arXiv subjects

Robert W. Boyd

Publications and source records attributed to Robert W. Boyd.

At least 55 records · Page 3Linked to original sources

arXiv2021

Cross-polarized surface lattice resonances in a rectangular lattice plasmonic metasurface

Multiresonant metasurfaces could enable many applications in filtering, sensing and nonlinear optics. However, developing a metasurface with more than one high-quality-factor or high-Q resonance at designated resonant wavelengths is challenging. Here, we experimentally demonstrate a plasmonic metasurface exhibiting different, narrow surface lattice resonances by exploiting the polarization degree of freedom where different lattice modes propagate along different dimensions of the lattice. The surface consists of aluminum nanostructures in a rectangular periodic lattice. The resulting surface lattice resonances were measured around 630 nm and 1160 nm with Q-factors of ~50 and ~800, respectively. The latter is a record-high plasmonic Q-factor within the near-infrared type-II window. Such metasurfaces could benefit applications such as frequency conversion and all-optical switching.

physics.optics↗

arXiv2021

A Comprehensive Multipolar Theory for Periodic Metasurfaces

Optical metasurfaces consist of a 2D arrangement of scatterers, and they control the amplitude, phase, and polarization of an incidence field on demand. Optical metasurfaces are the cornerstone for a future generation of flat optical devices in a wide range of applications. The rapidly growing advances in nanofabrication have made the versatile design and analysis of these ultra-thin surfaces an ever-growing necessity. However, despite their importance, a comprehensive theory to describe the optical response of periodic metasurfaces in closed-form and analytical expressions has not been formulated, and prior attempts were frequently approximate. Here, we develop a theory that analytically links the properties of the scatterer, from which a periodic metasurface is made, to its optical response via the lattice coupling matrix. The scatterers are represented by their polarizability or T matrix, and our theory works for normal and oblique incidence. We provide explicit expressions for the optical response up to octupolar order in both spherical and Cartesian coordinates. Several examples demonstrate that our analytical tool constitutes a paradigm shift in designing and understanding optical metasurfaces. Novel fully-diffracting metagratings and particle-independent polarization filters are proposed, and novel insights into the response of Huygens' metasurfaces under oblique incidence are provided. Our analytical expressions are a powerful tool for exploring the physics of metasurfaces and designing novel flat optics devices.

physics.optics↗

arXiv2021

Anomalous Optical Drag

A moving dielectric medium can displace the optical path of light passing through it, a phenomenon known as the Fresnel-Fizeau optical drag effect. The resulting displacement is proportional to the medium's velocity. In this article, we report on an anomalous optical drag effect, where the displacement is still proportional to the medium's speed but along the direction opposite to the medium's movement. We conduct an optical drag experiment under conditions of electromagnetically-induced transparency and observe the transition from normal, to null, to anomalous optical drag by modification of the two-photon detuning.

physics.optics↗

arXiv2021

Lattice-plasmon induced asymmetric transmission in two-dimensional chiral arrays

Asymmetric transmission - direction-selective control of electromagnetic transmission between two ports - is an important phenomenon typically exhibited by two-dimensional chiral systems. Here, we study this phenomenon in chiral plasmonic metasurfaces supporting lattice plasmons modes. We show, both numerically and experimentally, that asymmetric transmission can be achieved through an unbalanced excitation of such lattice modes by circularly polarized light of opposite handedness. The excitation efficiencies of the lattice modes, and hence the strength of the asymmetric transmission, can be controlled by engineering the in-plane scattering of the individual plasmonic nanoparticles such that the maximum scattering imbalance occurs along one of the in-plane diffraction orders of the metasurface. Our study also shows that, contrary to the case of a non-diffractive metasurface, the lattice-plasmon-enabled asymmetric transmission can occur at normal incidence for cases where the metasurface is composed of chiral or achiral nanoparticles possessing 4-fold rotational symmetry.

physics.optics↗

arXiv2021

Direct tomography of high-dimensional density matrices for general quantum states of photons

Quantum state tomography is the conventional method used to characterize density matrices for general quantum states. However, the data acquisition time generally scales linearly with the dimension of the Hilbert space, hindering the possibility of dynamic monitoring of a high-dimensional quantum system. Here, we demonstrate a direct tomography protocol to measure density matrices of photons in the position basis through the use of a polarization-resolving camera, where the dimension of density matrices can be as large as 580$\times$580 in our experiment. The use of the polarization-resolving camera enables parallel measurements in the position and polarization basis and as a result, the data acquisition time of our protocol does not increase with the dimension of the Hilbert space and is solely determined by the camera exposure time (on the order of 10 ms). Our method is potentially useful for the real-time monitoring of the dynamics of quantum states and paves the way for the development of high-dimensional, time-efficient quantum metrology techniques.

