arXiv subjects

R. Saldanha

Publications and source records attributed to R. Saldanha.

At least 19 recordsLinked to original sources

arXiv2026

The nEXO Radioassay Program

Material radioactivity compilations, such as the one presented here, are important enablers of science. They are useful for the selection of radiopure materials used in the design and construction of low-energy rare-event search experiments. They allow researchers developing such experiments to save time on material studies and avoid costly duplication of effort. The data presented here were generated in support of the planned nEXO double-beta decay search. This work contains among the most restrictive constraints on the natural radioactivity content of materials of general interest to the low-radioactivity community, found in any tabulation of this kind. In this study, various techniques were employed; they are described here.

physics.ins-det↗

arXiv2026

Design of a high voltage delivery system for noble liquid time projection chambers

Noble liquid time projection chambers (TPCs) are a leading technology in the detection of ionizing radiation, particularly in applications such as accelerator neutrino physics, dark matter detection, and neutrinoless double beta decay. This paper addresses the design considerations for implementing stable high voltage (HV) systems within large noble liquid TPCs, with a focus on the nEXO experiment. Utilizing insights from prior HV research and experimental investigations, we outline factors influencing HV stability and discuss design choices to improve stability and prevent electrical discharges. A novel HV delivery system concept is presented, tailored for the nEXO TPC, which incorporates these design considerations while also meeting the stringent radiopurity requirements of the nEXO neutrinoless double beta decay search. These design considerations and their specific implementation towards a HV delivery system offer guidance to future experiments applying high voltage in noble liquid environments.

physics.ins-det↗

arXiv2026

Enhanced sensitivity to trace $^{238}$U impurity of sapphire via coincidence neutron activation analysis

Sapphire has mechanical and electrical properties that are advantageous for the construction of internal components of radiation detectors such as time projection chambers and bolometers. However, it has proved difficult to assess its $\rm ^{232}Th$ and $\rm ^{238}U$ content down to the picogram per gram level. This work reports an experimental verification of a computational study that demonstrates $γγ$ coincidence counting, coupled with neutron activation analysis (NAA), can reach ppt sensitivities. Combining results from $γγ$ coincidence counting with those of earlier single-$γ$ counting based NAA shows that a sample of Saint Gobain sapphire has $\rm ^{232}Th$ and $\rm ^{238}U$ concentrations of $<0.26$ ppt and $<2.3$ ppt, respectively; the best constraints on the radiopurity of sapphire.

nucl-ex↗

arXiv2025

Removal of spallation-induced tritium from silicon through diffusion

Tritium, predominantly produced through spallation reactions caused by cosmic ray interactions, is a significant radioactive background for silicon-based rare event detection experiments, such as dark matter searches. We have investigated the feasibility of removing cosmogenic tritium from high-purity silicon intended for use in low-background experiments. We demonstrate that significant tritium removal is possible through diffusion by subjecting silicon to high-temperature (> 400C) baking. Using an analytical model for the de-trapping and diffusion of tritium in silicon, our measurements indicate that cosmogenic tritium diffusion constants are comparable to previous measurements of thermally-introduced tritium, with complete de-trapping and removal achievable above 750C. This approach has the potential to alleviate the stringent constraints of cosmic ray exposure prior to device fabrication and significantly reduce the cosmogenic tritium backgrounds of silicon-based detectors for next-generation rare event searches.

physics.ins-det↗

arXiv2025

Scintillation of liquid nitrogen

Liquid nitrogen is commonly used in cryogenic applications and is a promising medium for the direct immersion cooling of sensors used for nuclear and particle physics experiments. The scintillation properties of gaseous nitrogen are well-documented, but little is known about the scintillation of liquid nitrogen. If present, scintillation light from interactions of ambient radioactivity could produce backgrounds for rare event searches such as the direct detection of dark matter. Using a coincidence-tagged alpha decay, we demonstrate that liquid nitrogen exhibits measurable, albeit very faint, scintillation. Assuming the same scintillation wavelength spectrum as gaseous nitrogen, we estimate a relative scintillation yield of $Y_{\text{LN}}/Y^{\text{STP}}_{\text{GN}} = 0.0142 \pm 0.0005\text{(stat)} \pm 0.0030\text{(sys)}$ with respect to gaseous nitrogen at standard temperature and pressure. Considering the average scintillation yield from alpha decays in gaseous nitrogen, this implies a scintillation yield for alpha decays in liquid nitrogen of $Y_{\text{LN}} = 2.39 \pm 0.56$ photons per MeV. To our knowledge this is the first measurement of scintillation in liquid nitrogen.

