arXiv subjects

R. Lebrun

Publications and source records attributed to R. Lebrun.

At least 19 recordsLinked to original sources

arXiv2025

Multi-functional Wafer-Scale Van der Waals Heterostructures and Polymorphs

Van der Waals heterostructures have promised the realisation of artificial materials with multiple physical phenomena such as giant optical nonlinearities, spin-to-charge interconversion in spintronics and topological carrier protection, in a single layered device through an infinitely diverse set of quantum materials. However, most efforts have only focused on exfoliated material that inherently limits both the dimensions of the materials and the scalability for applications. Here, we show the epitaxial growth of large area heterostructures of topological insulators (Bi2Se3), transition metal dichalcogenides (TMDs, WSe2) and ferromagnets (Co), resulting in the combination of functionalities including tuneable optical nonlinearities, spin-to-charge conversion and magnetic proximity effects. This is demonstrated through coherent phase resolved terahertz currents, bringing novel functionalities beyond those achievable in simple homostructures. In particular, we show the role of different TMD polymorphs, with the simple change of one atomic monolayer of the artificial material stack entirely changing its optical, electrical and magnetic properties. This epitaxial integration of diverse two-dimensional materials offers foundational steps towards diverse perspectives in quantum material engineering, where the material polymorph can be controlled at technological relevant scales for coupling applications in, for example, van der Waals nonlinear optics, optoelectronics, spintronics, multiferroics and coherent current control.

cond-mat.mtrl-sci↗

arXiv2024

Inverse Rashba-Edelstein THz emission modulation induced by ferroelectricity in CoFeB/PtSe2/MoSe2//LiNbO3 systems

Spintronic Terahertz emitters, based on optically triggered spin-to-charge interconversion processes, have recently emerged as novel route towards compact and efficient THz sources. Yet, the next challenge for further technologically-relevant devices remains to modulate the emission, with low-energy consumption operation. To this aim, ferroelectric materials coupled to active spin-orbit layers such as two-dimensional transition metal dichalcogenides are suitable candidates. In this work, we present the realization of a large area heterostructure of CoFeB/PtSe2/MoSe2 on a bi-domain LiNbO3 substrate. Using THz time-domain spectroscopy, we show that the ferroelectric polarization direction induces a sizeable modulation of the THz emission. We rationalise these experimental results by using band structure and spin accumulation calculations that are consistent with an interfacial spin-to-charge conversion mediated by inverse Rashba-Edelstein effect at the MoSe2/PtSe2 interface and being tuned by ferroelectricity in the adjacent LiNbO3 surface. This work points out the relevance of field effect spin-orbit architectures for novel THz technologies.

cond-mat.mtrl-sci↗

arXiv2024

Controlling encirclement of an exceptional point using coupled spintronic nano-oscillators

Exceptional points (EPs), branch singularities parameter space of non-Hermitian eigenvalue manifolds, display unique topological phenomena linked to eigenvalue and eigenvector switching: the parameter space states are highly sensitive to the system's parameter changes. Therefore, we suggest investigating the parameter space in the presence of an EP by experimentally accessing and exploiting the topological nature of the coupled system around an EP. We demonstrate control over exceptional points in coupled vortex spin-transfer torque oscillators by adjusting the system's damping through the spin-transfer torque effect and their relative phase. This approach allows for precise manipulation of the coupling behavior in the vicinity of an exceptional point. We report the presence of both level attraction/repulsion by adjusting the system's parameters. Moreover, we evidence the topological nature of the EP by dynamically encircling it in the phase-current parameter space, leading to a switch of the eigenstates. Our study introduces a new method for exploring non-Hermitian physics in spintronic systems at room temperature.

cond-mat.mes-hall↗

arXiv2024

Probing nonlinear spin dynamics in canted easy-plane antiferromagnets using spin-rectification effects

