arXiv subjects

R. Moessner

Publications and source records attributed to R. Moessner.

At least 55 records · Page 3Linked to original sources

arXiv2015

Classical spin-liquid on the maximally frustrated honeycomb lattice

We show that the honeycomb Heisenberg antiferromagnet with $J_1/2=J_2=J_3$, where $J_{1/2/3}$ are first-, second- and third-neighbour couplings respectively, forms a classical spin liquid with pinch-point singularities in the structure factor at the Brillouin zone corners. Upon dilution with non-magnetic ions, fractionalised degrees of freedom carrying $1/3$ of the free moment emerge. Their effective description in the limit of low-temperature is that of spins randomly located on a triangular lattice, with a frustrated interaction of long-ranged logarithmic form. The XY version of this magnet exhibits nematic thermal order by disorder, which comes with a clear experimental diagnostic.

cond-mat.str-el↗

arXiv2015

Bosonic Integer Quantum Hall effect in an interacting lattice model

We study a bosonic model with correlated hopping on a honeycomb lattice, and show that its ground state is a bosonic integer quantum Hall (BIQH) phase, a prominent example of a symmetry protected topological (SPT) phase. By using the infinite density matrix renormalization group method, we establish the existence of the BIQH phase by providing clear numerical evidence: (i) a quantized Hall conductance with $|σ_{xy}|= 2$ (ii) two counter propagating gapless edge modes. Our simple model is an example of a novel class of systems that can stabilize SPT phases protected by a continuous symmetry on lattices and opens up new possibilities for the experimental realization of these exotic phases.

cond-mat.str-el↗

arXiv2015

Neutron scattering signatures of the 3D hyper-honeycomb Kitaev quantum spin-liquid

Motivated by recent synthesis of the hyper-honeycomb material $β$-$\mathrm{Li_2 Ir O_3}$, we study the dynamical structure factor (DSF) of the corresponding 3D Kitaev quantum spin-liquid (QSL), whose fractionalised degrees of freedom are Majorana fermions and emergent flux-loops. Properties of this 3D model are known to differ in important ways from those of its 2D counterpart -- it has finite-temperature phase transition, as well as distinct features in Raman response. We show, however, that the qualitative behaviour of the DSF is broadly dimension-independent. Characteristics of the 3D DSF include a response gap even in the gapless QSL phase and an energy dependence deriving from the Majorana fermion density of states. Since the majority of the response is from states containing a single Majorana excitation, our results suggest inelastic neutron scattering as the spectroscopy of choice to illuminate the physics of Majorana fermions in Kitaev QSLs.

cond-mat.str-el↗

arXiv2015

Analytical theory for proton correlations in common water ice $I_h$

We provide a fully analytical microscopic theory for the proton correlations in water ice $I_h$. We compute the full diffuse elastic neutron scattering structure factor, which we find to be in excellent quantitative agreement with Monte Carlo simulations. It is also in remarkable qualitative agreement with experiment, in the absence of any fitting parameters. Our theory thus provides a tractable analytical starting point to account for more delicate features of the proton correlations in water ice. In addition, it directly determines an effective field theory of water ice as a topological phase.

cond-mat.stat-mech↗

arXiv2015

Acoustic signatures of the phases and phase transitions in Yb$_2$Ti$_2$O$_7$

We report on measurements of the sound velocity and attenuation in a single crystal of the candidate quantum- spin-ice material Yb$_2$Ti$_2$O$_7$ as a function of temperature and magnetic field. The acoustic modes couple to the spins magneto-elastically and, hence, carry information about the spin correlations that sheds light on the intricate magnetic phase diagram of Yb$_2$Ti$_2$O$_7$ and the nature of spin dynamics in the material. Particularly, we find a pronounced thermal hysteresis in the acoustic data with a concomitant peak in the specific heat indicating a possible first-order phase transition at about $0.17$ K. At low temperatures, the acoustic response to magnetic field saturates hinting at the development of magnetic order. Furthermore, mean-field calculations suggest that Yb$_2$Ti$_2$O$_7$ undergoes a first-order phase transition from a cooperative paramagnetic phase to a ferromagnet below $T\approx 0.17$ K.