physics.ins-det↗

arXiv2025

First Production of Skipper-CCD Modules for the DAMIC-M Experiment

The DAMIC-M experiment will search for sub-GeV dark matter particles with a large array of silicon skipper charge-coupled devices (CCDs) at the Modane Underground Laboratory (LSM) in France. After five years of development, we recently completed the production of 28 CCD modules at the University of Washington, each consisting of four 9-megapixel skipper CCDs. Material screening and background controls were implemented to meet stringent radio-purity targets, while extensive testing was employed to select science-grade CCDs for the modules and confirm their excellent performance after fabrication. Further testing at LSM will select 26 of these modules (${\sim}$350 g active mass) to be installed and operated in the DAMIC-M detector in early 2026.

physics.ins-det↗

arXiv2025

Ultra-pure Nickel for Structural Components of Low-Radioactivity Instruments

The next generation of rare-event search experiments in nuclear and particle physics demand structural materials combining exceptional mechanical strength with ultra-low levels of radioactive contamination. This study evaluates chemical vapor deposition (CVD) nickel as a candidate structural material for such applications. Manufacturer-supplied CVD Ni grown on aluminum substrates underwent tensile testing before and after welding alongside standard Ni samples. CVD Ni exhibited a planar tensile strength of ~600 MPa, significantly surpassing standard nickel. However, welding and heat treatment were found to reduce the tensile strength to levels comparable to standard Ni, with observed porosity in the welds likely contributing to this reduction. Material assay via inductively coupled plasma mass spectrometry (ICP-MS) employing isotope-dilution produced measured bulk concentration of 232-Th, 238-U, and nat-K at the levels of ~70 ppq, <100 ppq, and ~900 ppt, respectively, which is the lowest reported in nickel. Surface-etch profiling uncovered higher concentrations of these contaminants extending ~10 micrometer beneath the surface, likely associated with the aluminum growth substrate. The results reported are compared to the one other well documented usage of CVD Ni in a low radioactive background physics research experiment and a discussion is provided on how the currently reported results may arise from changes in CVD fabrication or testing process. These results establish CVD Ni as a promising low-radioactivity structural material, while outlining the need for further development in welding and surface cleaning techniques to fully realize its potential in large-scale, low radioactive background rare-event search experiments.

nucl-ex↗

arXiv2025

Sensitivity of nEXO to $^{136}$Xe Charged-Current Interactions: Background-free Searches for Solar Neutrinos and Fermionic Dark Matter

We study the sensitivity of nEXO to solar neutrino charged-current interactions, $ν_e + ^{136}$Xe$\rightarrow ^{136}$Cs$^* + e^-$, as well as analogous interactions predicted by models of fermionic dark matter. Due to the recently observed low-lying isomeric states of $^{136}$Cs, these interactions will create a time-delayed coincident signal observable in the scintillation channel. Here we develop a detailed Monte Carlo of scintillation emission, propagation, and detection in the nEXO detector to model these signals under different assumptions about the timing resolution of the photosensor readout. We show this correlated signal can be used to achieve background discrimination on the order of $10^{-9}$, enabling nEXO to make background-free measurements of solar neutrinos above the reaction threshold of 0.668 MeV. We project that nEXO could measure the flux of CNO solar neutrinos with a statistical uncertainty of 25%, thus contributing a novel and competitive measurement towards addressing the solar metallicity problem. Additionally, nEXO could measure the mean energy of the $^7$Be neutrinos with a precision of $σ\leq 1.5$ keV and could determine the survival probability of $^{7}$Be and $pep$ solar $ν_e$ with precision comparable to state-of-the-art. These quantities are sensitive to the Sun's core temperature and to non-standard neutrino interactions, respectively. Furthermore, the strong background suppression would allow nEXO to search for for charged-current interactions of fermionic dark matter in the mass range $m_χ$ = $0.668$-$7$ MeV with a sensitivity up to three orders of magnitude better than current limits.

nucl-ex↗

arXiv2024

Report from the Workshop on Xenon Detector $0νββ$ Searches: Steps Towards the Kilotonne Scale

