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Romain Quidant

Publications and source records attributed to Romain Quidant.

At least 19 recordsLinked to original sources

3D trapping of a meta-atom in an intensity minimum

High-refractive-index particles have recently attracted a growing interest in optical levitation experiments, offering the ability to further engineer optical forces through electromagnetic Mie resonances. Unlike standard silica particles, which are predominantly trapped in the dipole regime and exhibit trap frequencies mainly determined by material density, resonant meta-atoms formed by high-index particles enable qualitatively new trapping behaviors. In this work, we experimentally investigate the trapping of resonant silicon particles in an optical standing wave. A direct comparison of silicon and silica highlights the fundamental differences in their optical force scaling and trapping dynamics. Beyond conventional trapping at intensity-maxima, we demonstrate deterministic and stable three-dimensional trapping of silicon nanoparticles in optical intensity minima, a regime that remains inaccessible for silica particles. Drawing a mesoscopic analogy with blue-detuned atom trapping, our results establish meta-atoms as a versatile approach to further extend the optical manipulation tool box towards accessing novel trapping regimes e.g. in close proximity to a surface.

physics.optics

Cooling of an optically levitated nanoparticle via measurement-free coherent feedback

We demonstrate coherent, measurement-free optical feedback control of a levitated nanoparticle, achieving phonon occupations down to a few hundred phonons. Unlike measurement-based feedback, this all-optical scheme preserves the correlations between mechanical motion and the feedback signal. Adjustment of the feedback phase and delay provides precise and tunable control over the system dynamics. The ultimate cooling performance is currently limited by phase noise, which we analyze within a theoretical framework that outlines the constraints and prospects for reaching the motional ground state. Our results establish coherent feedback as a powerful tool for quantum control of levitated systems, extending beyond center-of-mass cooling.

quant-ph

Controlling the sign of optical forces using metaoptics

Precise manipulation of small objects using light holds transformative potential across diverse fields. While research in optical trapping and manipulation predominantly relies on the attraction of solid matter to light intensity maxima, here we demonstrate that meta-optics enables a departure from this accepted behavior. Specifically, we present deterministic control over the sign of optical forces exerted on a metasurface integrated on a suspended silicon nanomembrane. By tailoring the geometry of the constituent meta-atoms, we engineer the coherent superposition of their multipolar modes, and consequently, the net optical force experienced by the metasurface within a phase-controlled optical standing wave. In excellent agreement with 3D numerical simulations, we experimentally realize both attractive and repulsive forces on distinct metasurface designs, directly mirroring the behavior of two-level systems interacting with optical fields. This work establishes a versatile platform for the optical control of nanoscale mechanical systems, opening new avenues for both fundamental research and engineering.

physics.optics

Leveraging partial coherence in interferometric microscopy to enhance nanoparticle detection sensitivity and throughput

Interferometric-based microscopies stand as powerful label-free approaches for monitoring and characterising chemical reactions and heterogeneous nanoparticle systems in real time with single particle sensitivity. Nevertheless, coherent artifacts, such as speckle and parasitic interferences, together with limited photon fluxes from spatially incoherent sources, pose an ongoing challenge in achieving both high sensitivity and throughput. In this study, we systematically characterise how partial coherence affects both the signal contrast and the background noise level; thus, it offers a route to improve the signal-to-noise ratio from single nanoparticles (NPs), irrespective of their size and composition; or the light source used. We first validate that lasers can be modified into partially coherent sources with performance matching that of spatially incoherent ones; while providing higher photon fluxes. Secondly, we demonstrate that tuning the degree of partial coherence not only enhances the detection sensitivity of both synthetic and biological NPs, but also affects how signal contrasts vary as a function of the focus position. Finally, we apply our findings to single-protein detection, confirming that these principles extend to differential imaging modalities, which deliver the highest sensitivity. Our results address a critical milestone in the detection of weakly scattering NPs in complex matrices, with wide-ranging applications in biotechnology, nanotechnology, chemical synthesis, and biosensing; ushering a new generation of microscopes that push both the sensitivity and throughput boundaries without requiring beam scanning.

