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Ramamoorthy Ramesh

Publications and source records attributed to Ramamoorthy Ramesh.

At least 37 records · Page 2Linked to original sources

Low-energy domain wall racetracks with multiferroic topologies

Conventional racetrack memories move information by pushing magnetic domain walls or other spin textures with spin-polarized currents, but the accompanying Joule heating inflates their energy budget and can hamper scaling. Here we present a voltage-controlled, magnetoelectric racetrack in which transverse electric fields translate coupled ferroelectric-antiferromagnetic walls along BiFeO3 nanostrips at room temperature. Because no charge traverses the track, the switching dissipates orders of magnitude less energy than the most efficient spin-torque devices with more favourable scaling, making the scheme significantly more attractive at the nanoscale. We further uncover noncollinear topological magnetoelectric textures that emerge at domain walls in BiFeO3, where the nature of these topologies influences their stability upon translation. Among these are polar bi-merons and polar vertices magnetoelectrically coupled with magnetic cycloid disclinations and previously unobserved, topological magnetic cycloid twist topologies. We observe domain wall velocities of at least kilometres per second - matching or surpassing the fastest ferrimagnetic and antiferromagnetic racetracks and approaching the acoustic-phonon limit of BiFeO3 - while preserving these topologies over tens of micrometres. The resulting high velocity, low-energy racetrack delivers nanosecond access times without the thermal overhead of current-driven schemes, charting a path toward dense, ultralow-power racetrack devices which rely on spin texture translation.

cond-mat.mtrl-sci↗

Electron-magnon coupling at the interface of a "twin-twisted" antiferromagnet

We identify a "twin-twist" angle in orthorhombic two-dimensional magnets that maximizes interlayer orbital overlap and enables strong interfacial coupling. Focusing on the van der Waals antiferromagnet CrSBr, we show that this twist angle, near 72 deg, aligns diagonal lattice vectors across the layers, enhancing the interlayer hopping that is spin-forbidden in pristine systems and orbital-forbidden in 90-deg-twisted samples. The enhanced hopping modifies the electronic structure and activates a novel mechanism for excitation of interfacial magnons. Using optical probes we discover that excitons on one side of the interface selectively excite magnons localized on the opposite side. We show that this cross-coupling phenomenon can be understood as a consequence of the spin-transfer torque as that arises as electrons tunnel across the twin-twisted interface. Our findings demonstrate that large-angle twisting in anisotropic 2D materials offers a powerful tool for engineering spin and charge transport through controlled interlayer hybridization, opening new avenues for twisted magnetism and strongly correlated moiré physics.

cond-mat.mes-hall↗

Emergence of Transverse Dielectric Response in Ferroelectric Dielectric Heterostructures

We report the emergence of a transverse dielectric response in PbTiO$_{3}$/SrTiO$_{3}$ superlattices hosting polar vortex structures. Using second-principles simulations, we find that an electric field applied along one direction induces significant local polarization responses along orthogonal directions, with magnitudes approaching half that of the diagonal susceptibility components. These off-diagonal responses are strongly dependent on the topology of the vortex structure and can be deterministically tuned or even reversed via homogeneous electric fields or epitaxial strain. Notably, the transverse susceptibilities become comparable to the diagonal components during a field- or strain-induced transition to a polarization wave state. This discovery opens avenues for engineering reconfigurable nanoscale dielectric responses in topologically textured ferroelectric systems.

cond-mat.mtrl-sci↗

Colossal enhancement of spin transmission through magnon confinement in an antiferromagnet

Since Felix Bloch's introduction of the concept of spin waves in 1930, magnons (the quanta of spin waves) have been extensively studied in a range of materials for spintronics, particularly for non-volatile logic-in-memory devices. Controlling magnons in conventional antiferromagnets and harnessing them in practical applications, however, remains a challenge. In this letter, we demonstrate highly efficient magnon transport in an LaFeO$_3$/BiFeO$_3$/LaFeO$_3$ all-antiferromagnetic system which can be controlled electrically, making it highly desirable for energy-efficient computation. Leveraging spin-orbit-driven spin-charge transduction, we demonstrate that this material architecture permits magnon confinement in ultrathin antiferromagnets, enhancing the output voltage generated by magnon transport by several orders of magnitude, which provides a pathway to enable magnetoelectric memory and logic functionalities. Additionally, its non-volatility enables ultralow-power logic-in-memory processing, where magnonic devices can be efficiently reconfigured via electrically controlled magnon spin currents within magnetoelectric channels.