These proceedings summarize the program and discussions of the ``Workshop on Xenon Detector $0νββ$ Searches: Steps Towards the Kilotonne Scale'' held on October 25-27 2023 at SLAC National Accelerator Laboratory. This workshop brought together experts from the communities of neutrinoless double-beta decay and dark matter detection, to discuss paths forward for the realization of monolithic experiments with xenon approaching the kilotonne scale.

nucl-ex↗

arXiv2023

Large Low Background kTon-Scale Liquid Argon Time Projection Chambers

We find that it is possible to increase sensitivity to low energy physics in a third or fourth DUNE-like module with careful controls over radiopurity and targeted modifications to a detector similar to the DUNE Far Detector design. In particular, sensitivity to supernova and solar neutrinos can be enhanced with improved MeV-scale reach. A neutrinoless double beta decay search with $^{136}$Xe loading appears feasible. Furthermore, sensitivity to Weakly-Interacting Massive Particle (WIMP) Dark Matter (DM) becomes competitive with the planned world program in such a detector, offering a unique seasonal variation detection that is characteristic for the nature of WIMPs.

hep-ex↗

arXiv2022

Cosmogenic activation of sodium iodide

The production of radioactive isotopes by interactions of cosmic-ray particles with sodium iodide (NaI) crystals can produce radioactive backgrounds in detectors used to search for rare events. Through controlled irradiation of NaI crystals with a neutron beam that matches the cosmic-ray neutron spectrum, followed by direct counting and fitting the resulting spectrum across a broad range of energies, we determined the integrated production rate of several long-lived radioisotopes. The measurements were then extrapolated to determine the sea-level cosmogenic neutron activation rate, including the first experimental determination of the tritium production rate: $(80 \pm 21)$ atoms/kg/day. These results will help constrain background estimates and determine the maximum time that NaI-based detectors can remain unshielded above ground before cosmogenic backgrounds impact the sensitivity of next-generation experiments.

hep-ex↗

arXiv2022

Low Background kTon-Scale Liquid Argon Time Projection Chambers

We find that it is possible to increase sensitivity to low energy physics in a third or fourth DUNE-like module with careful controls over radiopurity and some modifications to a detector similar to the DUNE Far Detector design. In particular, sensitivity to supernova and solar neutrinos can be enhanced with improved MeV-scale reach. A neutrinoless double beta decay search with $^{136}$Xe loading appears feasible. Furthermore, sensitivity to Weakly-Interacting Massive Particle (WIMP) Dark Matter (DM) becomes competitive with the planned world program in such a detector, offering a unique seasonal variation detection that is characteristic for the nature of WIMPs.

physics.ins-det↗

arXiv2022

Simulated Thick, Fully-Depleted CCD Exposures Analyzed with Deep Learning Techniques

Thick, Charge Coupled Devices (CCDs) have recently been explored for applied physics, such as nuclear explosion monitoring, and dark matter detection purposes. When run in fully-depleted mode, these devices are sensitive detectors for energy depositions by a variety of primary particles. In this study we are interested in applying the Deep Learning (DL) technique known as panoptic segmentation to simulated CCD images to identify, attribute and measure energy depositions from radioisotopes of interest. We simulate CCD exposures of a chosen radioxenon isotope, $^{135}$Xe, and overlay a simulated cosmic muon background appropriate for a surface-lab. We show that with this DL technique we can reproduce the beta spectrum to good accuracy, while suffering expected confusion with same-topology gammas and conversion electrons and identifying cosmic muons less than optimally.

physics.ins-det↗

arXiv2021

Kiloton-scale xenon detectors for neutrinoless double beta decay and other new physics searches

Large detectors employing xenon are a leading technology in existing and planned searches for new physics, including searches for neutrinoless double beta decay ($0νββ$) and dark matter. While upcoming detectors will employ target masses of a ton or more, further extending gas or liquid phase Xe detectors to the kton scale would enable extremely sensitive next-generation searches for rare phenomena. The key challenge to extending this technology to detectors well beyond the ton scale is the acquisition of the Xe itself. We describe the motivation for extending Xe time projection chambers (TPCs) to the kton scale and possible avenues for Xe acquisition that avoid existing supply chains. If acquisition of Xe in the required quantities is successful, kton-scale detectors of this type could enable a new generation of experiments, including searches for $0νββ$ at half-life sensitivities as long as $10^{30}$ yr.

