arXiv subjects

R. H. Heffner

Publications and source records attributed to R. H. Heffner.

At least 19 recordsLinked to original sources

arXiv2013

Project X: Broader Impacts

Part-3 of "Project X: Accelerator Reference Design, Physics Opportunities, Broader Impacts". The proposed Project X proton accelerator at Fermilab, with multi-MW beam power and highly versatile beam formatting, will be a unique world-class facility to explore particle physics at the intensity frontier. Concurrently, however, it can also facilitate important scientific research beyond traditional particle physics and provide unprecedented opportunities in applications to problems of great national importance in the nuclear energy and security sector. Part 1 is available as arXiv:1306.5022 [physics.acc-ph] and Part 2 is available as arXiv:1306.5009 [hep-ex].

physics.acc-ph↗

arXiv2009

Field-induced coupled superconductivity and spin density wave order in the Heavy Fermion compound CeCoIn5

The high field superconducting state in CeCoIn5 has been studied by transverse field muon spin rotation measurements with an applied field parallel to the crystallographic c-axis close to the upper critical field Hc2 = 4.97 T. At magnetic fields >= 4.8 T the muon Knight shift is enhanced and the superconducting transition changes from second order towards first order as predicted for Pauli-limited superconductors. The field and temperature dependence of the transverse muon spin relaxation rate sigma reveal paramagnetic spin fluctuations in the field regime from 2 T < H < 4.8 T. In the normal state close to Hc2 correlated spin fluctuations as described by the self consistent renormalization theory are observed. The results support the formation of a mode-coupled superconducting and antiferromagnetically ordered phase in CeCoIn5 for H directed parallel to the c-axis.

cond-mat.str-el↗

arXiv2009

Penetration depth, multiband superconductivity, and absence of muon-induced perturbation in superconducting PrOs$_{4}$Sb$_{12}$

Transverse-field muon spin rotation ($μ$SR) experiments in the heavy-fermion superconductor PrOs$_{4}$Sb$_{12}$ ($T_{c}=1.85$ K) suggest that the superconducting penetration depth $λ(T)$ is temperature-independent at low temperatures, consistent with a gapped quasiparticle excitation spectrum. In contrast, radiofrequency (rf) inductive measurements yield a stronger temperature dependence of $λ(T)$, indicative of point nodes in the gap. This discrepancy appears to be related to the multiband structure of PrOs$_{4}$Sb$_{12}$. Muon Knight shift measurements in PrOs$_{4}$Sb$_{12}$ suggest that the perturbing effect of the muon charge on the neighboring Pr$^{3+}$ crystalline electric field is negligibly small, and therefore is unlikely to cause the difference between the $μ$SR and rf results.

cond-mat.supr-con↗

arXiv2008

Unconventional spin freezing and fluctuations in the frustrated antiferromagnet NiGa2S4

Muon spin rotation (muSR) experiments reveal unconventional spin freezing and dynamics in the two-dimensional (2D) triangular lattice antiferromagnet NiGa2S4. Long-lived disordered Ni-spin freezing (correlation time > 10-6 s at 2 K) sets in below T_f = 8.5 +- 0.5 K with a mean-field-like temperature dependence. The observed exponential temperature dependence of the muon spin relaxation above T_f is strong evidence for 2D critical spin fluctuations. Slow Ni spin fluctuations coexist with quasistatic magnetism at low temperatures but are rapidly suppressed for fields > 10 mT, in marked contrast with the field-independent specific heat. The muSR and bulk susceptibility data indicate a well-defined 2D phase transition at T_f, below which NiGa2S4 is neither a conventional magnet nor a singlet spin liquid.