We investigate spin-rectification phenomena in canted antiferromagnets, closely connected to the family of altermagnetic materials. Our results show that excitation efficiency is significantly enhanced by the Dzyaloshinskii-Moriya interaction. Antiferromagnetic dynamics can be detected through spin-Hall magnetoresistance and bolometric effects, with an efficiency reaching up to mV/W. The rectified voltage shape is influenced by both the symmetry of the exciting torques, detection mechanisms (continuous spin-pumping and spin-Hall magnetoresistance), and the antiferromagnetic crystalline axis. Under high pumping power, we observe a saturation effect related to Suhl-like spin-wave instabilities and a nonlinear redshift of the antiferromagnetic resonance. These findings open new avenues for studying nonlinear dynamics in antiferromagnetic and altermagnetic spintronic devices.

cond-mat.mes-hall↗

arXiv2023

Antiferromagnetic magnon spintronic based on non-reciprocal and non-degenerated ultra-fast spin-waves in the canted antiferromagnet α-Fe2O3

Spin-waves in antiferromagnets hold the prospects for the development of faster, less power-hungry electronics, as well as promising physics based on spin-superfluids and coherent magnon-condensates. For both these perspectives, addressing electrically coherent antiferromagnetic spin-waves is of importance, a prerequisite that has so far been elusive, because unlike ferromagnets,antiferromagnets couple weakly to radiofrequency fields. Here, we demonstrate the detection of ultra-fast non-reciprocal spin-waves in the dipolar-exchange regime of a canted antiferromagnet using both inductive and spintronic transducers. Using time-of-flight spin-wave spectroscopy on hematite (α-Fe2O3), we find that the magnon wave packets can propagate as fast as 20 km/s for reciprocal bulk spin-wave modes and up to 6 km/s for surface-spin waves propagating parallel to the antiferromagnetic Neel vector. We finally achieve efficient electrical detection of non-reciprocal spin-wave transport using non-local inverse spin-Hall effects. The electrical detection of coherent non-reciprocal antiferromagnetic spin waves paves the way for the development of antiferromagnetic and altermagnet-based magnonic devices.

cond-mat.mes-hall↗

arXiv2023

Spin-momentum locking and ultrafast spin-charge conversion in ultrathin epitaxial Bi$_{1-x}$Sb$_x$ topological insulator

The helicity of 3D topological insulator surface states has drawn significant attention in spintronics owing to spin-momentum locking where the carriers' spin is oriented perpendicular to their momentum. This property can provide an efficient method to convert charge currents into spin currents, and vice-versa, through the Rashba-Edelstein effect. However, experimental signatures of these surface states to the spin-charge conversion are extremely difficult to disentangle from bulk state contributions. Here, we combine spin- and angle-resolved photo-emission spectroscopy, and time-resolved THz emission spectroscopy to categorically demonstrate that spin-charge conversion arises mainly from the surface state in Bi$_{1-x}$Sb$_x$ ultrathin films, down to few nanometers where confinement effects emerge. We correlate this large conversion efficiency, typically at the level of the bulk spin Hall effect from heavy metals, to the complex Fermi surface obtained from theoretical calculations of the inverse Rashba-Edelstein response. %We demonstrate this for film thickness down to a few nanometers, Both surface state robustness and sizeable conversion efficiency in epitaxial Bi$_{1-x}$Sb$_x$ thin films bring new perspectives for ultra-low power magnetic random-access memories and broadband THz generation.

cond-mat.mtrl-sci↗

arXiv2022

Emission of coherent THz magnons in an antiferromagnetic insulator triggered by ultrafast spin-phonon interactions

Antiferromagnetic materials have been proposed as new types of narrowband THz spintronic devices owing to their ultrafast spin dynamics. Manipulating coherently their spin dynamics, however, remains a key challenge that is envisioned to be accomplished by spin-orbit torques or direct optical excitations. Here, we demonstrate the combined generation of broadband THz (incoherent) magnons and narrowband (coherent) magnons at 1 THz in low damping thin films of NiO/Pt. We evidence, experimentally and through modelling, two excitation processes of magnetization dynamics in NiO, an off-resonant instantaneous optical spin torque and a strain-wave-induced THz torque induced by ultrafast Pt excitation. Both phenomena lead to the emission of a THz signal through the inverse spin Hall effect in the adjacent heavy metal layer. We unravel the characteristic timescales of the two excitation processes found to be < 50 fs and > 300 fs, respectively, and thus open new routes towards the development of fast opto-spintronic devices based on antiferromagnetic materials.

