genuine quantum mechanical nonlinearity, several orders of magnitude larger than for usual macroscopic media. This produces observable quadrature squeezing with an excitation beam containing on average only two photons per system lifetime. In sharp contrast to the emission of single photons, the squeezed light stems from the quantum coherence of photon pairs emitted from the system. The ability of a single atom to induce strong coherent interactions between propagating photons opens up new perspectives for photonic quantum logic with single emitters

quant-ph↗

arXiv2011

Cavity sideband cooling of trapped molecules

The efficiency of cavity sideband cooling of trapped molecules is theoretically investigated for the case where the IR transition between two rovibrational states is used as a cycling transition. The molecules are assumed to be trapped either by a radio-frequency or optical trapping potential, depending on whether they are charged or neutral, and confined inside a high-finesse optical resonator which enhances radiative emission into the cavity mode. Using realistic experimental parameters and COS as a representative molecular example, we show that in this setup cooling to the trap ground state is feasible.

quant-ph↗

arXiv2011

Controlling the quality factor of a tuning-fork resonance between 9 K and 300 K for scanning-probe microscopy

We study the dynamic response of a mechanical quartz tuning fork in the temperature range from 9 K to 300 K. Since the quality factor Q of the resonance strongly depends on temperature, we implement a procedure to control the quality factor of the resonance. We show that we are able to dynamically change the quality factor and keep it constant over the whole temperature range. This procedure is suitable for applications in scanning probe microscopy.

physics.optics↗

arXiv2010

Feedback Cooling of a Single Neutral Atom

We demonstrate feedback cooling of the motion of a single rubidium atom trapped in a high-finesse optical resonator to a temperature of about 160 μK. Time-dependent transmission and intensity-correlation measurements prove the reduction of the atomic position uncertainty. The feedback increases the 1/e storage time into the one second regime, 30 times longer than without feedback. Feedback cooling therefore rivals state-of-the-art laser cooling, but with the advantages that it requires less optical access and exhibits less optical pumping.

quant-ph↗

arXiv2010

Velocity-selected molecular pulses produced by an electric guide

Electrostatic velocity filtering is a technique for the production of continuous guided beams of slow polar molecules from a thermal gas. We extended this technique to produce pulses of slow molecules with a narrow velocity distribution around a tunable velocity. The pulses are generated by sequentially switching the voltages on adjacent segments of an electric quadrupole guide synchronously with the molecules propagating at the desired velocity. This technique is demonstrated for deuterated ammonia (ND$_{3}$), delivering pulses with a velocity in the range of $20-100\,\rm{m/s}$ and a relative velocity spread of $(16\pm 2)\,%$ at FWHM. At velocities around $60\,\rm{m/s}$, the pulses contain up to $10^6$ molecules each. The data are well reproduced by Monte-Carlo simulations, which provide useful insight into the mechanisms of velocity selection.

physics.chem-ph↗

arXiv2010

Cavity-Enhanced Rayleigh Scattering

We demonstrate Purcell-like enhancement of Rayleigh scattering into a single optical mode of a Fabry-Perot resonator for several thermal atomic and molecular gases. The light is detuned by more than an octave, in this case by hundreds of nanometers, from any optical transition, making particle excitation and spontaneous emission negligible. The enhancement of light scattering into the resonator is explained quantitatively as an interference effect of light waves emitted by a classical driven dipole oscillator. Applications of our method include the sensitive, non-destructive in-situ detection of ultracold molecules.

quant-ph↗

arXiv2010

Calculating the Fine Structure of a Fabry-Perot Resonator using Spheroidal Wave Functions

A new set of vector solutions to Maxwell's equations based on solutions to the wave equation in spheroidal coordinates allows laser beams to be described beyond the paraxial approximation. Using these solutions allows us to calculate the complete first-order corrections in the short-wavelength limit to eigenmodes and eigenfrequencies in a Fabry-Perot resonator with perfectly conducting mirrors. Experimentally relevant effects are predicted. Modes which are degenerate according to the paraxial approximation are split according to their total angular momentum. This includes a splitting due to coupling between orbital angular momentum and spin angular momentum.

physics.optics↗

arXiv2008

Collisional effects in the formation of cold guided beams of polar molecules

High fluxes of cold polar molecules are efficiently produced by electric guiding and velocity filtering. Here, we investigate different aspects of the beam formation. Variations of the source parameters such as density and temperature result in characteristic changes in the guided beam. These are observed in the velocity distribution of the guided molecules as well as in the dependence of the signal of guided molecules on the trapping electric field. A model taking into account velocity-dependent collisional losses of cold molecules in the region close to the nozzle accurately reproduces this behavior. This clarifies an open question on the parameter dependence of the detected signal and gives a more detailed understanding of the velocity filtering and guiding process.

physics.chem-ph↗

arXiv2008

Continuous guided beams of slow and internally cold polar molecules

We describe the combination of buffer-gas cooling with electrostatic velocity filtering to produce a high-flux continuous guided beam of internally cold and slow polar molecules. In a previous paper (L.D. van Buuren et al., arXiv:0806.2523v1) we presented results on density and state purity for guided beams of ammonia and formaldehyde using an optimized set-up. Here we describe in more detail the technical aspects of the cryogenic source, its operation, and the optimization experiments that we performed to obtain best performance. The versatility of the source is demonstrated by the production of guided beams of different molecular species.

physics.chem-ph↗

arXiv2008

Spectroscopy of formaldehyde in the 30140-30790cm^-1 range

Room-temperature absorption spectroscopy of formaldehyde has been performed in the 30140-30790cm^-1 range. Using tunable ultraviolet continuous-wave laser light, individual rotational lines are well resolved in the Doppler-broadened spectrum. Making use of genetic algorithms, the main features of the spectrum are reproduced. Spectral data is made available as Supporting Information.

physics.chem-ph↗

arXiv2007

Cavity cooling of translational and ro-vibrational motion of molecules: ab initio-based simulations for OH and NO

We present detailed calculations at the basis of our recent proposal for simultaneous cooling the rotational, vibrational and external molecular degrees of freedom. In this method, the molecular rovibronic states are coupled by an intense laser and an optical cavity via coherent Raman processes enhanced by the strong coupling with the cavity modes. For a prototype system, OH, we showed that the translational motion is cooled to few micro Kelvin and the molecule is brought to the internal ground state in about a second. Here, we investigate numerically the dependence of the cooling scheme on the molecular polarizability, selecting NO as a second example. Furthermore, we demonstrate the general applicability of the proposed cooling scheme to initially vibrationally and rotationally hot molecular systems.

quant-ph↗

arXiv2007

Cavity cooling of internal molecular motion

We predict that it is possible to cool rotational, vibrational and translational degrees of freedom of molecules by coupling a molecular dipole transition to an optical cavity. The dynamics is numerically simulated for a realistic set of experimental parameters using OH molecules. The results show that the translational motion is cooled to few $μ$K and the internal state is prepared in one of the two ground states of the two decoupled rotational ladders in few seconds. Shorter cooling times are expected for molecules with larger polarizability.

quant-ph↗