physics.ins-det↗

arXiv2020

Cosmogenic activation of silicon

The production of $^{3}$H, $^{7}$Be, and $^{22}$Na by interactions of cosmic-ray particles with silicon can produce radioactive backgrounds in detectors used to search for rare events. Through controlled irradiation of silicon CCDs and wafers with a neutron beam that mimics the cosmic-ray neutron spectrum, followed by direct counting, we determined that the production rate from cosmic-ray neutrons at sea level is ($112 \pm 24$) atoms/(kg day) for $^{3}$H, ($8.1 \pm 1.9 $) atoms/(kg day) for $^{7}$Be, and ($43.0 \pm 7.1 $) atoms/(kg day) for $^{22}$Na. Complementing these results with the current best estimates of activation cross sections for cosmic-ray particles other than neutrons, we obtain a total sea-level cosmic-ray production rate of ($124 \pm 24$) atoms/(kg day) for $^{3}$H, ($9.4 \pm 2.0 $) atoms/(kg day) for $^{7}$Be, and ($49.6 \pm 7.3 $) atoms/(kg day) for $^{22}$Na. These measurements will help constrain background estimates and determine the maximum time that silicon-based detectors can remain unshielded during detector fabrication before cosmogenic backgrounds impact the sensitivity of next-generation rare-event searches.

physics.ins-det↗

arXiv2020

Measurement of the onset of nucleate boiling in liquid xenon

We report the first precision measurement of the superheat temperature required for bubble nucleation in liquid xenon of $ΔT_{wall,ONB}$ = (16.9$\pm$0.5) K and $ΔT_{wall,ONB}$ = (19.2$^{+0.4}_{-1.1}$) K at pressures of P = $(0.98\pm0.02)$ bar and P = $(1.32^{+0.05}_{-0.01})$ bar, respectively. Both are measured at a subcooled bulk fluid temperature of $\sim$ 162 K. A dedicated liquid xenon setup is used to measure the temperature at which bubble nucleation first appears on the flat surface of a resistor. The associated average heat flux at the surface of the resistor is determined using fluid dynamics simulations. Future experiments can use these experimental results to determine the likelihood of boiling in liquid xenon and to design effective thermal sinks that prevent bubble nucleation.

physics.ins-det↗

arXiv2019

Cosmogenic production of $^{39}$Ar and $^{37}$Ar in argon

We have experimentally determined the production rate of $^{39}$Ar and $^{37}$Ar from cosmic ray neutron interactions in argon at sea level. Understanding these production rates is important for argon-based dark matter experiments that plan to utilize argon extracted from deep underground because it is imperative to know what the ingrowth of $^{39}$Ar will be during the production, transport, and storage of the underground argon. These measurements also allow for the prediction of $^{39}$Ar and $^{37}$Ar concentrations in the atmosphere which can be used to determine the presence of other sources of these isotopes. Through controlled irradiation with a neutron beam that mimics the cosmic ray neutron spectrum, followed by direct counting of $^{39}$Ar and $^{37}$Ar decays with sensitive ultra-low background proportional counters, we determined that the production rate from cosmic ray neutrons at sea-level is expected to be $(759 \pm 128)$ atoms/kg$_\text{Ar}$/day for $^{39}$Ar, and $(51.0 \pm 7.4)$ atoms/kg$_\text{Ar}$/day for $^{37}$Ar. We also performed a survey of the alternate production mechanisms based on the state-of-knowledge of the associated cross-sections to obtain a total sea-level cosmic ray production rate of $(1048 \pm 133)$ atoms/kg$_\text{Ar}$/day for $^{39}$Ar, $(56.7 \pm 7.5)$ atoms/kg$_\text{Ar}$/day for $^{37}$Ar in underground argon, and $(92 \pm 13)$ atoms/kg$_\text{Ar}$/day for $^{37}$Ar in atmospheric argon.

nucl-ex↗

arXiv2018

Treatment of material radioassay measurements in projecting sensitivity for low-background experiments

By analyzing sensitivity projections as a statisical estimation problem, we evaluated different ways of treating radioassay measurement results (values and upper limits) when projecting sensitivity for low-background experiments. We developed a figure of merit that incorporates a notion of conservativeness to quantitatively explore the consequences of attempts to bias sensitivity projections, and proposed a method to report sensitivity.

physics.data-an↗