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R. Moessner

Publications and source records attributed to R. Moessner.

At least 91 records · Page 5Linked to original sources

Vacancy-induced spin textures and their interactions in a classical spin liquid

Motivated by experiments on the archetypal frustrated magnet SrCr$_{9p}$Ga$_{12-9p}$O$_{19}$ (SCGO), we study the classical Heisenberg model on the pyrochlore slab (Kagomé bilayer) lattice with site-dilution $x=1-p$. This allows us to address generic aspects of the physics of non-magnetic vacancies in a classical spin liquid. We explicitly demonstrate that the pure ($x=0$) system remains a spin-liquid down to the lowest temperatures, with an unusual {\em non-monotonic} temperature dependence of the susceptibility, which even turns diamagnetic for the apical spins between the two kagome layers. For $x> 0$ but small, the low temperature magnetic response of the system is most naturally described in terms of the properties of spatially extended spin textures that cloak an "orphan" $S=3/2$ Cr$^{3+}$ spin in direct proximity to a pair of missing sites belonging to the same triangular simplex. In the $T \rightarrow 0$ limit, these orphan-texture complexes each carry a net magnetization that is exactly half the magnetic moment of an individual spin of the undiluted system. Furthermore, we demonstrate that they interact via an entropic {\em temperature dependent} {\em pair-wise exchange interaction} $J_{eff}(T,\vec{r}) \sim T {\mathcal J} (\vec{r} \sqrt{T})$ that has a logarithmic form at short-distances and decays exponentially beyond a thermal correlation length $ξ(T) \sim 1/\sqrt{T}$. The sign of $J_{eff}$ depends on whether the two orphan spins belong to the same Kagome layer or not. We provide a detailed analytical account of these properties using an effective field theory approach specifically tailored for the problem at hand. These results are in quantitative agreement with large-scale Monte Carlo numerics.

cond-mat.str-el↗

Quantum magnetism on the Cairo pentagonal lattice

We present an extensive analytical and numerical study of the antiferromagnetic Heisenberg model on the Cairo pentagonal lattice, the dual of the Shastry-Sutherland lattice with a close realization in the S=5/2 compound Bi2Fe4O9. We consider a model with two exchange couplings suggested by the symmetry of the lattice, and investigate the nature of the ground state as a function of their ratio x and the spin S. After establishing the classical phase diagram we switch on quantum mechanics in a gradual way that highlights the different role of quantum fluctuations on the two inequivalent sites of the lattice. The most important findings for S=1/2 include: (i) a surprising interplay between a collinear and a four-sublattice orthogonal phase due to an underlying order-by-disorder mechanism at small x (related to an emergent J1-J2 effective model with J2 >> J1), and (ii) a non-magnetic and possibly spin-nematic phase with d-wave symmetry at intermediate x.

cond-mat.str-el↗

Possible Quantum Diffusion of Polaronic Muons in Dy$_2$Ti$_2$O$_7$ Spin Ice

We interpret recent measurements of the zero field muon relaxation rate in the frustrated magnetic pyrochlore Dy$_2$Ti$_2$O$_7$ as resulting from the quantum diffusion of muons in the substance. In this scenario, the plateau observed at low temperature ($<7$ K) in the relaxation rate is due to coherent tunneling of the muons through a spatially disordered spin state and not to any magnetic fluctuations persisting at low temperature. Two further regimes either side of a maximum relaxation rate at $T^* = 50$ K correspond to a crossover between tunnelling and incoherent activated hopping motion of the muon. Our fit of the experimental data is compared with the case of muonium diffusion in KCl.

cond-mat.str-el↗

The quantum adiabatic algorithm and scaling of gaps at first order quantum phase transitions

Motivated by the quantum adiabatic algorithm (QAA), we consider the scaling of the Hamiltonian gap at quantum first order transitions, generally expected to be exponentially small in the size of the system. However, we show that a quantum antiferromagnetic Ising chain in a staggered field can exhibit a first order transition with only an algebraically small gap. In addition, we construct a simple classical translationally invariant one-dimensional Hamiltonian containing nearest-neighbour interactions only, which exhibits an exponential gap at a thermodynamic quantum first-order transition of essentially topological origin. This establishes that (i) the QAA can be successful even across first order transitions but also that (ii) it can fail on exceedingly simple problems readily solved by inspection, or by classical annealing.

