arXiv subjects

R. Moessner

Publications and source records attributed to R. Moessner.

At least 37 records · Page 2Linked to original sources

arXiv2018

Zero point fluctuations for magnetic spirals and Skyrmions, and the fate of the Casimir energy in the continuum limit

We study the role of zero-point quantum fluctuations in a range of magnetic states which on the classical level are close to spin-aligned ferromagnets. These include Skyrmion textures characterized by non-zero topological charge, and topologically-trivial spirals arising from the competition of the Heisenberg and Dzyaloshinskii-Moriya interactions. For the former, we extend our previous results on quantum exactness of classical Bogomolny-Prasad-Sommerfield (BPS) ground-state degeneracies to the general case of Kähler manifolds, with a specific example of Grassmann manifolds $\mathrm{Gr(M,N)}$. These are relevant to quantum Hall ferromagnets with $\mathrm{N}$ internal states and integer filling factor $\mathrm{M}$. A promising candidate for their experimental implementation is monolayer graphene with $\mathrm{N=4}$ corresponding to spin and valley degrees of freedom at the charge neutrality point with $\mathrm{M=2}$ filled Landau levels. We find that the vanishing of the zero-point fluctuations in taking the continuum limit occurs differently in the case of BPS states compared to the case of more general smooth textures, with the latter exhibiting more pronounced lattice effects. This motivates us to consider the vanishing of zero-point fluctuations in such near-ferromagnets more generally. We present a family of lattice spin models for which the vanishing of zero-point fluctuations is evident, and show that some spirals can be thought of as having nonzero but weak zero-point fluctuations on account of their closeness to this family. Between them, these instances provide concrete illustrations of how the Casimir energy, dependent on the full UV-structure of the theory, evolves as the continuum limit is taken.

cond-mat.str-el↗

arXiv2018

Inverted hysteresis and negative remanence in a homogeneous antiferromagnet

Magnetic remanence - found in bar magnets or magnetic storage devices - is probably the oldest and most ubiquitous phenomenon underpinning technological applications of magnetism. It is a macroscopic non-equilibrium phenomenon: a remanent magnetisation appears when a magnetic field is applied to an initially unmagnetised ferromagnet, and then taken away. Here, we present an inverted magnetic hysteresis loop in the pyrochlore compound Nd$_2$Hf$_2$O$_7$: the remanent magnetisation points in a direction opposite to the applied field. This phenomenon is exquisitely tunable as a function of the protocol in field and temperature, and it is reproducible as in a quasi-equilibrium setting. We account for this phenomenon in considerable detail in terms of the properties of non-equilibrium population of domain walls which exhibit a magnetic moment between domains of an ordered antiferromagnetic state which itself has zero net magnetisation. Properties and (non-equilibrium) dynamics of topological defects play an important role in modern spintronics, and our study adds an instance where a uniform field couples selectively to domain walls rather than the bulk.

cond-mat.str-el↗

arXiv2018

Topological Magnons in Kitaev Magnets at High Fields

We study the Kitaev-Heisenberg-$Γ$-$Γ'$ model that describes the magnetism in strong spin-orbit coupled honeycomb lattice Mott insulators. In strong $[111]$ magnetic fields that bring the system into the fully polarized paramagnetic phase, we find that the spin wave bands carry nontrivial Chern numbers over large regions of the phase diagram implying the presence of chiral magnon edge states. In contrast to other topological magnon systems, the topological nontriviality of these systems results from the presence of magnon number non-conserving terms in the Hamiltonian. Since the effects of interactions are suppressed by $J/h$, the validity of the single particle picture is tunable making paramagnetic phases particularly suitable for the exploration of this physics. Using time dependent DMRG and interacting spin wave theory, we demonstrate the presence of the chiral edge mode and its evolution with field.

cond-mat.str-el↗

arXiv2017

Neutron Scattering Signatures of Magnon Weyl Points

We study the inelastic neutron scattering cross section in the vicinity of touching points in magnon bands. Among the possible touching points are magnon Weyl points in three dimensional ordered magnets with significant spin-orbit coupling that are characterized by a linear dispersion in their vicinity. A Weyl point is topologically protected by its net chirality and here we show that this leads to a characteristic form for the dynamical structure factor. To address this question, we show that scattering intensities in the vicinity of arbitrary magnon two-band touching points are identical to expectation values of the pseudospin polarization along some direction $\hat{\boldsymbol{n}}$ in momentum space fixed by the magnetic Hamiltonian. This approach applied to Weyl points shows that they are singular points in the intensity of the form $\hat{\boldsymbol{n}}\cdot δ\hat{\boldsymbol{k}}$ regardless of the magnetic ground state. We make specific predictions for the experimental signatures of such intensity singularities in several spin models hosting Weyl magnons applicable to candidate materials.

