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Rembert A. Duine

Publications and source records attributed to Rembert A. Duine.

At least 73 records · Page 4Linked to original sources

Magnon antibunching in a nanomagnet

We investigate the correlations of magnons inside a nanomagnet and identify a regime of parameters where the magnons become antibunched, i.e., where there is a large probability for occupation of the single-magnon state. This antibunched state is very different from magnons at thermal equilibrium and microwave-driven coherent magnons. We further obtain the steady state analytically and describe the magnon dynamics numerically, and ascertain the stability of such antibunched magnons over a large window of magnetic anisotropy, damping and temperature. This means that the antibunched magnon state is feasible in a wide class of low-damping magnetic nanoparticles. To detect this quantum effect, we propose to transfer the quantum information of magnons to photons by magnon-photon coupling and then measure the correlations of photons to retrieve the magnon correlations. Our findings may provide a promising platform to study quantum-classical transitions and for designing a single magnon source.

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Layer effects on the magnetic textures in magnets with local inversion asymmetry

Magnets with broken local inversion symmetries are interesting candidates for chiral magnetic textures such as skyrmions and spin spirals. The property of these magnets is that each subsequent layer can possess a different Dzyaloshniskii-Moriya interaction (DMI) originating from the local inversion symmetry breaking. Given that new candidates of such systems are emerging, with the Van der Waals crystals and magnetic multilayer systems, it is interesting to investigate how the chiral magnetic textures depend on the number of layers and the coupling between them. In this article, we model the magnetic layers with a classical Heisenberg spin model, where the sign of the DMI alternates for each consecutive layer. We use Monte Carlo simulations to examine chiral magnetic textures and show that the pitch of magnetic spirals is influenced by the interlayer coupling and the number of layers. We observe even-odd effects in the number of layers, where we observe a suppression of the spin spirals for even layer numbers. We give an explanation for our findings by proposing a net DMI in systems with strongly coupled layers. Our results can be used to determine the DMI in systems with a known number of layers, and for new technologies based on the tunability of the spiral wave length.

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Stabilizing chiral spin-structures via an alternating Dzyaloshinskii-Moriya interaction

The stabilization of chiral magnetic spin-structures in thin films is often attributed to the interfacial Dzyaloshinskii-Moriya interaction (DMI). Very recently, however, it has been reported that the chirality induced by the DMI can be affected by dipolar interactions. These dipolar fields tend to form Néel caps, which entails the formation of a clockwise chirality at the top of the film and a counterclockwise chirality at the bottom. Here, we show that engineering an alternating DMI that changes sign across the film thickness, together with the tendency to form Néel caps, leads to an enhanced stability of chiral spin-structures. Micromagnetic simulations for skyrmions demonstrate that this can increase the effective DMI in a prototypical [Pt/Co/Ir] multilayer system by at least \SI{0.6}{mJ.m^{-2}}. These gains are comparable to what has been achieved using additive DMI, but more flexible as we are not limited to a select set of material combinations. We also present experimental results: by measuring equilibrium domain widths we quantify the effective DMI in [Pt/Co/Ir] multilayer systems typically used for skyrmion stabilization. Upon introducing an alternating DMI we demonstrate changes in the effective DMI that agree with our simulations. Our results provide a route towards enhancing the stability of chiral spin-structures that does not rely on enlarging the chiral interactions.

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Long-Range Phonon Spin Transport in Ferromagnet-Nonmagnetic Insulator Heterostructures

We investigate phonon spin transport in an insulating ferromagnet-nonmagnet-ferromagnet heterostructure. We show that the magnetoelastic interaction between the spins and the phonons leads to nonlocal spin transfer between the magnets. This transfer is mediated by a local phonon spin current and accompanied by a phonon spin accumulation. The spin conductance depends nontrivially on the system size, and decays over millimeter length scales for realistic material parameters, far exceeding the decay lengths of magnonic spin currents.

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Spin-accumulation induced magnetic texture in a metal-insulator bilayer

We consider the influence of a spin accumulation in a normal metal on the magnetic statics and dynamics in an adjacent magnetic insulator. In particular, we focus on arbitary angles between the spin accumulation and the easy-axis of the magnetic insulator. Based on Landau-Lifshitz-Gilbert phenomenology supplemented with magnetoelectronic circuit theory, we find that the magnetic texture twists into a stable configuration that turns out to be described by a virtual, or image, domain wall configuration, i.e., a domain wall outside the ferromagnet. We show that even when the spin accumulation is perpendicular to the anisotropy axis, the magnetic texture develops a component parallel to the spin accumulation for sufficiently large spin bias. The emergence of this parallel component gives rise to threshold behavior in the spin Hall magnetoresistance and nonlocal magnon transport. This threshold can be used to design novel spintronic and magnonic devices that can be operated without external magnetic fields.

