arXiv subjects

R. Prozorov

Publications and source records attributed to R. Prozorov.

At least 163 records · Page 9Linked to original sources

arXiv2008

The London penetration depth in single crystals of Ba(Fe_{1-x}Co_x)_2As_2 at various doping levels

The London penetration depth $λ(T)$ has been measured in single crystals of Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ using the tunnel diode resonator technique. The measured doping levels of $x=$~0.038, 0.047, 0.058, 0.074 and 0.10 range from underdoped to overdoped concentrations. The measurements have shown that the density of carriers participating in superconductivity decreases sharply in the underdoped regime, but the penetration depth as a function of temperature exhibits a robust power law, $Δλ(T)\sim T^{n}$, for all measured dopings, with $n$ between 2 and 2.5. We discuss the implications of these results and possible interpretations of such robust behavior.

cond-mat.supr-con↗

arXiv2008

Unconventional London penetration depth in Ba(Fe0.93Co0.07)2As2 single crystals

The London penetration depth, $λ(T)$, has been measured in several single crystals of Ba(Fe$_{0.93}$Co$_{0.07}$)$_2$As$_2$. Thermodynamic, electromagnetic, and structural characterization measurements confirm that these crystals are of excellent quality. The observed low temperature variation of $λ(T)$ follows a power-law, $Δλ(T) \sim T^n$ with $n=2.4 \pm 0.1$, indicating the existence of normal quasiparticles down to at least $0.02T_c$. This is in contrast to recent penetration depth measurements on single crystals of NdFeAsO$_{1-x}$F$_x$ and SmFeAsO$_{1-x}$F$_x$, which indicate an anisotropic but nodeless gap. We propose that a more three-dimensional character in the electronic structure of Ba(Fe$_{0.93}$Co$_{0.07}$)$_2$As$_2$ may lead to an anisotropic $s-$wave gap with point nodes that would explain the observed $λ(T)$.

cond-mat.supr-con↗

arXiv2008

Vortex phase diagram of Ba(Fe0.93Co0.07)2As2 single crystals

Detailed measurements of the global and local electromagnetic properties of Ba(Fe$_{0.93}$Co$_{0.07}$)$_{2}$As$_{2}$ single crystals are reported. Analysis of the irreversible magnetic response provides strong evidence for similar vortex physics in this Fe-based pnictide superconductor to the high-$T_{c}$ cuprates, such as Y-Ba-Cu-O or Nd-Ce-Cu-O. In particular, we have found a nonmonotonic "fishtail" magnetization in $M(H,T=const)$ loops and its signature is also present in $M(H=const,T)$ scans. The supercurrent density is evaluated by using several techniques, including direct transport measurements. At 5 K we estimate its value to be a moderate $j \approx 2.6 \pm 0.2 \times 10^5$ A/cm$^2$. Analysis of the magnetic relaxation is consistent with the collective pinning and creep models (weak pinning and fast creep) and suggests a crossover from the collective to the plastic creep regime in fields exceeding the value corresponding to the maximum in fishtail magnetization.

cond-mat.supr-con↗

arXiv2008

Coexistence of Long-Range Magnetic Order and Superconductivity from Campbell Penetration Depth Measurements

Application of a tunnel-diode resonator (TDR) technique for studies of the vortex response in magnetic superconductors is described. Operating at very small excitation fields and sufficiently high frequency, TDR was used to probe small-amplitude linear AC response in several types of single crystals where long-range magnetic order coexists with bulk superconductivity. Full local - moment ferromagnetism destroys superconductivity and can coexist with it only in a narrow temperature range ($\sim 0.3$ K). In contrast, weak ferromagnetic as well as antiferromagnetic orders can coexist with bulk superconductivity and may even lead to enhancements of vortex pinning. By analyzing the Campbell penetration depth we find sharp increase of the true critical current in the vicinity of the magnetic phase transitions. We conclude that critical magnetic fluctuations are responsible for this enhancement.