cond-mat.str-el↗

arXiv2017

Classical Dynamics of Harmonically Trapped Interacting Particles

Motivated by current interest in the dynamics of trapped quantum gases, we study the microcanonical dynamics of a trapped one-dimensional gas of classical particles interacting via a finite-range repulsive force of tunable strength. We examine two questions which have been of interest in quantum dynamics: (1) the breathing mode (size oscillation) dynamics of the trapped gas and the dependence of the breathing frequency on the interaction strength, and (2) the long-time relaxation and possible thermalization of the finite isolated gas. We show that the breathing mode frequency has non-monotonic dependence on the magnitude of the mutual repulsion, decreasing for small interactions and increasing for larger interactions. We explain these dependences in terms of slowing-down or speeding-up effects of two-body collision processes. We find that the gas thermalizes within a reasonable finite timescale in the sense of single-particle energies acquiring a Boltzmann distribution, only when the interaction strength is large compared to the energy per particle.

cond-mat.stat-mech↗

arXiv2017

Excitations in the field-induced quantum spin liquid state of alpha-RuCl3

The Kitaev model on a honeycomb lattice predicts a paradigmatic quantum spin liquid (QSL) exhibiting Majorana Fermion excitations. The insight that Kitaev physics might be realized in practice has stimulated investigations of candidate materials, recently including alpha-RuCl3. In all the systems studied to date, non-Kitaev interactions induce magnetic order at low temperature. However, in-plane magnetic fields of roughly 8 Tesla suppress the long-range magnetic order in alpha-RuCl3 raising the intriguing possibility of a field-induced QSL exhibiting non-Abelian quasiparticle excitations. Here we present inelastic neutron scattering in alpha-RuCl3 in an applied magnetic field. At a field of 8 Tesla, the spin waves characteristic of the ordered state vanish throughout the Brillouin zone. The remaining single dominant feature of the response is a broad continuum centered at the Gamma point, previously identified as a signature of fractionalized excitations. This provides compelling evidence that a field-induced QSL state has been achieved.

cond-mat.mtrl-sci↗

arXiv2017

Clustering in Hilbert space of a quantum optimization problem

The solution space of many classical optimization problems breaks up into clusters which are extensively distant from one another in the Hamming metric. Here, we show that an analogous quantum clustering phenomenon takes place in the ground state subspace of a certain quantum optimization problem. This involves extending the notion of clustering to Hilbert space, where the classical Hamming distance is not immediately useful. Quantum clusters correspond to macroscopically distinct subspaces of the full quantum ground state space which grow with the system size. We explicitly demonstrate that such clusters arise in the solution space of random quantum satisfiability (3-QSAT) at its satisfiability transition. We estimate both the number of these clusters and their internal entropy. The former are given by the number of hardcore dimer coverings of the core of the interaction graph, while the latter is related to the underconstrained degrees of freedom not touched by the dimers. We additionally provide new numerical evidence suggesting that the 3-QSAT satisfiability transition may coincide with the product satisfiability transition, which would imply the absence of an intermediate entangled satisfiable phase.

quant-ph↗

arXiv2017

Equilibration and Order in Quantum Floquet Matter

Equilibrium theormodynamics is characterized by two fundamental ideas: thermalisation--that systems approach a late time thermal state; and phase structure--that thermal states exhibit singular changes as various parameters characterizing the system are changed. We summarise recent progress that has established generalizations of these ideas to periodically driven, or Floquet, closed quantum systems. This has resulted in the discovery of entirely new phases which exist only out of equilibrium, such as the $π$-spin glass or Floquet time crystal.

cond-mat.dis-nn↗

arXiv2016

Quasiparticle interference from different impurities on the surface of pyrochlore iridates: signatures of the Weyl phase

