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Pratap Raychaudhuri

Publications and source records attributed to Pratap Raychaudhuri.

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Study of spin fluctuations in Ni3Al using point contact Andreev reflection spectroscopy

We report point contact Andreev reflection (PCAR) spectroscopy studies on Ni3Al with composition range (24, 26 and 27 at. % of Al in the solid solution) spanning the ferromagnetic to paramagnetic phase boundary. PCAR studies performed using Nb tip as counter electrode reveal that the superconducting quasiparticle lifetime (\tao) and superconducting energy gap (δ) decreases with increasing spin fluctuation in the normal metal electrode. Our study reveals that PCAR could be a useful probe to study spin fluctuations in systems which are on the verge of a magnetic instability.

cond-mat.supr-con↗

Superconducting properties and Hall Effect of epitaxial NbN thin films

We have measured the magnetotransport properties and Hall effect of a series of epitaxial NbN films grown on (100) oriented single crystalline MgO substrate under different conditions using reactive magnetron sputtering. Hall effect measurements reveal that the carrier density in NbN thin films is sensitive to the growth condition. The carrier density increases by a factor of 3 between the film with highest normal state resistivity (rho_n~3.83micro-Ohm-m) and lowest transition temperature (Tc~9.99K) and the film with lowest normal state resistivity (rho_n~0.94micro-Ohm-m) and highest transition temperature (Tc~16.11K) while the mobility of carriers does not change significantly except for the most resistive films. Our results show that the Tc of NbN is governed primarily by the carrier density rather than disorder scattering. By varying the carrier concentration during growth we can vary the effective disorder (kF_l) from the moderately clean limit to the dirty limit which makes this system ideal to study the interplay of carrier density and disorder on the superconducting properties of an s-wave superconductor.

cond-mat.supr-con↗

Non-intrinsic superconductivity in InN epilayers: role of Indium Oxide

In recent years there have been reports of anomalous electrical resistivity and the presence of superconductivity in semiconducting InN layers. By a careful correlation of the temperature dependence of resistivity and magnetic susceptibility with structural information from highresolution x-ray diffraction measurements we show that superconductivity is not intrinsic to InN and is seen only in samples that show traces of oxygen impurity. We hence believe that InN is not intrinsically a superconducting semiconductor.

cond-mat.mtrl-sci↗

Competing effects of surface phonon softening and quantum size effects on the superconducting properties of nanostructured Pb

The superconducting transition temperature (TC) in nanostructured Pb remains nearly constant as the particle size is reduced from 65 to 7nm, below which size the superconductivity is lost rather abruptly. In contrast, there is a large enhancement in the upper critical field (HC2) in the same size regime. We explore the origin of the unusual robustness of the TC over such a large particle size range in nanostructured Pb, by measuring the temperature dependence of the superconducting energy gap in planar tunnel junctions of Al/Al2O3/nano-Pb. We show that below 22nm, the electron phonon coupling strength increases monotonically with decreasing particle size, and almost exactly compensates for the quantum size effect, which is expected to suppress TC.

cond-mat.mes-hall↗

Size induced metal insulator transition in nanostructured Niobium thin films: Intragranular and intergranular contributions

With a reduction in the average grain size in nanostructured films of elemental Nb, we observe a systematic crossover from metallic to weakly-insulating behavior. An analysis of the temperature dependence of the resistivity in the insulating phase clearly indicates the existence of two distinct activation energies corresponding to inter-granular and intra-granular mechanisms of transport. While the high temperature behavior is dominated by grain boundary scattering of the conduction electrons, the effect of discretization of energy levels due to quantum confinement shows up at low temperatures. We show that the energy barrier at the grain boundary is proportional to the width of the largely disordered inter-granular region, which increases with a decrease in the grain size. For a metal-insulator transition to occur in nano-Nb due to the opening up of an energy gap at the grain boundary, the critical grain size is ~ 8nm and the corresponding grain boundary width is ~ 1.1nm.

cond-mat.mes-hall↗

Upper critical field in nanostructured Nb: Competing effects of the reduction in density of states and the mean free path

We show that the upper critical field in nanometer-sized Nb particles is governed by the changes in the effective Ginzburg-Landau coherence length occurring due to two competing factors: (i) the decrease in the grain size and consequent increase of disorder, and (ii) the effective decrease in the density of states at the Fermi level due to the formation of a Kubo gap. As a result, the upper critical field (HC2) and irreversibility fields (Hirr) in nanostructured Nb show non-monotonic grain size dependences. Between 60nm to 20nm, HC2 is found to increase by 2.5times while there is no appreciable decrease in the superconducting transition temperature (TC) from its bulk value of 9.4K. This can be ascribed to a decrease in the coherence length due to a reduction in the mean free path with decreasing size. Below 20 nm, however, HC2 decreases with decreasing size. In this size range (<20 nm), there also occurs a decrease in the TC as well as the superconducting energy gap. The decrease in HC2 in this regime can be ascribed to the decrease in the density of states at the Fermi level due to a quantization in the electronic energy levels.

cond-mat.mes-hall↗

Temperature dependence of transport spin polarization in NdNi5 measured using Point Contact Andreev reflection

We report a study in which Point contact Andreev reflection (PCAR) spectroscopy using superconducting Nb tip has been carried out on NdNi5, a ferromagnet with a Curie temperature of TC~7.7K. The measurements were carried out over a temperature range of 2-9K which spans across the ferromagnetic transition temperature. From an analysis of the spectra, we show that (i) the temperature dependence of the extracted value of transport spin polarization closely follows the temperature dependence of the spontaneous magnetization; (ii) the superconducting quasiparticle lifetime shows a large decrease close to the Curie temperature of the ferromagnet. We attribute the latter to the presence of strong ferromagnetic spin fluctuations in the ferromagnet close to the ferromagnetic transition temperature.

cond-mat.supr-con↗

CeMnNi4: A soft ferromagnet with a high degree of transport spin polarization

In this letter we introduce a new soft ferromagnetic compound, i.e. CeMnNi4, which exhibits a large moment (~4.95mu_B/Mn) and high degree of spin polarization. The system has a ferromagnetic transition temperature of 148K. Isothermal magnetization measurements at 5K reveal that the material is a soft ferromagnet with a magnetization saturating at about 500Oe and a coercive field of < 5 Oe. We determine the transport spin polarization of this material from Point Contact Andreev Reflection measurements to be 66% thereby making this material potentially important for spintronic applications.

cond-mat.mtrl-sci↗

Size dependence of the Tc and the superconducting energy gap in nanocrystalline thin films of Nb

In nanocrystalline Nb films, the superconducting Tc decreases with a reduction in the average particle size below 20nm. We correlate the decrease in Tc with a reduction in the superconducting energy gap measured by point contact spectroscopy. Consistent with the Anderson criterion, no superconducting transition was observed for sizes below 8 nm. We show that the size-dependence of the superconducting properties in this intermediate coupling Type II superconductor is governed by changes in the electronic density of states rather than by phonon softening.

cond-mat.supr-con↗