quant-ph↗

Itinerant electrons in the Coulomb phase

We study the interplay between magnetic frustration and itinerant electrons. For example, how does the coupling to mobile charges modify the properties of a spin liquid, and does the underlying frustration favor insulating or conducting states? Supported by Monte Carlo simulations, our goal is in particular to provide an analytical picture of the mechanisms involved. The models under considerations exhibit Coulomb phases in two and three dimensions, where the itinerant electrons are coupled to the localized spins via double exchange interactions. Because of the Hund coupling, magnetic loops naturally emerge from the Coulomb phase and serve as conducting channels for the mobile electrons, leading to doping-dependent rearrangements of the loop ensemble in order to minimize the electronic kinetic energy. At low electron density ρ, the double exchange coupling mainly tends to segment the very long loops winding around the system into smaller ones while it gradually lifts the extensive degeneracy of the Coulomb phase with increasing ρ. For higher doping, the results are strongly lattice dependent, displaying loop crystals with a given loop length for some specific values of ρ, which can melt into another loop crystal by varying ρ. Finally, we contrast this to the qualitatively different behavior of analogous models on kagome or triangular lattices.

cond-mat.stat-mech↗

Spin Ice, Fractionalization and Topological Order

The spin ice compounds {\dys} and {\holm} are highly unusual magnets which epitomize a set of concepts of great interest in modern condensed matter physics: their low-energy physics exhibits an emergent gauge field and their excitations are magnetic monopoles which arise from the fractionalization of the microscopic magnetic spin degrees of freedom. In this review, we provide an elementary introduction to these concepts and we survey the thermodynamics, statics and dynamics---in and out of equilibrium---of spin ice from these vantage points. Along the way, we touch on topics such as emergent Coulomb plasmas, observable "Dirac strings", and irrational charges. We close with the outlook for these unique materials.

cond-mat.str-el↗

Intrinsic and extrinsic nonstationary field-driven processes in the spin-ice compound Dy2Ti2O7

Nonequilibrium processes are probed by ultrasound waves in the spin-ice material Dy2Ti2O7 at low temperatures. The sound velocity and the sound attenuation exhibit a number of anomalies versus applied magnetic field for temperatures below the "freezing" temperature of ~500 mK. These robust anomalies can be seen for longitudinal and transverse acoustic modes for different field directions. The anomalies show a broad hysteresis. Most notable are peaks in the sound velocity, which exhibit two distinct regimes: an intrinsic (extrinsic) one in which the data collapse for different sweep rates when plotted as function of field strength (time). We discuss our observations in context of the emergent quasiparticles which govern the low-temperature dynamics of the spin ice.

cond-mat.str-el↗

Magnetic resonance from the interplay of frustration and superconductivity

Motivated by the iron-based superconductors, we develop a self-consistent electronic theory for the itinerant spin excitations in the regime of coexistence of the antiferromagnetic stripe order with wavevector ${\bf Q}_{1} = (π,0)$ and $s^{+-}$ superconductivity. The onset of superconductivity leads to the appearance of a {\em magnetic} resonance near the wavevector ${\bf Q}_{2} = (0,π)$ where magnetic order is absent. This resonance is isotropic in spin space, unlike the excitations near ${\bf Q}_{1}$ where the magnetic Goldstone mode resides. We discuss several features which can be observed experimentally.

cond-mat.supr-con↗

Site dilution in Kitaev's honeycomb model

We study the physical consequences of site dilution in Kitaev's honeycomb model, in both its gapped and gapless phases. We show that a vacancy binds a flux of the emergent $Z_2$ gauge field and induces a local moment. In the gapped phase this moment is free while in the gapless phase the susceptibility has the dependence $χ(h)\sim\ln(1/h)$ on field strength $h$. Vacancy moments have interactions that depend on their separation, their relative sublattice, and the phase of the model. Strikingly, in the gapless phase, two nearby vacancies on the same sublattice have a parametrically larger $χ(h)\sim(h[\ln(1/h)]^{3/2})^{-1}$. In the gapped phase, even a finite density of randomly distributed vacancies remains tractable, via a mapping to a bipartite random hopping problem. This leads to a strong disorder form of the low-energy thermodynamics, with a Dyson-type singularity in the density of states for excitations.

