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R. Brandt

Publications and source records attributed to R. Brandt.

14 recordsLinked to original sources
arXiv2022

X-ray diffraction with micrometer spatial resolution for highly absorbing samples

X-ray diffraction with high spatial resolution is commonly used to characterize (poly-)crystalline samples with, for example, respect to local strain, residual stress, grain boundaries and texture. However, the investigation of highly absorbing samples or the simultaneous assessment of high-Z materials by X-ray fluorescence have been limited due to the utilisation of low photon energies. Here, we report on a goniometer-based setup implemented at the P06 beamline of PETRA III that allows for micrometer spatial resolution with a photon energy of 35 keV and above. A highly focused beam was achieved by using compound refractive lenses and high precision sample manipulation was enabled by a goniometer that allows for up to 5D scans (3 rotations & 2 translations). As experimental examples, we demonstrate the determination of local strain variations in martensitic steel samples with micrometer spatial resolution as well as the simultaneous elemental distribution for high-Z materials in a thin film solar cell. Our proposed approach allows users from the materials science community to determine micro-structural properties even in highly absorbing samples.

cond-mat.mtrl-sci↗
arXiv2013

Size-dependent magnetization switching characteristics and spin wave modes of FePt nanostructures

We present a comprehensive investigation of the size-dependent switching characteristics and spin wave modes of FePt nanoelements. Curved nanomagnets ("caps") are compared to flat disks of identical diameter and volume over a size range of 100 to 300nm. Quasi-static magnetization reversal analysis using first-order reversal curves (FORC) shows that spherical caps have lower vortex nucleation and annihilation fields than the flat disks. As the element diameter decreases, the reversal mechanism in the caps crosses over sooner to coherent rotation than in the disks. The magnetization dynamics are studied using optically induced small angle precession and reveal a strong size dependence that differs for the two shapes. Flat disks exhibit well-known center and edge modes at all sizes, but as the diameter of the caps increases from 100 to 300 nm, additional oscillation modes appear in agreement with dynamic micromagnetic simulations. In addition, we show that the three-dimensional curvature of the cap causes a much greater sensitivity to the applied field angle which provides an additional way for controlling the ultrafast response of nanomagnetic elements.

cond-mat.mtrl-sci↗
arXiv2011

ICP-SFMS search for long-lived naturally-occurring heavy, superheavy and superactinide nuclei compared to AMS experiments

Negative results obtained in AMS searches by Dellinger et al. on mostly unrefined ores have led them to conclude that the very heavy long-lived species found in chemically processed samples with ICP-SFMS by Marinov et al. are artifacts. We argue that it may not be surprising that results obtained from small random samplings of inhomogeneous natural minerals would contrast with concentrations found in homogeneous materials extracted from large quantities of ore. We also point out that it is possible that the groups of counts at masses 296 and 294 seen by Dellinger et al. could be, within experimental uncertainties, due to $^{296}$Rg and $^{294}$eka-Bi in long-lived isomeric states. In such case, the experiments of Dellinger et al. lend support to the experiments of Marinov et al.

nucl-ex↗
arXiv2010

Enrichment of the Superheavy Element Rg in Natural Au

Based on the observation of the long-lived isotopes 261Rg and 265Rg (Z = 111, t(1/2) >= 10^(8) y) in natural Au, an experiment was performed to enrich Rg in 99.999% Au. 16 mg of Au were heated in vacuum for two weeks at a temperature of 1127 deg. C (63 deg. C above the melting point of Au). The content of 197Au and 261Rg in the residue was studied with high resolution inductively coupled plasma-sector field mass spectrometry (ICP-SFMS). The residue of Au was 3x10^(-6) of its original quantity. The recovery of Rg was a few percent. The abundance of Rg compared to Au in the enriched solution was about 2x10^(-6), which is a three to four orders of magnitude enrichment. It is concluded that the evaporation rate of Rg from an Au matrix in vacuum at 63 deg. C above the Au melting point is lower than that of Au. This experiment reinforces our first observation of Rg in a terrestrial material. As before it is concluded that a long-lived isomeric state exists in 261Rg and that it probably belongs to a new class of isomeric states, namely high spin super- or hyperdeformed isomeric states.

nucl-ex↗
arXiv2008

Evidence for a long-lived superheavy nucleus with atomic mass number A=292 and atomic number Z=~122 in natural Th

Evidence for the existence of a superheavy nucleus with atomic mass number A=292 and abundance (1-10)x10^(-12) relative to 232Th has been found in a study of natural Th using inductively coupled plasma-sector field mass spectrometry. The measured mass matches the predictions [1,2] for the mass of an isotope with atomic number Z=122 or a nearby element. Its estimated half-life of t1/2 >= 10^8 y suggests that a long-lived isomeric state exists in this isotope. The possibility that it might belong to a new class of long-lived high spin super- and hyperdeformed isomeric states is discussed.[3-6]

nucl-ex↗
arXiv2007

Existence of long-lived isotopes of a superheavy element in natural Au

Evidence for the existence of long-lived isotopes with atomic mass numbers 261 and 265 and abundance of (1-10)x10$^{-10}$ relative to Au has been found in a study of natural Au using an inductively coupled plasma - sector field mass spectrometer. The measured masses fit the predictions made for the masses of $^{261}$Rg and $^{265}$Rg (Z=111) and for some isotopes of nearby elements. The possibility that these isotopes belong to the recently discovered class of long-lived high spin super- and hyperdeformed isomeric states is discussed.