quant-ph↗

arXiv2021

Giant asymmetric second-harmonic generation in bianisotropic metasurfaces based on bound states in the continuum

Bianisotropy is a powerful concept enabling asymmetric optical response, including asymmetric reflection, absorption, optical forces, light trapping, and lasing. The physical origin of these asymmetric effects can be understood from magnetoelectric coupling and asymmetrical field enhancement. Here, we theoretically propose highly asymmetric second-harmonic generation (SHG) in bianisotropic AlGaAs metasurfaces. We show that around four orders of magnitude second-harmonic power difference for the forward and backward illuminations can be obtained by altering geometrical parameters that coincide with quasi-bound states in the continuum. Our study paves the way towards a directional generation of higher-order waves and can be potentially useful for nonlinear holograms.

physics.optics↗

arXiv2021

Designing high-performance propagation-compressing spaceplates using thin-film multilayer stacks

The development of metasurfaces has enabled unprecedented portability and functionality in flat optical devices. Spaceplates have recently been introduced as a complementary element to reduce the space between individual metalenses. This will further miniaturize entire imaging devices. However, a spaceplate necessitates a non-local optical response -- one which depends on the transverse spatial frequency component of a light field -- therefore making it challenging both to design them and to assess their ultimate performance and potential. Here, we employ inverse-design techniques to explore the behaviour of general thin-film-based spaceplates. We observe a tradeoff between the compression factor R and the numerical aperture NA of such devices; we obtained a compression factor of R = 5.5 for devices with an NA = 0.42 up to a record R = 340 with NA of 0.017. Our work illustrates that even simple designs consisting of realistic materials (i.e., silicon and glass) permit capable spaceplates for monochromatic applications.

physics.optics↗

arXiv2021

An optic to replace space and its application towards ultra-thin imaging systems

Centuries of effort to improve imaging has focused on perfecting and combining lenses to obtain better optical performance and new functionalities. The arrival of nanotechnology has brought to this effort engineered surfaces called metalenses, which promise to make imaging devices more compact. However, unaddressed by this promise is the space between the lenses, which is crucial for image formation but takes up by far the most room in imaging systems. Here, we address this issue by presenting the concept of and experimentally demonstrating an optical 'spaceplate', an optic that effectively propagates light for a distance that can be considerably longer than the plate thickness. Such an optic would shrink future imaging systems, opening the possibility for ultra-thin monolithic cameras. More broadly, a spaceplate can be applied to miniaturize important devices that implicitly manipulate the spatial profile of light, for example, solar concentrators, collimators for light sources, integrated optical components, and spectrometers.

physics.optics↗

arXiv2021

Selective Excitation of Subwavelength Atomic Clouds

A dense cloud of atoms with randomly changing positions exhibits coherent and incoherent scattering. We show that an atomic cloud of subwavelength dimensions can be modeled as a single scatterer where both coherent and incoherent components of the scattered photons can be fully explained based on effective multipole moments. This model allows us to arrive at a relation between the coherent and incoherent components of scattering based on the conservation of energy. Furthermore, using superposition of four plane waves, we show that one can selectively excite different multipole moments and thus tailor the scattering of the atomic cloud to control the cooperative shift, resonance linewidth, and the radiation pattern. Our approach provides a new insight into the scattering phenomena in atomic ensembles and opens a pathway towards controlling scattering for applications such as generation and manipulation of single-photon states.

quant-ph↗

arXiv2021

Ultrafast pulse measurement via time-domain single-pixel imaging

In contrast with imaging using position-resolving cameras, single-pixel imaging uses a bucket detector along with spatially structured illumination for image recovery. This emerging imaging technique is a promising candidate for a broad range of applications due to high signal-to-noise ratio (SNR) and sensitivity, and applicability in a wide range of frequency bands. Here, inspired by single-pixel imaging in the spatial domain, we demonstrate a temporal single-pixel imaging (TSPI) system that covers frequency bands including both terahertz (THz) and near-infrared (NIR) region. By implementing a programmable temporal fan-out (TFO) gate based on a digital micromirror device (DMD), we can deterministically prepare temporally structured pulses with a temporal sampling size down to 16.00$\pm$0.01 fs. By inheriting the advantages in detection efficiency and sensitivity from spatial single-pixel imaging, TSPI enables the compressive recovery of a 5 fJ THz pulse and two NIR pulses with over 97$\%$ fidelity. We demonstrate that the TSPI is robust against temporal distortions in the probe pulse train as well. As a direct application, we apply TSPI to machine-learning-aided THz spectroscopy and demonstrate a high sample identification accuracy (97.5$\%$) even under low SNRs (SNR $\sim$ 10).

