arXiv subjects

Peter Hommelhoff

Publications and source records attributed to Peter Hommelhoff.

At least 55 records · Page 3Linked to original sources

arXiv2020

Attosecond-fast internal photoemission

The photoelectric effect has a sister process relevant in optoelectronics called internal photoemission. Here an electron is photoemitted from a metal into a semiconductor. While the photoelectric effect takes place within less than 100 attoseconds, the attosecond time scale has so far not been measured for internal photoemission. Based on the new method CHArge transfer time MEasurement via Laser pulse duration-dependent saturation fluEnce determinatiON, CHAMELEON, we show that the atomically thin semi-metal graphene coupled to bulk silicon carbide, forming a Schottky junction, allows charge transfer times as fast as (300 $\pm$ 200) attoseconds. These results are supported by a simple quantum mechanical model simulation. With the obtained cut-off bandwidth of 3.3 PHz for the charge transfer rate, this semimetal-semiconductor interface represents the first functional solid-state interface offering the speed and design space required for future light-wave signal processing.

physics.app-ph↗

arXiv2019

Generation and Characterization of Attosecond Micro-Bunched Electron Pulse Trains via Dielectric Laser Acceleration

Dielectric laser acceleration is a versatile scheme to accelerate and control electrons with the help of femtosecond laser pulses in nanophotonic structures. We demonstrate here the generation of a train of electron pulses with individual pulse durations as short as $270\pm80$ attoseconds(FWHM), measured in an indirect fashion, based on two subsequent dielectric laser interaction regions connected by a free-space electron drift section, all on a single photonic chip. In the first interaction region (the modulator), an energy modulation is imprinted on the electron pulse. During free propagation, this energy modulation evolves into a charge density modulation, which we probe in the second interaction region (the analyzer). These results will lead to new ways of probing ultrafast dynamics in matter and are essential for future laser-based particle accelerators on a photonic chip.

physics.acc-ph↗

arXiv2019

Femtosecond laser-induced electron emission from nanodiamond-coated tungsten needle tips

We present femtosecond laser-induced electron emission from nanodiamond-coated tungsten tips. Based on the shortness of the femtosecond laser pulses, electrons can be photo-excited for wavelengths from the infrared (1932 nm) to the ultraviolet (235 nm) because multi-photon excitation becomes efficient over the entire spectral range. Depending on the laser wavelength, we find different dominant emission channels identified by the number of photons needed to emit electrons. Based on the band alignment between tungsten and nanodiamond, the relevant emission channels can be identified as specific transitions in diamond and its graphitic boundaries. It is the combination of the character of initial and final states (i.e. bulk or surface-near, direct or indirect excitation in the diamond band structure), the number of photons providing the excitation energy and the peak intensity of the laser pulses that determines the dominant excitation channel for photoemission. A specific feature of the hydrogen-terminated nanodiamond coating is its negative electron affinity that significantly lowers the work function and enables efficient emission from the conduction band minimum into vacuum without energy barrier. The properties of these tips are encouraging for their use as laser-triggered electron sources in applications such as ultrafast electron microscopy and diffraction and novel photonics-based laser accelerators. Emission is stable for bunch charges up to 400 electrons per laser pulse. We infer a normalized emittance of < 0.20~nm~rad and a normalized brightness of > $1.2 \cdot 10^{12} \text{A} \text{ m}^{-2} \text{ sr}^{-1}$.

physics.app-ph↗

arXiv2019

CEP-stable soliton-based pulse compression to 4.4 fs and UV generation at 800 kHz repetition rate

We report generation of a femtosecond supercontinuum extending from the ultraviolet to the near-infrared and detection of its carrier-envelope phase variation by f-to-2f interferometry. The spectrum is generated in a gas-filled hollow-core photonic crystal fiber where soliton dynamics allows CEP-stable self-compression of OPCPA pump pulses at 800 nm to a duration of 1.7 optical cycles, followed by dispersive wave emission. The source provides up to 1 μJ of pulse energy at 800 kHz repetition rate resulting in 0.8 W of average power, and can be extremely useful for example in strong-field physics, pump-probe measurements and ultraviolet frequency comb metrology.

