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Rembert A. Duine

Publications and source records attributed to Rembert A. Duine.

At least 91 records · Page 5Linked to original sources

Microscopic theory of magnon-drag electron flow in ferromagnetic metals

A temperature gradient applied to a ferromagnetic metal induces not only independent flows of electrons and magnons but also drag currents because of their mutual interaction. In this paper, we present a microscopic study of the electron flow induced by the drag due to magnons. The analysis is based on the $s$-$d$ model, which describes conduction electrons and magnons coupled via the $s$-$d$ exchange interaction. Magnetic impurities are introduced in the electron subsystem as a source of spin relaxation. The obtained magnon-drag electron current is proportional to the entropy of magnons and to $α- β$ (more precisely, to $1 - β/α$), where $α$ is the Gilbert damping constant and $β$ is the dissipative spin-transfer torque parameter. This result almost coincides with the previous phenomenological result based on the magnonic spin-motive forces, and consists of spin-transfer and momentum-transfer contributions, but with a slight disagreement in the former. The result is interpreted in terms of the nonequilibrium spin chemical potential generated by nonequilibrium magnons.

cond-mat.mes-hall↗

Spin current cross-correlations as a probe of magnon coherence

Motivated by the important role of the normalized second order coherence function, often called $g^{(2)}$, in the field of quantum optics, we propose a method to determine magnon coherence in solid-state devices. Namely, we show that the cross-correlations of pure spin-currents injected by a ferromagnet into two metal leads, normalized by their dc value, replicate the behavior of $g^{(2)}$ when magnons are driven far from equilibrium. We consider two scenarios: driving by ferromagnetic resonance, which leads to the coherent occupation of a single mode, and driving by heating of the magnons, which leads to an excess of incoherent magnons. We find an enhanced normalized cross-correlation in the latter case, thereby demonstrating bunching of nonequilibrium thermal magnons due to their bosonic statistics. Our results contribute to the burgeoning field of quantum magnonics, which seeks to explore and exploit the quantum nature of magnons.

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Quantum kinetic theory of spin-transfer torque and magnon-assisted transport in nanostructures

We theoretically investigate the role of spin fluctuations in charge transport through a magnetic junction. Motivated by recent experiments that measure a nonlinear dependence of the current on electrical bias, we develop a systematic understanding of the interplay of charge and spin dynamics in nanoscale magnetic junctions. Our model captures two distinct features arising from these fluctuations: magnon-assisted transport and the effect of spin-transfer torque on the magnetoconductance. The latter stems from magnetic misalignment in the junction induced by spin-current fluctuations. As the temperature is lowered, inelastic quantum scattering takes over thermal fluctuations, exhibiting signatures that make it readily distinguishable from magnon-assisted transport.

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Enhanced Spin Conductance of a Thin-Film Insulating Antiferromagnet

We investigate spin transport by thermally excited spin waves in an antiferromagnetic insulator. Starting from a stochastic Landau-Lifshitz-Gilbert phenomenology, we obtain the out-of-equilibrium spin-wave properties. In linear response to spin biasing and a temperature gradient, we compute the spin transport through a normal metal$|$antiferromagnet$|$normal metal heterostructure. We show that the spin conductance diverges as one approaches the spin-flop transition; this enhancement of the conductance should be readily observable by sweeping the magnetic field across the spin-flop transition. The results from such experiments may, on the one hand, enhance our understanding of spin transport near a phase transition, and on the other be useful for applications that require a large degree of tunability of spin currents. In contrast, the spin Seebeck coefficient does not diverge at the spin-flop transition. Furthermore, the spin Seebeck coefficient is finite even at zero magnetic field, provided that the normal metal contacts break the symmetry between the antiferromagnetic sublattices.

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Microwave control of thermal magnon spin transport

We observe that an rf microwave field strongly influences the transport of incoherent thermal magnons in yttrium iron garnet. Ferromagnetic resonance in the nonlinear regime suppresses thermal magnon transport by 95%. The transport is also modulated at non-resonant conditions in two cases, both related to the magnon band minimum. Firstly, a strong enhancement of the nonlocal signal appears at a static magnetic field below the resonance condition. This increase only occurs at one field polarity and can be as large as 800%. We attribute this effect to magnon kinetic processes, which give rise to band-minimum magnons and high-energy chiral surface modes. Secondly, the signal increases at a static field above the resonance condition, where the rf frequency coincides with the magnon band minimum. Our study gives insight into the interplay between coherent and incoherent spin dynamics: The rf field modifies the occupation of relevant magnon states and, via kinetic processes, the magnon spin transport.

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Many-body theory of spin-current driven instabilities in magnetic insulators

We consider a magnetic insulator in contact with a normal metal. We derive a self-consistent Keldysh effective action for the magnon gas that contains the effects of magnon-magnon interactions and contact with the metal to lowest order. Self-consistent expressions for the dispersion relation, temperature and chemical potential for magnons are derived. Based on this effective action, we study instabilities of the magnon gas that arise due to spin-current flowing across the interface between the normal metal and the magnetic insulator. We find that the stability phase diagram is modified by an interference between magnon-magnon interactions and interfacial magnon-electron coupling. These effects persist at low temperatures and for thin magnetic insulators.

