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Robert W. Boyd

Publications and source records attributed to Robert W. Boyd.

At least 73 records · Page 4Linked to original sources

Telecom C-Band Photon-Pair Generation using Standard SMF-28 Fiber

Photon-pair generation must satisfy both the energy conservation and phase-matching conditions with a specific pump wavelength and dispersion of nonlinear optical medium, but finding a photon-pair, which has a desired specific wavelength, generation medium is challenging. Here, we present a method to create photon pairs that functions efficiently even the pump wavelength is much larger than the zero GVD wavelength of medium. In this study, we employ short SMF-28 fibers having ~1310 nm zero GVD wavelength and C-band pump (1552.52 nm) to generate C-band photon pairs. The measured pair generation rate and coincidence-to-accidental ratios are comparable to those from a long dispersion-shifted fiber. Polarization-entangled states are prepared, and an S value of 2.659 +- 0.094 is achieved from Bell inequality measurements. Our results indicate that the use of a short SFWM medium yields adequate photon-pair generation rates regardless of its dispersion properties in almost any material at any pump wavelength.

quant-ph↗

Kelvin's Chirality of Optical Beams

Geometrical chirality is a property of objects that describes three-dimensional mirror-symmetry violation and therefore it requires a non-vanishing spatial extent. In contrary, optical chirality describes only the local handedness of electromagnetic fields and neglects the spatial geometrical structure of optical beams. In this manuscript, we put forward the physical significance of geometrical chirality of spatial structure of optical beams, which we term "Kelvin's chirality". Further, we report on an experiment revealing the coupling of Kelvin's chirality to optical chirality upon transmission of a focused beam through a planar medium. Our work emphasizes the importance of Kelvin's chirality in all light-matter interaction experiments involving structured light beams with spatially inhomogeneous phase and polarization distributions.

physics.optics↗

Superscattering, Superabsorption, and Nonreciprocity in Nonlinear Antennas

We propose tunable nonlinear antennas based on an epsilon-near-zero material with a large optical nonlinearity. We show that the absorption and scattering cross sections of the antennas can be controlled dynamically from a nearly superscatterer to a nearly superabsorber by changing the intensity of the laser beam. Moreover, we demonstrate that a hybrid nonlinear antenna, composed of epsilon-near-zero and high-index dielectric materials, exhibits nonreciprocal radiation patterns because of broken spatial inversion symmetry and large optical nonlinearity of the epsilon-near-zero material. By changing the intensity of the laser, the radiation pattern of the antenna can be tuned between a bidirectional and a unidirectional emission known as a Huygens source. Our study provides a novel approach toward ultrafast dynamical control of metamaterials, for applications such as beam steering and optical limiting.

physics.optics↗

Dependence of the Nonlinear-Optical Response of Materials on their Linear $ε$ and $μ$

We investigate, theoretically and numerically, the dependence of a material's nonlinear-optical response on the linear relative electric permittivity $ε$ and magnetic permeability $μ$. The conversion efficiency of low-order harmonic-generation processes, as well as the increase rate of Kerr-effect nonlinear phase shift and nonlinear losses from two-photon absorption (TPA), are seen to increase with decreasing $ε$ and/or increasing $μ$. We also discuss the rationale and physical insights behind this nonlinear response, particularly its enhancement in $ε$-near-zero (ENZ) media. This behavior is consistent with the experimental observation of intriguingly high effective nonlinear refractive index in degenerate semiconductors such as indium tin oxide [\textit{Alam et al., Science 352 (795), 2016}] (where the nonlinearity is attributed to a modification of the energy distribution of conduction-band electrons due to laser-induced electron heating) and aluminum zinc oxide [\textit{Caspani et al., Phys. Rev. Lett. 116 (233901), 2016}] at frequencies with vanishing real part of the linear permittivity. Such strong nonlinear response can pave the way for a new paradigm in nonlinear optics with much higher conversion efficiencies and therefore better miniaturization capabilities and power requirements for next-generation integrated nanophotonics.

physics.optics↗

Kerker Effect, Superscattering, and Scattering Dark State in Atomic Antennas

We study scattering phenomena such as the Kerker effect, superscattering, and scattering dark states in a subwavelength atomic antenna consisting of atoms with only electric dipole transitions. We show that an atomic antenna can exhibit arbitrarily large or small scattering cross sections depending on the geometry of the structure and the direction of the impinging light. We also demonstrate that atoms with only an electric dipole transition can exhibit a directional radiation pattern with zero backscattering when placed in a certain configuration. This is a special case of a phenomenon known as the Kerker effect, which typically occurs in the presence of both electric and magnetic transitions. Our findings open a pathway to design highly directional emitters, nonradiating sources, and highly scattering objects based on individually controlled atoms.

