arXiv subjects

Q. Yao

Publications and source records attributed to Q. Yao.

At least 19 recordsLinked to original sources

arXiv2024

Variational Scarring in Graphene Quantum Dots

A quantum eigenstate of a classically chaotic system is referred as scarred by an unstable periodic orbit if its probability density is concentrated in the vicinity of that orbit. Recently, a new class of scarring - variational scarring - was discovered in numerical studies of disordered quantum dots, arising from near-degeneracies in the quantum spectrum associated with classical resonances of the unperturbed system. Despite the increasing body of theoretical evidence on variational scarring, its experimental observation has remained out of reach. Motivated by this dearth, we argue and demonstrate that variational scarring can occur in an elliptical quantum dot fabricated on monolayer graphene, and locally perturbed by a nanotip. Then, we further show that the fingerprint of these variational scars can potentially be detected via scanning tunneling microscopy, thus offering an attractive experimental pathway for the first validation of this puzzling quantum-chaotic phenomenon.

cond-mat.mes-hall↗

arXiv2023

Topologically protected one-dimensional electronic states in group IV two-dimensional Dirac materials

In this report we give a brief introduction on the occurrence of topologically protected one-dimensional electronic states in group IV two-dimensional graphene-like materials. We discuss the effect of spin-orbit coupling on the electronic band structure and show that these materials are potential candidates to exhibit the quantum spin Hall effect. The quantum spin Hall effect is characterized by a gapped interior and metallic counter-propagating spin-polarized topologically protected edges states. We also elaborate on the electric-field induced formation of a hexagonal network of one-dimensional topologically protected electronic states in small-angle twisted bilayer graphene.

cond-mat.mes-hall↗

arXiv2023

Persistent, controllable circulation of a polariton ring condensate

Persistent circulation is a canonical effect of superfluidity. In previous experiments, quantized circulation has been observed in polariton condensates, usually far from equilibrium, but persistent current in the absence of any stirring has not been seen. We report here the direct observation of persistent circulation of a polariton condensate with no driving force and with no observable change in time. We can cause the condensate to circulate in either direction on demand using a short laser pulse, after which the condensate continues to circulate for dozens to hundreds of rotations around a ring trap without any further stimulation. Our theoretical model successfully shows how the pulse, despite not carrying any angular momentum, causes the circulation.

cond-mat.quant-gas↗

arXiv2021

Valley protected one-dimensional states in small-angle twisted bilayer graphene

Theory predicts that the application of an electric field breaks the inversion symmetry of AB and BA stacked domains in twisted bilayer graphene, resulting in the formation of a triangular network of one-dimensional valley-protected helical states. This two-dimensional network of one-dimensional states has been observed in several studies, but direct experimental evidence that the electronic transport in these one-dimensional states is valley-protected is still lacking. In this study, we report the existence of the network in small-angle twisted bilayer graphene at room temperature. Moreover, by analyzing Fourier transforms of atomically resolved scanning tunnelling microscopy images of minimally twisted bilayer graphene, we provide convincing experimental evidence that the electronic transport in the counter-propagating one-dimensional states is indeed valley protected.

cond-mat.mes-hall↗

arXiv2020

Colossal band renormalization and stoner ferromagnetism induced by electron-antiferromagnetic-magnon coupling

The interactions between electrons and antiferromagnetic magnons (AFMMs) are important for a large class of correlated materials. For example, they are the most plausible pairing glues in high-temperature superconductors, such as cuprates and iron pnictides. However, unlike electron-phonon interactions (EPIs), clear-cut observations regarding how electron-AFMM interactions (EAIs) affect the band structure are still lacking. Consequently, critical information on the EAIs, such as its strength and doping dependence, remains elusive. Here we directly observe that EAIs induces a kink structure in the band dispersion in Ba$_{1-x}$K$_x$Mn$_2$As$_2$, and subsequently unveil several key characteristics of EAIs. We found that the coupling constant of EAIs can be as large as 6, and it shows huge doping dependence and temperature dependence, all in stark contrast to the behaviors of EPI and beyond our current understanding of EAIs. Such a colossal renormalization of electronic bands by EAIs drives the system to the Stoner criteria, giving the intriguing ferromagnetic state in Ba$_{1-x}$K$_x$Mn$_2$As$_2$. Our results expand the current knowledge of EAIs, which may facilitate the further understanding of many correlated materials where EAIs play a critical role, such as high-temperature superconductors.

