arXiv subjects

R. Kadono

Publications and source records attributed to R. Kadono.

At least 55 records · Page 3Linked to original sources

arXiv2014

Bulk superconductivity in undoped T'-La$_{1.9}$Y$_{0.1}$CuO$_4$ probed by muon spin rotation

The Meissner effect has been directly demonstrated by depth-resolved muon spin rotation measurements in high-quality thin films of the T'-structured cuprate, T'-La$_{1.9}$Y$_{0.1}$CuO$_4$, to confirm bulk superconductivity ($T_c\simeq21$ K) in its {\sl undoped} state. The gradual expelling of an external magnetic field is observed over a depth range of $\sim$100 nm in films with a thickness of 275(15) nm, from which the penetration depth is deduced to be 466(22) nm. Based on this result, we argue that the true ground state of the "parent" compound of the $n$-type cuprates is not a Mott insulator but a strongly correlated metal with colossal sensitivity to apical oxygen impurities.

cond-mat.supr-con↗

arXiv2014

Cooperative order in the weakly magnetic domain of LaFeAsO$_{1-x}$F$_{x}$ near the doping phase boundary

Spatial phase separation into mesoscopic domains of non-magnetic [superconducting (SC) below Tc = 25.5 K] and two kinds of magnetic phases, one showing disordered spin density wave (d-SDW) order and another associated with glassy weak magnetism (WM), are observed below ~100 K by muon spin rotation (muSR) in LaFeAsO1-xFx for x = 0.057(3) which is near the boundary of these phases on the doping phase diagram. In contrast to the competing order observed in the regular SDW phase of Ba(Fe1-xCox)2As2, the WM domain exhibits cooperative coupling of superconducting and magnetic order parameters as inferred from strong diamagnetism and associated negative shift of muSR frequency just below Tc.

cond-mat.str-el↗

arXiv2012

muSR Investigation of magnetically ordered states in A-site ordered perovskite manganites RBaMn2O6 (R = Y and La)

The magnetically ordered states of the A-site ordered perovskite manganites LaBaMn2O6 and YBaMn2O6 have been investigated by muon spin relaxation in zero external magnetic field. Our data reveal striking differences in the nature of the magnetically ordered state of these materials. For LaBaMn2O6, the muSR time-spectra in the ferromagnetic state below ~ 330 K reveal a strongly inhomogeneous phase, reminiscent of a Griffiths phase. Within this magnetically inhomogeneous phase, an antiferromagnetic state develops below 150 K, which displays well defined static internal magnetic fields, but reaches only 30% of the volume fraction at low temperatures. A broad distribution of muSR relaxation rates is inferred down to the lowest temperatures. This behavior is similar to the A-site disordered La0.5Ba0.5MnO3. On the other hand, for YBaMn2O6, the muSR time spectra for both (i) the charge and orbital ordered and (ii) the paramagnetic phases reveal rather homogeneous states, namely, an exponential relaxation in the paramagnetic state and well defined muon spin oscillation in the antiferromagnetic state.

cond-mat.str-el↗

arXiv2011

Quasi-one-dimensional spin dynamics in LiV2O4: 1D-to-3D crossover as a possible origin of heavy fermion state

Spin fluctuation in LiV2O4 is revisited by examining the earlier result of muon spin rotation/ relaxation measurements. Instead of a relationship for the localized electron limit, one for itinerant electron systems between muon depolarization rate and spin fluctuation rate (ν_D) is employed to re-analyze data, which reveals that νD varies linearly with temperature (ν_D {\propto} T) over a range 10^8-10^{12} /s for 0.02 {\le} T < 102 K. Such a linear-T behavior as well as the magnitude of ν_D is fully consistent with that of the magnetic relaxation rate previously observed by inelastic neutron scattering (INS), demonstrating that μSR and INS have a common time window over the fluctuation spectrum. The linear-T dependence of ν_D is understood as a specific feature predicted by a Hubbard model for intersecting one-dimensional (1D) chains. This quasi-1D character, which is co-existent with enhanced uniform susceptibility at low temperatures, supports the scenario of 1D-to-3D crossover for the microscopic origin of heavy-fermion behavior in LiV2O4.