cond-mat.mes-hall↗

arXiv2022

Antiferromagnetic cavity magnon polaritons in collinear and canted phases of hematite

Cavity spintronics explores light matter interactions at the interface between spintronic and quantum phenomena. Until now, studies have focused on the hybridization between ferromagnets and cavity photons.In this article, we realize antiferromagnetic cavity-magnon polaritons. The collective spin motion in single hematite crystals (α-Fe2O3) hybridizes with 18 - 45 GHz microwave cavity photons with required specific symmetries. We show theoretically and experimentally that the photon-magnon coupling in the collinear phase is mediated by the dynamical Neel vector and the weak magnetic moment in the canted phase by measuring across the Morin transition. The coupling strength g is shown to scale with the anisotropy field in the collinear phase and with the Dzyaloshinskii-Moriya field in the canted phase. We achieve a strong coupling regime both in canted (C > 25 at 300 K) and noncolinear phases (C > 4 at 150 K) and thus coherent information exchange with antiferromagnets These results evidence a generic strategy to achieve cavity-magnon polaritons in antiferromagnets for different symmetries, opening the field of cavity spintronics to antiferromagnetic materials.

cond-mat.mes-hall↗

arXiv2022

Ultrafast spin-charge conversion at SnBi$_2$Te$_4$/Co topological insulator interfaces probed by terahertz emission spectroscopy

Spin-to-charge conversion (SCC) involving topological surface states (TSS) is one of the most promising routes for highly efficient spintronic devices for terahertz (THz) emission. Here, the THz generation generally occurs mainly via SCC consisting in efficient dynamical spin injection into spin-locked TSS. In this work, we demonstrate sizable THz emission from a nanometric thick topological insultator (TI)/ferromagnetic junction - SnBi$_2$Te$_4$/Co - specifically designed to avoid bulk band crossing with the TSS at the Fermi level, unlike its parent material Bi$_2$Te$_3$. THz emission time domain spectroscopy (TDS) is used to indicate the TSS contribution to the SCC by investigating the TI thickness and angular dependence of the THz emission. This work illustrates THz emission TDS as a powerful tool alongside angular resolved photoemission spectroscopy (ARPES) methods to investigate the interfacial spintronic properties of TI/ferromagnet bilayers.

cond-mat.mtrl-sci↗

arXiv2022

Spintronic THz emitters based on transition metals and semi-metals/Pt multilayers

Spintronic terahertz (THz) emitters (STE) based on the inverse spin Hall effect in ferromagnetic/heavy metal (FM/HM) heterostructures have become important sources for THz pulse generation. The design, materials and control of these interfaces at the nanometer level has become vital to engineer their THz emission properties.In this work, we present studies of the optimization of such structures through a multi-pronged approach, taking advantage of material and interface engineering to enhance the THz spintronic emission. This includes: the application of multi-stacks of HM/FM junctions and their application to trilayer structures, the use of spin-sinks to simultaneously enhance the THz emitted fields and reduce the use of thick Pt layers to reduce optical absorption, and the use of semi-metals to increase the spin polarization and thus the THz emission. Through these approaches, significant enhancements of the THz field can be achieved. Importantly, taking into account the optical absorption permits to elucidate novel phenomena such as the relation between the spin diffusion length and the spin-sink using THz spectroscopy, as well as possibly distinguishing between self and interface spin-to-charge conversion in semi-metals.

cond-mat.mtrl-sci↗

arXiv2021

Anisotropic long-range spin transport in canted antiferromagnetic orthoferrite YFeO$_3$

