arXiv subjects

Qinghai Song

Publications and source records attributed to Qinghai Song.

At least 19 recordsLinked to original sources

arXiv2026

Transition of Photonic Dissipative Dynamics through the Exceptional Point

The decay of light in an optical structure depends not only on the intrinsic properties of the material but also on the surrounding electromagnetic environment. This principle has laid the foundation for the engineering of dissipation in photonic emitters. In the conventional wisdom, dissipation is governed by a fixed set of decay channels, each defined by the eigenstates of the structure, and energy leaks through and interacts with these channels. Here we provide experimental evidence that this paradigm fails in non-Hermitian systems. Specifically, we observe an accelerated transient decay in a pair of coupled microcavities tuned near the exceptional point, revealing that photonic dissipation can be governed not by reconfiguring existing loss channels, but rather by restructuring the underlying state space. The universality of this phenomenon is corroborated through two independent control parameters.The finding provides a new perspective on dissipative dynamics in open optical systems and offers a distinct mechanism for controlling transient decay in ultrafast photonic systems.

physics.optics↗

arXiv2026

Rare Earth Ion Coupling Implements Attention-Like Reservoir Computing

We present a physical computing paradigm that harnesses the intrinsic nonlinear dynamics of rare earth doped core shell nanoparticles as a computational substrate. By directly exploiting cross relaxation and energy transfer upconversion processes, the system realizes a state dependent transfer function whose effective decay rate evolves with the instantaneous Er3+ population, which mathematically analogous to gating and attention mechanisms in recurrent neural networks. The three spectrally resolved emission channels inherently span disparate timescales, endowing the reservoir with native multitimescale feature extraction without auxiliary engineering. Under the reservoir computing framework, the coupled three channel system achieves a total memory capacity exceeding fourfold that of a single ion reservoir; capacity decomposition further reveals that the nonzero cross memory capacity is a direct signature of many body Tm3+@Er3+ coupling. On the Mackey Glass and Santa Fe chaotic benchmarks, the system attains normalized mean squared errors of 1.2x10-3 and 2.1x10-2, respectively, with only 125 virtual nodes. These results establish rare earth nanoparticles as a compelling platform for compact and hardware integrable neuromorphic computing, and introduce "inward evolution", the deliberate exploitation of intra material quantum dynamics, as a generalizable design principle for next generation physical computing systems.

physics.optics↗

arXiv2026

Bound state in the continuum induced room-temperature superfluorescence

Superfluorescence is a collective emission from several quantum emitters that initially have random phases and are then synchronized through vacuum field interactions. Despite its fascinating prospects in quantum information processing, optical computing and advanced photonic devices, a key challenge in harnessing superfluorescence is alleviating its reliance on cryogenic conditions. Recently, room-temperature superfluorescence has been successfully achieved using upconverted nanoparticles and quasi two-dimensional lead halide perovskites. These approaches, however, are restricted to a few specific material designs and unsuitable for wide promotion. Here, we report a universal strategy to elevate the operating temperature of superfluorescence. We reveal that the symmetry-protected optical bound state in the continuum (BIC) can break the size limitation of superfluorescence ({\lambda}^3) and correlate distant but similar emitters without violating the selection rules, significantly accelerating synchronization process and promoting the possibility of room-temperature superfluorescence. This effect has been experimentally verified using a series of BIC metasurfaces made of different lead halide perovskites. Key features such as the quadratic increase in transient peak intensity and the reduction in pulse width and build-up time at the BIC wavelength confirm the realization of room-temperature superfluorescence that is absent in the pristine material. A theoretical model is also built to explain the experimental observations. This research demonstrates that the operating temperatures of coherent macroscopic states can be effectively improved by artificial field, paving a critical step towards constructing building blocks for optical and quantum applications.

physics.optics↗

arXiv2025

Nonlinear chiral light generation from resonant metasurfaces

Chiral nonlinear response has been explored for decades due to its extreme sensitivity to molecular and structural dissymmetry. Conventional approaches often require bulky systems and produce only static nonlinear chirality. Here, we report on a generic mechanism for the generation and control of nonlinear chiral light in resonant optical systems. We reveal that nonlinear resonant generation of circularly polarized light from achiral dielectric metasurfaces is extremely sensitive to the polarization state of the fundamental wave, and a resonant metasurface can produce light with arbitrary degree of nonlinear chirality (DNC). Experimentally, we demonstrate that the chirality of nonlinear radiation from one metasurface can be continuously tuned from DNC = -0.86 to DNC = 0.94 by simply varying the polarization angle of the incident wave. By further exploiting the instantaneous polarization state, nonlinear chirality has been switched in a delay time step of 3.2 fs, which is orders of magnitude more sensitive than the current state-of-the-art polarization modulation. These results promise to enrich our understanding of nonlinear processes in chiral structures and their manipulation with resonant photonic structures.

