arXiv subjects

Quynh Le-Van

Publications and source records attributed to Quynh Le-Van.

8 recordsLinked to original sources

arXiv2026

Nanoscale Fluorescence Thermometry: Probes, Recent Advances and Emerging Directions

The transition of materials and devices to nanometer, atomic, and quantum scales makes thermal characterization increasingly challenging, driving the need for advanced nanoscale thermometry. Fluorescence nanothermometry has emerged as a powerful approach, enabling remote, spatially resolved temperature measurements with sub-micrometer-to-nanometer precision across applications in nanoelectronics, microfluidics, and biological systems. In these systems, temperature is inferred from variations in fluorescence observables, including spectral position, intensity, linewidth, and excited-state dynamics. This review provides a comprehensive and critical overview of fluorescence nanothermometry, covering fundamental mechanisms, material platforms, recent advances, and emerging applications. It further presents a critical evaluation of key challenges and discusses emerging strategies and future research directions toward achieving robust, real-time thermometry. It is anticipated that this review will stimulate further advances in material platforms and system design, accelerating the development of accurate, scalable, and application-ready nanoscale thermometers.

physics.optics↗

arXiv2025

Generalized Non-Hermitian Hamiltonian for Guided Resonances in Photonic Crystal Slabs

We develop a generalized non-Hermitian Hamiltonian formalism for guided resonances in photonic crystal slabs, derived directly from Maxwell's equations through a systematic guided-mode expansion. By expanding the electromagnetic fields over the complete mode basis of an unpatterned slab and systematically integrating out radiative Fabry--Pérot channels, we obtain the analytical operator structure of the Hamiltonian, which treats guided-mode coupling and radiation losses on equal footing. The resulting Hamiltonian provides explicit expressions for both dispersive and radiative coupling terms in terms of modal overlap integrals and Fourier components of the permittivity modulation. For specific geometries, the Hamiltonian coefficients can be extracted from full-wave simulations enabling accurate modeling without phenomenological assumptions. As a case study, we investigate hexagonal lattices with both preserved and broken $C_6$ symmetry, demonstrating predictive agreement for complex band structures, near-field distributions, and far-field polarization patterns. In particular, the formalism reproduces symmetry-protected bound states in the continuum (BICs) at the $Γ$ point, accidental off-$Γ$ BICs near the $Γ$ point, and the emergence of chiral exceptional points (EPs). It also captures the tunable behavior of eigenmodes near the $K$ point, including Dirac-point shifts and the emergence of quasi-BICs or bandgap openings, depending on the nature of $C_6$ symmetry breaking. We further demonstrate in the Appendix that the same formalism extends naturally to other symmetry classes, including $C_2$ (1D grating) and $C_4$ (square lattice) photonic crystal slabs. This approach enables predictive and efficient modeling of complex photonic resonances, revealing their topological and symmetry-protected characteristics in non-Hermitian systems.

physics.optics↗

arXiv2024

Micrometer-resolution fluorescence and lifetime mappings of CsPbBr$_3$ nanocrystal films coupled with a TiO$_2$ grating

Enhancing light emission from perovskite nanocrystal (NC) films is essential in light-emitting devices, as their conventional stacks often restrict the escape of emitted light. This work addresses this challenge by employing a TiO$_2$ grating to enhance light extraction and shape the emission of CsPbBr$_3$ nanocrystal films. Angle-resolved photoluminescence (PL) demonstrated a tenfold increase in emission intensity by coupling the Bloch resonances of the grating with the spontaneous emission of the perovskite NCs. Fluorescence lifetime imaging microscopy (FLIM) provided micrometer-resolution mapping of both PL intensity and lifetime across a large area, revealing a decrease in PL lifetime from 8.2 ns for NC films on glass to 6.1 ns on the TiO$_2$ grating. Back focal plane (BFP) spectroscopy confirmed how the Bloch resonances transformed the unpolarized, spatially incoherent emission of NCs into polarized and directed light. These findings provide further insights into the interactions between dielectric nanostructures and perovskite NC films, offering possible pathways for designing better performing perovskite optoelectronic devices.

physics.optics↗

arXiv2023

Direct Observation of Exceptional Points in Photonic Crystal by Cross-Polarization Imaging in Momentum Space

This study explores exceptional points (EPs) in photonic crystals (PhCs) and introduces a novel method for their single-shot observation. Exceptional points are spectral singularities found in non-Hermitian systems, such as leaky PhC slabs. However, directly observing EPs in PhC systems using regular reflectivity spectroscopy is a considerable challenge due to interference between guided resonances and background signals. In this work, we present a simple, nondestructive technique that employs crossed polarizations to directly observe EPs in momentum-resolved resonant scattering. This approach effectively suppresses the background signal, enabling exclusive probing of the guided resonances where EPs manifest. Our results demonstrate the formation of EPs in both energy-momentum mapping and isofrequency imaging. All experimental findings align seamlessly with numerical simulations and analytical models. Our approach holds great potential as a robust tool for studying non-Hermitian physics in PhC platform.