In antiferromagnets, the efficient propagation of spin-waves has until now only been observed in the insulating antiferromagnet hematite, where circularly (or a superposition of pairs of linearly) polarized spin-waves propagate over long distances. Here, we report long-distance spin-transport in the antiferromagnetic orthoferrite YFeO$_3$, where a different transport mechanism is enabled by the combined presence of the Dzyaloshinskii-Moriya interaction and externally applied fields. The magnon decay length is shown to exceed hundreds of nano-meters, in line with resonance measurements that highlight the low magnetic damping. We observe a strong anisotropy in the magnon decay lengths that we can attribute to the role of the magnon group velocity in the propagation of spin-waves in antiferromagnets. This unique mode of transport identified in YFeO$_3$ opens up the possibility of a large and technologically relevant class of materials, i.e., canted antiferromagnets, for long-distance spin transport.

cond-mat.str-el↗

arXiv2021

Evidence for spin current driven Bose-Einstein condensation of magnons

The quanta of magnetic excitations - magnons - are known for their unique ability to undergo Bose-Einstein condensation at room temperature. This fascinating phenomenon reveals itself as a spontaneous formation of a macroscopic coherent state under the influence of incoherent stimuli. Spin currents have been predicted to offer electronic control of magnon Bose-Einstein condensates, but this phenomenon has not been experimentally evidenced up to now. Here we experimentally show that current-driven Bose-Einstein condensation can be achieved in nanometer-thick films of magnetic insulators with tailored dynamic magnetic nonlinearities and minimized magnon-magnon interactions. We demonstrate that, above a certain threshold, magnons injected by the spin current overpopulate the lowest-energy level forming a highly coherent spatially extended state. By accessing magnons with essentially different energies, we quantify the chemical potential of the driven magnon gas and show that, at the critical current, it reaches the energy of the lowest magnon level. Our results pave the way for implementation of integrated microscopic quantum magnonic and spintronic devices.

cond-mat.mes-hall↗

arXiv2021

Roadmap on Spin-Wave Computing

Magnonics is a field of science that addresses the physical properties of spin waves and utilizes them for data processing. Scalability down to atomic dimensions, operations in the GHz-to-THz frequency range, utilization of nonlinear and nonreciprocal phenomena, and compatibility with CMOS are just a few of many advantages offered by magnons. Although magnonics is still primarily positioned in the academic domain, the scientific and technological challenges of the field are being extensively investigated, and many proof-of-concept prototypes have already been realized in laboratories. This roadmap is a product of the collective work of many authors that covers versatile spin-wave computing approaches, conceptual building blocks, and underlying physical phenomena. In particular, the roadmap discusses the computation operations with Boolean digital data, unconventional approaches like neuromorphic computing, and the progress towards magnon-based quantum computing. The article is organized as a collection of sub-sections grouped into seven large thematic sections. Each sub-section is prepared by one or a group of authors and concludes with a brief description of the current challenges and the outlook of the further development of the research directions.

physics.app-ph↗

arXiv2021

Size-dependent enhancement of passive microwave rectification in magnetic tunnel junctions with perpendicular magnetic anisotropy

Spintronic rf detectors were demonstrated, recently, for energy harvesting and wireless communication at low input power. Here we report on the optimization of the rectified output dc voltage using magnetic tunnel junctions (MTJ) with strong perpendicular anisotropy (PMA) of both the polarizing and the free layer. The magnetization of the polarizing layer is fixed out of plane, while the free layer thickness is adjusted so that its magnetization orientation changes from in plane to out of plane. The rectification dc output voltage lies in the mV range for moderate rf powers, with a signal to noise ratio of 10 to 100 for Prf = -25dBm. It shows a strong dependence on the dimensions of the MTJ: it increases by a factor of 5 to 6 when reducing the diameter from 150nm to 20nm. This enhancement can be doubled when reducing the FL thickness from 1.8nm to 1.6nm. This dimensional enhancement is attributed to the change of the effective anisotropy of the excited free layer, and the MTJ resistance. The results are of interest for the design of spintronic based rf detectors with optimized sensitivity.

