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R. Gross

Publications and source records attributed to R. Gross.

At least 73 records · Page 4Linked to original sources

Giant magnetic anisotropy changes in Sr2CrReO6 thin films on BaTiO3

The integration of ferromagnetic and ferroelectric materials into hybrid heterostructures yields multifunctional systems with improved or novel functionality. We here report on the structural, electronic and magnetic properties of the ferromagnetic double perovskite Sr2CrReO6, grown as epitaxial thin film onto ferroelectric BaTiO3. As a function of temperature, the crystal-structure of BaTiO3 undergoes phase transitions, which induce qualitative changes in the magnetic anisotropy of the ferromagnet. We observe abrupt changes in the coercive field of up to 1.2T along with resistance changes of up to 6.5%. These results are attributed to the high sensitivity of the double perovskites to mechanical deformation.

cond-mat.mtrl-sci↗

Mesoscopic Shelving Readout of Superconducting Qubits in Circuit QED

We present a method for measuring the internal state of a superconducting qubit inside an on-chip microwave resonator. We show that one qubit state can be associated with the generation of an increasingly large cavity coherent field, while the other remains associated with the vacuum. By measuring the outgoing resonator field with conventional devices, an efficient single-shot QND-like qubit readout can be achieved, enabling a high-fidelity measurement in the spirit of the electron-shelving technique for trapped ions. We expect that the proposed ideas can be adapted to different superconducting qubit designs and contribute to the further improvement of qubit readout fidelity.

cond-mat.mes-hall↗

Epitaxial growth and magnetic properties of Sr2CrReO6 thin films

The double perovskite Sr2CrReO6 is an interesting material for spintronics, showing ferrimagnetism up to 635 K with a predicted high spin polarization of about 86%. We fabricated Sr2CrReO6 epitaxial films by pulsed laser deposition on (001)-oriented SrTiO3 substrates. Phase-pure films with optimum crystallographic and magnetic properties were obtained by growing at a substrate temperature of 700 degree C in pure O2 of 6.6x10-4 mbar. The films are c-axis oriented, coherently strained, and show less than 20% anti-site defects. The magnetization curves reveal high saturation magnetization of 0.8 muB per formula unit and high coercivity of 1.1 T, as well as a strong magnetic anisotropy.

cond-mat.mtrl-sci↗

Fabrication Technology of and Symmetry Breaking in Superconducting Quantum Circuits

Superconducting quantum circuits are promising systems for experiments testing fundamental quantum mechanics on a macroscopic scale and for applications in quantum information processing. We report on the fabrication and characterization of superconducting flux qubits, readout dc SQUIDs, on-chip shunting capacitors, and high-quality coplanar waveguide resonators. Furthermore, we discuss the tunability and fundamental symmetry aspects inherent to all superconducting qubits, which can be regarded as artificial solid-state atoms. Comparing them to their natural counterparts, we discuss first and second-order energy shifts due to static control fields. Additionally, we present an intuitive derivation of the first- and second-order matrix elements for level transitions in the presence of a coherent microwave driving.

cond-mat.supr-con↗

Voltage controlled inversion of magnetic anisotropy in a ferromagnetic thin film at room temperature

The control of magnetic properties by means of an electric field is an important aspect in magnetism and magnetoelectronics. We here utilize magnetoelastic coupling in ferromagnetic/piezoelectric hybrids to realize a voltage control of magnetization orientation at room temperature. The samples consist of polycrystalline nickel thin films evaporated onto piezoelectric actuators. The magnetic properties of these multifunctional hybrids are investigated at room temperature as a function of the voltage controlled stress exerted by the actuator on the Ni film. Ferromagnetic resonance spectroscopy shows that the magnetic easy axis in the Ni film plane is rotated by 90 degree upon changing the polarity of the voltage Vp applied to the actuator. In other words, the in-plane uniaxial magnetic anisotropy of the Ni film can be inverted via the application of an appropriate voltage Vp. Using SQUID magnetometry, the evolution of the magnetization vector is recorded as a function of Vp and of the external magnetic field. Changing Vp allows to reversibly adjust the magnetization orientation in the Ni film plane within a range of approximately 70 degree. All magnetometry data can be quantitatively understood in terms of the magnetic free energy determined from the ferromagnetic resonance experiments. These results demonstrate that magnetoelastic coupling in hybrid structures indeed is a viable option to control magnetization orientation in technologically relevant ferromagnetic thin films at room temperature.