cond-mat.str-el↗

arXiv2019

Electronic structure and 4f-electron character in Ce2PdIn8 studied by angle-resolved photoemission spectroscopy

The localized-to-itinerant transition of f electrons lies at the heart of heavy-fermion physics, but has only been directly observed in single-layer Ce-based materials. Here, we report a comprehensive study on the electronic structure and nature of the Ce 4f electrons in the heavy-fermion superconductor Ce2PdIn8, a typical n=2 CenMmIn3n+2m compound, using high-resolution and 4d-4f resonance photoemission spectroscopies. The electronic structure of this material has been studied over a wide temperature range, and hybridization between f and conduction electrons can be clearly observed to form a Kondo resonance near the Fermi level at low temperatures. The characteristic temperature of the localized-to-itinerant transition is around 120K, which is much higher than its coherence temperature Tcoh~30K.

cond-mat.str-el↗

arXiv2018

Pushing Photons with Electrons: Observation of the Polariton Drag Effect

We show the direct effect of free electrons colliding with polaritons, changing their momentum. The result of this interaction of the electrons with the polaritons is a change in the angle of emission of the photons from our cavity structure. Because the experiment is a photon-in, photon-out system, this is equivalent to optical beam steering of photons using a direct electrical current. The effect is asymmetric, significantly slowing down the polaritons when they move oppositely to the electrons, while the polariton momentum only slightly increases when electrons moving in the same direction. We present a theoretical model which describes this effect.

cond-mat.quant-gas↗

arXiv2018

On-chip III-V monolithic integration of heralded single photon sources and beamsplitters

We demonstrate a monolithic III-V photonic circuit combining a heralded single photon source with a beamsplitter, at room temperature and telecom wavelength. Pulsed parametric down-conversion in an AlGaAs waveguide generates counterpropagating photons, one of which is used to herald the injection of its twin into the beamsplitter. We use this configuration to implement an integrated Hanbury-Brown and Twiss experiment, yielding a heralded second-order correlation $g^{(2)}_{\rm her}(0)=0.10 \pm 0.02$ that confirms single-photon operation. The demonstrated generation and manipulation of quantum states on a single III-V semiconductor chip opens promising avenues towards real-world applications in quantum information.

quant-ph↗

arXiv2018

Charge Transfer Effects in Naturally Occurring van der Waals Heterostructures (PbSe)1.16(TiSe2)m (m=1, 2)

Van der Waals heterostructures (VDWHs) exhibit rich properties and thus has potential for applications, and charge transfer between different layers in a heterostructure often dominates its properties and device performance. It is thus critical to reveal and understand the charge transfer effects in VDWHs, for which electronic structure measurements have proven to be effective. Using angle-resolved photoemission spectroscopy, we studied the electronic structures of (PbSe)1.16(TiSe2)m(m=1, 2), which are naturally occurring VDWHs, and discovered several striking charge transfer effects. When the thickness of the TiSe2 layers is halved from m=2 to m=1, the amount of charge transferred increases unexpectedly by more than 250%. This is accompanied by a dramatic drop in the electron-phonon interaction strength far beyond the prediction by first-principles calculations and, consequently, superconductivity only exists in the m=2 compound with strong electron-phonon interaction, albeit with lower carrier density. Furthermore, we found that the amount of charge transferred in both compounds is nearly halved when warmed from below 10 K to room temperature, due to the different thermal expansion coefficients of the constituent layers of these misfit compounds. These unprecedentedly large charge transfer effects might widely exist in VDWHs composed of metal-semiconductor contacts; thus, our results provide important insights for further understanding and applications of VDWHs.

cond-mat.str-el↗

arXiv2018

Unveiling the superconducting mechanism of Ba$_{0.51}$K$_{0.49}$BiO$_3$

Bismuthates were the first family of oxide high-temperature superconductors, exhibiting superconducting transition temperatures (Tc) up to 32K, but the superconducting mechanism remains under debate despite more than 30 years of extensive research. Our angle-resolved photoemission spectroscopy studies on Ba$_{0.51}$K$_{0.49}$BiO$_3$ reveal an unexpectedly 34% larger bandwidth than in conventional density functional theory calculations. This can be reproduced by calculations that fully account for long-range Coulomb interactions --- the first direct demonstration of bandwidth expansion due to the Fock exchange term, a long-accepted and yet uncorroborated fundamental effect in many body physics. Furthermore, we observe an isotropic superconducting gap with 2Δ$_0$/k$_B$ T$_c$ = 3.51 $\pm$ 0.05, and strong electron-phonon interactions with a coupling constant λ$\sim$ 1.3 $\pm$ 0.2. These findings solve a long-standing mystery --- Ba$_{0.51}$K$_{0.49}$BiO$_3$ is an extraordinary Bardeen-Cooper-Schrieffer (BCS) superconductor, where long-range Coulomb interactions expand the bandwidth, enhance electron-phonon coupling, and generate the high Tc. Such effects will also be critical for finding new superconductors.