physics.optics↗

arXiv2025

Deterministic and Scalable Coupling of Single 4H-SiC Spin Defects into Bullseye Cavities

Silicon carbide (SiC) has attracted significant attention as a promising quantum material due to its ability to host long-lived, optically addressable color centers with solid-state photonic interfaces. The CMOS compatibility of 4H-SiCOI (silicon-carbide-on-insulator) makes it an ideal platform for integrated quantum photonic devices and circuits. However, the deterministic integration of single spin defects into high-performance photonic cavities on this platform has remained a key challenge. In this work, we demonstrate the deterministic and scalable coupling of both ensemble (PL4) and single PL6 spin defects into monolithic bullseye cavities on the 4H-SiCOI platform. By tuning the cavity resonance, we achieve a 40-fold enhancement of the zero-phonon line (ZPL) intensity from ensemble PL4 defects, corresponding to a Purcell factor of approximately 5.0. For deterministically coupled single PL6 defects, we observe a threefold increase in the saturated photon count rate, confirm single-photon emission, and demonstrate coherent control of the spin state through optically detected magnetic resonance (ODMR), resonant excitation, and Rabi oscillations. These advancements establish a viable pathway for developing scalable, high-performance SiC-based quantum photonic circuits.

quant-ph↗

arXiv2025

Strain Enhanced Spin Readout Contrast in Silicon Carbide Membranes

Quantum defects in solids have emerged as a transformative platform for advancing quantum technologies. A key requirement for these applications is achieving high-fidelity single-spin readout, particularly at room temperature for quantum biosensing. Here, we demonstrate through ab initio simulations of a primary quantum defect in 4H silicon carbide that strain is an effective control parameter for significantly enhancing readout contrast. We validate this principle experimentally by inducing local strain in silicon carbide-on-insulator membranes, achieving a readout contrast exceeding 60% while preserving the favorable coherence properties of single spins. Our findings establish strain engineering as a powerful and versatile strategy for optimizing coherent spin-photon interfaces in solid-state quantum systems.

quant-ph↗

arXiv2025

Monoclinic nonlinear metasurfaces for resonant engineering of polarization states

Polarization is a fundamental property of light that can be engineered and controlled efficiently with optical metasurfaces. Here, we employ chiral metasurfaces with monoclinic lattice geometry and achiral meta-atoms for resonant engineering of polarization states of light. We demonstrate, both theoretically and experimentally, that a monoclinic metasurface can convert linearly polarized light into elliptically polarized light not only in the linear regime but also in the nonlinear regime with the resonant generation of the third-harmonic field. We reveal that the ellipticity of the fundamental and higher-harmonic fields depends critically on the angle of the input linear polarization, and the effective chiral response of a monoclinic lattice plays a significant role in the polarization conversion.

physics.optics↗

arXiv2024

Tunable cavity coupling to spin defects in 4H-silicon-carbide-on-insulator platform

Silicon carbide (SiC) has attracted significant attention as a promising quantum material due to its ability to host long-lived, optically addressable color centers with solid-state photonic interfaces. The CMOS compatibility of 4H-SiCOI (silicon-carbide-on-insulator) makes it an ideal platform for integrated quantum photonic devices and circuits. While micro-ring cavities have been extensively studied in SiC and other materials, the integration of 4H-SiC spin defects into these critical structures, along with continuous mode tunability, remains unexplored. In this work, we demonstrate the integration of PL4 divacancy spin defects into tunable micro-ring cavities in scalable thin-film 4H-SiC nanophotonics. Comparing on- and off-resonance conditions, we observed an enhancement of the Purcell factor by approximately 5.0. This enhancement effectively confined coherent photons within the coupled waveguide, leading to a twofold increase in the ODMR (optically detected magnetic resonance) contrast and coherent control of PL4 spins. These advancements lay the foundation for developing SiC-based quantum photonic circuits.