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Ellipticity and Dissipation Effects in Magnon Spin Valves

We consider alignment-dependent spin and heat transport across a magnon spin valve in the tunneling regime, i.e., a junction consisting of two weakly coupled ferromagnetic insulators. We determine the difference in spin and heat conductance between the parallel and antiparallel configuration of the magnetization direction. The dependence of these conductances on both the Gilbert damping and ellipticity is studied. We find that both magnon ellipticity and dissipation open channels for magnons to tunnel through in the antiparallel configuration. Our results highlight an important difference between electronic and magnon spin transport in spin-valve structures and may be important for the development of devices based on magnetic insulators.

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Angular Momentum Conservation and Phonon Spin in Magnetic Insulators

We develop a microscopic theory of spin-lattice interactions in magnetic insulators, separating rigid-body rotations and the internal angular momentum, or spin, of the phonons, while conserving the total angular momentum. In the low-energy limit, the microscopic couplings are mapped onto experimentally accessible magnetoelastic constants. We show that the transient phonon spin contribution of the excited system can dominate over the magnon spin, leading to nontrivial Einstein-de Haas physics.

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Non-Hermitian topology of one-dimensional spin-torque oscillator arrays

Magnetic systems have been extensively studied both from a fundamental physics perspective and as building blocks for a variety of applications. Their topological properties, in particular those of excitations, remain relatively unexplored due to their inherently dissipative nature. The recent introduction of non-Hermitian topological classifications opens up new opportunities for engineering topological phases in dissipative systems. Here, we propose a magnonic realization of a non-Hermitian topological system. A crucial ingredient of our proposal is the injection of spin current into the magnetic system, which alters and can even change the sign of terms describing dissipation. We show that the magnetic dynamics of an array of spin-torque oscillators can be mapped onto a non-Hermitian Su-Schrieffer-Heeger model exhibiting topologically protected edge states. Using exact diagonalization of the linearized dynamics and numerical solutions of the non-linear equations of motion, we find that a topological magnonic phase can be accessed by tuning the spin current injected into the array. In the topologically nontrivial regime, a single spin-torque oscillator on the edge of the array is driven into auto-oscillation and emits a microwave signal, while the bulk oscillators remain inactive. Our findings have practical utility for memory devices and spintronics neural networks relying on spin-torque oscillators as constituent units.

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Spin Transport in Thick Insulating Antiferromagnetic Films

Spin transport of magnonic excitations in uniaxial insulating antiferromagnets (AFs) is investigated. In linear response to spin biasing and a temperature gradient, the spin transport properties of normal-metal--insulating antiferromagnet--normal-metal heterostructures are calculated. We focus on the thick-film regime, where the AF is thicker than the magnon equilibration length. This regime allows the use of a drift-diffusion approach, which is opposed to the thin-film limit considered by Bender {\it et al.} 2017, where a stochastic approach is justified. We obtain the temperature- and thickness-dependence of the structural spin Seebeck coefficient $\mathcal{S}$ and magnon conductance $\mathcal{G}$. In their evaluation we incorporate effects from field- and temperature-dependent spin conserving inter-magnon scattering processes. Furthermore, the interfacial spin transport is studied by evaluating the contact magnon conductances in a microscopic model that accounts for the sub-lattice symmetry breaking at the interface. We find that while inter-magnon scattering does slightly suppress the spin Seebeck effect, transport is generally unaffected, with the relevant spin decay length being determined by non-magnon-conserving processes such as Gilbert damping. In addition, we find that while the structural spin conductance may be enhanced near the spin flip transition, it does not diverge due to spin impedance at the normal metal|magnet interfaces.

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Antiferromagnetic magnons as highly squeezed Fock states underlying quantum correlations

Employing the concept of two-mode squeezed states from quantum optics, we demonstrate a revealing physical picture for the antiferromagnetic ground state and excitations. Superimposed on a N{é}el ordered configuration, a spin-flip restricted to one of the sublattices is called a sublattice-magnon. We show that an antiferromagnetic spin-up magnon is comprised by a quantum superposition of states with $n+1$ spin-up and $n$ spin-down sublattice-magnons, and is thus an enormous excitation despite its unit net spin. Consequently, its large sublattice-spin can amplify its coupling to other excitations. Employing von Neumann entropy as a measure, we show that the antiferromagnetic eigenmodes manifest a high degree of entanglement between the two sublattices, thereby establishing antiferromagnets as reservoirs for strong quantum correlations. Based on these novel insights, we outline strategies for exploiting the strong quantum character of antiferromagetic (squeezed-)magnons and give an intuitive explanation for recent experimental and theoretical findings in antiferromagnetic magnon spintronics.