cond-mat.str-el↗

arXiv2011

Quasi-One-Dimensional Spin Dynamics in $d$-Electron Heavy-Fermion Metal Y$_{1-x}$Sc$_x$Mn$_2$

Slow spin fluctuations ($ν< 10^{12}$ s$^-1$) observed by the muon spin relaxation technique in Y$_{1-x}$Sc$_x$Mn$_2$ exhibits a power law dependence on temperature ($ν\propto T^α$), where the power converges asymptotically to unity ($α\rightarrow 1$) as the system moves away from spin-glass instability with increasing Sc content $x$. This linear $T$ dependence, which is common to that observed in LiV$_2$O$_4$, is in line with the prediction of the "intersecting Hubbard chains" model for a metallic pyrochlore lattice, suggesting that the geometrical constraints to t2g bands specific to the pyrochlore structure serve as a basis of the $d$-electron heavy-fermion state.

cond-mat.str-el↗

arXiv2011

Suppression of time reversal symmetry breaking superconductivity in Pr(Os,Ru)_4Sb_12 and (Pr,La)Os_4Sb_12

Zero-field muon spin relaxation experiments have been carried out in the Pr(Os_{1-x}Ru_x)_4Sb_12 and Pr_{1-y}La_yOs_4Sb_12 alloy systems to investigate broken time-reversal symmetry (TRS) in the superconducting state, signaled by the onset of a spontaneous static local magnetic field B_s. In both alloy series B_s initially decreases linearly with solute concentration. Ru doping is considerably more efficient than La doping, with a ~50% faster initial decrease. The data suggest that broken TRS is suppressed for Ru concentration x >~ 0.6, but persists for essentially all La concentrations. Our data support a crystal-field excitonic Cooper pairing mechanism for TRS-breaking superconductivity.

cond-mat.supr-con↗

arXiv2010

Magnetic ground state of pyrochlore oxides close to metal-insulator boundary probed by muon spin rotation

Magnetism of ruthernium pyrochlore oxides A2Ru2O7 (A = Hg, Cd, Ca), whose electronic properties within a localized ion picture are characterized by non-degenerate t2g orbitals (Ru5+, 4d3) and thereby subject to geometrical frustration, has been investigated by muon spin rotation/relaxation (muSR) technique. The A cation (mostly divalent) was varied to examine the effect of covalency (Hg > Cd > Ca) on their electronic property. In a sample with A = Hg that exhibits a clear metal-insulator (MI) transition below >> 100 K (which is associated with a weak structural transition), a nearly commensurate magnetic order is observed to develop in accordance with the MI transition. Meanwhile, in the case of A = Cd where the MI transition is suppressed to the level of small anomaly in the resistivity, the local field distribution probed by muon indicates emergence of a certain magnetic inhomogeneity below » 30 K. Moreover, in Ca2Ru2O7 that remains metallic, we find a highly inhomogeneous local magnetism below >>25 K that comes from randomly oriented Ru moments and thus described as a "frozen spin liquid" state. The systematic trend of increasing randomness and itinerant character with decreasing covalency suggests close relationship between these two characters. As a reference for the effect of orbital degeneracy and associated Jahn-Teller instability, we examine a tetravalent ruthernium pyrochlore, Tl2Ru2O7 (Ru4+, 4d4), where the result of muSR indicates a non-magnetic ground state that is consistent with the formation of the Haldane chains suggested by neutron diffraction experiment.

cond-mat.str-el↗

arXiv2010

Incommensurate spin correlations induced by magnetic Fe ions substituted into overdoped Bi1.75Pb0.35Sr1.90CuO6+z