cond-mat.str-el↗

arXiv2015

Dynamics of Fractionalization in Quantum Spin Liquids

We present the theory of dynamical spin-response for the Kitaev honeycomb model, obtaining exact results for the structure factor (SF) in gapped and gapless, Abelian and non-Abelian quantum spin-liquid (QSL) phases. We also describe the advances in methodology necessary to compute these results. The structure factor shows signatures of spin-fractionalization into emergent quasiparticles -- Majorana fermions and fluxes of $Z_2$ gauge field. In addition to a broad continuum from spin-fractionalization, we find sharp ($δ$-function) features in the response. These arise in two distinct ways: from excited states containing only (static) fluxes and no (mobile) fermions; and from excited states in which fermions are bound to fluxes. The SF is markedly different in Abelian and non-Abelian QSLs, and bound fermion-flux composites appear only in the non-Abelian phase.

cond-mat.str-el↗

arXiv2015

Nonequilibrium transport and statistics of Schwinger pair production in Weyl semimetals

The non-equilibrium dynamics beyond linear response of Weyl semimetals is studied after a sudden switching on of a DC electric field. The resulting current is a nonmonotonic function of time, with an initial quick increase of polarization current followed by a power-law decay. Particle-hole creation à la Schwinger dominates for long times when the conduction current takes over the leading role, with the total current increasing again. The conductivity estimated from a dynamical calculation within a Drude picture agrees with the one obtained from Kubo's formula. The full distribution function of electron-hole pairs changes from Poissonian for short perturbations to a Gaussian in the long perturbation (Landau-Zener) regime. The vacuum persistence probability of high energy physics manifests itself in a finite probability of no pair creation and no induced current at all times.

cond-mat.str-el↗

arXiv2015

Random Coulomb antiferromagnets: from diluted spin liquids to Euclidean random matrices

We study a disordered classical Heisenberg magnet with uniformly antiferromagnetic interactions which are frustrated on account of their long-range Coulomb form, {\em i.e.} $J(r)\sim -A\ln r$ in $d=2$ and $J(r)\sim A/r$ in $d=3$. This arises naturally as the $T\rightarrow 0$ limit of the emergent interactions between vacancy-induced degrees of freedom in a class of diluted Coulomb spin liquids (including the classical Heisenberg antiferromagnets on checkerboard, SCGO and pyrochlore lattices) and presents a novel variant of a disordered long-range spin Hamiltonian. Using detailed analytical and numerical studies we establish that this model exhibits a very broad paramagnetic regime that extends to very large values of $A$ in both $d=2$ and $d=3$. In $d=2$, using the lattice-Green function based finite-size regularization of the Coulomb potential (which corresponds naturally to the underlying low-temperature limit of the emergent interactions between orphan-spins), we only find evidence that freezing into a glassy state occurs in the limit of strong coupling, $A=\infty$, while no such transition seems to exist at all in $d=3$. We also demonstrate the presence and importance of screening for such a magnet. We analyse the spectrum of the Euclidean random matrices describing a Gaussian version of this problem, and identify a corresponding quantum mechanical scattering problem.

cond-mat.str-el↗

arXiv2015

Proximate Kitaev Quantum Spin Liquid Behaviour in α-RuCl$_3$

Topological states of matter such as quantum spin liquids (QSLs) are of great interest because of their remarkable predicted properties including protection of quantum information and the emergence of Majorana fermions. Such QSLs, however, have proven difficult to identify experimentally. The most promising approach is to study their exotic nature via the wave-vector and intensity dependence of their dynamical response in neutron scattering. A major search has centered on iridate materials which are proposed to realize the celebrated Kitaev model on a honeycomb lattice - a prototypical topological QSL system in two dimensions (2D). The difficulties of iridium for neutron measurements have, however, impeded progress significantly. Here we provide experimental evidence that a material based on ruthenium, α-RuCl$_3$ realizes the same Kitaev physics but is highly amenable to neutron investigation. Our measurements confirm the requisite strong spin-orbit coupling, and a low temperature magnetic order that matches the predicted phase proximate to the QSL. We also show that stacking faults, inherent to the highly 2D nature of the material, readily explain some puzzling results to date. Measurements of the dynamical response functions, especially at energies and temperatures above that where interlayer effects are manifest, are naturally accounted for in terms of deconfinement physics expected for QSLs. Via a comparison to the recently calculated dynamics from gauge flux excitations and Majorana fermions of the pure Kitaev model we propose α-RuCl$_3$ as the prime candidate for experimental realization of fractionalized Kitaev physics.