physics.optics↗

arXiv2022

Coexistence of Surface Lattice Resonances and Bound states In the Continuum in a Plasmonic Lattice

We present a numerical study on a 2D array of plasmonic structures covered by a subwavelength film. We explain the origin of surface lattice resonances (SLRs) using coupled dipole approximation and show that the diffraction-assisted plasmonic resonances and formation of bound states in the continuum (BICs) can be controlled by altering the optical environment. Our study shows that when the refractive index contrast is small ( $Δ$n < -0.1), the SLR cannot be excited, while a significant contrast ($Δ$n > 0.3) not only sustains plasmonic-induced resonances but also forms both symmetry-protected and accidental BICs. The results can aid the streamlined design of plasmonic lattices in studies on light-matter interaction and applications in biosensors and optoelectronic devices.

physics.optics↗

arXiv2019

Enhanced Delayed Fluorescence in Tetracene Crystals by Strong Light-Matter Coupling

We demonstrate experimentally an enhanced delayed fluorescence in tetracene single crystals strongly coupled to optical modes in open cavities formed by arrays of plasmonic nanoparticles. Hybridization of singlet excitons with collective plasmonic resonances in the arrays leads to the splitting of the material dispersion into a lower and an upper polariton band. This splitting significantly modifies the dynamics of the photo-excited tetracene crystal, resulting in an increase of the delayed fluorescence by a factor of four. The enhanced delayed fluorescence is attributed to the emergence of an additional radiative decay channel, where the lower polariton band harvests long-lived triplet states. There is also an increase in total emission, which is wavelength dependent, and can be explained by the direct emission from the lower polariton band, the more effcient light out-coupling and the enhancement of the excitation intensity. The observed enhanced fluorescence opens the possibility of effcient radiative triplet harvesting in open optical cavities, to improve the performance of organic light emitting diodes.

cond-mat.mes-hall↗

arXiv2019

Unified Weak-to-Strong Coupling Transitions and Radiation Interference Induced by Vertical-Symmetry Breaking in Photonic Crystal Slabs

Vertical-symmetry breaking provides a versatile means of coupling leaky photonic-crystal resonances that are otherwise protected by opposite out-of-plane parity. Here, we develop a unified two-mode framework for the weak-to-strong coupling transition induced by vertical-symmetry breaking in photonic crystal slabs. The symmetry-breaking perturbation simultaneously generates a near-field coherent coupling and modifies the overlap of the radiation channels of the two parent resonances. Their interplay drives the transition from frequency crossings to avoided crossings through an exceptional point (EP), while also governing radiative linewidth exchange through Friedrich-Wintgen interference. Using a radiation-vector description resolved into the upper and lower half-spaces, we show that total radiation cancellation and one-sided radiation cancellation correspond, respectively, to quasi-bound states in the continuum (quasi-BIC) and quasi-unidirectional guided resonances (quasi-UGR). This framework distinguishes the spectral condition for EP formation from the far-field conditions controlling linewidth suppression and directional emission. We validate this picture numerically and experimentally in square-lattice photonic crystal slabs. Tuning the superstrate index drives a weak-to-strong coupling transition through an EP, while partial etching yields a broad off-$\Gamma$ quasi-BIC regime with strongly asymmetric top and bottom radiation. We further apply the same radiation-vector framework to a laterally shifted bilayer grating, where quasi-BICs and quasi-UGR emerge along a continuous symmetry-breaking pathway. These results establish vertical-symmetry breaking as a general route for controlling hybridization, radiation interference, and directional leakage in photonic crystal slabs.

physics.optics↗

arXiv2018

Screened Strong Coupling of Excitons in Multilayer WS2 with Collective Plasmonic Resonances

We demonstrate the strong coupling of direct transition excitons in tungsten disulfide (WS2) with collective plasmonic resonances at room temperature. We use open plasmonic cavities formed by periodic arrays of metallic nanoparticles. We show clear anti-crossings with monolayer, bilayer and thicker multilayer WS2 on top of the nanoparticle array. The Rabi energy of such hybrid system varies from 50 to 110 meV from monolayer to sixteen layers, while it does not scale with the square root of the number of layers as expected for collective strong coupling. We prove that out-of-plane coupling components can be disregarded since the normal field is screened due to the high refractive index contrast of the dielectric layers. Even though the in-plane dipole moments of the excitons decrease beyond monolayers, the strong in-plane field distributed in the flake can still enhance the coupling strength with multilayers. However, the screened out-of-plane field leads to the saturation of the Rabi energy. The achieved coherent coupling of TMD multilayers with open cavities could be exploited for manipulating the dynamics and transport of excitons in 2D semiconductors and developing ultrafast valley/spintronic devices.

cond-mat.mtrl-sci↗