physics.optics↗

Fast Generation and Detection of Spatial Modes of Light using an Acousto-Optic Modulator

Spatial modes of light provide a high-dimensional space that can be used to encode both classical and quantum information. Current approaches for dynamically generating and measuring these modes are slow, due to the need to reconfigure a high-resolution phase mask such as a spatial light modulator or digital micromirror device. The process of updating the spatial mode of light can be greatly accelerated by multiplexing a set of static phase masks with a fast, image-preserving optical switch, such as an acousto-optic modulator (AOM). We experimentally realize this approach, using a double-pass AOM to generate one of five orbital angular momentum states with a switching rate of up to 500 kHz. We then apply this system to perform fast quantum state tomography of spatial modes of light in a 2-dimensional Hilbert space, by projecting the unknown state onto six spatial modes comprising three mutually unbiased bases. We are able to reconstruct arbitrary states in under 1 ms with an average fidelity of 96.9%.

physics.optics↗

Dynamic coherent perfect absorption in nonlinear metasurfaces

We propose a tunable coherent perfect absorber based on ultrathin nonlinear metasurfaces. The nonlinear metasurface is made of plasmonic nanoantennas coupled to an epsilon-near-zero material with a large optical nonlinearity. The coherent perfect absorption is achieved by controlling the relative phases of the input beams. We show that the optical response of the nonlinear metasurface can be tuned from a complete to a partial absorption by changing the intensity of the pump beam. The proposed nonlinear metasurface can be used to design optically tunable thermal emitters, modulators, and sensors.

physics.optics↗

Terahertz Nonlinear Optical Response of Water Vapor

We report on the nonlinear spectroscopy of water vapor at THz frequencies. Atmospheric water vapor has a rich spectrum with several strong resonances at frequencies below 3 THz, falling within the range of operation of most existing THz sources. We observe an extremely large nonlinear response to THz radiation at the positions of these resonances. Using the optical Kerr model for the nonlinear response, we estimate a minimum nonlinear refractive index of the order of 10^2 m^2/W. Our results provide insight into the energy levels of the water molecule and give a more accurate picture of its response to electromagnetic radiation, paving the way to more accurate THz spectroscopy, imaging and sensing systems, and thereby facilitating future emerging THz technologies.

physics.optics↗

A nonreciprocal optical resonator with broken time-invariance for arbitrarily high time-bandwidth performance

Most present-day resonant systems, throughout physics and engineering, are characterized by a strict time-reversal symmetry between the rates of energy coupled in and out of the system, which leads to a trade-off between how long a wave can be stored in the system and the system bandwidth. Any attempt to reduce the losses of the resonant system, and hence store a (mechanical, acoustic, electronic, optical, atomic, or of any other nature) wave for more time, will inevitably also reduce the bandwidth of the system. Until recently, this time-bandwidth limit has been considered fundamental, arising from basic Fourier reciprocity. A recent theory suggested that it might in fact be overcome by breaking Lorentz reciprocity in the resonant system, reinvigorated a debate about whether (or not) this was indeed the case. Here, we report an experimental realization of a cavity where, inducing nonreciprocity by breaking the time invariance, we do overcome the fundamental time-bandwidth limit of ordinary resonant systems by a factor of 30, in full agreement with accompanying numerical simulations. We show that, although in practice experimental constraints limit our scheme, the time bandwidth product can be arbitrarily large, simply dictated by the finesse of the cavity. Our experimental realization uses a simple macroscopic, time-variant, fiber-optic cavity, where we break Lorentz reciprocity by non-adiabatically opening the cavity, injecting a pulse of large bandwidth, and then closing the cavity, storing the pulse which can be released on-demand at a later time. Our results open the path for designing resonant systems, ubiquitous in physics and engineering, that can simultaneously be broadband (i.e., ultrafast) and possessing long storage times, thereby unleashing fundamentally new functionalities in wave physics and wave-matter interactions.