cond-mat.mtrl-sci↗

arXiv2015

Quantum simulations made easy plane

Ever since Heisenberg's proposal of a quantum-mechanical origin of ferromagnetism in 1928, the spin model named after him has been central to advances in magnetism, featuring in proposals of novel many-body states such as antiferromagnets, emergent gauge fields in their confined (valence bond crystal) and deconfined (resonating valence bond spin liquids) versions. Between them, these cover much of our understanding of modern magnetism specifically and topological states of matter in general. Many exciting phenomena predicted theoretically still await experimental realisation, and cold atomic systems hold the promise of acting as analogue 'quantum simulators' of the relevant theoretical models, for which ingenious and intricate set-ups have been proposed. Here, we identify a new class of particularly simple quantum simulators exhibiting many such phenomena but obviating the need for fine-tuning and for amplifying perturbatively weak superexchange or longer-range interactions. Instead they require only moderate on-site interactions on top of uncorrelated, one-body hopping--ingredients already available with present experimental technology. Between them, they realise some of the most interesting phenomena, such as emergent synthetic gauge fields, resonating valence bond phases, and even the celebrated yet enigmatic spin liquid phase of the kagome lattice.

cond-mat.quant-gas↗

arXiv2015

Multiferroicity in spin ice: towards a magnetic crystallography of Tb2Ti2O7 in a field

We combine two aspects of magnetic frustration, multiferroicity and emergent quasi-particles in spin liquids, by studying magneto-electric monopoles. Spin ice offers to couple these emergent topological defects to external fields, and to each other, in unusual ways, making possible to lift the degeneracy underpinning the spin liquid and to potentially stabilize novel forms of charge crystals, opening the path to a "magnetic crystallography". In developing the general phase diagram including nearest-neighbour coupling, Zeeman energy, electric and magnetic dipolar interactions, we uncover the emergence of a bi-layered crystal of singly-charged monopoles, whose stability, remarkably, is strengthened by an external [110] magnetic field. Our theory is able to account for the ordering process of Tb2Ti2O7 in large field for reasonably small electric energy scales.

cond-mat.str-el↗

arXiv2015

Topology and Interactions in a Frustrated Slab: Tuning from Weyl Semimetals to C > 1 Fractional Chern Insulators

We show that, quite generically, a [111] slab of spin-orbit coupled pyrochlore lattice exhibits surface states whose constant energy curves take the shape of Fermi arcs, localized to different surfaces depending on their quasimomentum. Remarkably, these persist independently of the existence of Weyl points in the bulk. Considering interacting electrons in slabs of finite thickness, we find a plethora of known fractional Chern insulating phases, to which we add the discovery of a new higher Chern number state which is likely a generalization of the Moore-Read fermionic fractional quantum Hall state. By contrast, in the three-dimensional limit, we argue for the absence of gapped states of the flat surface band due to a topologically protected coupling of the surface to gapless states in the bulk. We comment on generalizations as well as experimental perspectives in thin slabs of pyrochlore iridates.

cond-mat.str-el↗

arXiv2014

Quantum annealing: the fastest route to quantum computation?

In this review we consider the performance of the quantum adiabatic algorithm for the solution of decision problems. We divide the possible failure mechanisms into two sets: small gaps due to quantum phase transitions and small gaps due to avoided crossings inside a phase. We argue that the thermodynamic order of the phase transitions is not predictive of the scaling of the gap with the system size. On the contrary, we also argue that, if the phase surrounding the problem Hamiltonian is a Many-Body Localized (MBL) phase, the gaps are going to be typically exponentially small and that this follows naturally from the existence of local integrals of motion in the MBL phase.

quant-ph↗

arXiv2014

Ultrasonic investigations of spin-ices Dy$_2$Ti$_2$O$_7$ and Ho$_2$Ti$_2$O$_7$ in and out of equilibrium

