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R. Prozorov

Publications and source records attributed to R. Prozorov.

At least 145 records · Page 8Linked to original sources

Doping dependence of heat transport in the iron-arsenide superconductor Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$: from isotropic to strongly $k$-dependent gap structure

The temperature and magnetic field dependence of the in-plane thermal conductivity $κ$ of the iron-arsenide superconductor Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ was measured down to $T \simeq 50$ mK and up to $H = 15$ T as a function of Co concentration $x$ in the range 0.048 $ \leq x \leq $ 0.114. In zero magnetic field, a negligible residual linear term in $κ/T$ as $T \to 0$ at all $x$ shows that there are no zero-energy quasiparticles and hence the superconducting gap has no nodes in the $ab$-plane anywhere in the phase diagram. However, the field dependence of $κ$ reveals a systematic evolution of the superconducting gap with doping $x$, from large everywhere on the Fermi surface in the underdoped regime, as evidenced by a flat $κ(H)$ at $T \to 0$, to strongly $k$-dependent in the overdoped regime, where a small magnetic field can induce a large residual linear term, indicative of a deep minimum in the gap magnitude somewhere on the Fermi surface. This shows that the superconducting gap structure has a strongly $k$-dependent amplitude around the Fermi surface only outside the antiferromagnetic/orthorhombic phase.

cond-mat.supr-con↗

Magneto-optical study of Ba(Fe$_{1-x}$T$_{x}$)$_2$As$_2$ (T=Co, Ni) single crystals irradiated with heavy-ions

Optimally doped single crystals of Ba(Fe$_{1-x}$T$_x$)$_2$As$_2$ (T=Co, Ni) were irradiated with 1.4 GeV $^{208}$Pb$^{56+}$ ions at fluences corresponding to matching fields of $B_ϕ=0.1, 0.5, 1$ and 2 T. Magneto-optical imaging has been used to map the distribution of the magnetic induction in the irradiated samples. The imaging is complemented by the magnetization measurements. The results show a substantial enhancement of the apparent critical current densities as revealed by the much larger Bean penetration fields and an increase of the hysteretic magnetization. However, the effect depends on the compound, temperature and applied magnetic field. In \FeCo crystals, at 15 K and low fields, the enhancement appears to scale with the irradiation dose at a rate of about 0.27 MA$\cdot$cm$^{-2}$T$^{-1}$, whereas in \FeNi crystals, higher irradiation doses are less effective. Our results suggest that moderate irradiation with heavy ions is a an effective way to \emph{homogeneously} enhance the current-currying capabilities of pnictide superconductors.

cond-mat.supr-con↗

London penetration depth and superfluid density in single crystals of Fe(Te,Se) and Fe(Te,S) superconductors

The in-plane London penetration depth, $λ(T)$, was measured in single crystals of the iron-chalcogenide superconductors Fe$_{1.03}$(Te$_{0.63}$Se$_{0.37}$) and Fe$_{1.06}$(Te$_{0.88}$S$_{0.14}$) by using a radio-frequency tunnel diode resonator. As is also the case for the iron-pnictides, these iron-chalcogenides exhibit a nearly quadratic temperature variation of $λ(T)$ at low temperatures. The absolute value of the penetration depth in the $T \to 0$ limit was determined for Fe$_{1.03}$(Te$_{0.63}$Se$_{0.37})$ by using an Al coating technique, giving $λ(0)\approx560 \pm 20$ nm. The superfluid density $ρ_s(T)=λ^2(0)/λ^2(T)$ was fitted with a self-consistent two-gap $γ-$model. While two different gaps are needed to describe the full-range temperature variation of $ρ_s(T)$, a non-exponential behavior at low temperatures requires additional factors, such as scattering and/or significant gap anisotropy.

cond-mat.supr-con↗

London penetration depth and strong pair-breaking in iron-based superconductors

The low temperature variation of the London penetration depth for a number of iron-pnictide and iron-chalcogenide superconductors is nearly quadratic, $Δλ(T) = βT^n$ with $n\approx 2$. The coefficient in this dependence shows a robust scaling, $β\propto 1/T_c^3$ across different families of these materials. We associate the scaling with a strong pair-breaking. The same mechanism have recently been suggested to explain the scalings of the specific heat jump, $ΔC \propto T_c^3$, and of the slopes of the upper critical field, $dH_{c2}/dT\propto T_c$ in these materials. This suggests that thermodynamic and electromagnetic properties of the iron-based superconductors can be described within a strong pair-breaking scenario.