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Magnetic chirality controlled by the interlayer exchange interaction

Chiral magnetism, wherein there is a preferred sense of rotation of the magnetization, has become a key aspect for future spintronic applications. It determines the chiral nature of magnetic textures, such as skyrmions, domain walls or spin spirals, and a specific magnetic chirality is often required for spintronic applications. Current research focuses on identifying and controlling the interactions that define the magnetic chirality. The influence of the interfacial Dzyaloshinskii-Moriya interaction (iDMI) and, recently, the dipolar interactions have previously been reported. Here, we experimentally demonstrate that an indirect interlayer exchange interaction can be used as an additional tool to effectively manipulate the magnetic chirality. We image the chirality of magnetic domain walls in a coupled bilayer system using scanning electron microscopy with polarization analysis (SEMPA). Upon increasing the interlayer exchange coupling, we induce a transition of the magnetic chirality from clockwise rotating Néel walls to degenerate Bloch-Néel domain walls and we confirm our findings with micromagnetic simulations. In multi-layered systems relevant for skyrmion research a uniform magnetic chirality across the magnetic layers is often desired. Additional simulations show that this can be achieved for reduced iDMI values when exploiting the interlayer exchange interaction. This work opens up new ways to control and tailor the magnetic chirality by the interlayer exchange interaction.

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Magnon-Mediated Indirect Exciton Condensation through Antiferromagnetic Insulators

Electrons and holes residing on the opposing sides of an insulating barrier and experiencing an attractive Coulomb interaction can spontaneously form a coherent state known as an indirect exciton condensate. We study a trilayer system where the barrier is an antiferromagnetic insulator. The electrons and holes here additionally interact via interfacial coupling to the antiferromagnetic magnons. We show that by employing magnetically uncompensated interfaces, we can design the magnon-mediated interaction to be attractive or repulsive by varying the thickness of the antiferromagnetic insulator by a single atomic layer. We derive an analytical expression for the critical temperature $T_c$ of the indirect exciton condensation. Within our model, anisotropy is found to be crucial for achieving a finite $T_c$, which increases with the strength of the exchange interaction in the antiferromagnetic bulk. For realistic material parameters, we estimate $T_c$ to be around 7 K, the same order of magnitude as the current experimentally achievable exciton condensation where the attraction is solely due to the Coulomb interaction. The magnon-mediated interaction is expected to cooperate with the Coulomb interaction for condensation of indirect excitons, thereby providing a means to significantly increase the exciton condensation temperature range.

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Extraction of Dzyaloshinksii-Moriya interaction from propagating spin waves validated

The interfacial Dzyaloshinksii-Moriya interaction (iDMI) is of great interest in thin-film magnetism because of its ability to stabilize chiral spin textures. It can be quantified by investigating the frequency non-reciprocity of oppositely propagating spin waves. However, as the iDMI is an interface interaction the relative effect reduces when the films become thicker making quantification more difficult. Here, we utilize all-electrical Propagating Spin Wave Spectroscopy (PSWS) to disentangle multiple contributions to spin wave frequency non-reciprocity to determine the iDMI. This is done by investigating non-reciprocities across a wide range of magnetic layer thicknesses (from 4 to 26 nm) in Pt/Co/Ir, Pt/Co/Pt, and Ir/Co/Pt stacks. We find the expected sign change in the iDMI when inverting the stack order, and a negligible iDMI for the symmetric Pt/Co/Pt. We additionally extract a difference in surface anisotropies and find a large contribution due to the formation of different crystalline phases of the Co, which is corroborated using nuclear magnetic resonance and high-resolution transmission-electron-microscopy measurements. These insights will open up new avenues to investigate, quantify and disentangle the fundamental mechanisms governing the iDMI, and pave a way towards engineered large spin-wave non-reciprocities for magnonic applications.