cond-mat.supr-con↗

arXiv2018

Tracing crystal-field splittings in the rare earth-based intermetallic CeIrIn$_5$

Crystal electric field states in rare earth intermetallics show an intricate entanglement with the many-body physics that occurs in these systems and that is known to lead to a plethora of electronic phases. Here, we attempt to trace different contributions to the crystal electric field (CEF) splittings in CeIrIn$_5$, a heavy-fermion compound and member of the Ce$M$In$_5$ ($M$= Co, Rh, Ir) family. To this end, we utilize high-resolution resonant angle-resolved photoemission spectroscopy (ARPES) and present a spectroscopic study of the electronic structure of this unconventional superconductor over a wide temperature range. As a result, we show how ARPES can be used in combination with thermodynamic measurements or neutron scattering to disentangle different contributions to the CEF splitting in rare earth intermetallics. We also find that the hybridization is stronger in CeIrIn$_5$ than CeCoIn$_5$ and the effects of the hybridization on the Fermi volume increase is much smaller than predicted. By providing the first experimental evidence for $4f_{7/2}^{1}$ splittings which, in CeIrIn$_5$, split the octet into four doublets, we clearly demonstrate the many-body origin of the so-called $4f_{7/2}^{1}$ state.

cond-mat.str-el↗

arXiv2017

Phonon-enhanced superconductivity at the FeSe/SrTiO3 interface

The dream of room temperature superconductors has inspired intense research effort to find routes for enhancing the superconducting transition temperature (Tc). Therefore, single-layer FeSe on a SrTiO3 substrate, with its extraordinarily high Tc amongst all interfacial superconductors and iron based superconductors, is particularly interesting, but the mechanism underlying its high Tc has remained mysterious. Here we show through isotope effects that electrons in FeSe couple with the oxygen phonons in the substrate, and the superconductivity is enhanced linearly with the coupling strength atop the intrinsic superconductivity of heavily-electron-doped FeSe. Our observations solve the enigma of FeSe/SrTiO3, and experimentally establish the critical role and unique behavior of electron-phonon forward scattering in a correlated high-Tc superconductor. The effective cooperation between interlayer electron-phonon interactions and correlations suggests a path forward in developing more high-Tc interfacial superconductors, and may shed light on understanding the high Tc of bulk high temperature superconductors with layered structures.

cond-mat.supr-con↗

arXiv2017

Optomechanical properties of GaAs/AlAs micropillar resonators operating in the 18 GHz range

Recent experiments demonstrated that GaAs-AlAs based micropillar cavities are promising systems for quantum optomechanics, allowing the simultaneous three-dimensional confinement of near-infrared photons and acoustic phonons in the 18-100 GHz range. Here, we investigate through numerical simulations the optomechanical properties of this new platform. We evidence how the Poisson's ratio and semiconductor-vacuum boundary conditions lead to very distinct features in the mechanical and optical three dimensional confinement. We find a strong dependence of the mechanical quality factor and strain distribution on the micropillar radius, in great contrast to what is predicted and observed in the optical domain. The derived optomechanical coupling constants g_0 reach ultra-large values in the 10^6 rad/s range.

cond-mat.mes-hall↗

arXiv2017

Structural and electronic properties of germanene on MoS$_2$

To date, germanene has only been synthesized on metallic substrates. A metallic substrate is usually detrimental for the two-dimensional Dirac nature of germanene because the important electronic states near the Fermi level of germanene can hybridize with the electronic states of the metallic substrate. Here we report the successful synthesis of germanene on molybdenum disulfide (MoS$_2$), a band gap material. Pre-existing defects in the MoS$_2$ surface act as preferential nucleation sites for the germanene islands. The lattice constant of the germanene layer (3.8 $\pm$ 0.2 Å) is about 20\% larger than the lattice constant of the MoS$_2$ substrate (3.16 Å). Scanning tunneling spectroscopy measurements and density functional theory calculations reveal that there are, besides the linearly dispersing bands at the $K$ points, two parabolic bands that cross the Fermi level at the $Γ$ point.