cond-mat.supr-con↗

Three-dimensional nodal superconducting gap in single crystals Ba(Fe$_{1-x}$Ni$_x$)$_2$As$_2$

The London penetration depth, $λ$, is directly related to the density, $n_{s}$, of the Cooper pairs ($λ^{2}\propto 1/n_{s}$) and its variation with temperature provides valuable insight into the pairing mechanism. Here we study the evolution with doping of the temperature dependence of the in-plane ($λ_{ab}$) and out-of-plane ($λ_{c}$) penetration depths in single crystals of electron-doped Ba(Fe$_{1-x}$Ni$_x$)$_2$As$_2$. As is the case for other pnictides, $λ(T) \sim T^n$ over the whole doping range and this behavior extends down to at least $T=T_c/100$, setting a very small upper limit on the gap minimum. Furthermore, in the overdoped regime: 1) the exponent $n$ becomes substantially smaller than 2, which is incompatible with the models that explain power-law behavior to be due to scattering; 2) the exponent $n$ becomes anisotropic, with $λ_{c}(T)$ showing a clear $T$-linear behavior over a large temperature interval. These findings suggest that in the overdoped regime the superconducting gap in iron-based pnictide superconductors develops nodal structure, which unlike in the cuprates, cannot be understood within a two-dimensional picture.

cond-mat.supr-con↗

Intrinsic pinning on structural domains in underdoped single crystals of Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$

Critical current density was studied in single crystals of Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ for the values of $x$ spanning the entire doping phase diagram. A noticeable enhancement was found for slightly underdoped crystals with the peak at $x = 0.058$. Using a combination of polarized-light imaging, x-ray diffraction and magnetic measurements we associate this behavior with the intrinsic pinning on structural domains in the orthorhombic phase. Domain walls extend throughout the sample thickness in the direction of vortices and act as extended pinning centers. With the increasing $x$ domain structure becomes more intertwined and fine due to a decrease of the orthorhombic distortion. This results in the energy landscape with maze-like spatial modulations favorable for pinning. This finding shows that iron-based pnictide superconductors, characterized by high values of the transition temperature, high upper critical fields, and low anisotropy may intrinsically have relatively high critical current densities.

cond-mat.supr-con↗

Local-moment ferromagnetism and unusual magnetic domains in Fe$_{1/4}$TaS$_{2}$ crystals

Single crystals of Fe$_{1/4}$TaS$_{2}$ have been studied by using magneto-optical (MO) imaging and radio-frequency (rf) magnetic susceptibility, $χ$. Real time MO images reveal unusual, slow dynamics of dendritic domain formation, the details of which are strongly dependent upon magnetic and thermal history. Measurements of $χ(T)$ show well-defined, local moment ferromagnetic transition at $T\approx 155$ K as well as thermal hysteresis for 50 K$<T<$60 K. This temperature range corresponds to the domain formation temperature as determined by MO. Together these observations provide strong evidence for local moment ferromagnetism in Fe$_{1/4}$TaS$_{2}$ crystals with large, temperature dependent magnetic anisotropy.

cond-mat.str-el↗

Superfluid density and specific heat within self-consistent scheme for two-band superconductor

The two gaps in a two-band clean s-wave superconductor are evaluated self-consistently within the quasiclassical Eilenberger weak-coupling formalism with two in-band and one inter-band pairing potentials. Superfluid density, free energy and specific heat are given in the form amenable for fitting the experimental data. Well-known two-band MgB$_2$ and V$_3$Si superconductors are used to test the developed approach. The pairing potentials obtained from the fit of the superfluid density data in MgB$_2$ crystal were used to calculate temperature-dependent specific heat, $C(T)$. The calculated $C(T)$ compares very well with the experimental data. Advantages and validity of this, what we call the "$γ$-model", are discussed and compared with the commonly used empirical (and \textit{not self-consistent}) "$α$-model". Correlation between the sign of the inter-band coupling and the signs of the two order parameters is discussed. Suppression of the critical temperature by the inter-band scattering is evaluated and shown to be severe for the inter-band repulsion as compared to the attraction. The data on a strong $T_c$ suppression in MgB$_2$ crystals by impurities suggest that the order parameters on two effective bands of this material may have opposite signs, i.e., may have the $s_{\pm}$ structure similar to the current proposals in iron-based pnictide superconductors.