nucl-ex↗
arXiv2004

Comments on the question of the discovery of element 112 as early as 1971

There are two independent claims for the discovery of element 112: The claim by Hofmann et al. from 1996 and the older claim from 1971 by Marinov et al. This Comment will not challenge the experimental results of Hofmann et al., but it will discuss one aspect of the claimed discovery of element 112 by Marinov et al., as their experiment has never been reproduced in exactly the form in which the original experiment has been carried out. The reasons for this deficiency may not be found in the field of science, but possibly in radioprotection restrictions for researchers who want to carry out such an experiment. However, such is not a sufficient reason to exclude the original claim from all considerations of the responsible international authorities, who have to settle such priority questions. It may be in agreement with scientific traditions, that when the responsible international committees do not feel to be able to come to a positive decision on the "1971" claim, they could keep the priority problem unsettled for the time being.

nucl-ex↗
arXiv2004

The Chemical Separation of Eka-Hg from CERN W Targets in view of Recent Relativistic Calculations

In 1971 evidence for the production of element 112 via secondary reactions in CERN W targets was obtained. The evidence was mainly based on the observation of fission fragments in Hg sources separated from the W targets, on the measured masses of the fissioning nuclei and on the assumption that element 112 (Eka-Hg) actually behaves like Hg in the chemical separation process. This assumption is analyzed in view of recent relativistic calculations of the electronic structure of element 112. It is shown that in the superheavy element region only the chemistry of element 112 is similar to that of Hg.

nucl-ex↗
arXiv2004

Analysis of the JINR p(660 MeV) + 129I, 237Np, and 241Am Measurements with Eleven Different Models

We have analyzed the recent JINR measurements on nuclide production cross sections from interaction of 660 MeV proton beams with radioactive targets of enriched 129I (85% 129I and 15% 127I), 237Np, and 241Am with eleven different models, realized in eight transport codes and event-generators: LAHET (Bertini, ISABEL, INCL+ABLA, and INCL+RAL options), CASCADE, CEM95, CEM2k, LAQGSM+GEM2, CEM2k+GEM2, LAQGSM+GEMINI, and CEM2k+GEMINI. We found out that all these models have problems in a correct description of many of these cross sections, though some of these models describe very well most of the recent measurements done at GSI using inverse kinematics, as well as many other reactions. None of the tested here models is able to reproduce well all the JINR data and all of them should be further improved. Development of a better universal evaporation/fission model should be of a highest priority. We conclude that it is impossible to make a correct choice between fission and fragmentation reaction mechanisms analyzing only measurements on product cross sections; addressing this question would require analysis of two- or multi-particle correlation measurements.

nucl-th↗
arXiv2004

Super- and Hyperdeformed Isomeric States and Long-Lived Superheavy Elements

The recent discoveries of the long-lived high spin super- and hyperdeformed isomeric states and their unusual radioactive decay properties are described. Based on their existence a consistent interpretation is given to the production of the long-lived superheavy element with Z = 112, via secondary reactions in CERN W targets, and to the low energy and very enhanced alpha-particle groups seen in various actinide fractions separated from the same W target. In addition, consistent interpretations are suggested for previously unexplained phenomena seen in nature. These are the Po halos, the low-energy enhanced 4.5 MeV alpha-particle group proposed to be due to an isotope of a superheavy element with Z = 108, and the giant halos.

nucl-ex↗
arXiv2004

Study of Proton Induced Reactions in a Radioactive 129-I Target at Ep=660 MeV

Two NaI (85% 129-I and 15% 127-I) targets were exposed to a beam of 660-MeV protons. Cross sections for formation of 76 residual nuclei were obtained by the induced activity method. The results are compared with other experimental data on 127-I and theoretical calculations by eleven models contained in the codes LAHET3 (using the Bertini+Dresner, ISABEL+Dresner, INCL+Dresner, and INCL+ABLA options), CASCADE, CEM95, CEM2K, LAQGSM+GEM2, CEM2k+GEM2, LAQGSM+GEMINI, and CEM2k+GEMINI. Most of the models describe spallation products with masses close to the target reasonably well while the reliability of the codes differs greatly in the deep spallation and fission/fragmentation regions. The difficulties in describing products with A=40-80 by all of the codes tested here except for CEM2k+GEMINI and LAQGSM+GEMINI is related to the neglect of fission (and fragmentation) processes for targets as light as 129-I.

nucl-ex↗
arXiv2003

Coherent Description for Hitherto Unexplained Radioactivities by Super- and Hyperdeformed Isomeric States

Recently long-lived high spin super- and hyperdeformed isomeric states with unusual radioactive decay properties have been discovered. Based on these newly observed modes of radioactive decay, consistent interpretations are suggested for previously unexplained phenomena seen in nature. These are the Po halos, the low-energy enhanced 4.5 MeV alpha-particle group proposed to be due to an isotope of a superheavy element with Z = 108, and the giant halos.

nucl-th↗
arXiv2002

New Outlook on the Possible Existence of Superheavy Elements in Nature

A consistent interpretation is given to some previously unexplained phenomena seen in nature in terms of the recently discovered long-lived high spin super- and hyper-deformed isomeric states. The Po halos seen in mica are interpreted as due to the existence of such isomeric states in corresponding Po or nearby nuclei which eventually decay by gamma- or beta-decay to the ground states of 210Po, 214Po and 218Po nuclei. The low-energy 4.5 MeV alpha-particle group observed in several minerals is interpreted as due to a very enhanced alpha transition from the third minimum of the potential-energy surface in a superheavy nucleus with atomic number Z=108 (Hs) and atomic mass number around 271 to the corresponding minimum in the daughter.

nucl-ex↗