quant-ph↗

arXiv2024

Intrinsically chiral exciton polaritons in an atomically-thin semiconductor

Photonic bound states in the continuum (BICs) have emerged as a versatile tool for enhancing light-matter interactions by strongly confining light fields. Chiral BICs are photonic resonances with a high degree of circular polarisation, which hold great promise for spin-selective applications in quantum optics and nanophotonics. Here, we demonstrate a novel application of a chiral BIC for inducing strong coupling between the circularly polarised photons and spin-polarised (valley) excitons (bound electron-hole pairs) in atomically-thin transition metal dichalcogenide crystals (TMDCs). By placing monolayer WS$_2$ onto the BIC-hosting metasurface, we observe the formation of intrinsically chiral, valley-selective exciton polaritons, evidenced by circularly polarised photoluminescence (PL) at two distinct energy levels. The PL intensity and degree of circular polarisation of polaritons exceed those of uncoupled excitons in our structure by an order of magnitude. Our microscopic model shows that this enhancement is due to folding of the Brillouin zone creating a direct emission path for high-momenta polaritonic states far outside the light cone, thereby providing a shortcut to thermalisation (energy relaxation) and suppressing depolarisation. Moreover, while the polarisation of the upper polariton is determined by the valley excitons, the lower polariton behaves like an intrinsic chiral emitter with its polarisation fixed by the BIC. Therefore, the spin alignment of the upper and lower polaritons ($\uparrow\downarrow$ and $\uparrow \uparrow$) can be controlled by $\sigma^+$ and $\sigma^-$ polarised optical excitation, respectively. Our work introduces a new type of chiral light-matter quasi-particles in atomically-thin semiconductors and provides an insight into their energy relaxation dynamics.

cond-mat.mes-hall↗

arXiv2024

Chiral Dichroism in Resonant Metasurfaces with Monoclinic Lattices

We demonstrate that chiral response can be achieved in resonant metasurfaces with a monoclinic lattice symmetry (the so-called Bravais oblique lattices) where the mirror symmetry is broken by the lattice asymmetry and also by a substrate, whereas each individual meta-atom remains fully achiral. We describe the underlying physics by introducing a mode chirality parameter as a quantitative measure of the lattice chiral eigenmodes. We confirm experimentally selective linear and nonlinear chiral interaction of resonant silicon metasurfaces with circularly polarized light.

physics.optics↗

arXiv2024

Even-order optical harmonics generated from centrosymmetric-material metasurfaces

Generation of even-order optical harmonics requires noncentrosymmetric structures being conventionally observed in crystals lacking the center of inversion. In centrosymmetric systems, even-order harmonics may arise, e.g., at surfaces but such effects are usually very weak. Here we observe optical harmonics up to 4-th order generated under the normal incidence from centrosymmetric dielectric metasurfaces empowered by resonances. We design silicon metasurfaces supporting optical quasibound states in the continuum and guided-mode resonances, and demonstrate the enhancement of second-harmonic signals by over three orders of magnitude compared to nonresonant thin films. Under the optimal conditions, the brightness of the second harmonic approaches that of the third harmonic, and the 4th-order harmonic becomes detectable.

physics.optics↗

arXiv2024

Controllable distant interactions at bound state in the continuum

Distant interactions at arbitrary locations and their dynamic control are fundamentally important for realizing large-scale photonic and quantum circuits. Conventional approaches suffer from short coupling distance, poor controllability, fixed locations and low wavelength uniformity, significantly restricting the scalability of photonic and quantum networks. Here, we exploit the intrinsic advantages of optical bound state in the continuum (BIC) and demonstrate an all-in-one solution for dynamically controllable long-range interactions. BIC metasurface can support a series of finite-sized quasi-BIC microlasers at arbitrary locations. The quasi-BICs microlasers have the same wavelength and are inherently connected through BIC waveguide. Consequently, the coupling distances in experiment increase significantly from subwavelength to tens of micrometers. Such long-range interaction in BIC metasurface enables scaling to two-dimensional architectures and ultrafast control of internal laser actions, e.g., non-Hermitian zero-mode lasing and enhanced optical gain. This research shall facilitate the advancement of scalable and reconfigurable photonic networks.

physics.optics↗

arXiv2024

Chirality tuning and reversing with resonant phase-change metasurfaces

Dynamic control of circular dichroism in photonic structures is critically important for compact spectrometers, stereoscopic displays, and information processing exploiting multiple degrees of freedom. Metasurfaces can help miniaturize chiral devices but only produce static and limited chiral responses. While external stimuli are able to tune resonances, their modulations are often weak, and reversing continuously the sign of circular dichroism is extremely challenging. Here, we demonstrate dynamically tunable chiral response of resonant metasurfaces supporting chiral bound states in the continuum combining them with phase-change materials. Phase transition between amorphous and crystalline phases allows to control chiral response and vary chirality rapidly from -0.947 to +0.958 backward and forward via chirality continuum. Our demonstrations underpin the rapid development of chiral photonics and its applications.

physics.optics↗

arXiv2023

Room-Temperature entangled quantum processor on integrated semiconductor photonics platform

