arXiv subjects

Pratap Raychaudhuri

Publications and source records attributed to Pratap Raychaudhuri.

At least 73 records · Page 4Linked to original sources

arXiv2013

A 350 mK, 9 T scanning tunneling microscope for the study of superconducting thin films and single crystals

We report the construction and performance of a low temperature, high field scanning tunneling microscope (STM) operating down to 350mK and in magnetic fields up to 9T, with thin film deposition and in-situ cleaving capabilities. The main focus lies on the simple design of STM head allowing top loading of the sample and innovative sample holder design that allows us to get spectroscopic data on superconducting thin films grown in-situ on insulating substrates. Other design details on sample transport, chamber and vibration isolation scheme are also described. We demonstrate the capability of our instrument through the atomic resolution imaging and spectroscopy on NbSe2 single crystal and spectroscopic maps obtained on homogeneously disordered NbN thin film.

cond-mat.supr-con↗

arXiv2013

A two-coil mutual inductance technique to study matching effect in disordered NbN thin films

Although matching effects in superconducting anti-dot arrays have been studied extensively through magneto-resistance oscillations, these investigations have been restricted to a very narrow temperature window close to the superconducting transition. Here we report a "two coil" mutual inductance technique, which allows the study of this phenomenon deep in the superconducting state, through a direct measurement of the magnetic field variation of the shielding response. We demonstrate how this technique can be used to resolve outstanding issues on the origin of matching effects in superconducting thin films with periodic array of holes grown on anodized alumina membranes.

cond-mat.supr-con↗

arXiv2013

Probing long-range correlations in the Berezinskii-Kosterlitz-Thouless fluctuation regime of ultra-thin NbN superconducting films using transport noise measurements

We probe the presence of long-range correlations in phase fluctuations by analyzing the higher-order spectrum of resistance fluctuations in ultra-thin NbN superconducting films. The non-Gaussian component of resistance fluctuations is found to be sensitive to film thickness close to the transition, which allows us to distinguish between mean field and Berezinskii-Kosterlitz-Thouless (BKT) type superconducting transitions. The extent of non-Gaussianity was found to be bounded by the BKT and mean field transition temperatures and depend strongly on the roughness and structural inhomogeneity of the superconducting films. Our experiment outlines a novel fluctuation-based kinetic probe in detecting the nature of superconductivity in disordered low-dimensional materials.

cond-mat.supr-con↗

arXiv2013

Emergence of nanoscale inhomogeneity in the superconducting state of a homogeneously disordered conventional superconductor, NbN

The notion of spontaneous formation of an inhomogeneous superconducting state is at the heart of most theories attempting to understand the superconducting state in the presence of strong disorder. Using scanning tunneling spectroscopy and high resolution scanning transmission electron microscopy, we experimentally demonstrate that under the competing effects of strong homogeneous disorder and superconducting correlations, the superconducting state of a conventional superconductor, NbN, spontaneously segregates into domains. Tracking these domains as a function of temperature we observe that the superconducting domains persist across the bulk superconducting transition, Tc, and disappear close to the pseudogap temperature, T*, where signatures of superconducting correlations disappear from the tunneling spectrum and the superfluid response of the system.

cond-mat.supr-con↗

arXiv2013

The effect of Coulomb interactions on the disorder driven superconductor-insulator transition: THz versus tunneling spectroscopy

The interplay between disorder and superconductivity has intrigued physicists for decades. Of particular interest is the influence of disorder on the superconducting energy gap $Δ$. In the absence of Coulomb interactions between electrons, disorder leads to emergent granularity of the local order parameter resulting in a pseudogap at temperatures above the critical temperature $T_c$, as well as a finite gap $Δ$ on the insulating side of the disorder-driven superconductor-insulator transition (SIT). At the same time, disorder also enhances the Coulomb interactions, which subsequently may influence $Δ$ in a manner that is still not fully understood. Here we investigate the evolution of the energy gap through the SIT by two different experimental methods: tunneling spectroscopy, in which a metallic electrode is placed close to the studied sample thus screening the Coulomb interactions, and terahertz (THz) spectroscopy, which probes the unscreened sample. The comparison between the two methods illustrates the role played by electronic interactions in determining the nature of the phases across the SIT and sheds light on the mechanisms involved in the destruction of superconductivity.

cond-mat.supr-con↗

arXiv2012

Frequency dependent superfluid stiffness in the pseudogap regime in strongly disordered NbN thin films

