arXiv subjects

R. Lebrun

Publications and source records attributed to R. Lebrun.

31 records · Page 2Linked to original sources

arXiv2021

Effective strain manipulation of the antiferromagnetic state of polycrystalline NiO

As a candidate material for applications such as magnetic memory, polycrystalline antiferromagnets offer the same robustness to external magnetic fields, THz spin dynamics, and lack of stray field as their single crystalline counterparts, but without the limitation of epitaxial growth and lattice matched substrates. Here, we first report the detection of the average Neel vector orientiation in polycrystalline NiO via spin Hall magnetoresistance (SMR). Secondly, by applying strain through a piezo-electric substrate, we reduce the critical magnetic field required to reach a saturation of the SMR signal, indicating a change of the anisotropy. Our results are consistent with polycrystalline NiO exhibiting a positive sign of the in-plane magnetostriction. This method of anisotropy-tuning offers an energy efficient, on-chip alternative to manipulate a polycrystalline antiferromagnets magnetic state.

cond-mat.mtrl-sci↗

arXiv2020

Ultrafast spin-currents and charge conversion at 3d-5d interfaces probed by time-domain terahertz spectroscopy

Spintronic structures are extensively investigated for their spin orbit torque properties, required for magnetic commutation functionalities. Current progress in these materials is dependent on the interface engineering for the optimization of spin transmission. Here, we advance the analysis of ultrafast spin-charge conversion phenomena at ferromagnetic-transition metal interfaces due to their inverse spin-Hall effect properties. In particular the intrinsic inverse spin Hall effect of Pt-based systems and extrinsic inverse spin-Hall effect of Au:W and Au:Ta in NiFe/Au:(W,Ta) bilayers are investigated. The spin-charge conversion is probed by complementary techniques -- ultrafast THz time domain spectroscopy in the dynamic regime for THz pulse emission and ferromagnetic resonance spin-pumping measurements in the GHz regime in the steady state -- to determine the role played by the material properties, resistivities, spin transmission at metallic interfaces and spin-flip rates. These measurements show the correspondence between the THz time domain spectroscopy and ferromagnetic spin-pumping for the different set of samples in term of the spin mixing conductance. The latter quantity is a critical parameter, determining the strength of the THz emission from spintronic interfaces. This is further supported by ab-initio calculations, simulations and analysis of the spin-diffusion and spin relaxation of carriers within the multilayers in the time domain, permitting to determine the main trends and the role of spin transmission at interfaces. This work illustrates that time domain spectroscopy for spin-based THz emission is a powerful technique to probe spin-dynamics at active spintronic interfaces and to extract key material properties for spin-charge conversion.

physics.app-ph↗

arXiv2019

Spin structure and spin Hall magnetoresistance of epitaxial thin films of the insulating non-collinear antiferromagnet SmFeO$_3$

We report a combined study of imaging the antiferromagnetic (AFM) spin structure and measuring the spin Hall magnetoresistance (SMR) in epitaxial thin films of the insulating non-collinear antiferromagnet SmFeO$_3$. X-ray magnetic linear dichroism photoemission electron microscopy measurements reveal that the AFM spins of the SmFeO$_3$(110) align in the plane of the film. Angularly dependent magnetoresistance measurements show that SmFeO$_3$/Ta bilayers exhibit a positive SMR, in contrast to the negative SMR expected in previously studied collinear AFMs. The SMR amplitude increases linearly with increasing external magnetic field at higher magnetic field, suggesting that field-induced canting of the AFM spins plays an important role. In contrast, around the coercive field, no detectable SMR signal is observed, indicating that SMR of AFM and canting magnetization components cancel out. Below 50~K, the SMR amplitude increases sizably by a factor of two as compared to room temperature, which likely correlates with the long-range ordering of the Sm ions. Our results show that the SMR is a sensitive technique for non-equilibrium spin system of non-collinear AFM systems.

cond-mat.mtrl-sci↗

arXiv2019

Enhancing the injection locking range of spin torque oscillators through mutual coupling

We investigate how the ability of the vortex oscillation mode of a spin-torque nano-oscillator to lock to an external microwave signal is modified when it is coupled to another oscillator. We show experimentally that mutual electrical coupling can lead to locking range enhancements of a factor 1.64. Furthermore, we analyze the evolution of the locking range as a function of the coupling strength through experiments and numerical simulations. By uncovering the mechanisms at stake in the locking range enhancement, our results will be useful for designing spin-torque nano-oscillators arrays with high sensitivities to external microwave stimuli.