cond-mat.mtrl-sci↗

Magnon thermal conductivity in multiferroics with spin cycloids

Multiferroic materials, characterized by the occurrence of two or more ferroic properties, hold potential in future technological applications and also exhibit intriguing phenomena caused by the interplay of multiple orders. One such example is the formation of spin cycloid structures within multiferroic materials, which we investigate in this work by focusing on their magnon excitations and transport based on a general multiferroic Hamiltonian with an antiferromagnetic order. More specifically, we identify the ground state and explore the dynamics of magnon modes, revealing distinct in-plane and out-of-plane modes with anisotropic dispersion relations.The magnon modes include a massless excitation, known as the Goldstone boson, originating from the spontaneous breaking of the translational symmetry by the formation of the cycloid structures. By employing the Boltzmann transport formalism, the magnonic thermal conductivity with spin cycloids and low-temperature anisotropic behaviors is discussed. This work provides pathways to envision the spin-textured multiferroics, which may serve as a fertile ground to look for novel thermal and spin transport with the rich interplay of quasiparticles such as magnons and phonons.

cond-mat.mtrl-sci↗

Improper Ferroelectricity at the Monolayer Limit

Ultrathin ferroelectric films with out-of-plane polarization and high Curie temperatures are key to miniaturizing electronic devices. Most ferroelectrics employed in devices are proper ferroelectrics, where spontaneous polarization is the primary order parameter. Unfortunately, the Curie temperature of proper ferroelectrics is drastically reduced as the ferroelectric becomes thin; nearly all proper ferroelectrics need to be thicker than several unit cells. The absence of an ultrathin limit has been predicted, but not verified for improper ferroelectrics. These are ferroelectrics where the polarization emerges secondary to the primary order parameter, such as a structural distortion. Here we report improper ferroelectricity with an undiminished Curie temperature in a 0.75-unit-cell-thick hexagonal LuFeO3 (h-LuFeO3) film grown on a SrCo2Ru4O11 bottom electrode with an atomically engineered monolayer bridging layer. Our results demonstrate the absence of a critical thickness for improper ferroelectricity and provide a methodology for creating ultrathin improper ferroelectrics by stabilizing their primary order parameters.

cond-mat.mtrl-sci↗

Spin frustration and unconventional spin twisting state in van der Waals ferromagnet/antiferromagnet heterostructures

Atomically flat surfaces of van der Waals (vdW) materials pave an avenue for addressing a long-standing fundamental issue of how a perfectly compensated antiferromagnet (AFM) surface frustrates a ferromagnetic (FM) overlayer in FM/AFM heterostructures. By revealing the AFM and FM spin structures separately in vdW Fe5GeTe2/NiPS3 heterostructures, we find that C-type in-plane AFM NiPS3 develops three equivalent AFM domains which are robust against external magnetic field and magnetic coupling with Fe5GeTe2. Consequently, spin frustration at the Fe5GeTe2/NiPS3 interface was shown to develop a perpendicular Fe5GeTe2 magnetization in the interfacial region that switches separately from the bulk of the Fe5GeTe2 magnetizations. In particular, we discover an unconventional spin twisting state that the Fe5GeTe2 spins twist from perpendicular direction near the interface to in-plane direction away from the interface in Fe5GeTe2/NiPS3. Our finding of the twisting spin texture is a unique property of spin frustration in van der Waals magnetic heterostructures.