We report ultrasound studies of spin-lattice and single-ion effects in the spin-ice materials Dy$_2$Ti$_2$O$_7$ (DTO) and Ho$_2$Ti$_2$O$_7$ (HTO) across a broad field range up to 60 T, covering phase transformations, interactions with low-energy magnetic excitations, as well as single-ion effects. In particular, a sharp dip observed in the sound attenuation in DTO at the gas-liquid transition of the magnetic monopoles is explained based on an approach involving negative relaxation processes. Furthermore, quasi-periodic peaks in the acoustic properties of DTO due to non-equilibrium processes are found to be strongly affected by {\em macroscopic} thermal-coupling conditions: the thermal runaway observed in previous studies in DTO can be suppressed altogether by immersing the sample in liquid helium. Crystal-electric-field effects having higher energy scale lead to a renormalization of the sound velocity and sound attenuation at very high magnetic fields. We analyze our observations using an approach based on an analysis of exchange-striction couplings and single-ion effects.

cond-mat.str-el↗

arXiv2014

Doping a topological quantum spin liquid: slow holes in the Kitaev honeycomb model

We present a controlled microscopic study of mobile holes in the spatially anisotropic (Abelian) gapped phase of the Kitaev honeycomb model. We address the properties of (i) a single hole [its internal degrees of freedom as well as its hopping properties]; (ii) a pair of holes [their (relative) particle statistics and interactions]; (iii) the collective state for a finite density of holes. We find that each hole in the doped model has an eight-dimensional internal space, characterized by three internal quantum numbers: the first two "fractional" quantum numbers describe the binding to the hole of the fractional excitations (fluxes and fermions) of the undoped model, while the third "spin" quantum number determines the local magnetization around the hole. The fractional quantum numbers also encode fundamentally distinct particle properties, topologically robust against small local perturbations: some holes are free to hop in two dimensions, while others are confined to hop in one dimension only; distinct hole types have different particle statistics, and in particular, some of them exhibit non-trivial (anyonic) relative statistics. These particle properties in turn determine the physical properties of the multi-hole ground state at finite doping, and we identify two distinct ground states with different hole types that are stable for different model parameters. The respective hopping dimensionalities manifest themselves in an electrical conductivity approximately isotropic in one ground state and extremely anisotropic in the other one. We also compare our microscopic study with related mean-field treatments, and discuss the main discrepancies between the two approaches, which in particular involve the possibility of binding fractional excitations as well as the particle statistics of the holes.

cond-mat.str-el↗

arXiv2014

Raman Scattering Signatures of Kitaev Spin Liquids in A$_2$ IrO$_3$ Iridates

We study theoretically the Raman scattering response $I(ω)$ in the gapless quantum spin liquid phase of the Kitaev-Heisenberg model. The dominant polarization-independent contribution $I_K (ω)$ reflects the density of states of the emergent Majorana fermions in the ground-state flux-sector. The integrability-breaking Heisenberg exchange generates a second contribution, whose dominant part $I_H (ω)$ has the form of a quantum quench corresponding to an abrupt insertion of four $Z_2$ gauge fluxes. This results in a weakly polarization dependent response with a sharp peak at the energy of the flux excitation accompanied by broad features, which can be related to Majorana fermions in the presence of the perturbed gauge field. We discuss the experimental situation and explore more generally the influence of integrability breaking for Kitaev spin liquid response functions.

cond-mat.str-el↗

arXiv2014

A topological spin glass in diluted spin ice

It is a salient experimental fact that a large fraction of candidate spin liquid materials freeze as the temperature is lowered. The question naturally arises whether such freezing is intrinsic to the spin liquid ("disorder-free glassiness") or extrinsic, in the sense that a topological phase simply coexists with standard freezing of impurities. Here, we demonstrate a surprising third alternative, namely that freezing and topological liquidity are inseparably linked. The topological phase reacts to the introduction of disorder by generating degrees of freedom of a new type (along with interactions between them), which in turn undergo a freezing transition while the topological phase supporting them remains intact.

cond-mat.str-el↗

arXiv2014

Nature of finite-temperature transition in anisotropic pyrochlore Er2Ti2O7

We study the finite-temperature transition in a model XY antiferromagnet on a pyrochlore lattice, which describes the pyrochlore material Er2Ti2O7. The ordered magnetic structure selected by thermal fluctuations is six-fold degenerate. Nevertheless, our classical Monte Carlo simulations show that the critical behavior corresponds to the three-dimensional XY universality class. We determine an additional critical exponent nu_6=0.75>nu characteristic of a dangerously irrelevant scaling variable. Persistent thermal fluctuations in the ordered phase are revealed in Monte Carlo simulations by the peculiar coexistence of Bragg peaks and diffuse magnetic scattering, the feature also observed in neutron diffraction experiments.

cond-mat.str-el↗