physics.optics↗

arXiv2021

Confocal super-resolution microscopy based on a spatial mode sorter

Spatial resolution is one of the most important specifications of an imaging system. Recent results in quantum parameter estimation theory reveal that an arbitrarily small distance between two incoherent point sources can always be efficiently determined through the use of a spatial mode sorter. However, extending this procedure to a general object consisting of many incoherent point sources remains challenging, due to the intrinsic complexity of multi-parameter estimation problems. Here, we generalize the Richardson-Lucy (RL) deconvolution algorithm to address this challenge. We simulate its application to an incoherent confocal microscope, with a Zernike spatial mode sorter replacing the pinhole used in a conventional confocal microscope. We test different spatially incoherent objects of arbitrary geometry, and we find that the resolution enhancement of sorter-based microscopy is on average over 30% higher than that of a conventional confocal microscope using the standard RL deconvolution algorithm. Our method could potentially be used in diverse applications such as fluorescence microscopy and astronomical imaging.

physics.optics↗

arXiv2021

High-fidelity spatial mode transmission through a 1-km-long multimode fiber via vectorial time reversal

The large number of spatial modes supported by standard multimode fibers is a promising platform for boosting the channel capacity of quantum and classical communications by orders of magnitude. However, the practical use of long multimode fibers is severely hampered by modal crosstalk and polarization mixing. To overcome these challenges, we develop and experimentally demonstrate a vectorial time reversal technique, which is accomplished by digitally pre-shaping the wavefront and polarization of the forward-propagating signal beam to be the phase conjugate of an auxiliary, backward-propagating probe beam. Here, we report an average modal fidelity above 80% for 210 Laguerre-Gauss and Hermite-Gauss modes by using vectorial time reversal over an unstabilized 1-km-long fiber. We also propose a practical and scalable spatial-mode-multiplexed quantum communication protocol over long multimode fibers to illustrate potential applications that can be enabled by our technique.

physics.optics↗

arXiv2021

Experimental demonstration of superresolution of partially coherent light sources using parity sorting

Analyses based on quantum metrology have shown that the ability to localize the positions of two incoherent point sources can be significantly enhanced through the use of mode sorting. Here we theoretically and experimentally investigate the effect of partial coherence on the sub-diffraction limit localization of two sources based on parity sorting. With the prior information of a negative and real-valued degree of coherence, higher Fisher information is obtained than that for the incoherent case. Our results pave the way to clarifying the role of coherence in quantum limited metrology.

physics.optics↗

arXiv2021

Multiprobe time reversal for high-fidelity vortex-mode-division multiplexing over a turbulent free-space link

The orbital angular momentum (OAM) of photons presents a degree of freedom for enhancing the secure key rate of free-space quantum key distribution (QKD) through mode-division multiplexing (MDM). However, atmospheric turbulence can lead to substantial modal crosstalk, which is a long-standing challenge to MDM for free-space QKD. Here, we show that the digital generation of time-reversed wavefronts for multiple probe beams is an effective method for mitigating atmospheric turbulence. We experimentally characterize seven OAM modes after propagation through a 340-m outdoor free-space link and observe an average modal crosstalk as low as 13.2% by implementing real-time time reversal. The crosstalk can be further reduced to 3.4% when adopting a mode spacing $Δ\ell$ of 2. We implement a classical MDM system as a proof-of-principle demonstration, and the bit error rate is reduced from $3.6\times 10^{-3}$ to be less than $1.3\times 10^{-7}$ through the use of time reversal. We also propose a practical and scalable scheme for high-speed, mode-multiplexed QKD through a turbulent link. The modal crosstalk can be further reduced by using faster equipment. Our method can be useful to various free-space applications that require crosstalk suppression.

physics.optics↗

arXiv2021

Relaxed phase-matching constraints in zero-index waveguides

The nonlinear optical response of materials is the foundation upon which applications such as frequency conversion, all-optical signal processing, molecular spectroscopy, and nonlinear microscopy are built. However, the utility of all such parametric nonlinear optical processes is hampered by phase-matching requirements. Quasi-phase-matching, birefringent phase matching, and higher-order-mode phase matching have all been developed to address this constraint, but the methods demonstrated to date suffer from the inconvenience of only being phase-matched for a single, specific arrangement of beams, typically co-propagating, resulting in cumbersome experimental configurations and large footprints for integrated devices. Here, we experimentally demonstrate that these phase-matching requirements may be satisfied in a parametric nonlinear optical process for multiple, if not all, configurations of input and output beams when using low-index media. Our measurement constitutes the first experimental observation of direction-independent phase matching for a medium sufficiently long for phase matching concerns to be relevant. We demonstrate four-wave mixing from spectrally distinct co- and counter-propagating pump and probe beams, the backward-generation of a nonlinear signal, and excitation by an out-of-plane probe beam. These results explicitly show that the unique properties of low-index media relax traditional phase-matching constraints, which can be exploited to facilitate nonlinear interactions and miniaturize nonlinear devices, thus adding to the established exceptional properties of low-index materials.