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Anomalous direction for skyrmion bubble motion

Magnetic skyrmions are localized topological excitations that behave as particles and can be mobile, with great potential for novel data storage devices. In this work, the current-induced dynamics of large skyrmion bubbles is studied. When skyrmion motion in the direction opposite to the electron flow is observed, this is usually interpreted as a perpendicular spin current generated by the spin Hall effect exerting a torque on the chiral Néel skyrmion. By designing samples in which the direction of the net generated spin current can be carefully controlled, we surprisingly show that skyrmion motion is always against the electron flow, irrespective of the net vertical spin-current direction. We find that a negative bulk spin-transfer torque is the most plausible explanation for the observed results, which is qualitatively justified by a simple model that captures the essential behaviour. These findings demonstrate that claims about the skyrmion chirality based on their current-induced motion should be taken with great caution.

cond-mat.mtrl-sci↗

Theory of the Interfacial Dzyaloshinskii-Moriya Interaction in Rashba Antiferromagnets

In antiferromagnetic (AFM) thin films, broken inversion symmetry or coupling to adjacent heavy metals can induce Dzyaloshinskii-Moriya (DM) interactions. Knowledge of the DM parameters is essential for understanding and designing exotic spin structures, such as hedgehog Skyrmions and chiral Néel walls, which are attractive for use in novel information storage technologies. We introduce a framework for computing the DM interaction in two-dimensional Rashba antiferromagnets. Unlike in Rashba ferromagnets, the DM interaction is not suppressed even at low temperatures. The material parameters control both the strength and the sign of the interfacial DM interaction. Our results suggest a route toward controlling the DM interaction in AFM materials by means of doping and electric fields.

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Bulk and edge spin transport in topological magnon insulators

We investigate the spin transport properties of a topological magnon insulator, a magnetic insulator characterized by topologically nontrivial bulk magnon bands and protected magnon edge modes located in the bulk band gaps. Employing the Landau-Lifshitz-Gilbert phenomenology, we calculate the spin current driven through a normal metal$|$topological magnon insulator$|$normal metal heterostructure by a spin accumulation imbalance between the metals, with and without random lattice defects. We show that bulk and edge transport are characterized by different length scales. This results in a characteristic system size where the magnon transport crosses over from being bulk-dominated for small systems to edge-dominated for larger systems. These findings are generic and relevant for topological transport in systems of nonconserved bosons.

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Thickness dependence of unidirectional spin-Hall magnetoresistance in metallic bilayers

A nonlinear magnetoresistance - called unidirectional spin-Hall magnetoresistance - is recently experimentally discovered in metallic bilayers consisting of a heavy metal and a ferromagnetic metal. To study the fundamental mechanism of the USMR, both ferromagnetic and heavy metallic layer thickness dependence of the USMR are presented in a Pt/Co/AlOx trilayer at room temperature. To avoid ambiguities, second harmonic Hall measurements are used for separating spin-Hall and thermal contributions to the non-linear magnetoresistance. The experimental results are fitted by using a drift-diffusion theory, with parameters extracted from an analysis of longitudinal resistivity of the Co layer within the framework of the Fuchs-Sondheimer model. A good agreement with the theory is found, demonstrating that the USMR is governed by both the spin-Hall effect in the heavy metallic layer and the metallic diffusion process in the ferromagnetic layer.

cond-mat.mtrl-sci↗

Scanning electron microscopy with polarization analysis for multilayered chiral spin textures

We show that scanning electron microscopy with polarization analysis (SEMPA) that is sensitive to both in-plane magnetization components can be used to image the out-of-plane magnetized multi-domain state in multilayered chiral spin textures. By depositing a thin layer of Fe on top of the multilayer we image the underlying out-of-plane domain state through the mapping of its stray fields in the Fe. We also demonstrate that SEMPA can be used to image the domain wall chirality in these systems after milling away the capping layer and imaging the topmost magnetic layer directly.

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Theory of magnon-mediated tunnel magneto-Seebeck effect

The tunnel magneto-Seebeck effect is the dependence of the thermopower of magnetic tunnel junctions on the magnetic configuration. It is conventionally interpreted in terms of a thermoelectric generalization of the tunnel magnetoresistance. Here, we investigate the heat-driven electron transport in these junctions associated with electron-magnon scattering, using stochastic Landau-Lifshitz phenomenology and quantum kinetic theory. Our findings challenge the widely accepted single-electron picture of the tunneling thermopower in magnetic junctions.