cond-mat.supr-con↗

Direct imaging of the structural domains in iron pnictides AFe2As2 (A = Ca, Sr, Ba)

The parent compounds of recently discovered iron-arsenide superconductors, $A$Fe$_2$As$_2$ with alkaline earth $A$=Ca, Sr, Ba, undergo simultaneous structural and magnetic phase transitions at a temperature $T_{SM}$. Using a combination of polarized light microscopy and spatially resolved high-energy synchrotron X-ray diffraction we show that the orthorhombic distortion leads to the formation of 45$^o$-type structural domains in all parent compounds. Domains penetrate through the sample thickness in the $c$- direction and are not affected by crystal defects such as growth terraces. The domains form regular stripe patterns in the plane with a characteristic dimension of 10 to 50 $μm$. The direction of the stripes is fixed with respect to the tetragonal (100) and (010) directions but can change by 90$^o$ on thermal cycling through the transition. This domain pattern may have profound implications for intrinsic disorder and anisotropy of iron arsenides.

cond-mat.supr-con↗

Non-exponential London penetration depth in RFeAsO$_{0.9}$F$_{0.1}$ (R=La,Nd) single crystals

The superconducting penetration depth, $λ(T)$, has been measured in RFeAsO$_{0.9}$F$_{0.1}$ (R=La,Nd) single crystals (R-1111). In Nd-1111, we find an upturn in $λ(T)$ upon cooling and attribute it to the paramagnetism of the Nd ions, similar to the case of the electron-doped cuprate Nd-Ce-Cu-O. After the correction for paramagnetism, the London penetration depth variation is found to follow a power-law behavior, $Δλ_L(T)\propto T^{2}$ at low temperatures. The same $T^2$ variation of $λ(T)$ was found in non-magnetic La-1111 crystals. Analysis of the superfluid density and of penetration depth anisotropy over the full temperature range is consistent with two-gap superconductivity. Based on this and on our previous work, we conclude that both the RFeAsO (1111) and BaFe$_2$As$_2$ (122) families of pnictide superconductors exhibit unconventional two-gap superconductivity.

cond-mat.supr-con↗

Resistivity Anisotropy of $AE$Fe$_2$As$_2$ ($AE$ =Ca, Sr, Ba): direct versus Montgomery technique measurements

The anisotropy of electrical resistivity was measured in parent compounds of the iron-arsenic high temperature superconductors, AEFe2As2 with Alkali Earth elements AE=Ca,Sr, Ba. Measurements were performed using both the Montgomery technique and direct resistivity measurements on samples cut along principal crystallographic directions. The anisotropy ratio γ_ρ=ρ_c/ρ_a is well below 10 for all compounds in the whole temperature range studied (4 to 300 K), in notable contrast to previous reports. The anisotropy at room temperature increases from about 2 in Ca, to about 4 in Sr and Ba. In all compounds the resistivity ratio decreases on cooling through the structural/antiferromagnetic transition temperature T_{SM}, with the change mainly coming from stronger variation in ρ_a as compared with ρ_c. This suggests that the transitions stronger affect the two-dimensional parts of the Fermi surface. We compare our experimental observations with band structure calculations, and find similar trend in the evolution of anisotropy with the size of AE ion. Our results show that the electronic structure of the iron pnictides has large contribution from three-dimensional areas of the Fermi surface.

cond-mat.supr-con↗

Non-exponential London penetration depth in Ba$_{1-}$K$_{x}$Fe$_{2}$As$_{2}$ single crystals

We have studied the in- and out-of-plane magnetic penetration depths in the hole- doped iron based superconductor Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$ ($T_{c}\approx$ 30K). The study was performed on single crystals grown from different fluxes and we find that the results are nearly the same. The in-plane London penetration depth $λ_{ab}$ does not show exponential saturation at low temperature, as would be expected from a fully gapped superconductor. Instead, $λ_{ab}(T)$ shows a power-law behavior, $λ\propto T^{n}$ ($n\approx 2$), down to $T\approx 0.02 T_{c}$, similar to the electron doped Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$. The penetration depth anisotropy $γ_λ=λ_{c}(T)/λ_{ab}(T)$ increases upon cooling, opposite to the trend observed in the anisotropy of the upper critical field, $γ_ξ=H_{c2}^{\perp c}(0)/H_{c2}^{\parallel c}(0)$. These are universal characteristics of both the electron and hole doped 122 systems, suggesting unconventional superconductivity. The behavior of the in-plane superfluid density $ρ_{ab}(T)$ is discussed in light of existing theoretical models proposed for the iron pnictides superconductors.