cond-mat.supr-con↗

arXiv2008

Effect of doping on irreversible Campbell length in MgB$_2$ single crystals

We have measured small-amplitude rf penetration depth $λ(H,T)$ in pure and C, Li and (Li+C) doped single crystals of MgB$_2$. The effect of doping on the critical temperature T$_c$ and on the upper critical field H$_{c2}$ was found to be in good agreement with previous results. We report the presence of clear signatures of irreversibility in $λ(H,T)$, associated with the peak effect. Carbon doping enhances the signature and shifts its position on the H-T phase diagram to higher temperatures. Contrary to this, Li substitution has the effect of suppressing the peak effect to lower temperatures. Analysis of both zero field (ZFC) and field cooled (FC) measurements suggests that the hysteresis associated with the peak effect is due to macroscopic screening supercurrents, $j$, generated during the magnetic field ramp.

cond-mat.supr-con↗

arXiv2008

Field-dependent AC susceptibility of itinerant ferromagnets

Whereas dc measurements of magnetic susceptibility, $χ$, fail to distinguish between local and weak itinerant ferromagnets, radio-frequency (rf) measurements of $χ$ in the ferromagnetic state show dramatic differences between the two. We present sensitive tunnel-diode resonator measurements of $χ$ in the weak itinerant ferromagnet ZrZn$_2$ at a frequency of 23 MHz. Below Curie temperature, $T_C \approx 26$ K, the susceptibility is seen to increase and pass through a broad maximum at approximately 15 K in zero applied dc magnetic field. Application of a magnetic field reduces the amplitude of the maximum and shifts it to lower temperatures. The existence and evolution this maximum with applied field is not predicted by either the Stoner or self-consistent renormalized (SCR) spin fluctuations theories. For temperatures below $T_C$ both theories derive a zero-field limit expression for $χ$. We propose a semi-phenomenological model that considers the effect of the internal field from the polarized fraction of the conduction band on the remaining, unpolarized conduction band electrons. The developed model accurate describes the experimental data.

cond-mat.str-el↗

arXiv2008

Current-driven transformations of the intermediate state patterns in type-I superconductors

Dynamic structure of the intermediate state was studied in pinning-free thick Pb strips using real-time magneto-optical visualization. It is found that topological hysteresis can be lifted by applying sufficiently large current. Namely, laminar structure that appears on flux exit in a static case is turned into tubular when the sufficiently large transport current is present. Size and distribution of the flux tubes in static and dynamic regimes are different. Temperature, magnetic field and current phase diagram is discussed.

cond-mat.supr-con↗

arXiv2008

Fermi surface and strong coupling superconductivity in single crystal NdFeAsO_{1-x}F_x

We use angle-resolved photoemission spectroscopy (ARPES) to investigate the electronic properties of the newly discovered oxypnictide superconductor, NdFeAsO_{1-x}F_x. We find a well-defined Fermi surface that consists of a large hole pocket at the Brillouin zone center and a smaller electron pocket in each corner of the Brillouin zone. The overall location and shape of the Fermi surface agrees reasonably well with calculations. The band dispersion is quite complicated with many flat bands located just below the chemical potential. We observe a superconducting gap of 20 meV, which indicates that this system is in the strong coupling regime. The emergence of a coherent peak below the critical temperature Tc and diminished spectral weight at the chemical potential above Tc closely resembles the spectral characteristics of the cuprates.

cond-mat.supr-con↗

arXiv2008

Interplay of Local-Moment Ferromagnetism and Superconductivity in ErRh$_4$B$_4$ Single Crystals

Tunnel-diode resonator technique was used to study crystals of ferromagnetic re-entrant superconductor, ErRh$_{4}$B$_{4}$. At the boundary between ferromagnetism (FM) and superconductivity (SC), dynamic magnetic susceptibility, $χ(T,H)$, exhibits highly asymmetric behavior upon warming and cooling as well as enhanced diamagnetism on the SC side. SC phase nucleates upon warming in a cascade of discontinuous jumps in magnetic susceptibility $χ(T,H)$, whereas FM phase develops gradually as reported in detail in \cite{prozorov2008}. Here we further investigate enhanced diamagnetism. We find that when a magnetic field is applied along the magnetic easy axes, a region of enhanced diamagnetic screening is smaller than in the perpendicular orientation. A discussion of possible causes of this effect is provided.

cond-mat.supr-con↗

arXiv2008

Effect of high-intensity ultrasound on superconducting properties of polycrystalline YBCO