Weyl semimetals are gapless three-dimensional topological materials where two bands touch at an even number of points in the bulk Brillouin zone. These semimetals exhibit topologically protected surface Fermi arcs, which pairwise connect the projected bulk band touchings in the surface Brillouin zone. Here, we analyze the quasiparticle interference patterns of the Weyl phase when time-reversal symmetry is explicitly broken. We use a multi-band $d$-electron Hubbard Hamiltonian on a pyrochlore lattice, relevant for the pyrochlore iridate R$_2$Ir$_2$O$_7$ (where R is a rare earth). Using exact diagonalization, we compute the surface spectrum and quasiparticle interference (QPI) patterns for various surface terminations and impurities. We show that the spin and orbital texture of the surface states can be inferred from the absence of certain backscattering processes and from the symmetries of the QPI features for non-magnetic and magnetic impurities. Furthermore, we show that the QPI patterns of the Weyl phase in pyrochlore iridates may exhibit additional interesting features that go beyond those found previously in TaAs.

cond-mat.str-el↗

arXiv2016

A fractionalised "$\mathbb{Z}_2$" classical Heisenberg spin liquid

Quantum spin systems are by now known to exhibit a large number of different classes of spin liquid phases. By contrast, for \textit{classical} Heisenberg models, only one kind of fractionalised spin liquid phase, the so-called Coulomb or $U(1)$ spin liquid, has until recently been identified: this exhibits algebraic spin correlations and impurity moments, `orphan spins', whose size is a fraction of that of the underlying microscopic degrees of freedom. Here, we present two Heisenberg models exhibiting fractionalisation in combination with exponentially decaying correlations. These can be thought of as a classical continuous spin version of a $\mathbb{Z}_2$ spin liquid. Our work suggests a systematic search and classification of classical spin liquids as a worthwhile endeavour.

cond-mat.str-el↗

arXiv2016

Spin glass behavior in a random Coulomb antiferromagnet

We study spin glass behavior in a random Ising Coulomb antiferromagnet in two and three dimensions using Monte Carlo simulations. In two dimensions, we find a transition at zero temperature with critical exponents consistent with those of the Edwards Anderson model, though with large uncertainties. In three dimensions, evidence for a finite-temperature transition, as occurs in the Edwards-Anderson model, is rather weak. This may indicate that the sizes are too small to probe the asymptotic critical behavior, or possibly that the universality class is different from that of the Edwards-Anderson model and has a lower critical dimension equal to three.

cond-mat.dis-nn↗

arXiv2016

Majorana spectroscopy of 3D Kitaev spin-liquids

We analyse the dynamical response of a range of 3D Kitaev quantum spin-liquids, using lattice models chosen to explore the different possible low-energy spectra for gapless Majorana fermions, with either Fermi surfaces, nodal lines or Weyl points. We find that the behaviour of the dynamical structure factor is distinct in all three cases, reflecting the quasiparticle density of states in two fundamentally different ways. First, the low-energy response is either straightforwardly related to the power with which the low-energy density of states vanishes; or for a non-vanishing density of states, to the phase shifts encountered in the corresponding X-ray edge problem, whose phenomenology we extend to the case of Majorana fermions. Second, at higher energies, there is a rich fine-structure, determined by microscopic features of the Majorana spectrum. Our theoretical results test the usefulness of inelastic neutron scattering as a probe of these quantum spin liquids: we find that although spin flips fractionalise, the main features of the dynamical spin response nevertheless admit straightforward interpretations in terms of Majorana and flux loop excitations.

cond-mat.str-el↗

arXiv2016

Maxwell electromagnetism as an emergent phenomenon in condensed matter

The formulation of a complete theory of classical electromagnetism by Maxwell is one of the milestones of science. The capacity of many-body systems to provide emergent mini-universes with vacua quite distinct from the one we inhabit was only recognised much later. Here, we provide an account of how simple systems of localised spins manage to emulate Maxwell electromagnetism in their low-energy behaviour. They are much less constrained by symmetry considerations than the relativistically invariant electromagnetic vacuum, as their substrate provides a non-relativistic background with even translational invariance broken. They can exhibit rich behaviour not encountered in conventional electromagnetism. This includes the existence of magnetic monopole excitations arising from fractionalisation of magnetic dipoles; as well as the capacity of disorder, by generating defects on the lattice scale, to produce novel physics, as exemplified by topological spin glassiness or random Coulomb magnetism.

cond-mat.str-el↗

arXiv2016

Low-field behavior of an XY pyrochlore antiferromagnet: emergent clock anisotropies