Spin correlations in the overdoped region of Bi1.75Pb0.35Sr1.90CuO6+z have been explored with Fe-doped single crystals characterized by neutron scattering, muon-spin-rotation (muSR) spectroscopy, and magnetic susceptibility measurements. Static incommensurate spin correlations induced by the Fe spins are revealed by elastic neutron scattering. The resultant incommensurability delta is unexpectedly large (~0.2 r.l.u.), as compared with delta ~ 1/8 in overdoped superconductor La2-xSrxCuO4. Intriguingly, the large delta in this overdoped region is close to the hole concentration p. This result is reminiscent of the delta ~ p trend observed in underdoped La2-xSrxCuO4; however, it is inconsistent with the saturation of delta in the latter compound in the overdoped regime. While our findings in Fe-doped Bi1.75Pb0.35Sr1.90CuO6+z support the commonality of incommensurate spin correlations in high-Tc cuprate superconductors, they also suggest that the magnetic response might be dominated by a distinct mechanism in the overdoped region.

cond-mat.supr-con↗

arXiv2010

Anisotropic order parameter in Li-intercalated layered superconductor Li$_x$ZrNCl

In this study, it is shown that in a layered nitride superconductor, i.e., LixZrNCl (0.07<=x<=0.21), the superconducting order parameter is highly anisotropic in a sample with x=0.12, as inferred from both the temperature and the magnetic field dependences of the muon depolarization rate (sigma_s, proportional to the superfluid density). Moreover, the tendency of strong anisotropy with an increase in x is indicated by the T dependence of sigma_s. These observations are in good agreement with the recent theory that predicts the development of anisotropy in a d+id' gap upon carrier filling to the bands with disconnected Fermi surfaces on a honeycomb lattice.

cond-mat.supr-con↗

arXiv2009

Field-induced magnetism in the high-$T_c$ superconductor Ca$_{2-x}$Na$_x$CuO$_2$Cl$_2$ with flat CuO$_2$ planes

The internal magnetic field distribution in a mixed state of a cuprate superconductor, Ca$_{2-x}$Na$_x$CuO$_2$Cl$_2$ ($T_{\rm c}\simeq28.5$ K, near the optimal doping), was measured by muon spin rotation ($μ$SR) technique up to 60 kOe. The $μ$SR linewidth $Λ(B)$ which exhibits excess broadening at higher fields ($B>5$ kOe) due to field-induced magnetism (FIM), is described by a relation, $Λ(B)\propto\sqrt{B}$. This suggests that the orbital current and associated quasiparticle excitation plays predominant roles in stabilizing the quasistatic correlation. Moreover, a slowing down of the vortex fluctuation sets in well above $T_{\rm c}$, as inferred from the trace of FIM observed up to $\sim80$ K, and develops continuously without a singularity at $T_{\rm c}$ as the temperature decreases.

cond-mat.supr-con↗

arXiv2009

Insular superconductivity in Co-doped iron pnictide CaFe$_{1-x}$Co$_x$AsF

The presence of macroscopic phase separation between the superconducting and magnetic phases in \cfcaf is demonstrated by muon spin rotation (muSR) measurements conducted across their phase boundaries (x=0.05-0.15). The magnetic phase tends to retain the high transition temperature (T_m > T_c), while Co-doping induces strong randomness. The volumetric fraction of superconducting phase is nearly proportional to the Co content $x$ with constant superfluid density. These observations suggest the formation of superconducting "islands" (or domains) associated with Co ions in the Fe$_2$As$_2$ layers, indicating a very short coherence length.

cond-mat.supr-con↗

arXiv2009

Competition/Coexisitence of Magnetism and Superconductivity in Iron Pnictides Probed by Muon Spin Rotation