physics.optics↗

arXiv2019

A nanoscale vacuum-tube diode triggered by few-cycle laser pulses

We propose and demonstrate a nanoscale vacuum-tube diode triggered by few-cycle near-infrared laser pulses. It represents an ultrafast electronic device based on light fields, exploiting near-field optical enhancement at surfaces of two metal nanotips. The sharper of the two tips displays a stronger field-enhancement, resulting in larger photoemission yields at its surface. One laser pulse with a peak intensity of $4.7\times 10^{11}$ W/cm$^2$ triggers photoemission of ${\sim }16$ electrons from the sharper cathode tip, while emission from the blunter anode tip is suppressed by $19$ dB to ${\sim }0.2$ electrons per pulse. Thus, the laser-triggered current between two tips exhibit a rectifying behavior, in analogy to classical vacuum-tube diodes. According to the kinetic energy of the emitted electrons and the distance between tips, the total operation time of this laser-triggered nanoscale diode is estimated to be below 1 ps.

physics.optics↗

arXiv2019

Non-adiabatic ponderomotive effects in photoemission from nanotips in intense mid-infrared laser fields

Transient near-fields around metallic nanotips drive many applications, including the generation of ultrafast electron pulses and their use in electron microscopy. We have investigated the electron emission from a gold nanotip driven by mid-infrared few-cycle laser pulses. We identify a low-energy peak in the kinetic energy spectrum and study its shift to higher energies with increasing laser intensities from $1.7$ to $3.7\cdot10^{11} \mathrm{W}/\mathrm{cm}^2$. The experimental observation of the upshift of the low-energy peak is compared to a simple model and numerical simulations, which show that the decay of the near-field on a nanometer scale results in non-adiabatic transfer of the ponderomotive potential to the kinetic energy of emitted electrons and in turn to a shift of the peak. We derive an analytic expression for the non-adiabatic ponderomotive shift, which, after the previously found quenching of the quiver motion, completes the understanding of the role of inhomogeneous fields in strong-field photoemission from nanostructures.

physics.optics↗

arXiv2019

Dielectric-laser electron acceleration in a dual pillar grating with a distributed Bragg reflector

We report on the efficacy of a novel design for dielectric laser accelerators by adding a distributed Bragg reflector (DBR) to a dual pillar grating accelerating structure. This mimics a double-sided laser illumination, resulting in an enhanced longitudinal electric field while reducing the deflecting transverse effects, when compared to single-sided illumination. We improve the coupling efficiency of the incident electric field into the accelerating mode by 57 percent. The 12 $μ$m long structures accelerate sub-relativistic 28 keV electrons with gradients of up to 200 MeV/m in theory and 133 MeV/m in practice. Our work shows how lithographically produced nano-structures help to make novel laser accelerators more efficient.

physics.acc-ph↗

arXiv2019

Inelastic ponderomotive scattering of electrons at a high-intensity optical travelling wave in vacuum

In the early days of quantum mechanics Kapitza and Dirac predicted that matter waves would scatter off the optical intensity grating formed by two counter-propagating light waves [1]. This interaction, driven by the ponderomotive potential of the optical standing wave, was both studied theoretically and demonstrated experimentally for atoms [2] and electrons [3-5]. In the original version of the experiment [1,5], only the transverse momentum of particles was varied, but their energy and longitudinal momentum remained unchanged after the interaction. Here, we report on the generalization of the Kapitza-Dirac effect. We demonstrate that the energy of sub-relativistic electrons is strongly modulated on the few-femtosecond time scale via the interaction with a travelling wave created in vacuum by two colliding laser pulses at different frequencies. This effect extends the possibilities of temporal control of freely propagating particles with coherent light and can serve the attosecond ballistic bunching of electrons [6], or for the acceleration of neutral atoms or molecules by light.

physics.optics↗

arXiv2019

Ponderomotive generation and detection of attosecond free-electron pulse trains

Atomic motion dynamics during structural changes or chemical reactions have been visualized by picosecond and femtosecond pulsed electron beams via ultrafast electron diffraction and microscopy. Imaging the even faster dynamics of electrons in atoms, molecules and solids requires electron pulses with sub-femtosecond durations. We demonstrate here the all-optical generation of trains of attosecond free-electron pulses. The concept is based on the periodic energy modulation of a pulsed electron beam via an inelastic interaction with the ponderomotive potential of an optical travelling wave generated by two femtosecond laser pulses at different frequencies in vacuum. The subsequent dispersive propagation leads to a compression of the electrons and the formation of ultrashort pulses. The longitudinal phase space evolution of the electrons after compression is mapped by a second phase-locked interaction. The comparison of measured and calculated spectrograms reveals the attosecond temporal structure of the compressed electron pulse trains with individual pulse durations of less than 300 as. This technique can be utilized for tailoring and initial characterization of sub-optical cycle free-electron pulses at high repetition rates for stroboscopic time-resolved experiments with sub-femtosecond time resolution.