cond-mat.mtrl-sci↗

arXiv2017

Electronic structure of FeS

Here we report the electronic structure of FeS, a recently identified iron-based superconductor. Our high-resolution angle-resolved photoemission spectroscopy studies show two hole-like ($α$ and $β$) and two electron-like ($η$ and $δ$) Fermi pockets around the Brillouin zone center and corner, respectively, all of which exhibit moderate dispersion along $k_z$. However, a third hole-like band ($γ$) is not observed, which is expected around the zone center from band calculations and is common in iron-based superconductors. Since this band has the highest renormalization factor and is known to be the most vulnerable to defects, its absence in our data is likely due to defect scattering --- and yet superconductivity can exist without coherent quasiparticles in the $γ$ band. This may help resolve the current controversy on the superconducting gap structure of FeS. Moreover, by comparing the $β$ bandwidths of various iron chalcogenides, including FeS, FeSe$_{1-x}$S$_x$, FeSe, and FeSe$_{1-x}$ Te$_x$, we find that the $β$ bandwidth of FeS is the broadest. However, the band renormalization factor of FeS is still quite large, when compared with the band calculations, which indicates sizable electron correlations. This explains why the unconventional superconductivity can persist over such a broad range of isovalent substitution in FeSe$_{1-x}$Te$_{x}$ and FeSe$_{1-x}$S$_{x}$.

cond-mat.supr-con↗

arXiv2016

Direct observation of the Dirac nodes lifting in semimetallic perovskite SrIrO3 thin films

Perovskite SrIrO3 has long been proposed as an exotic semimetal induced by the interplay between the spin-orbit coupling and electron correlations. However, its low-lying electronic structure is still lacking. We synthesize high-quality perovskite SrIrO3 (100) films by means of oxide molecular beam epitaxy, and then systemically investigate their low energy electronic structure using in-situ angle-resolved photoemission spectroscopy. We find that the hole-like bands around R and the electron-like bands around U(T) intersect the Fermi level simultaneously, providing the direct evidence of the semimetallic ground state in this compound. Comparing with the density functional theory, we discover that the bandwidth of states near Fermi level is extremely small, and there exists a pronounced mixing between the Jeff = 1/2 and Jeff = 3/2 states. Moreover, our data reveal that the predicted Dirac degeneracy protected by the mirror-symmetry, which was theoretically suggested to be the key to realize the non-trivial topological properties, is actually lifted in perovskite SrIrO3 thin films. Our findings pose strong constraints on the current theoretical models for the 5d iridates.

cond-mat.str-el↗

arXiv2016

Observation of the anisotropic Dirac cone in the band dispersion of 112-structured iron-based superconductor Ca0.9La0.1FeAs2

CaFeAs2 is a parent compound of recently discovered 112-type iron-based superconductors. It is predicted to be a staggered intercalation compound that naturally integrates both quantum spin Hall insulating and superconducting layers and an ideal system for the realization of Majorana modes. We performed a systematical angle-resolved photoemission spectroscopy and first-principle calculation study of the slightly electron-doped CaFeAs2. We found that the zigzag As chain of 112-type iron-based superconductors play a considerable role in the low-energy electronic structure, resulting in the characteristic Dirac-cone like band dispersion as the prediction. Our experimental results further confirm that these Dirac cones only exists around the X but not Y points in the Brillouin zone, breaking the S4 symmetry at iron sites. Our findings present the compelling support to the theoretical prediction that the 112-type iron-based superconductors might host the topological nontrivial edge states. The slightly electron doped CaFeAs2 would provide us a unique opportunity to realize and explore Majorana fermion physics.

cond-mat.supr-con↗

arXiv2016

Bulk and surface electronic structure of trigonal structured PtBi2 studied by angle-resolved photoemission spectroscopy

PtBi2 with a layered trigonal crystal structure was recently reported to exhibit an unconventional large linear magnetoresistance, while the mechanism involved is still elusive. Using high resolution angle-resolved photoemission spectroscopy, we present a systematic study on its bulk and surface electronic structure. Through careful comparison with first-principle calculations, our experiment distinguishes the low-lying bulk bands from entangled surface states, allowing the estimation of the real stoichiometry of samples. We find significant electron doping in PtBi2, implying a substantial Bi deficiency induced disorder therein. We discover a Dirac-cone-like surface state on the boundary of the Brillouin zone, which is identified as an accidental Dirac band without topological protection. Our findings exclude quantum-limit-induced linear band dispersion as the cause of the unconventional large linear magnetoresistance.

cond-mat.str-el↗