cond-mat.mtrl-sci↗

Epitaxial Strain Tuning of Er3+ in Ferroelectric Thin Films

Er3+ color centers are promising candidates for quantum science and technology due to their long electron and nuclear spin coherence times, as well as their desirable emission wavelength. By selecting host materials with suitable, controllable properties, we introduce new parameters that can be used to tailor the Er3+ emission spectrum. PbTiO3 is a well-studied ferroelectric material with known methods of engineering different domain configurations through epitaxial strain. By distorting the structure of Er3+-doped PbTiO3 thin films, we can manipulate the crystal fields around the Er3+ dopant. This is resolved through changes in the Er3+ resonant fluorescence spectra, tying the optical properties of the defect directly to the domain configurations of the ferroelectic matrix. Additionally, we are able to resolve a second set of peaks for films with in-plane ferroelectric polarization. We hypothesize these results to be due to either the Er3+ substituting different sites of the PbTiO3 crystal, differences in charges between the Er3+ dopant and the original substituent ion, or selection rules. Systematically studying the relationship between the Er3+ emission and the epitaxial strain of the ferroelectric matrix lays the pathway for future optical studies of spin manipulation by altering ferroelectric order parameters

cond-mat.mtrl-sci↗

Continuous Collapse of the Spin Cycloid in BiFeO3 Thin Films under an Applied Magnetic Field probed by Neutron Scattering

Bismuth ferrite (BiFeO3) is one of the rare materials that exhibits multiferroic properties already at room-temperature. Therefore, it offers tremendous potential for future technological applications, such as memory and logic. However, a weak magnetoelectric coupling together with the presence of a noncollinear cycloidal spin order restricts various practical applications of BiFeO3. Therefore, there is a large interest in the search for suitable methods for the modulation of the spin cycloid in BiFeO3. By performing neutron diffraction experiments using a triple-axis instrument we have determined that the spin cycloid can be systematically suppressed by applying a high magnetic field of 10 T in a BiFeO3 thin film of about 100 nm grown on a (110)-oriented SrTiO3 substrate. As predicted by previous theoretical calculations, we observed that the required critical magnetic field to suppress the spin cycloid in a BiFeO3 thin film was lower as compared to the previously reported critical magnetic field for bulk BiFeO3 single crystals. Our experiment reveals that the spin cycloid continuously expands with increasing magnetic field before the complete transformation into a G-type antiferromagnetic spin order. Such tuning of the length of the spin cycloid up to a complete suppression offers new functionalities for future technological applications as in spintronics or magnonics.

cond-mat.mtrl-sci↗

Low-Field Regime of Magnon Transport in Yttrium Iron Garnet

Diffusive propagation of spin waves and their quanta - magnons - in the archetypal magnetic insulator yttrium iron garnet (YIG) is under a surge of research for low-power and low-loss data communication. However, operation under external magnetic fields reduces magnon diffusion length, attenuates the voltage amplitude at measurement terminals, and complicates the architecture of magnonic devices. Here, we explore the low-field and field-free regime of diffusive magnon transport in YIG films. We demonstrate that the field-induced suppression of magnon diffusion length can be fully inhibited only at the zero-field limit. Even a modest field of 10mT attenuates the non-local spin voltage by $\sim$ 20$\%$ in a transport channel of $\sim$ 1$μ$m long. Using Stoner-Wohlfarth macrospin simulations, we reveal that an often overlooked, in-plane uniaxial anisotropy becomes the critical parameter governing the field-free operation of magnonic devices. We further demonstrate a tenfold enhancement in the effective field associated with the in-plane uniaxial anisotropy of YIG films at low temperatures - a key finding for field-free operation of magnonic devices under cryogenic conditions.

cond-mat.mes-hall↗

Symmetry-based phenomenological model for magnon transport in a multiferroic

Magnons carriers of spin information can be controlled by electric fields in the multiferroic BiFeO$_3$ (BFO), a milestone that brings magnons closer to application in future devices. The origin of magnon-spin currents in BFO, however, is not fully understood due to BFO's complicated magnetic texture. In this letter, we present a phenomenological model to elucidate the existence of magnon spin currents in generalized multiferroics by examining the symmetries inherent to their magnetic and polar structures. This model is grounded in experimental data obtained from BFO and its derivatives, which informs the symmetry operations and resultant magnon behavior. By doing so, we address the issue of symmetry-allowed, switchable magnon spin transport in multiferroics, thereby establishing a critical framework for comprehending magnon transport within complex magnetic textures.

cond-mat.mtrl-sci↗

Voltage-based magnetization switching and reading in magnetoelectric spin-orbit nanodevices