physics.optics↗

arXiv2021

Enhanced Nonlinear Optical Responses of Layered Epsilon-Near-Zero Metamaterials at Visible Frequencies

Optical materials with vanishing dielectric permittivity, known as epsilon-near-zero (ENZ) materials, have been shown to possess enhanced nonlinear optical responses in their ENZ region. These strong nonlinear optical properties have been firmly established in homogeneous materials; however, it is as of yet unclear whether metamaterials with effective optical parameters can exhibit a similar enhancement. Here, we probe an optical ENZ metamaterial composed of a subwavelength periodic stack of alternating Ag and SiO$_2$ layers and measure a nonlinear refractive index $n_2 = (1.2 \pm 0.1) \times 10^{-12}$ m$^2$/W and nonlinear absorption coefficient $β= (-1.5 \pm 0.2) \times 10^{-5}$ m/W at its effective zero-permittivity wavelength. The measured $n_2$ is $10^7$ times larger than $n_2$ of fused silica and four times larger than that the $n_2$ of silver. We observe that the nonlinear enhancement in $n_2$ scales as $1/(n_0 \mathrm{Re}[n_0])$, where $n_0$ is the linear effective refractive index. As opposed to homogeneous ENZ materials, whose optical properties are dictated by their intrinsic material properties and hence are not widely tunable, the zero-permittivity wavelength of the demonstrated metamaterials may be chosen to lie anywhere within the visible spectrum by selecting the right thicknesses of the sub-wavelength layers. Consequently, our results offer the promise of a means to design metamaterials with large nonlinearities for applications in nanophotonics at any specified optical wavelength.

physics.optics↗

arXiv2021

Ultra-high-Q resonances in plasmonic metasurfaces

Plasmonic nanostructures hold promise for the realization of ultra-thin sub-wavelength devices, reducing power operating thresholds and enabling nonlinear optical functionality in metasurfaces. However, this promise is substantially undercut by absorption introduced by resistive losses, causing the metasurface community to turn away from plasmonics in favour of alternative material platforms (e.g., dielectrics) that provide weaker field enhancement, but more tolerable losses. Here, we report a plasmonic metasurface with a quality-factor (Q-factor) of 2340 in the telecommunication C band by exploiting surface lattice resonances (SLRs), exceeding the record by an order of magnitude. Additionally, we show that SLRs retain many of the same benefits as localized plasmonic resonances, such as field enhancement and strong confinement of light along the metal surface. Our results demonstrate that SLRs provide an exciting and unexplored method to tailor incident light fields, and could pave the way to flexible wavelength-scale devices for any optical resonating application.

physics.optics↗

arXiv2021

Turbulence-Resilient Coherent Free-Space Optical Communications using Automatic Power-Efficient Pilot-Assisted Optoelectronic Beam Mixing of Many Modes

Atmospheric turbulence generally limits free-space optical (FSO) communications, and this problem is severely exacerbated when implementing highly sensitive and spectrally efficient coherent detection. Specifically, turbulence induces power coupling from the transmitted Gaussian mode to higher-order Laguerre-Gaussian (LG) modes, resulting in a significant decrease of the power that mixes with a single-mode local oscillator (LO). Instead, we transmit a frequency-offset Gaussian pilot tone along with the data signal, such that both experience similar turbulence and modal power coupling. Subsequently, the photodetector (PD) optoelectronically mixes all corresponding pairs of the beams' modes. During mixing, a conjugate of the turbulence experienced by the pilot tone is automatically generated and compensates the turbulence experienced by the data, and nearly all orders of the same corresponding modes efficiently mix. We demonstrate a 12-Gbit/s 16-quadrature-amplitude-modulation (16-QAM) polarization-multiplexed (PolM) FSO link that exhibits resilience to emulated turbulence. Experimental results for turbulence D/r_0~5.5 show up to ~20 dB reduction in the mixing power loss over a conventional coherent receiver. Therefore, our approach automatically recovers nearly all the captured data power to enable high-performance coherent FSO systems.

physics.optics↗