physics.optics↗

arXiv2019

Interaction of carrier envelope phase-stable laser pulses with graphene: the transition from the weak-field to the strong-field regime

Ultrafast control of electron dynamics in solid state systems has recently found particular attention. By increasing the electric field strength of laser pulses, the light-matter interaction in solids might turn from a perturbative into a novel non-perturbative regime, where interband transitions from the valence to the conduction band become strongly affected by intraband motion. We have demonstrated experimentally and numerically that this combined dynamics can be controlled in graphene with the electric field waveform of phase-stabilized few-cycle laser pulses. Here we show new experimental data and matching simulation results at comparably low optical fields, which allows us to focus on the highly interesting transition regime where the light-matter interaction turns from perturbative to non-perturbative. We find a 5th order power-law scaling of the laser induced waveform-dependent current at low optical fields, which breaks down for higher optical fields, indicating the transition.

physics.optics↗

arXiv2019

Fabrication and structural characterization of diamond-coated tungsten tips

Coating metal nanotips with a negative electron affinity material like hydrogen-terminated diamond bears promise for a high brightness photocathode. We report a recipe on the fabrication of diamond coated tungsten tips. A tungsten wire is etched electrochemically to a nanometer sharp tip, dip-seeded in diamond suspension and subsequently overgrown with a diamond film by plasma-enhanced chemical vapor deposition. With dip-seeding only, the seeding density declines towards the tip apex due to seed migration during solvent evaporation. The migration of seeds can be counteracted by nitrogen gas flow towards the apex, which makes coating of the apex with nanometer-thin diamond possible. At moderate gas flow, diamond grows homogeneously at shaft and apex whereas at high flow diamond grows in the apex region only. With this technique, we achieve a thickness of a few tens of nanometers of diamond coating within less than 1 $μ$m away from the apex. Conventional transmission electron microscopy (TEM), electron diffraction and electron energy loss spectroscopy confirm that the coating is composed of dense nanocrystalline diamond with a typical grain size of 20 nm. High resolution TEM reveals graphitic paths between the diamond grains.

cond-mat.mtrl-sci↗

arXiv2018

High spatial coherence in multiphoton-photoemitted electron beams

Nanometer-sharp metallic tips are known to be excellent electron emitters. They are used in highest-resolution electron microscopes in cold field emission mode to generate the most coherent electron beam in continuous-wave operation. For time-resolved operation, sharp metal needle tips have recently been triggered with femtosecond laser pulses. We show here that electrons emitted with near-infrared femtosecond laser pulses at laser oscillator repetition rates show the same spatial coherence properties as electrons in cold field emission mode in cw operation. From electron interference fringes, obtained with the help of a carbon nanotube biprism beam splitter, we deduce a virtual source size of less than $(0.65\pm0.06)\,$nm for both operation modes, a factor of ten smaller than the geometrical source size. These results bear promise for ultrafast electron diffraction, ultrafast electron microscopy and other techniques relying on highly coherent and ultrafast electron beams.

physics.app-ph↗

arXiv2018

Coherent electron trajectory control in graphene

We investigate coherent electron dynamics in graphene, interacting with the electric field waveform of two orthogonally polarized, few-cycle laser pulses. Recently, we demonstrated that linearly polarized driving pulses lead to sub-optical-cycle Landau-Zener quantum path interference by virtue of the combination of intraband motion and interband transition [Higuchi $\textit{et al.}$, Nature $\textbf{550}$, 224 (2017)]. Here we introduce a pulsed control laser beam, orthogonally polarized to the driving pulses, and observe the ensuing electron dynamics. The relative delay between the two pulses is a tuning parameter to control the electron trajectory, now in a complex fashion exploring the full two-dimensional reciprocal space in graphene. Depending on the relative phase, the electron trajectory in the reciprocal space can, for example, be deformed to suppress the quantum path interference resulting from the driving laser pulse. Intriguingly, this strong-field-based complex matter wave manipulation in a two-dimensional conductor is driven by a high repetition rate \textit{laser oscillator}, rendering unnecessary complex and expensive amplified laser systems.

cond-mat.mes-hall↗

arXiv2018

Silicon dual pillar structure with a distributed Bragg reflector for dielectric laser accelerators: Design and fabrication