cond-mat.mes-hall↗

arXiv2021

Magnon Transport in the Presence of Antisymmetric Exchange in a Weak Antiferromagnet

The Dzyaloshinskii-Moriya interaction (DMI) is at the heart of many modern developments in the research field of spintronics. DMI is known to generate noncollinear magnetic textures, and can take two forms in antiferromagnets: homogeneous or inter-sublattice, leading to small, canted moments and inhomogeneous or intra-sublattice, leading to formation of chiral structures. In this work, we first determine the strength of the effective field created by the DMI, using SQUID based magnetometry and transport measurements, in thin films of the antiferromagnetic iron oxide hematite, $α$-Fe$_2$O$_3$. We demonstrate that DMI additionally introduces reconfigurability in the long distance magnon transport in these films under different orientations of a magnetic field. This arises as a hysteresis centred around the easy-axis direction for an external field rotated in opposing directions whose width decreases with increasing magnetic field as the Zeeman energy competes with the effective field created by the DMI.

cond-mat.mtrl-sci↗

arXiv2021

Dispersionless propagation of ultra-short spin-wave pulses in ultrathin yttrium iron garnet waveguides

We study experimentally the propagation of nanosecond spin-wave pulses in microscopic waveguides made of nanometer-thick yttrium iron garnet films. For these studies, we use micro-focus Brillouin light scattering spectroscopy, which provides the possibility to observe propagation of the pulses with high spatial and temporal resolution. We show that, for most spin-wave frequencies, dispersion leads to broadening of the pulse by several times at propagation distances of 10 micrometers. However, for certain frequency interval, the dispersion broadening is suppressed almost completely resulting in a dispersionless pulse propagation. We show that the formation of the dispersion-free region is caused by the competing effects of the dipolar and the exchange interaction, which can be controlled by the variation of the waveguide geometry. These conclusions are supported by micromagnetic simulations and analytical calculations. Our findings provide a simple solution for the implementation of high-speed magnonic systems that require undisturbed propagation of short information-carrying spin-wave pulses.

cond-mat.mes-hall↗

arXiv2021

Exceptional sign changes of the non-local spin Seebeck effect in antiferromagnetic hematite

Low power spintronic devices based on the propagation of pure magnonic spin currents in antiferromagnetic insulator materials offer several distinct advantages over ferromagnetic components including higher frequency magnons and a stability against disturbing external magnetic fields. In this work, we make use of the insulating antiferromagnetic phase of iron oxide, the mineral hematite $α$-Fe$_2$O$_3$ to investigate the long distance transport of thermally generated magnonic spin currents. We report on the excitation of magnons generated by the spin Seebeck effect, transported both parallel and perpendicular to the antiferromagnetic easy-axis under an applied magnetic field. Making use of an atomistic hematite toy model, we calculate the transport characteristics from the deviation of the antiferromagnetic ordering from equilibrium under an applied field. We resolve the role of the magnetic order parameters in the transport, and experimentally we find significant thermal spin transport without the need for a net magnetization.

cond-mat.mtrl-sci↗

arXiv2021

Room temperature antiferromagnetic resonance and inverse spin-Hall voltage in canted antiferromagnets

We study theoretically and experimentally the spin pumping signals induced by the resonance of canted antiferromagnets with Dzyaloshinskii-Moriya interaction and demonstrate that they can generate easily observable inverse spin-Hall voltages. Using a bilayer of hematite/heavy metal as a model system, we measure at room temperature the antiferromagnetic resonance and an associated inverse spin-Hall voltage, as large as in collinear antiferromagnets. As expected for coherent spin-pumping, we observe that the sign of the inverse spin-Hall voltage provides direct information about the mode handedness as deduced by comparing hematite, chromium oxide and the ferrimagnet Yttrium-Iron Garnet. Our results open new means to generate and detect spin-currents at terahertz frequencies by functionalizing antiferromagnets with low damping and canted moments.

cond-mat.mes-hall↗