We measure the frequency dependence of the complex ac conductivity of NbN films with different levels of disorder in frequency range 0.4-20 GHz. Films with low disorder exhibit a narrow dynamic fluctuation regime above T_c as expected for a conventional superconductor. However, for strongly disordered samples, the fluctuation regime extends well above T_c, with a strongly frequency-dependent superfluid stiffness which disappears only at a temperature T* close to the pseudogap temperature obtained from scanning tunneling measurements. Such a finite-frequency response is associated to a marked slowing down of the superconducting fluctuations already below T*. The corresponding large length-scale fluctuations suggest a scenario of thermal phase fluctuations between superconducting domains in a strongly disordered s-wave superconductor.

cond-mat.supr-con↗

arXiv2012

Observation of Andreev bound state and multiple energy gaps in the non-centrosymmetric superconductor BiPd

We report directional point contact Andreev reflection (PCAR) measurements on high-quality single crystals of the non-centrosymmetric superconductor, BiPd. The PCAR spectra measured on different crystallographic faces of the single crystal clearly show the presence of multiple superconducting energy gaps. For point contacts with low resistance, in addition to the superconducting gap feature, a pronounced zero bias conductance peak is observed. These observations provide strong evidence of the presence of unconventional order parameter in this material.

cond-mat.supr-con↗

arXiv2011

Phase diagram of a strongly disordered s-wave superconductor, NbN, close to the metal-insulator transition

We present a phase diagram as a function of disorder in three-dimensional NbN thin films, as the system enters the critical disorder for the destruction of the superconducting state. The superconducting state is investigated using a combination of magnetotransport and tunneling spectroscopy measurements. Our studies reveal 3 different disorder regimes. At low disorder the (k_{F}l~10-4), the system follows the mean field Bardeen-Cooper-Schrieffer behavior where the superconducting energy gap vanishes at the temperature where electrical resistance appears. For stronger disorder (k_{F}l<4) a "pseudogap" state emerges where a gap in the electronic spectrum persists up to temperatures much higher than Tc, suggesting that Cooper pairs continue to exist in the system even after the zero resistance state is destroyed. Finally, very strongly disordered samples (k_{F}l<1) exhibit a pronounced magnetoresistance peak at low temperatures, suggesting that localized Cooper pairs continue to survive in the system even after the global superconducting ground state is completely destroyed.

cond-mat.supr-con↗

arXiv2011

Role of the vortex-core energy on the Beresinkii-Kosterlitz-Thouless transition in thin films of NbN

We analyze the occurrence of the Beresinkii-Kosterlitz-Thouless transition in thin films of NbN at various film thickness, by probing the effect of vortex fluctuations on the temperature dependence of the superfluid density below $T_{BKT}$ and of the resistivity above $T_{BKT}$. By direct comparison between the experimental data and the theory we show the crucial role played by the vortex-core energy in determining the characteristic signatures of the BKT physics, and we estimate its dependence on the disorder level. Our work provides a paradigmatic example of BKT physics in a quasi-two-dimensional superconductor.

cond-mat.supr-con↗

arXiv2010

Phase fluctuations in a strongly disordered s-wave superconductor close to the metal-insulator transition

We explore the role of phase fluctuations in a 3-dimensional s-wave superconductor, NbN, as we approach the critical disorder for the destruction of the superconducting state. Scanning tunneling spectroscopy measurements reveal that in the presence of strong disorder, a finite gap in the electronic spectrum continues to persist at temperatures above Tc. With increase in disorder, the superfluid density is strongly suppressed at low temperatures and evolves towards a linear-T variation at higher temperatures. These observations provide strong evidence that phase fluctuation leads to the formation of a pseudogap state in a disordered conventional superconductor.

cond-mat.supr-con↗

arXiv2010

Phase diagram and upper critical field of homogenously disordered epitaxial 3-dimensional NbN films

We report the evolution of superconducting properties with disorder, in 3-dimensional homogeneously disordered epitaxial NbN thin films. The effective disorder in NbN is controlled from moderately clean limit down to Anderson metal-insulator transition by changing the deposition conditions. We propose a phase diagram for NbN in temperature-disorder plane. With increasing disorder we observe that as kFl-->1 the superconducting transition temperature (Tc) and minimum conductivity (sigma_0) go to zero. The phase diagram shows that in homogeneously disordered 3-D NbN films, the metal-insulator transition and the superconductor-insulator transition occur at a single quantum critical point at kFl~1.

cond-mat.supr-con↗

arXiv2010

Effect of Phase Fluctuations on the Superconducting Properties of Strongly Disordered 3D NbN Thin Films