As CMOS technologies face challenges in dimensional and voltage scaling, the demand for novel logic devices has never been greater, with spin-based devices offering scaling potential, at the cost of significantly high switching energies. Alternatively, magnetoelectric materials are predicted to enable low-power magnetization control, a solution with limited device-level results. Here, we demonstrate voltage-based magnetization switching and reading in nanodevices at room temperature, enabled by exchange coupling between multiferroic BiFeO$_3$ and ferromagnetic CoFe, for writing, and spin-to-charge current conversion between CoFe and Pt, for reading. We show that upon the electrical switching of the BiFeO$_3$, the magnetization of the CoFe can be reversed, giving rise to different voltage outputs. Through additional microscopy techniques, magnetization reversal is linked with the polarization state and antiferromagnetic cycloid propagation direction in the BiFeO$_3$. This study constitutes the building block for magnetoelectric spin-orbit logic, opening a new avenue for low-power beyond-CMOS technologies.

cond-mat.mes-hall↗

Morphogenesis of Spin Cycloids in a Non-collinear Antiferromagnet

Pattern formation in spin systems with continuous-rotational symmetry (CRS) provides a powerful platform to study emergent complex magnetic phases and topological defects in condensed-matter physics. However, its understanding and correlation with unconventional magnetic order along with high-resolution nanoscale imaging is challenging. Here, we employ scanning NV magnetometry to unveil the morphogenesis of spin cycloids at both the local and global scales within a single ferroelectric domain of (111)-oriented BiFeO$_3$ (which is a non-collinear antiferromagnet), resulting in formation of a glassy labyrinthine pattern. We find that the domains of locally oriented cycloids are interconnected by an array of topological defects and exhibit isotropic energy landscape predicted by first-principles calculations. We propose that the CRS of spin-cycloid propagation directions within the (111) drives the formation of the labyrinthine pattern and the associated topological defects such as antiferromagnetic skyrmions. Unexpectedly, reversing the as-grown ferroelectric polarization from [$\bar{1}$$\bar{1}$$\bar{1}$] to [111] induces a magnetic phase transition, destroying the labyrinthine pattern and producing a deterministic non-volatile non cycloidal, uniformly magnetized state. These findings highlight that (111)-oriented BiFeO$_3$ is not only important for studying the fascinating subject of pattern formation but could also be utilized as an ideal platform for integrating novel topological defects in the field of antiferromagnetic spintronics.

cond-mat.mtrl-sci↗

Optical Control of Adaptive Nanoscale Domain Networks

Adaptive networks can sense and adjust to dynamic environments to optimize their performance. Understanding their nanoscale responses to external stimuli is essential for applications in nanodevices and neuromorphic computing. However, it is challenging to image such responses on the nanoscale with crystallographic sensitivity. Here, the evolution of nanodomain networks in (PbTiO3)n/(SrTiO3)n superlattices was directly visualized in real space as the system adapts to ultrafast repetitive optical excitations that emulate controlled neural inputs. The adaptive response allows the system to explore a wealth of metastable states that were previously inaccessible. Their reconfiguration and competition were quantitatively measured by scanning x-ray nanodiffraction as a function of the number of applied pulses, in which crystallographic characteristics were quantitatively assessed by assorted diffraction patterns using unsupervised machine-learning methods. The corresponding domain boundaries and their connectivity were drastically altered by light, holding promise for light-programmable nanocircuits in analogy to neuroplasticity. Phase-field simulations elucidate that the reconfiguration of the domain networks is a result of the interplay between photocarriers and transient lattice temperature. The demonstrated optical control scheme and the uncovered nanoscopic insights open opportunities for remote control of adaptive nanoscale domain networks.

cond-mat.mes-hall↗

Non-volatile spin transport in a single domain multiferroic

Antiferromagnets have attracted significant attention in the field of magnonics, as promising candidates for ultralow-energy carriers for information transfer for future computing. The role of crystalline orientation distribution on magnon transport has received very little attention. In multiferroics such as BiFeO$_3$ the coupling between antiferromagnetic and polar order imposes yet another boundary condition on spin transport. Thus, understanding the fundamentals of spin transport in such systems requires a single domain, a single crystal. We show that through Lanthanum(La) substitution, a single ferroelectric domain can be engineered with a stable, single-variant spin cycloid, controllable by an electric field. The spin transport in such a single domain displays a strong anisotropy, arising from the underlying spin cycloid lattice. Our work shows a pathway to understand the fundamental origins of spin transport in such a single domain multiferroic.