Using $\rm Er_2Ti_2O_7$ as a motivation, we investigate finite-field properties of $XY$ pyrochlore antiferromagnets. In addition to a fluctuation-induced six-fold anisotropy present in zero field, an external magnetic field induces a combination of two-, three-, and six-fold clock terms as a function of its orientation providing for a rich and controllable magnetothermodynamics. For $\rm Er_2Ti_2O_7$, we predict a new phase transition for ${\bf H}\parallel [001]$. Re-entrant transitions are also found for ${\bf H}\parallel [111]$. We extend these results to the whole family the $XY$ pyrochlore antiferromagnets and show that presence and number of low-field transitions for different orientations can be used for locating a given material in the parameter space of anisotropic pyrochlores. Finite-temperature classical Monte Carlo simulations serve to confirm and illustrate these analytic predictions.

cond-mat.str-el↗

arXiv2016

Fermionic response from fractionalization in an insulating two-dimensional magnet

Conventionally ordered magnets possess bosonic elementary excitations, called magnons. By contrast, no magnetic insulators in more than one dimension are known whose excitations are not bosons but fermions. Theoretically, some quantum spin liquids (QSLs) -- new topological phases which can occur when quantum fluctuations preclude an ordered state -- are known to exhibit Majorana fermions as quasiparticles arising from fractionalization of spins. Alas, despite much searching, their experimental observation remains elusive. Here, we show that fermionic excitations are remarkably directly evident in experimental Raman scattering data across a broad energy and temperature range in the two-dimensional material $α$-RuCl$_3$. This shows the importance of magnetic materials as hosts of Majorana fermions. In turn, this first systematic evaluation of the dynamics of a QSL at finite temperature emphasizes the role of excited states for detecting such exotic properties associated with otherwise hard-to-identify topological QSLs.

cond-mat.str-el↗

arXiv2016

Large and exact quantum degeneracy in a Skyrmion magnet

We identify a large family of ground states of a topological Skyrmion magnet whose classical degeneracy persists to all orders in a semiclassical expansion. This goes along with an exceptional robustness of the concomitant ground state configurations, which are not at all dressed by quantum fluctuations. We trace these twin observations back to a common root: this class of topological ground states saturates a Bogomolny inequality. A similar phenomenology occurs in high-energy physics for some field theories exhibiting supersymmetry. We propose quantum Hall ferromagnets, where these Skyrmions configurations arise naturally as ground states away from integer filling, as the best available laboratory realisations.

cond-mat.str-el↗

arXiv2016

Kagome chiral spin liquid as a gauged U(1) symmetry protected topological phase

While the existence of a chiral spin liquid (CSL) on a class of spin-1/2 kagome antiferromagnets is by now well-established numerically, a controlled theoretical path from the lattice model leading to a low energy topological field theory is still lacking. This we provide via an explicit construction, starting from reformulating a microscopic model for a CSL as a lattice gauge theory, and deriving the low-energy form of its continuum limit. A crucial ingredient is the realisation that the bosonic spinons of the gauge theory exhibit a $U(1)$ symmetry-protected topological (SPT) phase, which upon promoting its $U(1)$ global symmetry to a local gauge structure ("gauging") yields the CSL. We suggest that such an explicit lattice-based construction involving gauging of an SPT phase can be applied more generally to understand topological spin liquids.

cond-mat.str-el↗

arXiv2015

Vacancies in the Kitaev quantum spin liquids on the 3D hyper-honeycomb lattice

We study the effect of adding disorder to the exactly solvable Kitaev model on the hyper-honeycomb lattice, which hosts both gapped and gapless spin liquid phases with an emergent $\mathbb{Z}_2$ gauge field. The latter has an unusual gapless spectrum of Majorana fermion excitations, with a co-dimension-two Fermi ring. We thus address the question of the interplay of topological physics and disorder by considering the properties of isolated single and pair of vacancies. We show that near the vacancies, the local magnetic response to a field $h_z$ is parametrically enhanced in comparison to the pristine bulk. Unlike the previously studied case of the 2D honeycomb Kitaev model, the vacancies do not bind a flux of the $\mathbb{Z}_2$ gauge field. In the gapped phase, an isolated vacancy gives rise to effectively free spin-half moments with a non-universal coupling to an external field. In the gapless phase, the low-field magnetization is suppressed parametrically, to $(-\ln h_z)^{-1/2}$ because of interactions with the surrounding spin-liquid. We also show that a pair of vacancies is subject to a sublattice-dependent interaction on account of coupling through the bulk spin liquid, which is spatially anisotropic even when all Kitaev couplings have equal strength. This coupling is thus exponentially suppressed with distance in the gapped phase. In the gapless phase, two vacancies on the same (opposite) sublattice exhibit an enhanced (suppressed) low-field response, amounting to an effectively (anti-)ferromagnetic interaction.

cond-mat.str-el↗