We present transport, Hall effect, electronic tunnelling and penetration depth studies in 3D homogeneously disordered epitaxial NbN thin films with disorder ranging from the moderately clean limit (k_Fl~10.12) to the very dirty limit (k_Fl~1.24). The superconducting transition temperature (T_c) decreases from ~17K to less than 350mK with increasing disorder. The T_c and conductivity at the lowest temperature both asymptotically approach zero as k_Fl tends to 1, indicating a coincidence of the metal-insulator transition (MIT) and the superconductor-insulator transition. Close to critical disorder there is spatial inhomogeneity in the superconducting density of states (DOS) and the superconducting state is governed by quantum phase fluctuations. This results in suppression of the superfluid density (n_s) and a pseudogap state where the resistance is no longer zero but the energy gap remains finite

cond-mat.supr-con↗

arXiv2010

Observation of Vortex Matching Phenomena in Antidot Array of NbN Thin Film

We report vortex matching phenomenon in rectangular antidot array fabricated on epitaxial NbN thin film. The antidot array was fabricated using Focussed Ion Beam milling technique. The magneto-transport measurements points to a period doubling transition at higher magnetic field for rectangular lattices. The results are discussed within the light of several models including the multi-vortex model, the matched lattice model and the super-matched lattice model.

cond-mat.supr-con↗

arXiv2010

Penetration depth and tunneling studies in very thin epitaxial NbN films

We investigate evolution of the magnetic penetration depth and superconducting energy gap in epitaxial NbN films using a low frequency mutual inductance technique and tunneling spectroscopy using a low temperature scanning tunneling microscope (STM). The superconducting transition temperature (Tc) for films grown under optimal growth conditions decreases monotonically from 15.87K to 9.16K as the film thickness is decreased from 50nm to 3nm. With decrease in film thickness delta(0) monotonically decreases, whereas lambda(0) monotonically increases. We observe that Tc, lambda(o) and delta(0) are well described by Bardeen-Cooper-Schrieffer (BCS) theory in all films other than the two thinnest ones where we see evidence of the Kosterlitz-Thouless-Berezinski (KTB) transition close to Tc.

cond-mat.supr-con↗

arXiv2009

Temperature dependence of resistivity and Hall-coefficient in a strongly disordered metal: NbN

We report the temperature dependence of resistivity (rho) and Hall coefficient (R_H) in the normal state of homogeneously disordered epitaxial NbN thin films with kFl~3.27-10.12. The superconducting transition temperature (Tc) of these films varies from 8.13K to 16.8K. While our least disordered film displays usual metallic behavior, for all the films with kFl<8.13, both and are negative up to 300K. We observe that R_H(T) varies linearly with rho(T) for all the films. Measurements performed on a 2nm thick Be film shows similar behavior >. This behavior is inconsistent with existing theories of localization and e-e interactions in a disordered metal.

cond-mat.dis-nn↗

arXiv2009

Vortex matching effect in engineered thin films of NbN

We report robust vortex matching effects in antidot arrays fabricated on thin films of NbN. The near absence of hysteresis between field sweep directions indicates a negligible residual pinning in the host thin film. Owing to the very small coherence length of NbN thin films ($ξ< 5 nm$), the observations suggests the possibility of probing physics of vortices at true nanometer length scales in suitably fabricated structures.

cond-mat.supr-con↗

arXiv2008

Tunneling studies in a homogeneously disordered s-wave superconductor: NbN

We report the evolution of superconducting properties as a function of disorder in homogeneously disordered epitaxial NbN thin films grown on (100) MgO substrates, studied through a combination of electrical transport, Hall Effect and tunneling measurements. The thickness of all our films are >50nm much larger than the coherence length ~5nm. The effective disorder in different films encompasses a large range, with the Ioffe-Regel parameter varying in the range kFl~1.38-8.77. Tunneling measurements on films with different disorder reveals that for films with large disorder the bulk superconducting transition temperature (Tc) is not associated with a vanishing of the superconducting energy gap, but rather a large broadening of the superconducting density of states. Our results provide strong evidence of the loss of superconductivity via phase-fluctuations in a disordered s-wave superconductor.

cond-mat.supr-con↗

arXiv2008

Effect of Pt doping on the critical temperature and upper critical field in YNi2-xPtxB2C (x=0-0.2)

We investigate the evolution of superconducting properties by doping non-magnetic impurity in single crystals of YNi2-xPtxB2C (x=0-0.2). With increasing Pt doping the critical temperature (Tc) monotonically decreases from 15.85K and saturates to a value ~13K for x>0.14. However, unlike conventional s-wave superconductors, the upper critical field (HC2) along both crystallographic directions a and c decreases with increasing Pt doping. Specific heat measurements show that the density of states (N(EF)) at the Fermi level (EF) and the Debye temperatures (Theta_D) in this series remains constant within the error bars of our measurement. We explain our results based on the increase in intraband scattering in the multiband superconductor YNi2B2C.

cond-mat.supr-con↗