High intensity ultrasonic irradiation (sonication) of alkane slurries of polycrystalline \ybco leads to a significant modification of the grain morphology and, if performed with enforced oxygen flow, results in the increase of the superconducting transition temperature. Sonication with added Fe(CO)$_5$ produces magnetic \fe2o3 nanoparticles deposited on the surface of \ybco (YBCO) granules. Upon sintering these nanoparticles should act as efficient pinning centers utilizing both condensation and magnetic contributions to the free energy. The developed method could become a major technique to produce practically useful high-pinning nanocomposite materials based on \ybco superconductor.

cond-mat.supr-con↗

arXiv2008

Dynamic Formation of Metastable Intermediate State Patterns in Type-I Superconductors

Structure of the intermediate state in type-I superconducting lead (Pb) is shown to be very sensitive to the ramp rate of an applied magnetic field. The configurations of resulting static patterns depend sensitively on the shape of the specimen. In particular, geometric barrier, present in the samples with rectangular cross-section, plays an important role in determining the sharp boundary between the phases of different topology. We propose that seemingly laminar (stripe) pattern obtained as a result of the fast field ramp is simply an imprint left behind by the fast-moving flux tubes. Our results confirm that flux tube phase is topologically favorable.

cond-mat.supr-con↗

arXiv2008

Intrinsic magnetic properties of NdFeAsO$_{0.9}$F$_{0.1}$ superconductor from local and global measurements

Magneto-optical imaging was used to study the local magnetization in polycrystalline NdFeAsO$_{0.9}$F$_{0.1}$ (NFAOF). Individual crystallites up to $\sim200\times100\times30$ $μm^{3}$ in size could be mapped at various temperatures. The in-grain, persistent current density is about $j\sim10^{5}$ A/cm$^{2}$ and the magnetic relaxation rate in a remanent state peaks at about $T_{m}\sim38$ K. By comparison with with the total magnetization measured in a bar-shaped, dense, polycrystalline sample, we suggest that NdFeAsO$_{0.9}$F$_{0.1}$ is similar to a layered high-$T_{c}$, compound such as Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+x}$ and exhibits a $3D\to2D$ crossover in the vortex structure. The 2D Ginzburg parameter is about $Gi^{2D}% \simeq10^{-2}$ implying electromagnetic anisotropy as large as $ε\sim1/30$. Below $T_{m}$, the static and dynamic behaviors are consistent with collective pinning and creep.

cond-mat.supr-con↗

arXiv2008

^{7}Li NMR Study of Heavy Fermion LiV2O4 Containing Magnetic Defects

We present a systematic study of the variations of the ^{7}Li NMR properties versus magnetic defect concentration up to 0.83 mol% within the spinel structure of polycrystalline powder samples and a collection of small single crystals of LiV2O4 in the temperature range from 0.5 to 4.2 K. We also report static magnetization measurements and ac magnetic susceptibility measurements at 14 MHz on the samples at low temperatures. Both the NMR spectrum and nuclear spin-lattice relaxation rate are inhomogeneous in the presence of the magnetic defects. The NMR data for the powders are well explained by assuming that (i) there is a random distribution of magnetic point defects, (ii) the same heavy Fermi liquid is present in the samples containing the magnetic defects as in magnetically pure LiV2O4, and (iii) the influences of the magnetic defects and of the Fermi liquid on the magnetization and NMR properties are separable. In the single crystals, somewhat different behaviors are observed. Remarkably, the magnetic defects in the powder samples show evidence of spin freezing below T ~ 1.0 K, whereas in the single crystals with similar magnetic defect concentration no spin freezing was found down to 0.5 K. Thus different types of magnetic defects and/or interactions between them appear to arise in the powders versus the crystals, possibly due to the substantially different synthesis conditions of the powders and crystals.

cond-mat.str-el↗

arXiv2008

Exotic (anti)ferromagnetism in single crystals of Pr6Ni2Si3

The ternary intermetallic compound Pr6Ni2Si3, is a member of a structure series of compounds based on a triangular structure where the number of Pr atoms in the prism cross section can be systematically varied. Pr6Ni2Si3 contains two distinct Pr lattice sites which result in complex interactions between the magnetic ions. Extensive measurements of specific heat and magnetization on single crystal samples indicate that Pr6Ni2Si3 orders with both a ferromagnet and an antiferromagnet component, with ordering temperatures of 39.6 K and ~ 32 K, respectively. The ferromagnetic component // c-axis is accompanied by a large hysteresis, and the antiferromagnetic component,_|_ c-axis is accompanied by a spin-flop-type transition. More detailed measurements, of the vector magnetization, indicate that the ferromagnetic and the antiferromagnetic order appear independent of each other. These results not only clarify the behavior of Pr6Ni2Si3 itself, but also of the other members of the structure series, Pr5Ni2Si3 and Pr15Ni7Si10.