cond-mat.mes-hall↗

arXiv2018

Electrically controlled long-distance spin transport through an antiferromagnetic insulator

Spintronics uses spins, the intrinsic angular momentum of electrons, as an alternative for the electron charge. Its long-term goal is in the development of beyond-Moore low dissipation technology devices. Recent progress demonstrated the long-distance transport of spin signals across ferromagnetic insulators. Antiferromagnetically ordered materials are however the most common class of magnetic materials with several crucial advantages over ferromagnetic systems. In contrast to the latter, antiferromagnets exhibit no net magnetic moment, which renders them stable and impervious to external fields. In addition, they can be operated at THz frequencies. While fundamentally their properties bode well for spin transport, previous indirect observations indicate that spin transmission through antiferromagnets is limited to short distances of a few nanometers. Here we demonstrate the long-distance, over tens of micrometers, propagation of spin currents through hematite (α-Fe2O3), the most common antiferromagnetic iron oxide, exploiting the spin Hall effect for spin injection. We control the spin current flow by the interfacial spin-bias and by tuning the antiferromagnetic resonance frequency with an external magnetic field. This simple antiferromagnetic insulator is shown to convey spin information parallel to the compensated moment (Néel order) over distances exceeding tens of micrometers. This newly-discovered mechanism transports spin as efficiently as the net magnetic moments in the best-suited complex ferromagnets. Our results pave the way to ultra-fast, low-power antiferromagnet-insulator-based spin-logic devices that operate at room temperature and in the absence of magnetic fields.

cond-mat.mes-hall↗

arXiv2016

Driven energy transfer between coupled modes in spin-torque oscillators

The mutual interaction between the different eigenmodes of a spin-torque oscillator can lead to a large variety of physical mechanisms from mode hopping to multi-mode generation, that usually reduce their performances as radio-frequency devices. To tackle this issue for the future applications, we investigate the properties of a model spin-torque oscillator that is composed of two coupled vortices with one vortex in each of the two magnetic layers of the oscillator. In such double-vortex system, the remarkable properties of energy transfer between the coupled modes, one being excited by spin transfer torque while the second one being damped, result into an alteration of the damping parameters. As a consequence, the oscillator nonlinear behavior is concomitantly drastically impacted. This efficient coupling mechanism, driven mainly by the dynamic dipolar field generated by the spin transfer torque induced motion of the vortices, gives rise to an unexpected dynamical regime of self-resonance excitation. These results show that mode coupling can be leveraged for controlling the synchronization process as well as the frequency tunability of spin-torque oscillators.

cond-mat.mes-hall↗

arXiv2016

Controlling the phase locking of unstable magnetic bits for ultra-low power computation

When fabricating magnetic memories, one of the main challenges is to maintain the bit stability while downscaling. Indeed, for magnetic volumes of a few thousand nm3, the energy barrier between magnetic configurations becomes comparable to the thermal energy at room temperature. Then, switches of the magnetization spontaneously occur. These volatile, superparamagnetic nanomagnets are generally considered useless. But what if we could use them as low power computational building blocks? Remarkably, they can oscillate without the need of any external dc drive, and despite their stochastic nature, they can beat in unison with an external periodic signal. Here we show that the phase locking of superparamagnetic tunnel junctions can be induced and suppressed by electrical noise injection. We develop a comprehensive model giving the conditions for synchronization, and predict that it can be achieved with a total energy cost lower than 10-^13 J. Our results open the path to ultra-low power computation based on the controlled synchronization of oscillators.

cond-mat.mtrl-sci↗

arXiv2016

Mutual synchronization of spin torque nano-oscillators through a non-local and tunable electrical coupling

The concept of spin torque driven high frequency magnetization dynamics has opened up the field of spintronics to non-linear physics, potentially in complex networks of dynamical systems. In the scarce demonstrations of synchronized spin-torque oscillators, the local nature of the magnetic coupling that is used have largely hampered a good understanding and thus the control of the synchronization process. Here we take advantage of the non-local nature of an electrical coupling to mutually synchronize spin-torque oscillators through their self-emitted microwave currents. The control of the synchronized state is achieved at the nanoscale through two active components of spin transfer torques, but also externally through an electrical delay line. These additional levels of control of the synchronization capability provide new approaches to underlie a large variety of nanoscale collective dynamics in complex networks.