cond-mat.mtrl-sci↗

Tuning magnetic chirality by dipolar interactions

Chiral magnetism has gained enormous interest in recent years because of the anticipated wealth of applications in nanoelectronics. The demonstrated stabilization of chiral magnetic domain walls and skyrmions has been attributed to the actively investigated Dzyaloshinskii-Moriya interaction. Recently, however, predictions were made that suggest dipolar interactions can also stabilize chiral domain walls and skyrmions, but direct experimental evidence has been lacking. Here we show that dipolar interactions can indeed stabilize chiral domain walls by directly imaging the magnetic domain walls using scanning electron microscopy with polarization analysis. We further show that the competition between the Dzyaloshinskii-Moriya and dipolar interactions can reverse the domain-wall chirality. Finally, we suggest that this competition can be tailored by a Ruderman-Kittel-Kasuya-Yosida interaction. Our work therefore reveals that dipolar interactions play a key role in the stabilization of chiral spin textures. This insight will open up new routes towards balancing interactions for the stabilization of chiral magnetism.

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Investigating optically-excited THz standing spin waves using noncollinear magnetic bilayers

We investigate optically excited THz standing spin waves in noncollinear magnetic bilayers. Using femtosecond laser-pulse excitation, a spin current is generated in the first ferromagnetic (FM) layer, and flows through a conductive spacer layer to be injected into the second (transverse) FM layer, where it exerts a spin-transfer torque on the magnetization and excites higher-order standing spin waves. We show that the noncollinear magnetic bilayer is a convenient tool that allows easy excitation of THz spin waves, and can be used to investigate the dispersion and thereby the spin wave stiffness parameter in the thin-film regime. This is experimentally demonstrated using wedge-shaped Co and CoB (absorption) layers. Furthermore, the damping of these THz spin waves is investigated, showing a strong increase of the damping with decreasing absorption layer thickness, much stronger than expected from interface spin pumping effects. Additionally, a previously unseen sudden decrease in the damping for the thinnest films is observed. A model for the additional damping contribution incorporating both these observations is proposed.

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Optimizing propagating spin wave spectroscopy

The frequency difference between two oppositely propagating spin waves can be used to probe several interesting magnetic properties, such as the Dzyaloshinkii-Moriya interaction (DMI). Propagating spin wave spectroscopy is a technique that is very sensitive to this frequency difference. Here we show several elements that are important to optimize devices for such a measurement. We demonstrate that for wide magnetic strips there is a need for de-embedding. Additionally, for these wide strips there is a large parasitic antenna-antenna coupling that obfuscates any spin wave transmission signal, which is remedied by moving to smaller strips. The conventional antenna design excites spin waves with two different wave vectors. As the magnetic layers become thinner, the resulting resonances move closer together and become very difficult to disentangle. In the last part we therefore propose and verify a new antenna design that excites spin waves with only one wave vector. We suggest to use this antenna design to measure the DMI in thin magnetic layers.

cond-mat.mtrl-sci↗

Structural transitions of skyrmion lattices in synthetic antiferromagnets

Thin magnetic films with Dzyaloshinskii-Moriya interactions are known to host skyrmion crystals, which typically have a hexagonal lattice structure. We investigate skyrmion-lattice configurations in synthetic antiferromagnets, i.e., a bilayer of thin magnetic films that is coupled antiferromagnetically. By means of Monte-Carlo simulations, we find that by tuning the interlayer coupling the skyrmion lattice structure can be tuned from square to hexagonal. We give a simple interpretation for the existence of this transition based on the fact that for synthetic antiferromagnetic coupling the skyrmions in different layers repel each other and form each others' dual lattice. Our findings may be useful to experimentally switch between two lattice configurations to, for example, modify spin-wave propagation.

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Creep of Chiral Domain Walls

Recent experimental studies of magnetic domain expansion under easy-axis drive fields in materials with a perpendicular magnetic anisotropy have shown that the domain wall velocity is asymmetric as a function of an external in plane magnetic field. This is understood as a consequence of the inversion asymmetry of the system, yielding a finite chiral Dzyaloshinskii-Moriya interaction. Numerous attempts have been made to explain these observations using creep theory, but, in doing so, these have not included all contributions to the domain wall energy or have introduced additional free parameters. In this article we present a theory for creep motion of chiral domain walls in the creep regime that includes the most important contributions to the domain-wall energy and does not introduce new free parameters beyond the usual parameters that are included in the micromagnetic energy. Furthermore, we present experimental measurements of domain wall velocities as a function of in-plane field that are well decribed by our model, and from which material properties such as the strength of the Dzyaloshinskii-Moriya interaction and the demagnetization field are extracted.

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