cond-mat.str-el↗

arXiv2008

Weak quasistatic magnetism in the frustrated Kondo lattice Pr_2Ir_2O_7

Muon spin relaxation experiments have been performed in the pyrochlore iridate Pr_2Ir_2O_7 for temperatures in the range 0.025-250 K. Kubo-Toyabe relaxation functions are observed up to > 200 K, indicating static magnetism over this temperature range. The T -> 0 static muon spin relaxation rate Delta(0) ~ 8 mus^-1 implies a weak quasistatic moment (~0.1 mu_B). The temperature dependence of Delta is highly non-mean-field-like, decreasing smoothly by orders of magnitude but remaining nonzero below ~150 K. The data rule out ordering of the full Pr^3+ CEF ground-state moment (3.0 mu_B) down to 0.025 K. The weak static magnetism is most likely due to hyperfine-enhanced ^141Pr nuclear magnetism. The dynamic relaxation rate lambda increases markedly below ~20 K, probably due to slowing down of spin fluctuations in the spin-liquid state. At low temperatures lambda is strong and temperature-independent, indicative of a high density of low-lying spin excitations as is common in frustrated antiferromagnets.

cond-mat.str-el↗

arXiv2007

Muon spin rotation measurements of the superfluid density in fresh and aged superconducting PuCoGa$_5$

We have measured the temperature dependence and magnitude of the superfluid density $ρ_{\rm s}(T)$ via the magnetic field penetration depth $λ(T)$ in PuCoGa$_5$ (nominal critical temperature $T_{c0} = 18.5$ K) using the muon spin rotation technique in order to investigate the symmetry of the order parameter, and to study the effects of aging on the superconducting properties of a radioactive material. The same single crystals were measured after 25 days ($T_c = 18.25$ K) and 400 days ($T_c = 15.0$ K) of aging at room temperature. The temperature dependence of the superfluid density is well described in both materials by a model using d-wave gap symmetry. The magnitude of the muon spin relaxation rate $σ$ in the aged sample, $σ\propto 1/λ^2\proptoρ_s/m^*$, where $m^*$ is the effective mass, is reduced by about 70% compared to fresh sample. This indicates that the scattering from self-irradiation induced defects is not in the limit of the conventional Abrikosov-Gor'kov pair-breaking theory, but rather in the limit of short coherence length (about 2 nm in PuCoGa$_5$) superconductivity.

cond-mat.str-el↗

arXiv2007

Multiband superconductivity and penetration depth in PrOs4Sb12

The effective superconducting penetration depth measured in the vortex state of PrOs4Sb12 using transverse-field muon spin rotation (TF-muSR) exhibits an activated temperature dependence at low temperatures, consistent with a nonzero gap for quasiparticle excitations. In contrast, Meissner-state radiofrequency (rf) inductive measurements of the penetration depth yield a T^2 temperature dependence, suggestive of point nodes in the gap. A scenario based on the recent discovery of extreme two-band superconductivity in PrOs4Sb12 is proposed to resolve this difference. In this picture a large difference between large- and small-gap coherence lengths renders the field distribution in the vortex state controlled mainly by supercurrents from a fully-gapped large-gap band. In zero field all bands contribute, yielding a stronger temperature dependence to the rf inductive measurements.

cond-mat.supr-con↗

arXiv2007

Muon spin relaxation and hyperfine-enhanced 141Pr nuclear spin dynamic in Pr(Os,Ru)4Sb12 and (Pr,La)Os4Sb12

Zero- and longitudinal-field muon spin relaxation (MuSR) experiments have been carried out in the alloy series Pr(Os1-xRux)4Sb12 and Pr1-yLayOs4Sb12 to elucidate the anomalous dynamic muon spin relaxation observed in these materials. The damping rate associated with this relaxation varies with temperature, applied magnetic field, and dopant concentrations x and y in a manner consistent with the ``hyperfine enhancement'' of 141Pr nuclear spins first discussed by Bleaney in 1973. This mechanism arises from Van Vleck-like admixture of magnetic Pr3+ crystalline-electric-field-split excited states into the nonmagnetic singlet ground state by the nuclear hyperfine coupling, thereby increasing the strengths of spin-spin interactions between 141Pr and muon spins and within the 141Pr spin system. We find qualitative agreement with this scenario, and conclude that electronic spin fluctuations are not directly involved in the dynamic muon spin relaxation.

cond-mat.str-el↗

arXiv2005

Critical slowing down in the geometrically frustrated pyrochlore antiferromagnet Gd_2Ti_2O_7