cond-mat.mtrl-sci↗

Designed spin-texture-lattice to control anisotropic magnon transport in antiferromagnets

Spin waves in magnetic materials are promising information carriers for future computing technologies due to their ultra-low energy dissipation and long coherence length. Antiferromagnets are strong candidate materials due, in part, to their stability to external fields and larger group velocities. Multiferroic aniferromagnets, such as BiFeO$_3$ (BFO), have an additional degree of freedom stemming from magnetoelectric coupling, allowing for control of the magnetic structure, and thus spin waves, with electric field. Unfortunately, spin-wave propagation in BFO is not well understood due to the complexity of the magnetic structure. In this work, we explore long-range spin transport within an epitaxially engineered, electrically tunable, one-dimensional (1D) magnonic crystal. We discover a striking anisotropy in the spin transport parallel and perpendicular to the 1D crystal axis. Multiscale theory and simulation suggests that this preferential magnon conduction emerges from a combination of a population imbalance in its dispersion, as well as anisotropic structural scattering. This work provides a pathway to electrically-reconfigurable magnonic crystals in antiferromagnets.

cond-mat.mtrl-sci↗

Non-equilibrium pathways to emergent polar supertextures

Ultrafast stimuli can stabilize metastable states of matter inaccessible by equilibrium means. Establishing the spatiotemporal link between ultrafast excitation and metastability is crucial to understanding these phenomena. Here, we use single-shot optical-pump, X-ray-probe measurements to provide snapshots of the emergence of a persistent polar vortex supercrystal in a heterostructure that hosts a fine balance between built-in electrostatic and elastic frustrations by design. By perturbing this balance with photoinduced charges, a starting heterogenous mixture of polar phases disorders within a few picoseconds, resulting in a soup state composed of disordered ferroelectric and suppressed vortex orders. On the pico-to-nanosecond timescales, transient labyrinthine fluctuations form in this soup along with a recovering vortex order. On longer timescales, these fluctuations are progressively quenched by dynamical strain modulations, which drive the collective emergence of a single supercrystal phase. Our results, corroborated by dynamical phase-field modeling, reveal how ultrafast excitation of designer systems generates pathways for persistent metastability.

cond-mat.mtrl-sci↗

Electrical control of magnetism by electric field and current-induced torques

While early magnetic memory designs relied on magnetization switching by locally generated magnetic fields, key insights in condensed matter physics later suggested the possibility to do it electrically. In the 1990s, Slonczewzki and Berger formulated the concept of current-induced spin torques in magnetic multilayers through which a spin-polarized current may switch the magnetization of a ferromagnet. This discovery drove the development of spin-transfer-torque magnetic random-access memories (STT-MRAMs). More recent research unveiled spin-orbit-torques (SOTs) and will lead to a new generation of devices including SOT-MRAMs. Parallel to these advances, multiferroics and their magnetoelectric coupling experienced a renaissance, leading to novel device concepts for information and communication technology such as the MESO transistor. The story of the electrical control of magnetization is that of a dance between fundamental research (in spintronics, condensed matter physics, and materials science) and technology (MRAMs, MESO, microwave emitters, spin-diodes, skyrmion-based devices, components for neuromorphics, etc). This pas de deux led to major breakthroughs over the last decades (pure spin currents, magnetic skyrmions, spin-charge interconversion, etc). As a result, this field has propelled MRAMs into consumer electronics products but also fueled discoveries in adjacent research areas such as ferroelectrics or magnonics. Here, we cover recent advances in the control of magnetism by electric fields and by current-induced torques. We first review fundamental concepts in these two directions, then discuss their combination, and finally present various families of devices harnessing the electrical control of magnetic properties for various application fields. We conclude by giving perspectives in terms of both emerging fundamental physics concepts and new directions in materials science.

physics.app-ph↗