The presence of macroscopic phase separation into superconducting and magnetic phases in LaFeAsO$_{1-x}$F$_x$ (LFAOF) and CaFe$_{1-x}$Co$_x$AsF (CFCAF) is demonstrated by muon spin rotation (muSR) measurement across their phase boundaries ($x=0.06$ for LFAOF and $x=0.075$--0.15 for CFCAF). In LFAOF, both magnetism and superconductivity develop simultaneously below a common critical temperature, $T_m =~ T_c =~ 18$ K, where the magnetism is characterized by strong randomness. A similar, but more distinct segregation of these two phases is observed in CFCAF, where the magnetic phase retains $T_m$ as close to that of the parent compound ($T_c << T_m =~ 80$--120 K) and the superconducting volume fraction is proportional to the Co content $x$. The close relationship between magnetism and superconductivity is discussed based on these experimental observations. Concerning superconducting phase, an assessment is made on the anisotropy of order parameter in the superconducting state of LFAOF, CFCAF, and Ba$_{1-x}$K$_x$Fe$_2$As$_2$ (BKFA, $x=0.4$) based on the temperature dependence of superfluid density [$n_s(T)$] measured by muSR. The gap parameter, $2Δ/k_BT_c$, determined from $n_s(T)$ exhibits a tendency that hole-doped pnictides (BKFA) is much greater than those in electron-doped ones (LFAOF, CFCAF), suggesting difference in the coupling to bosons mediating the Cooper pairs between relevant $d$ electron bands.

cond-mat.supr-con↗

arXiv2008

Full Gap Superconductivity in Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ Probed by Muon Spin Rotation

Superfluid density ($n_s$) in the mixed state of an iron pnictide superconductor Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ is determined by muon spin rotation for a sample with optimal doping ($x=0.4$). The temperature dependence of $n_s$ is perfectly reproduced by the conventional BCS model for s-wave paring, where the order parameter can be either a single-gap with $Δ=8.35(6)$ meV [$2Δ/k_BT_c=5.09(4)$], or double-gap structure with $Δ_1=12$ meV (fixed) [$2Δ_1/k_BT_c=7.3$] and $Δ_2=6.8(3)$ meV [$2Δ_2/k_BT_c=4.1(2)$]. The latter is consistent with the recent result of angle-resolved photo-emssion spectroscopy. The large gap parameters ($2Δ/k_BT_c$) indicate extremely strong coupling of carriers to bosons that mediate the Cooper pairing.

cond-mat.supr-con↗

arXiv2008

Magnetic response of noncentrosymmetric superconductor La2C3: Effect of double-gap and spin-orbit interaction

The presence of spin-orbit (SO) interaction in a noncentrosymmetric superconductor, La2C3 (T_c~11 K) is demonstrated by muon spin rotation (muSR) in its normal state, where muSR spectra exhibit field-induced weak depolarization due to van Vleck-like local susceptibility. In the mixed state, muon spin relaxation due to inhomogeneity of internal field (sigma_v) exhibits a field dependence that is characterized by a kink, where sigma_v (and hence the superfluid density) is more strongly reduced at lower fields. This is perfectly in line with the presence of a secondary energy gap previously inferred from the temperature dependence of sigma_v, and also consistent with the possible influence of asymmetric deformation of the Fermi surface due to the SO interaction.

cond-mat.supr-con↗

arXiv2008

Effect of Zn substitution for Cu on Ca$_{2-x}$Na$_{x}$CuO$_{2}$Cl$_{2}$ near the hole concentration of 1/8 per Cu

A weakening of superconductivity upon substitution of Cu by Zn (0.5~1 %) is observed in a high-T_c cuprate, Ca_{2-x}Na_xCuO2Cl2, near the hole concentration of 1/8 per Cu. The superconducting transition temperature and its volume fraction, estimated by magnetic susceptibility, exhibit a sizable anomaly for x=0.12~0.14, where the slowing down of Cu spin fluctuations below 5 K is demonstrated by muon spin relaxation experiments. These observations are in close resemblance to other typical cuprates including YBa2Cu3O_{7-d}, and Bi2Sr2Ca_{1-x}Y_xCu2O_{8+d}, providing further evidence that Zn-induced "stripe" correlation is a universal feature of high-T_c cuprate superconductors common to that of La_{2-x}A_{x}CuO4 (A=Ba, Sr).