Longitudinal-field muon spin relaxation experiments have been carried out in the paramagnetic state of single-crystal Gd_2Ti_2O_7 just above the phase transition at T_m = 1.0 K. At high applied fields the exponential relaxation time T_1 is proportional to field, whereas T_1 saturates below a crossover field B_c that is ~2.5 T at 1.5 K and decreases as T_m is approached. At low fields the relaxation rate increases markedly as the freezing temperature is approached, as expected for critical slowing down of the spin fluctuations, but the increase is suppressed by applied field. This behavior is consistent with the very long autocorrelation function cutoff time implied by the low value of B_c.

cond-mat.str-el↗

arXiv2005

Susceptibility inhomogeneity and non-Fermi liquid behavior in UCu_{5-x}Pt_x

Transverse-field muSR shifts and relaxation rates have been measured in the non-Fermi liquid (NFL) alloy system UCu_{5-x}Pt_x, x = 1.0, 1.5, and 2.5. At low temperatures the fractional spread in Knight shifts delta K/K approx deltachi/chi is gtrsim 2 for x = 1, but is only half this value for x = 1.5 and 2.5. In a disorder-driven scenario where the NFL behavior is due to a broadly distributed (Kondo or Griffiths-phase cluster) characteristic energy E, our results indicate that delta E/E_{rm av} approx (delta K/K)_{T=0} is similar for UCu_{5-x}Pd_x (x = 1 and 1.5) and UCu_4Pt, but is reduced for UCu_{5-x}Pt_x, x = 1.5 and 2.5. This reduction is due to a marked increase of E with increasing x; the spread delta E is found to be roughly independent of x. Our results correlate with the observed suppression of other NFL anomalies for x > 1 in UCu_{5-x}Pt_x but not in UCu_{5-x}Pd_x, and are further evidence for the importance of disorder in the NFL behavior of both these alloy systems.

cond-mat.str-el↗

arXiv2005

Effect of annealing on glassy dynamics and non-Fermi liquid behavior in UCu_4Pd

Longitudinal-field muon spin relaxation (LF-muSR) experiments have been performed in unannealed and annealed samples of the heavy-fermion compound UCu_4Pd to study the effect of disorder on non-Fermi liquid behavior in this material. The muon spin relaxation functions G(t,H) obey the time-field scaling relation G(t,H) = G(t/H^gamma) previously observed in this compound. The observed scaling exponent gamma = 0.3 pm 0.1, independent of annealing. Fits of the stretched-exponential relaxation function G(t) = exp[-(Lambda t)^K] to the data yielded stretching exponentials K < 1 for all samples. Annealed samples exhibited a reduction of the relaxation rate at low temperatures, indicating that annealing shifts fluctuation noise power to higher frequencies. There was no tendency of the inhomogeneous spread in rates to decrease with annealing, which modifies but does not eliminate the glassy spin dynamics reported previously in this compound. The correlation with residual resistivity previously observed for a number of NFL heavy-electron materials is also found in the present work.

cond-mat.str-el↗

arXiv2005

New limits on the ordered moments in alpha-Pu and Ga-stabilized delta-Pu

We present the first muon spin relaxation measurements ever performed on elemental Pu, and set the most stringent upper limits to date on the magnitude of the ordered moment in alpha-Pu and delta-stabilized Pu (alloyed with 4.3 at. % Ga). Assuming a nominal hyperfine coupling field of 1 kOe per Bohr magneton we set an upper limit of 0.001 Bohr magnetons for both materials at T = 4 K.

cond-mat.str-el↗

arXiv2005

Evolution of the heavy fermion state in Ce2IrIn8

We report muon spin rotation Knight shift and susceptibility studies for 1 T applied field along the crystalline c- and a-axes of the heavy fermion compound Ce2IrIn8. Below a characteristic temperature T* one observes a `Knight-shift anomaly' in which the Knight shift constant K no longer scales linearly with susceptibility chi. This anomaly is consistent with a scaling law in which chi is composed of a high-temperature component corresponding to non-interacting local moments and a low-temperature component chi_cf proportional to (1-T/T*)\ln(T*/T) which characterizes the heavy-electron state below T*. We find that T* is anisotropic, with T_a* = 59(3)K and T_c* = 24(1)K, and derive the magnitudes of chi_cf for H along the a- and c-axes.