cond-mat.mtrl-sci↗

Two-resonator circuit QED: A superconducting quantum switch

We introduce a systematic formalism for two-resonator circuit QED, where two on-chip microwave resonators are simultaneously coupled to one superconducting qubit. Within this framework, we demonstrate that the qubit can function as a quantum switch between the two resonators, which are assumed to be originally independent. In this three-circuit network, the qubit mediates a geometric second-order circuit interaction between the otherwise decoupled resonators. In the dispersive regime, it also gives rise to a dynamic second-order perturbative interaction. The geometric and dynamic coupling strengths can be tuned to be equal, thus permitting to switch on and off the interaction between the two resonators via a qubit population inversion or a shifting of the qubit operation point. We also show that our quantum switch represents a flexible architecture for the manipulation and generation of nonclassical microwave field states as well as the creation of controlled multipartite entanglement in circuit QED. In addition, we clarify the role played by the geometric interaction, which constitutes a fundamental property characteristic of superconducting quantum circuits without counterpart in quantum-optical systems. We develop a detailed theory of the geometric second-order coupling by means of circuit transformations for superconducting charge and flux qubits. Furthermore, we show the robustness of the quantum switch operation with respect to decoherence mechanisms. Finally, we propose a realistic design for a two-resonator circuit QED setup based on a flux qubit and estimate all the related parameters. In this manner, we show that this setup can be used to implement a superconducting quantum switch with available technology.

cond-mat.mes-hall↗

Phase-Coherent Dynamics of a Superconducting Flux Qubit with Capacitive-Bias Readout

We present a systematic study of the phase-coherent dynamics of a superconducting three-Josephson-junction flux qubit. The qubit state is detected with the integrated-pulse method, which is a variant of the pulsed switching DC SQUID method. In this scheme the DC SQUID bias current pulse is applied via a capacitor instead of a resistor, giving rise to a narrow band-pass instead of a pure low-pass filter configuration of the electromagnetic environment. Measuring one and the same qubit with both setups allows a direct comparison. With the capacitive method about four times faster switching pulses and an increased visibility are achieved. Furthermore, the deliberate engineering of the electromagnetic environment, which minimizes the noise due to the bias circuit, is facilitated. Right at the degeneracy point the qubit coherence is limited by energy relaxation. We find two main noise contributions. White noise is limiting the energy relaxation and contributing to the dephasing far from the degeneracy point. 1/f-noise is the dominant source of dephasing in the direct vicinity of the optimal point. The influence of 1/f-noise is also supported by non-random beatings in the Ramsey and spin echo decay traces. Numeric simulations of a coupled qubit-oscillator system indicate that these beatings are due to the resonant interaction of the qubit with at least one point-like fluctuator, coupled especially strongly to the qubit.

cond-mat.supr-con↗

All Oxide Ferromagnet/Semiconductor Epitaxial Heterostructures

Oxide based ferromagnet/semiconductor heterostructures offer substantial advantages for spin electronics. We have grown (111) oriented Fe3O4 thin films and Fe3O4/ZnO heterostructures on ZnO(0001) and Al2O3(0001) substrates by pulsed laser deposition. High quality crystalline films with mosaic spread as small as 0.03 degree, sharp interfaces, and rms surface roughness of 0.3 nm were achieved. Magnetization measurements show clear ferromagnetic behavior of the magnetite layers with a saturation magnetization of 3.2 muB/f.u. at 300 K. Our results demonstrate that the Fe3O4/ZnO system is an intriguing and promising candidate for the realization of multi-functional heterostructures.

cond-mat.mtrl-sci↗

Two-photon probe of the Jaynes-Cummings model and symmetry breaking in circuit QED