cond-mat.supr-con↗

arXiv2008

Coexistence of Supercondcutivity and Magnetism in LaFeAs(O0.94F0.06) Probed by Muon Spin Relaxation

Recent discovery of oxypnictide superconductor LaFeAs(O,F) (LFAO-F) with the critical temperature (Tc) of 26 K and succeeding revelation of much increased Tc upon substitution of La for other rare earth elements (such as Sm, leading to ~43 K) and application of pressure for LFAO-F (~ 43 K) has triggered broad interest in the mechanism yielding relatively high Tc in this new class of compounds. While they share a feature with high-Tc cuprates that superconductivity occurs upon carrier doping to pristine compound which exhibits magnetism, they also resemble the heavy-fermion compounds in the sense that superconductivity appears in the vicinity of magnetic phase. Investigation of electronic states near the boundary between these two phases might provide some useful information on the mechanism of superconductivity, as it has been proved to be the case in many exotic superconductors. Here we show by muon experiment in the LFAO-F compound that a macroscopic phase separation into superconducting and spin glass-like magnetic phases occurs at x=0.06 that is near the phase boundary, where both the magnetism and superconductivity develop simultaneously below a common Tc ~ 18 K. This accordance strongly suggests intimate relationship between magnetism and superconductivity typically found in heavy-fermion systems near the quantum critical point.

cond-mat.mtrl-sci↗

arXiv2008

Multigap superconductivity in sesquicarbides La$_2$C$_3$ and Y$_2$C$_3$

A complex structure of the superconducting order parameter in $Ln_2$C$_3$ ($Ln$ = La, Y) is demonstrated by muon spin relaxation ($μ$SR) measurements in their mixed state. The muon depolarization rate [$σ_{\rm v}(T)$] exhibits a characteristic temperature dependence that can be perfectly described by a phenomenological double-gap model for nodeless superconductivity. While the magnitude of two gaps is similar between La$_2$C$_3$ and Y$_2$C$_3$, a significant difference in the interband coupling between those two cases is clearly observed in the behavior of $σ_{\rm v}(T)$.

cond-mat.supr-con↗

arXiv2008

t'- and t"-dependence of the bulk-limit superconducting condensation energy of the 2D Hubbard model

The 2D Hubbard model having the 2nd- and 3rd-neighbor transfer energies t' and t" is investigated by use of the variational Monte Carlo method. At the nearly optimal doping with on-site Coulomb energy U=6 (energy unit is t) the condensation energy Econd for the d-wave superconductivity (SC) is computed for lattices of sizes from 10x10 to 28x28 with the aim to get its bulk-limit value. t" is fixed at -t'/2. Outside and in the neighborhood of the SDW region of -0.16=<t'=<-0.08 the SC Econd dominates over the SDW Econd. At t'=-0.05 and -0.10 we obtained a definitely finite bulk-limit SC Econd of the order of the experimental value for YBCO. At t'=0 Econd nearly vanishes. For t'=<-0.18, the SC Econd strongly oscillates as a function of the lattice size, when periodic boundary conditions (b.c.'s) are imposed to both axes. In the case of periodic and antiperiodic b.c.'s, a finite bulk-limit value is obtained at t'=-0.22. Econd tends to vanish with further decrease of t'. With our results the SC of LSCO is understandable with t'~ -0.10. The t' values of Hg1201, Tl2201 and Na-CCOC seem close to -0.20 so that they locate in the boundary zone of SC indicated in the present work. Slightly larger U improves the situation by increasing Econd.

cond-mat.supr-con↗