Dielectric laser accelerators (DLAs) have proven to be good candidates for miniaturized particle accelerators. They rely on micro-fabricated dielectrics which are able to modulate the kinetic energy of the incoming electron beam under a proper laser illumination. In this paper we demonstrate a dual pillar structure with a distributed Bragg reflector to mimic a double sided illumination to the electron path. The structure is fabricated by an electron beam lithography technique followed by a cryogenic reactive ion etching process. Such a structure can accelerate the injected 28 keV electrons by a gradient of approximately 150 MeV/m which can be further optimized towards the GeV/m regime.

physics.acc-ph↗

arXiv2018

Alternating Phase Focusing for Dielectric Laser Acceleration

The concept of Dielectric Laser Acceleration (DLA) provides highest gradients among non-plasma particle accelerators. However, stable beam transport and staging have not been shown experimentally yet. We present a scheme that confines the beam longitudinally and in one transverse direction. Confinement in the other direction is obtained by a single conventional quadrupole magnet. Within the small aperture of 420 nm we find the matched distributions, which allow an optimized injection into pure transport, bunching, and accelerating structures. The combination of these resembles the photonics analogue of the Radio Frequency Quadrupole (RFQ), but since our setup is entirely twodimensional, it can be manufactured on a microchip by lithographic techniques. This is a crucial step towards relativistic electrons in the MeV range from low-cost, handheld devices.

physics.acc-ph↗

arXiv2018

Tracing the phase of focused broadband laser pulses

Precise knowledge of the behaviour of the phase of light in a focused beam is fundamental to understanding and controlling laser-driven processes. More than a hundred years ago an axial phase anomaly for focused monochromatic light beams was discovered and is now commonly known as the Gouy phase. Recent theoretical work has brought into question the validity of applying this monochromatic phase formulation to the broadband pulses becoming ubiquitous today. Based on electron back-scattering at sharp nanometre-scale metal tips, a method is available to measure light fields with sub-wavelength spatial resolution and sub-optical cycle time resolution. Here we report such a direct, three-dimensional measurement of the spatial dependence of the optical phase of a focused, 4-fs, near-infrared laser pulse. The observed optical phase deviates substantially from the monochromatic Gouy phase - exhibiting a much more complex spatial dependence, both along the propagation axis and in the radial direction. In our measurements, these significant deviations are the rule and not the exception for focused, broadband laser pulses. Therefore, we expect wide ramifications for all broadband laser-matter interactions, such as in high-harmonic and attosecond pulse generation, femtochemistry, ophthalmological optical coherence tomography and light-wave electronics.

physics.optics↗

arXiv2018

High-order above-threshold photoemission from nanotips controlled with two-color laser fields

We investigate the process of phase-controlled high-order above-threshold photoemission from sharp metallic nanotips under bichromatic laser fields. Experimental photoelectron spectra resulting from two-color excitation with a moderately intense near-infrared fundamental field (1560 nm) and its weak second harmonic show a strong sensitivity on the relative phase and clear indications for a plateau-like structure that is attributed to elastic backscattering. To explore the relevant control mechanisms, characteristic features, and particular signatures from near-field inhomogeneity, we performed systematic quantum simulations employing a one-dimensional nanotip model. Besides rich phase-dependent structures in the simulated above-threshold ionization (ATI) photoelectron spectra we find ponderomotive shifts as well as substantial modifications of the rescattering cutoff as function of the decay length of the near-field. To explore the quantum or classical nature of the observed features and to discriminate the two-color effects stemming from electron propagation and from the ionization rate we compare the quantum results to classical trajectory simulations. We show that signatures from direct electrons as well as the modulations in the plateau region mainly stem from control of the ionization probability, while the modulation in the cutoff region can only be explained by the impact of the two-color field on the electron trajectory. Despite the complexity of the phase-dependent features that render two-color strong-field photoemission from nanotips intriguing for sub-cycle strong-field control, our findings support that the recollision features in the cutoff region provide a robust and reliable method to calibrate the relative two-color phase.

physics.atom-ph↗

arXiv2017

High Visibility in Two-Color Above-Threshold Photoemission from Tungsten Nanotips in a Coherent Control Scheme

In this article we present coherent control of above-threshold photoemission from a tungsten nanotip achieving nearly perfect modulation. Depending on the pulse delay between fundamental (1560 nm) and second harmonic (780 nm) pulses of a femtosecond fiber laser at the nanotip, electron emission is significantly enhanced or depressed during temporal overlap. Electron emission is studied as a function of pulse delay, optical near-field intensities, DC bias field, and final photoelectron energy. Under optimized conditions modulation amplitudes of the electron emission of 97.5% are achieved. Experimental observations are discussed in the framework of quantum- pathway interference supported by local density of states (LDOS) simulations.

physics.optics↗