cond-mat.supr-con↗

Doping dependent Irreversible Magnetic Properties of Ba(Fe1-xCox)2As2 Single Crystals

We discuss the irreversible magnetic properties of self-flux grown Ba(Fe1-xCox)2As2 single crystals for a wide range of concentrations covering the whole phase diagram from the underdoped to the overdoped regime, x=0.038, 0.047, 0.058, 0.071, 0.074, 0.10, 0.106 and 0.118. Samples were characterized by a magneto-optical method and show excellent spatial uniformity of the superconducting state. The overall behavior closely follows classical Bean model of the critical state. The field-dependent magnetization exhibits second peak at a temperature and doping - dependent magnetic field, Hp. The evolution of this fishtail feature with doping is discussed. Magnetic relaxation is time-logarithmic and unusually fast. Similar to cuprates, there is an apparent crossover from collective elastic to plastic flux creep above Hp. At high fields, the field dependence of the relaxation rate becomes doping independent. We discuss our results in the framework of the weak collective pinning and show that vortex physics in iron-based pnictide crystals is much closer to high-Tc cuprates than to conventional s-wave (including MgB2) superconductors.

cond-mat.supr-con↗

Anisotropic London Penetration Depth and Superfluid Density in Single Crystals of Iron-based Pnictide Superconductors

In- and out-of-plane magnetic penetration depths were measured in three iron-based pnictide superconducting systems. All studied samples of both 122 systems show a robust power-law behavior, $λ(T) T^n$, with the sample-dependent exponent n=2-2.5, which is indicative of unconventional pairing. This scenario could be possible either through scattering in a $s_{\pm }$ state or due to nodes in the superconducting gap. In the Nd-1111 system, the interpretation of data may be obscured by the magnetism of rare-earth ions. The overall anisotropy of the pnictide superconductors is small. The 1111 system is about two times more anisotropic than the 122 system. Our data and analysis suggest that the iron-based pnictides are complex superconductors in which a multiband three-dimensional electronic structure and strong magnetic fluctuations play important roles.

cond-mat.supr-con↗

Probing fractal magnetic domains on multiple length scales in Nd2Fe14B

Using small-angle neutron scattering, we demonstrate that the complex magnetic domain patterns at the surface of Nd2Fe14B, revealed by quantitative Kerr and Faraday microscopy, propagate into the bulk and exhibit structural features with dimensions down to 6 nm, the domain wall thickness. The observed fractal nature of the domain structures provides an explanation for the anomalous increase in the bulk magnetization of Nd2Fe14B below the spin-reorientation transition. These measurements open up a rich playground for studies of fractal structures in highly anisotropic magnetic systems.

cond-mat.mtrl-sci↗

Anisotropy of the Optimally-Doped Iron Pnictide Superconductor Ba(Fe0.926Co0.074)2As2

Anisotropies of electrical resistivity, upper critical field, London penetration depth and critical currents have been measured in single crystals of the optimally doped iron pnictide superconductor Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, $x$=0.074 and $T_c \sim$23 K. The normal state resistivity anisotropy was obtained by employing both the Montgomery technique and direct measurements on samples cut along principal crystallographic directions. The ratio $γ_ρ = ρ_c /ρ_a$ is about 4$\pm$1 just above $T_c$ and becomes half of that at room temperature. The anisotropy of the upper critical field, $γ_{H} = H_{c2,ab} /H_{c2,c} $, as determined from specific heat measurements close to $T_c$, is in the range of 2.1 to 2.6, depending on the criterion used. A comparable low anisotropy of the London penetration depth, $γ_λ=λ_{c}/λ_{ab}$, was recorded from TDR measurements and found to persist deep into the superconducting state. An anisotropy of comparable magnitude was also found in the critical currents, $γ_j=j_{c,ab}/j_{c,c}$, as determined from both direct transport measurements ($\sim$1.5) and from the analysis of the magnetization data ($\sim$3). Overall, our results show that iron pnictide superconductors manifest anisotropies consistent with essentially three-dimensional intermetallic compound and bear little resemblance to cuprates.

cond-mat.supr-con↗