cond-mat.mes-hall↗

arXiv2015

Efficient Synchronization of Dipolarly Coupled Vortex-Based Spin Transfer Nano-Oscillators

Due to their nonlinear properties, spin transfer nano-oscillators can easily adapt their frequency to external stimuli. This makes them interesting model systems to study the effects of synchronization and brings some opportunities to improve their microwave characteristics in view of their applications in information and communication technologies and to design innovative computing architectures. So far, mutual synchronization of spin transfer nano-oscillators through propagating spin-waves and exchange coupling in a common magnetic layer has been demonstrated. Here we show that the dipolar interaction is also an efficient mechanism to synchronize neighbouring oscillators. We experimentally study a pair of vortex-based spin-transfer nano-oscillators, in which mutual synchronization can be achieved despite a significant frequency mismatch between oscillators. Importantly, the coupling efficiency is controlled by the magnetic configuration of the vortices, as confirmed by an analytical model highlighting the physics at play in the synchronization process as well as by micromagnetic simulations.

cond-mat.mes-hall↗

arXiv2015

Self-injection locking of a vortex spin torque oscillator by delayed feedback

The self-synchronization of spin torque oscillators is investigated experimentally by re-injecting its radiofrequency (rf) current after a certain delay time. We demonstrate that the emission power and the spectral linewidth are improved for optimal delay times. Moreover by varying the phase difference between the emitted power and the re-injected one, we find a clear oscillatory dependence with a 2π periodicity of the frequency of the oscillator as well as its power and linewidth. Such periodical behavior within the self-injection regime is well described by the general model of nonlinear auto-oscillators including not only a delayed rf current but also all spin torque forces responsible for the self-synchronization. Our results reveal new approaches for controlling the non-autonomous dynamics of spin torque oscillators, a key issue for rf spintronics applications as well as for the development of neuro-inspired spin-torque oscillators based devices.

cond-mat.mes-hall↗

arXiv2015

Optimizing magneto-dipolar interactions for synchronizing vortex based spin-torque nano-oscillators

We report on a theoretical study about the magneto-dipolar coupling and synchronization between two vortex-based spin-torque nano-oscillators. In this work we study the dependence of the coupling efficiency on the relative magnetization parameters of the vortices in the system. For that purpose, we combine micromagnetic simulations, Thiele equation approach, and analytical macro-dipole approximation model to identify the optimized configuration for achieving phase-locking between neighboring oscillators. Notably, we compare vortices configurations with parallel (P) polarities and with opposite (AP) polarities. We demonstrate that the AP core configuration exhibits a coupling strength about three times larger than in the P core configuration.

cond-mat.mes-hall↗

arXiv2015

Spin torque resonant vortex core expulsion for an efficient radio-frequency detection scheme

Spin-polarised radio-frequency currents, whose frequency is equal to that of the gyrotropic mode, will cause an excitation of the core of a magnetic vortex confined in a magnetic tunnel junction. When the excitation radius of the vortex core is greater than that of the junction radius, vortex core expulsion is observed, leading to a large change in resistance, as the layer enters a predominantly uniform magnetisation state. Unlike the conventional spin-torque diode effect, this highly tunable resonant effect will generate a voltage which does not decrease as a function of rf power, and has the potential to form the basis of a new generation of tunable nanoscale radio-frequency detectors.

cond-mat.mes-hall↗

arXiv2015

Understanding of phase noise squeezing under fractional synchronization of non-linear spin transfer vortex oscillator

We investigate experimentally the synchronization of a vortex based spin transfer oscillator to an external rf current whose frequency is at multiple integers, as well as half integer, of the oscillator frequency. Through a theoretical study of the locking process, we highlight both the crucial role of the symmetries of the spin torques acting on the magnetic vortex and the nonlinear properties of the oscillator on the phase locking process. Through the achievement of a perfect injection locking state, we report a record phase noise reduction down to -90dBc/Hz at 1 kHz offset frequency. The phase noise of these nanoscale oscillators is demonstrating as being low and controllable which is of significant importance for real applications using spin transfer devices.

cond-mat.mes-hall↗