cond-mat.mtrl-sci↗

arXiv2008

Two-gap superconductivity in single crystal Lu$_2$Fe$_3$Si$_5$ from penetration depth measurements

Single crystal of Lu$_2$Fe$_3$Si$_5$ was studied with the tunnel-diode resonator technique in Meissner and mixed states. Temperature dependence of the superfluid density provides strong evidence for the two-gap superconductivity with almost equal contributions from each gap of magnitudes $Δ_1/k_BT_c=1.86$ and $Δ_1/k_BT_c=0.54$. In the vortex state, pinning strength shows unusually strong temperature dependence and is non-monotonic with the magnetic field (peak effect). The irreversibility line is sharply defined and is quite distant from the $H_{c2}(T)$, which hints on to enhanced vortex fluctuations in this two-gap system. Altogether our findings provide strong electromagnetic - measurements support to the two-gap superconductivity in Lu$_2$Fe$_3$Si$_5$ previously suggested from specific heat measurements.

cond-mat.supr-con↗

arXiv2007

Superfluid density in gapless superconductor CeCoIn5

Temperature dependence of the London penetration depth $λ$ measured in single crystals of CeCoIn$_5$ is interpreted as caused by a strong pair-breaking scattering that makes the superconductivity in this compound gapless. For a gapless d-wave superconductor, we derive $λ=λ_0/\sqrt{1-(T/T_c)^2}$ caused by combined effect of magnetic and non-magnetic scattering in excellent agreement with the data in the full temperature range and with the gapless s-wave case of Abrikosov and Gor'kov. We also obtain the slope of the upper critical field at $T_c$ that compares well with the measured slope.

cond-mat.supr-con↗

arXiv2007

Superconducting and normal state properties of the layered boride OsB2

OsB_2 crystallizes in an orthorhombic structure (Pmmn) which contains alternate boron and osmium layers stacked along the c-axis. The boron layers consist of puckered hexagons as opposed to the flat graphite-like boron layers in MgB_2. OsB_2 is reported to become superconducting below 2.1 K. We report results of the dynamic and static magnetic susceptibility, electrical resistivity, Hall effect, heat capacity and penetration depth measurements on arc-melted polycrystalline samples of OsB_2 to characterize its superconducting and normal state properties. These measurements confirmed that OsB_2 becomes a bulk superconductor below T_ c = 2.1 K. Our results indicate that OsB_2 is a moderate-coupling Type-II superconductor with an electron-phonon coupling constant λ_{ep} \approx 0.4 to 0.5, a small Ginzburg-Landau parameter κ\sim 1 to 2 and an upper critical magnetic field H_{c2}(0.5 K) \sim 420 Oe for an unannealed sample and H_{c2}(1 K) \sim 330 Oe for an annealed sample. The temperature dependence of the superfluid density n_{s}(T) for the unannealed sample is consistent with an s-wave superconductor with a slightly enhanced zero temperature gap Δ(0) = 1.9 k_{B}T_c and a zero temperature London penetration depth λ(0) = 0.38(2) μm. The n_{s}(T) data for the annealed sample shows deviations from the predictions of the single-band s-wave BCS model. The magnetic, transport and thermal properties in the normal state of isostructural and isoelectronic RuB_2, which is reported to become superconducting below 1.6 K, are also reported.

cond-mat.supr-con↗

arXiv2007

s-Wave superconductivity in non-centrosymmetric Re_3W probed by magnetic penetration depth

We report measurements of the temperature dependence of the magnetic penetration depth λ(T) in non-centrosymmetric superconductor Re_3W. We employed two experimental techniques: extraction of λ(T) from magnetic {\em dc}-susceptibility, measured on a powder sample, and the rf tunnel diode resonator technique, where a bulk polycrystalline sample was used. The results of both techniques agree: the temperature dependence of the penetration depth can be well described by weak-coupling, dirty-limit, s-wave BCS theory where we obtain $Δ(0)/k_BT_C=1.76$. No evidence for unconventional pairing resulting from the absence of the inversion symmetry is found.

cond-mat.supr-con↗