cond-mat.str-el↗

Interplay of Spin and Lattice Degrees of Freedom in the Frustrated Antiferromagnet CdCr_2O_4: High-field and Temperature Induced Anomalies of the Elastic Constants

Temperature and magnetic field studies of the elastic constants of the chromium spinel CdCr_2O_4 show pronounced anomalies related to strong spin-phonon coupling in this frustrated antiferromagnet. A detailed comparison of the longitudinal acoustic mode propagating along the [111] direction with theory based on an exchange-striction mechanism leads to an estimate of the strength of the magneto-elastic interaction. The derived spin-phonon coupling constant is in good agreement with previous determinations based on infrared absorption. Further insight is gained from intermediate and high magnetic field experiments in the field regime of the magnetization plateau. The role of the antisymmetric Dzyaloshinskii-Moriya interaction discussed and we compare the spin-phonon coupling in CdCr_2O_4 in both the ordered and disordered states.

cond-mat.str-el↗

Analysis of a fully packed loop model arising in a magnetic Coulomb phase

The Coulomb phase of spin ice, and indeed the Ic phase of water ice, naturally realise a fully-packed two-colour loop model in three dimensions. We present a detailed analysis of the statistics of these loops, which avoid themselves and other loops of the same colour, and contrast their behaviour to an analogous two-dimensional model. The properties of another extended degree of freedom are also addressed, flux lines of the emergent gauge field of the Coulomb phase, which appear as "Dirac strings" in spin ice. We mention implications of these results for related models, and experiments.

cond-mat.stat-mech↗

Multiorbital Spin Susceptibility in a Magnetically Ordered State - Orbital versus Excitonic Spin Density Wave Scenario

We present a general theory of multiorbital spin waves in magnetically ordered metallic systems. Motivated by the itinerant magnetism of iron-based superconductors, we compare the magnetic excitations for two different scenarios: when the magnetic order either sets in on the on-site orbital level; or when it appears as an electron-hole pairing between different bands of electron and hole character. As an example we treat the two-orbital model for iron-based superconductors. For small magnetic moments the spin excitations look similar in both scenarios. Going to larger interactions and larger magnetic moments, the difference between both scenarios becomes striking. While in the excitonic scenario the spin waves form a closed structure over the entire Brillouin zone and the particle-hole continuum is gapped, the spin excitations in the orbital scenario can be treated as spin waves only in a close vicinity to the ordering momenta. The origin of this is a gapless electronic structure with Dirac cones which is a source of large damping. We analyze our results in connection with recent neutron scattering measurements and show that certain features of the orbital scenario with multiple order parameters can be observed experimentally.

cond-mat.supr-con↗

Symmetry Breaking on the Three-Dimensional Hyperkagome Lattice of Na_4Ir_3O_8

We study the antiferromagnetic spin-1/2 Heisenberg model on the highly frustrated, three-dimensional, hyperkagome lattice of Na_4Ir_3O_8 using a series expansion method. We propose a valence bond crystal with a 72 site unit cell as a ground state that supports many, very low lying, singlet excitations. Low energy spinons and triplons are confined to emergent lower-dimensional motifs. Here, and for analogous kagome and pyrochlore states, we suggest finite temperature signatures, including an Ising transition, in the magnetic specific heat due to a multistep breaking of discrete symmetries.