physics.optics↗

Ultrafast Topological Engineering in Metamaterials

Transient optical heating provides an efficient way to trigger phase transitions in naturally occurring media through ultrashort laser pulse irradiation. A similar approach could be used to induce topological phase transitions in the photonic response of suitably engineered artificial structures known as metamaterials. Here, we predict a topological transition in the isofrequency dispersion contours of a layered graphene metamaterial under optical pumping. We show that the contour topology transforms from elliptic to hyperbolic within a subpicosecond timescale by exploiting the extraordinary photothermal properties of graphene. This new phenomenon allows us to theoretically demonstrate applications in engineering the decay rate of proximal optical emitters, ultrafast beam steering, and dynamical far-field subwavelength imaging. Our study opens a disruptive approach toward ultrafast control of light emission, beam steering, and optical image processing.

cond-mat.mes-hall↗

On modifications of fundamental radiative processes in near-zero-index media of various dimensions

Spontaneous emission, stimulated emission and absorption are the three fundamental radiative processes describing light-matter interactions. Here, we theoretically study the behaviour of these fundamental processes inside an unbounded medium exhibiting a vanishingly small refractive index, i.e., a near-zero-index (NZI) host medium. We present a generalized framework to study these processes and find that the spatial dimension of the NZI medium has profound effects on the nature of the fundamental radiative processes. Our formalism highlights the role of the number of available optical modes as well as the ability of an emitter to couple to these modes as a function of the dimension and the class of NZI media. We demonstrate that the fundamental radiative processes are inhibited in 3D homogeneous lossless zero index materials but may be strongly enhanced in a zero index medium of reduced dimensionality. Our findings have implications in thermal, nonlinear and quantum optics as well as in designing quantum metamaterials at optical or microwave frequencies.

physics.optics↗

Performance of real-time adaptive optics compensation in a turbulent channel with high-dimensional spatial-mode encoding

The orbital angular momentum (OAM) of photons is a promising degree of freedom for high-dimensional quantum key distribution (QKD). However, effectively mitigating the adverse effects of atmospheric turbulence is a persistent challenge in OAM QKD systems operating over free-space communication channels. In contrast to previous works focusing on correcting static simulated turbulence, we investigate the performance of OAM QKD in real atmospheric turbulence with real-time adaptive optics (AO) correction. We show that, even our AO system provides a limited correction, it is possible to mitigate the errors induced by weak turbulence and establish a secure channel. The crosstalk induced by turbulence and the performance of AO systems is investigated in two configurations: a lab-scale link with controllable turbulence, and a 340 m long cross-campus link with dynamic atmospheric turbulence. Our experimental results suggest that an advanced AO system with fine beam tracking, reliable beam stabilization, precise wavefront sensing, and accurate wavefront correction is necessary to adequately correct turbulence-induced error. We also propose and demonstrate different solutions to improve the performance of OAM QKD with turbulence, which could enable the possibility of OAM encoding in strong turbulence.

eess.SP↗

Theory of Four-Wave Mixing of Cylindrical Vector Beams in Optical Fibers

Cylindrical vector (CV) beams are a set of transverse spatial modes that exhibit a cylindrically symmetric intensity profile and a variable polarization about the beam axis. They are composed of a non-separable superposition of orbital and spin angular momentum. Critically, CV beams are also the eigenmodes of optical fiber and, as such, are of wide-spread practical importance in photonics and have the potential to increase communications bandwidth through spatial multiplexing. Here, we derive the coupled amplitude equations that describe the four-wave mixing (FWM) of CV beams in optical fibers. These equations allow us to determine the selection rules that govern the interconversion of CV modes in FWM processes. With these selection rules, we show that FWM conserves the total angular momentum, the sum of orbital and spin angular momentum, in the conversion of two input photons to two output photons. When applied to spontaneous four-wave mixing, the selection rules show that photon pairs can be generated in CV modes directly and can be entangled in those modes. Such quantum states of light in CV modes could benefit technologies such as quantum key distribution with satellites.

physics.optics↗

Entanglement: Quantum or Classical?