cond-mat.str-el↗

arXiv2005

Penetration depth, symmetry breaking, and gap nodes in superconducting PrOs4Sb12

Transverse-field muon spin relaxation rates in single crystals of the heavy-fermion superconductor PrOs4Sb12 (Tc = 1.85 K) are nearly constant in the vortex state for temperatures below ~0.5Tc. This suggests that the superconducting penetration depth lambda(T) is temperature-independent at low temperatures, consistent with a gapped quasiparticle excitation spectrum. In contrast, radiofrequency measurements yield a stronger temperature dependence of lambda(T), indicative of point nodes in the gap. A similar discrepancy exists in superconducting Sr2RuO4 which, like PrOs4Sb12, breaks time-reversal symmetry (TRS) below Tc, but not in a number of non-TRS-breaking superconductors.

cond-mat.supr-con↗

arXiv2005

The symmetry of the superconducting order parameter in PuCoGa$_5$

The symmetry of the superconducting order parameter in single-crystalline PuCoGa$_5$ ($T_{\rm c} = 18.5$ K) is investigated via zero- and transverse- field muon spin relaxation ($μ$SR) measurements, probing the possible existence of orbital and/or spin moments (time reversal-symmetry violation TRV) associated with the superconducting phase and the in-plane magnetic-field penetration depth $λ(T)$ in the mixed state, respectively. We find no evidence for TRV, and show that the superfluid density, or alternatively, $Δλ(T) = λ(T) - λ(0)$, are $\propto T$ for $T/T_{\rm c} \leq 0.5$. Taken together these measurements are consistent with an even-parity (pseudo-spin singlet), d-wave pairing state.

cond-mat.supr-con↗

arXiv2004

Direct observation of the formation of polar nanoregions in Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_3$ using neutron pair distribution function analysis

Using neutron pair distribution function (PDF) analysis over the temperature range from 1000 K to 15 K, we demonstrate the existence of local polarization and the formation of medium-range, polar nanoregions (PNRs) with local rhombohedral order in a prototypical relaxor ferroelectric Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_3$. We estimate the volume fraction of the PNRs as a function of temperature and show that this fraction steadily increases from 0 % to a maximum of $\sim$ 30% as the temperature decreases from 650 K to 15 K. Below T$\sim$200 K the PNRs start to overlap as their volume fraction reaches the percolation threshold. We propose that percolating PNRs and their concomitant overlap play a significant role in the relaxor behavior of Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_3$.

cond-mat.dis-nn↗

arXiv2004

Local Distortion Induced Metal-to-Insulator Phase Transition in PrRu$_4$P$_{12}$

Extended X-ray Absorption Fine Structure (EXAFS) experiments have been carried out on PrRu$_4$P$_{12}$ and PrOs$_4$P$_{12}$ to study the metal-to-insulator (MI) phase transition in PrRu$_4$P$_{12}$. No Pr displacement was observed across the MI transition temperature from the EXAFS data. Instead, our EXAFS data clearly show that a Ru displacement is associated with this MI transition. The very high Debye temperature for the Ru-P bond ($Θ_D$=690 K) suggests that a slight rotation/displacement of relatively rigid RuP$_6$ octahedra leads to this small Ru displacement, which accompanies the MI transition at 62 K in PrRu$_4$P$_{12}$.

cond-mat.mtrl-sci↗

arXiv2004

Disorder, inhomogeneity and spin dynamics in f-electron non-Fermi liquid systems

Muon spin rotation and relaxation ($μ$SR) experiments have yielded evidence that structural disorder is an important factor in many f-electron-based non-Fermi-liquid (NFL) systems. Disorder-driven mechanisms for NFL behaviour are suggested by the observed broad and strongly temperature-dependent $μ$SR (and NMR) linewidths in several NFL compounds and alloys. Local disorder-driven theories (Kondo disorder, Griffiths-McCoy singularity) are, however, not capable of describing the time-field scaling seen in muon spin relaxation experiments, which suggest cooperative and critical spin fluctuations rather than a distribution of local fluctuation rates. A strong empirical correlation is established between electronic disorder and slow spin fluctuations in NFL materials

cond-mat.str-el↗