cond-mat.str-el↗

Diagnosing Deconfinement and Topological Order

Topological or deconfined phases are characterized by emergent, weakly fluctuating, gauge fields. In condensed matter settings they inevitably come coupled to excitations that carry the corresponding gauge charges which invalidate the standard diagnostic of deconfinement---the Wilson loop. Inspired by a mapping between symmetric sponges and the deconfined phase of the $Z_2$ gauge theory, we construct a diagnostic for deconfinement that has the interpretation of a line tension. One operator version of this diagnostic turns out to be the Fredenhagen-Marcu order parameter known to lattice gauge theorists and we show that a different version is best suited to condensed matter systems. We discuss generalizations of the diagnostic, use it to establish the existence of finite temperature topological phases in $d \ge 3$ dimensions and show that multiplets of the diagnostic are useful in settings with multiple phases such as $U(1)$ gauge theories with charge $q$ matter. [Additionally we present an exact reduction of the partition function of the toric code in general dimensions to a well studied problem.]

cond-mat.str-el↗

Quasiparticle interference in iron-based superconductors

We systematically calculate quasiparticle interference (QPI) signatures for the whole phase diagram of iron-based superconductors. Impurities inherent in the sample together with ordered phases lead to distinct features in the QPI images that are believed to be measured in spectroscopic imaging-scanning tunneling microscopy (SI-STM). In the spin-density wave phase the rotational symmetry of the electronic structure is broken, signatures of which are also seen in the coexistence regime with both superconducting and magnetic order. In the superconducting regime we show how the different scattering behavior for magnetic and non-magnetic impurities allows to verify the $s^{+-}$ symmetry of the order parameter. The effect of possible gap minima or nodes is discussed.

cond-mat.supr-con↗

Dirac Strings and Magnetic Monopoles in Spin Ice Dy2Ti2O7

While sources of magnetic fields - magnetic monopoles - have so far proven elusive as elementary particles, several scenarios have been proposed recently in condensed matter physics of emergent quasiparticles resembling monopoles. A particularly simple proposition pertains to spin ice on the highly frustrated pyrochlore lattice. The spin ice state is argued to be well-described by networks of aligned dipoles resembling solenoidal tubes - classical, and observable, versions of a Dirac string. Where these tubes end, the resulting defect looks like a magnetic monopole. We demonstrate, by diffuse neutron scattering, the presence of such strings in the spin-ice Dy2Ti2O7. This is achieved by applying a symmetry-breaking magnetic field with which we can manipulate density and orientation of the strings. In turn, heat capacity is described by a gas of magnetic monopoles interacting via a magnetic Coulomb interaction.

cond-mat.mtrl-sci↗

Unconventional magnetization processes and thermal runaway in spin-ice Dy$_2$Ti$_2$O$_7$

We investigate the non-equilibrium behavior of the spin-ice material Dy$_2$Ti$_2$O$_7$ by studying its magnetization as a function of the rate at which an external field is swept. At temperatures below the enigmatic "freezing" temperature $T_{\rm equil}\approx600$ mK, we find that even the slowest sweeps fail to yield the equilibrium magnetization curve and instead give a smooth, initially much flatter curve. For higher sweep rates, the magnetization develops sharp steps accompanied by similarly sharp peaks in the temperature of the sample. We ascribe the former behavior to the energy barriers encountered in the magnetization process, which proceeds via flipping of spins on filaments traced out by the field-driven motion of the gapped, long-range interacting magnetic monopole excitations. In contrast, the peaks in temperature result from the released Zeeman energy not being carried away efficiently into the bath, with the resulting heating triggering a chain reaction.

cond-mat.mtrl-sci↗

Magnetic properties of the Hubbard model on kagome stripes

We consider the one-orbital $N$-site repulsive Hubbard model on two kagome-like chains, both of which yield a completely dispersionless (flat) one-electron band. Using exact many-electron ground states in the subspaces with $n\le n_{\max}$ ($n_{\max}\propto N$) electrons, we calculate the square of the total spin in the ground state to discuss magnetic properties of the models. We have found that although for $n<n_{\max}$ the ground states contain fully polarized states, there is no finite region of electron densities $n/{\cal{N}} <1$ (${\cal{N}}=N/3$ or ${\cal{N}}=N/5$) where ground-state ferromagnetism survives for ${\cal{N}}\to\infty$.

cond-mat.str-el↗