From its seemingly non-intuitive and puzzling nature, most evident in numerous EPR-like gedankenexperiments to its almost ubiquitous presence in quantum technologies, entanglement is at the heart of modern quantum physics. First introduced by Erwin Schrödinger nearly a century ago, entanglement has remained one of the most fascinating ideas that came out of quantum mechanics. Here, we attempt to explain what makes entanglement fundamentally different from any classical phenomenon. To this end, we start with a historical overview of entanglement and discuss several hidden variables models that were conceived to provide a classical explanation and demystify quantum entanglement. We discuss some inequalities and bounds that are violated by quantum states thereby falsifying the existence of some of the classical hidden variables theories. We also discuss some exciting manifestations of entanglement, such as N00N states and the non-separable single particle states. We conclude by discussing some contemporary results regarding quantum correlations and present a future outlook for the research of quantum entanglement.

quant-ph↗

Compensation-Free High-Capacity Free-Space Optical Communication Using Turbulence-Resilient Vector Beams

Free-space optical communication is a promising means to establish versatile, secure and high-bandwidth communication for many critical point-to-point applications. While the spatial modes of light offer an additional degree of freedom to increase the information capacity of an optical link, atmospheric turbulence can introduce severe distortion to the spatial modes and lead to data degradation. Here, we propose and demonstrate a vector-beam-based, turbulence-resilient communication protocol, namely spatial polarization differential phase shift keying (SPDPSK), that can encode a large number of information levels using orthogonal spatial polarization states of light. We show experimentally that the spatial polarization profiles of the vector modes are resilient to atmospheric turbulence, and therefore can reliably transmit high-dimensional information through a turbid channel without the need of any adaptive optics for beam compensation. We construct a proof-of-principle experiment with a controllable turbulence cell. Using 34 vector modes, we have measured a channel capacity of 4.84 bits per pulse (corresponding to a data error rate of 4.3\%) through a turbulent channel with a scintillation index larger than 1. Our SPDPSK protocol can also effectively transmit 4.02 bits of information per pulse using 18 vector modes through even stronger turbulence with a scintillation index of 1.54. Our study provides direct experimental evidence on how the spatial polarization profiles of vector beams are resilient to atmospheric turbulence and paves the way towards practical, high-capacity, free-space communication solutions with robust performance under harsh turbulent environments.

physics.optics↗

Multi-resonant high-Q plasmonic metasurfaces

Resonant metasurfaces are devices composed of nanostructured sub-wavelength scatterers that generate narrow optical resonances, enabling applications in filtering, nonlinear optics, and molecular fingerprinting. It is highly desirable for these applications to incorporate such devices with multiple, high-quality-factor resonances; however, it can be challenging to obtain more than a pair of narrow resonances in a single plasmonic surface. Here, we demonstrate a multi-resonant metasurface that operates by extending the functionality of surface lattice resonances, which are the collective responses of arrays of metallic nanoparticles. This device features a series of resonances with high quality factors (Q ~ 40), an order of magnitude larger than what is typically achievable with plasmonic nanoparticles, as well as a narrow free spectral range. This design methodology can be used to better tailor the transmission spectrum of resonant metasurfaces and represents an important step towards the miniaturization of optical devices.

physics.optics↗

Quantum, Nonlocal Aberration Cancellation

Phase distortions, or aberrations, can negatively influence the performance of an optical imaging system. Through the use of position-momentum entangled photons, we nonlocally correct for aberrations in one photon's optical path by intentionally introducing the complementary aberrations in the optical path of the other photon. In particular, we demonstrate the simultaneous nonlocal cancellation of aberrations that are of both even and odd order in the photons' transverse degrees of freedom. We also demonstrate a potential application of this technique by nonlocally cancelling the effect of defocus in a quantum imaging experiment and thereby recover the original spatial resolution.

quant-ph↗

Towards Polarization-based Excitation Tailoring for Extended Raman Spectroscopy

Undoubtedly, Raman spectroscopy is one of the most elaborated spectroscopy tools in materials science, chemistry, medicine and optics. However, when it comes to the analysis of nanostructured specimens, accessing the Raman spectra resulting from an exciting electric field component oriented perpendicularly to the substrate plane is a difficult task and conventionally can only be achieved by mechanically tilting the sample, or by sophisticated sample preparation. Here, we propose a novel experimental method based on the utilization of polarization tailored light for Raman spectroscopy of individual nanostructures. As a proof of principle, we create three-dimensional electromagnetic field distributions at the nanoscale using tightly focused cylindrical vector beams impinging normally onto the specimen, hence keeping the conventional beam-path of commercial Raman systems. Using this excitation scheme, we experimentally show that the recorded Raman spectra of individual gallium-nitride nanostructures of sub-wavelength diameter used as a test platform depend sensitively on their location relative to the focal vector field. The observed Raman spectra can be attributed to the interaction with transverse or longitudinal electric field components. This novel technique may pave the way towards a characterization of Raman active nanosystems using full information of all Raman modes.

physics.optics↗