Superconducting qubits behave as artificial two-level atoms and are used to investigate fundamental quantum phenomena. In this context, the study of multi-photon excitations occupies a central role. Moreover, coupling superconducting qubits to on-chip microwave resonators has given rise to the field of circuit QED. In contrast to quantum-optical cavity QED, circuit QED offers the tunability inherent to solid-state circuits. In this work, we report on the observation of key signatures of a two-photon driven Jaynes-Cummings model, which unveils the upconversion dynamics of a superconducting flux qubit coupled to an on-chip resonator. Our experiment and theoretical analysis show clear evidence for the coexistence of one- and two-photon driven level anticrossings of the qubit-resonator system. This results from the symmetry breaking of the system Hamiltonian, when parity becomes a not well-defined property. Our study provides deep insight into the interplay of multiphoton processes and symmetries in a qubit-resonator system.

cond-mat.supr-con↗

Piezo-control of magnetic anisotropy in GaMnAs: Reversible manipulation of magnetization orientation and irreversible magnetization switching

We have investigated the magnetic properties of a piezoelectric actuator/ferromagnetic semiconductor hybrid structure. Using a GaMnAs epilayer as the ferromagnetic semiconductor and applying the piezo-stress along its [110] direction, we quantify the magnetic anisotropy as a function of the voltage V_p applied to the piezoelectric actuator using anisotropic magnetoresistance techniques. We find that the easy axis of the strain-induced uniaxial magnetic anisotropy contribution can be inverted from the [110] to the [1-10] direction via the application of appropriate voltages V_p. At T=5K the magnetoelastic term is a minor contribution to the magnetic anisotropy. Nevertheless, we show that the switching fields of rho(H) loops are shifted as a function of V_p at this temperature. At 50K - where the magnetoelastic term dominates the magnetic anisotropy - we are able to tune the magnetization orientation by about 70 degree solely by means of the electrical voltage V_p applied. Furthermore, we derive the magnetostrictive constant lambda_111 as a function of temperature and find values consistent with earlier results. We argue that the piezo-voltage control of magnetization orientation is directly transferable to other ferromagnetic/piezoelectric hybrid structures, paving the way to innovative multifunctional device concepts. As an example, we demonstrate piezo-voltage induced irreversible magnetization switching at T=40K, which constitutes the basic principle of a nonvolatile memory element.

cond-mat.mtrl-sci↗

Andreev bound states at a cuprate grain boundary junction: A lower bound for the upper critical field

We investigate in-plane quasiparticle tunneling across thin film grain boundary junctions (GBJs) of the electron-doped cuprate La$_{2-x}$Ce$_{x}$CuO$_4$ in magnetic fields up to $B=16 $T, perpendicular to the CuO$_2$ layers. The differential conductance in the superconducting state shows a zero bias conductance peak (ZBCP) due to zero energy surface Andreev bound states. With increasing temperature $T$, the ZBCP vanishes at the critical temperature $T_c\approx29 $K if B=0, and at $T=12 $K for B=16 T. As the ZBCP is related to the macroscopic phase coherence of the superconducting state, we argue that the disappearance of the ZBCP at a field $B_{ZBCP}(T)$ must occur below the upper critical field $B_{c2}(T)$ of the superconductor. We find $B_{ZBCP}(0) \approx 25 $T which is at least a factor of 2.5 higher than previous estimates of $B_{c2}(0)$.

cond-mat.supr-con↗

Orthogonally-Driven Superconducting Qubit in Circuit QED

We consider a superconducting charge qubit coupled to distinct orthogonal electromagnetic field modes belonging to a coplanar wave guide and a microstrip transmission line resonators. This architecture allows the simultaneous implementation of a Jaynes-Cummings and anti-Jaynes-Cummings dynamics, a resonant method for generating mesoscopic qubit-field superpositions and for field-state reconstruction. Furthermore, we utilize this setup to propose a field measurement technique that is, in principle, robust to qubit dephasing and field relaxation due to a fast pre-measurement.

cond-mat.mes-hall↗

Magnetic and structural properties of GeMn films: precipitation of intermetallic nanomagnets