The rise of the 4H-silicon-carbide-on-insulator (SiCOI) platform marks a promising pathway towards the realization of monolithic quantum photonic networks. However, the challenge of establishing room-temperature entangled registers on these integrated photonics platforms remains unresolved. Herein, we demonstrate the first entangled processor on the SiCOI platform. We show that both deterministic generation of single divacancy electron spins and near-unity spin initialization of a single $^{13}$C nuclear spin can be achieved on SiCOI at room temperature. Besides coherently manipulating the single nuclear spin, a maximally entangled state with a fidelity of 0.89 has been prepared on this CMOS-compatible semiconductor-integrated photonics system. This work establishes the foundation for compact and on-chip solutions within existing defect-based computing and sensing protocols, positioning the SiCOI platform as the most promising candidate for integrated monolithic quantum photonic networks.

quant-ph↗

arXiv2022

Giant superchiral field at merged bound states in the continuum

Superchiral field is highly important for ultrasensitive detection of chiral objects and has been intensively explored. Despite the progress, the construction of electromagnetic field in achiral nanostructures with giant chirality (C) is fundamentally restricted. Here, we demonstrate a novel approach to construct superchiral field in achiral dielectric metasurfaces. Due to the quantum spin-hall effect, each symmetry-protected bound state in the continuum (BIC) exhibits the ability to support a superchiral field in vicinity of \Gamma point. By merging two BICs with orthogonal polarizations, all the criteria for a superchiral field are satisfied and the dramatic enhancement of chirality becomes more robust. Using typical photonic crystal slabs, we have produced a superchiral field with enhancement factor (C/C_CPL) orders of magnitude higher than state-of-the-art in nanostructures. By further introducing active chiral medium, a chiral mode splitting associated with giant enhancement of circular dichroism (CD) has been formed by the chiral light-matter interaction.

physics.optics↗

arXiv2020

Suppressing meta-holographic artifacts by laser coherence tuning

A metasurface hologram combines fine spatial resolution and large viewing angles with a planar form factor and compact size. However, it suffers coherent artifacts originating from electromagnetic cross-talk between closely packed meta-atoms and fabrication defects of nanoscale features. Here, we introduce an efficient method to remove all artifacts by fine-tuning the spatial coherence of illumination. Our method is implemented with a degenerate cavity laser, which allows precise, continuous tuning of spatial coherence over a wide range with little variation in emission spectrum and total power. We find the optimal degree of spatial coherence to remove the coherent artifacts of a meta-hologram while maintaining the image sharpness. This work paves the way to compact and dynamical holographic display free of coherent defects.

physics.optics↗

arXiv2019

Enhancing the Three-Photon Luminesce via the Resonance in Lead Halide Perovskite Metasurfaces

Lead halide perovskites (MAPbX3) have emerged as promising materials for photovoltaic and optoelectronic devices. However, their exceptional nonlinear properties have not been fully exploited in nanophotonics yet. Herein we fabricate MAPbX3 perovskite metasurfaces and explore their internal nonlinear processes. While both of third-order harmonic generation (THG) and three-photon luminescence are generated, the latter one is less affected by the material loss and has been significantly enhanced by a factor of 60. The corresponding simulation reveals that the improvement is caused by the resonant enhancement of incident laser in perovskite metasurface. Interestingly, such kind of resonance-enhanced three-photon luminescence holds true for metasurfaces with a small period number of 4, enabling new applications of perovskite metasurface in high-resolution nonlinear color nanoprinting and optical encoding. The encoded information "NANO" is visible only when the incident laser is on-resonance. The off-resonance pumping and the single-photon excitation just produce a uniform dark or photoluminescence background.

physics.app-ph↗

arXiv2019

Lead Halide Perovskite based Dynamic Metasurfaces

Lead halide perovskites (MAPbX3) are known to have high refractive index and controllable bandgap, making them attractive for all-dielectric and tunable metasurfaces. Till now, perovskite metasurfaces have only been used in structural colors. More interesting meta-devices with 2π phase control are still absent. Here we experimentally demonstrate the MAPbX3 perovskite based metasurfaces with a complete control of phase shift in a reflection mode. By utilizing MAPbBr3 cut-wires as meta-atoms on a ground metal film, we find that the MAPbBr3 perovskite metasurface can produce full phase control from 0 to 2π and high reflection efficiency simultaneously. Consequently, high-efficiency polarization conversion, anomalous reflection and meta-hologram have been successfully produced. Most interestingly, the bandgap of MAPbX3 perovskite can be post-synthetically and reversibly tuned via anion exchange, providing a new approach to dynamically control of the all-dielectric meta-devices with novel function such as anomalous reflection and hologram et al.

physics.app-ph↗