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Magnon-polaron transport in magnetic insulators

We theoretically study the effects of strong magnetoelastic coupling on the transport properties of magnetic insulators. We develop a Boltzmann transport theory for the mixed magnon-phonon modes (magnon polarons) and determine transport coefficients and spin diffusion length. Magnon-polaron formation causes anomalous features in the magnetic field and temperature dependence of the spin Seebeck effect when the disorder scattering in the magnetic and elastic subsystems is sufficiently different. Experimental data by Kikkawa et al. [PRL 117, 207203 (2016)] on yttrium iron garnet films can be explained by an acoustic quality that is much better than the magnetic quality of the material. We predict similar anomalous features in the spin and heat conductivity and non-local spin transport experiments.

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Magnon Polarons in the Spin Seebeck Effect

Sharp structures in magnetic field-dependent spin Seebeck effect (SSE) voltages of Pt/Y$_{3}$Fe$_{5}$O$_{12}$ (YIG) at low temperatures are attributed to the magnon-phonon interaction. Experimental results are well reproduced by a Boltzmann theory that includes the magnetoelastic coupling (MEC). The SSE anomalies coincide with magnetic fields tuned to the threshold of magnon-polaron formation. The effect gives insight into the relative quality of the lattice and magnetization dynamics.

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Local thermomagnonic torques in two-fluid spin dynamics

We develop a general phenomenology describing the interplay between coherent and incoherent dynamics in ferromagnetic insulators. Using the Onsager reciprocity and Neumann's principle, we derive expressions for the local thermomagnonic torques exerted by thermal magnons on the order-parameter dynamics and the reciprocal pumping processes, which are in close analogy to the spin-transfer torque and spin pumping at metallic interfaces. Our formalism is applicable to general long-wavelength dynamics and, although here we explicitly focus on ferromagnetic insulators possessing U(1) symmetry, our approach can be easily extended to other classes of magnetic materials. As an illustrative example, we apply our theory to investigate a domain wall floating over a spin superfluid, whose dynamics is triggered thermally at the system's edge. Our results demonstrate that the local pumping of coherent spin dynamics by a thermal magnon gas offers an alternative route - with no need for conducting components and thus devoid of Ohmic losses - for the control and manipulation of topological solitons.

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Magnon-drag thermopower and Nernst coefficient in Fe, Co, and Ni

Magnon-drag is shown to dominate the thermopower of elemental Fe from 2 to 80 K and of elemental Co from 150 to 600 K; it is also shown to contribute to the thermopower of elemental Ni from 50 to 500 K. Two theoretical models are presented for magnon-drag thermopower. One is a hydrodynamic theory based purely on non-relativistic, Galilean, spin-preserving electron-magnon scattering. The second is based on spin-motive forces, where the thermopower results from the electric current pumped by the dynamic magnetization associated with a magnon heat flux. In spite of their very different microscopic origins, the two give similar predictions for pure metals at low temperature, allowing us to semi-quantitatively explain the observed thermopower of elemental Fe and Co without adjustable parameters. We also find that magnon-drag may contribute to the thermopower of Ni. A spin-mixing model is presented that describes the magnon-drag contribution to the Anomalous Nernst Effect in Fe, again enabling a semi-quantitative match to the experimental data without fitting parameters. Our work suggests that particle non-conserving processes may play an important role in other types of drag phenomena, and also gives a predicative theory for improving metals as thermoelectric materials.

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Influence of yttrium iron garnet thickness and heater opacity on the nonlocal transport of electrically and thermally excited magnons

We studied the nonlocal transport behavior of both electrically and thermally excited magnons in yttrium iron garnet (YIG) as a function of its thickness. For electrically injected magnons, the nonlocal signals decrease monotonically as the YIG thickness increases. For the nonlocal behavior of the thermally generated magnons, or the nonlocal spin Seebeck effect (SSE), we observed a sign reversal which occurs at a certain heater-detector distance, and it is influenced by both the opacity of the YIG/heater interface and the YIG thickness. Our nonlocal SSE results can be qualitatively explained by the bulk-driven SSE mechanism together with the magnon diffusion model. Using a two-dimensional finite element model (2D-FEM), we estimated the bulk spin Seebeck coefficient of YIG at room temperature. The quantitative disagreement between the experimental and modeled results indicates more complex processes going on in addition to magnon diffusion and relaxation, especially close to the contacts.

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Landau-Lifshitz theory of the magnon-drag thermopower

Metallic ferromagnets subjected to a temperature gradient exhibit a magnonic drag of the electric current. We address this problem by solving a stochastic Landau-Lifshitz equation to calculate the magnon-drag thermopower. The long-wavelength magnetic dynamics result in two contributions to the electromotive force acting on electrons: (1) An adiabatic Berry-phase force related to the solid angle subtended by the magnetic precession and (2) a dissipative correction thereof, which is rooted microscopically in the spin-dephasing scattering. The first contribution results in a net force pushing the electrons towards the hot side, while the second contribution drags electrons towards the cold side, i.e., in the direction of the magnonic drift. The ratio between the two forces is proportional to the ratio between the Gilbert damping coefficient $α$ and the coefficient $β$ parametrizing the dissipative contribution to the electromotive force.

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