We present a comprehensive study relating the nanostructure of Ge_0.95Mn_0.05 films to their magnetic properties. The formation of ferromagnetic nanometer sized inclusions in a defect free Ge matrix fabricated by low temperature molecular beam epitaxy is observed down to substrate temperatures T_S as low as 70 deg. Celsius. A combined transmission electron microscopy (TEM) and electron energy-loss spectroscopy (EELS) analysis of the films identifies the inclusions as precipitates of the ferromagnetic compound Mn_5Ge_3. The volume and amount of these precipitates decreases with decreasing T_S. Magnetometry of the films containing precipitates reveals distinct temperature ranges: Between the characteristic ferromagnetic transition temperature of Mn_5Ge_3 at approximately room temperature and a lower, T_S dependent blocking temperature T_B the magnetic properties are dominated by superparamagnetism of the Mn_5Ge_3 precipitates. Below T_B, the magnetic signature of ferromagnetic precipitates with blocked magnetic moments is observed. At the lowest temperatures, the films show features characteristic for a metastable state.

cond-mat.mtrl-sci↗

Spin-glass-like behavior of Ge:Mn

We present a detailed study of the magnetic properties of low-temperature-molecular-beam-epitaxy grown Ge:Mn dilute magnetic semiconductor films. We find strong indications for a frozen state of Ge_{1-x}Mn_{x}, with freezing temperatures of T_f=12K and T_f=15K for samples with x=0.04 and x=0.2, respectively, determined from the difference between field-cooled and zero-field-cooled magnetization. For Ge_{0.96}Mn_{0.04}, ac susceptibility measurements show a peak around T_f, with the peak position T'_f shifting as a function of the driving frequency f by Delta T_f' / [T_f' Delta log f] ~ 0.06, whereas for sample Ge_{0.8}Mn_{0.2} a more complicated behavior is observed. Furthermore, both samples exhibit relaxation effects of the magnetization after switching the magnitude of the external magnetic field below T_f which are in qualitative agreement with the field- and zero-field-cooled magnetization measurements. These findings consistently show that Ge:Mn exhibits a frozen magnetic state at low temperatures and that it is not a conventional ferromagnet.

cond-mat.mtrl-sci↗

On-Chip Microwave Fock States and Quantum Homodyne Measurements

We propose a method to couple metastable flux-based qubits to superconductive resonators based on a quantum-optical Raman excitation scheme that allows for the deterministic generation of stationary and propagating microwave Fock states and other weak quantum fields. Moreover, we introduce a suitable microwave quantum homodyne technique, with no optical counterpart, that enables the measurement of relevant field observables, even in the presence of noisy amplification devices.

cond-mat.mes-hall↗

X-ray magnetic circular dichroism study of Re 5d magnetism in Sr2CrReO6

We have measured Re 5d spin and orbital magnetic moments in the ferrimagnetic double perovskite Sr2CrReO6 by X-ray magnetic circular dichroism at the L_{2,3} edges. In fair agreement with recent band-structure calculations [Vaitheeswaran et. al., Ref 1], at the Re site a large 5d spin magnetic moment of -0.68 mu_B and a considerable orbital moment of +0.25 mu_B have been detected. We found that the Curie temperature of the double perovskites A2BB'O6 scales with the spin magnetic moment of the 'non-magnetic' B' ion.

cond-mat.mtrl-sci↗

Laser microscopy of tunneling magnetoresistance in manganite grain-boundary junctions

Using low-temperature scanning laser microscopy we directly image electric transport in a magnetoresistive element, a manganite thin film intersected by a grain boundary (GB). Imaging at variable temperature allows reconstruction and comparison of the local resistance vs temperature for both, the manganite film and the GB. Imaging at low temperature also shows that the GB switches between different resistive states due to the formation and growth of magnetic domains along the GB. We observe different types of domain wall growth; in most cases a domain wall nucleates at one edge of the bridge and then proceeds towards the other edge.

cond-mat.str-el↗

Magnetic moments of W 5d in Ca2CrWO6 and Sr2CrWO6 double perovskites

We have investigated the magnetic moment of the W ion in the ferrimagnetic double perovskites Sr2CrWO6 and Ca2CrWO6 by X-ray magnetic circular dichroism (XMCD) at the W L(2,3) edges. In both compounds a finite negative spin and positive orbital magnetic moment was detected. The experimental results are in good agreement with band-structure calculations for (Sr/Ca)2CrWO6 using the full-potential linear muffin-tin orbital method. It is remarkable, that the magnetic ordering temperature, TC, is correlated with the magnetic moment at the 'non-magnetic' W atom.

cond-mat.mtrl-sci↗