physics.optics

Accelerated State Expansion of a Nanoparticle in a Dark Inverted Potential

While the wave packet of a massive particle grows linearly under free dynamics, it grows exponentially in an inverted harmonic potential, offering a pathway to rapidly increase quantum fluctuations to macroscopic dimensions. In this work, we experimentally demonstrate this principle by expanding the center-of-mass thermal state of a 125nm silica nanoparticle to a position uncertainty of 43.4nm within 260 $\mu$s. This expansion, achieved using an inverted dark potential to minimize decoherence from photon recoil, represents a 952-fold increase, reaching a scale comparable to the nanoparticle's physical size. This work represents a key advancement toward preparing macroscopic quantum superpositions at unprecedented mass and length scales.

quant-ph

Thermally Adaptive Surface Microscopy for brain functional imaging

Fluorescence microscopes can record the dynamics of living cells with high spatio-temporal resolution in a single plane. However, monitoring rapid and dim fluorescence fluctuations, e.g induced by neuronal activity in the brain, remains challenging for 3D-distributed emitters due to out-of-focus fluorescence background, a restricted photon budget, and the speed limit of conventional scanning systems. Here, we introduce a Thermally Adaptive Surface strategy, capable of simultaneously recording, at camera framerate, the activity of 3D-distributed objects. This innovative microscope leverages on an array of thermally tuneable microlenses that offer low chromatic aberration and high transmission, and can be combined with patterned illumination to provide optical sectioning. We demonstrate its potential in vivo, by simultaneously monitoring fast fluorescent dynamics at different depths in the zebrafish larval brain, at a rate of 0.5 kHz and over a large field of view (360um x 360um).

physics.optics

Optical Supertorque Induced by Mie-Resonant Modes

We introduce the concept of resonant optical torque that allows enhancing substantially a transfer of optical angular momentum (AM) of light to a subwavelength particle. We consider high-index cylindrical dielectric nanoparticles supporting Mie resonances, and explore a transfer of AM and how it is affected by absorption and particle shape. We analyze a simple trapping geometry of standing wave patterns created by opposite helical light waves. We uncover stable rotation of particles in both nodes and anti-nodes, and also study how specific particle properties influence the resonant optical torque. We demonstrate that adjusting particle asymmetry and losses can maximize spinning torque, and we predict "supertorque" originating from the scattering channel mixing. Our study offers a deeper understanding of the physics of resonant optical torque and its importance in manipulating AM transfer in optical systems, with promising implications for various fields and inspiring further research in resonant light-matter interactions.

physics.optics

Hybrid dielectrophoretic-optical trap for microparticles in aqueous suspension

We demonstrate that a set of microfabricated electrodes can be coupled to a commercial optical tweezers device, implementing a hybrid electro-optical trap with multiple functionalities to manipulate micro/nanoparticles in suspension. Our design allows us to simultaneously trap tens of particles in a single potential well generated in the low electric field region of the electrode arrangement, taking advantage of negative dielectrophoresis. Together with the optical tweezers, we show that the hybrid scheme allows enhanced manipulation capabilities, including controlled loading and accumulation in the dielectrophoretic trap from the optical tweezers, selectivity, and tracking of the individual trajectories of trapped particles.

cond-mat.mes-hall

3D Optofluidic Control Using Reconfigurable Thermal Barriers

Microfluidics has revolutionized control over small volumes through the use of physical barriers. However, the rigidity of these barriers limits flexibility in applications. We present an optofluidic toolbox that leverages structured light and photothermal conversion to create dynamic, reconfigurable fluidic boundaries. This system enables precise manipulation of fluids and particles by generating 3D thermal landscapes with high spatial control. Our approach replicates the functions of traditional barriers while additionally allowing real-time reconfiguration for complex tasks, such as individual particle steering and size-based sorting in heterogeneous mixtures. These results highlight the platform's potential for adaptive and multifunctional microfluidic systems in applications such as chemical synthesis, lab-on-chip devices, and microbiology, seamlessly integrating with existing setups due to its flexibility and minimal operation requirements.

cond-mat.soft

High throughput spectroscopy of pL droplets

Droplet microfluidics offers a versatile platform for analyzing liquid samples. Despite its potential, there is a lack of techniques that allow to reliably probe individual circulating droplets. The prospect of combining droplet microfluidics with sensitive, broadband spectroscopic techniques would therefore unlock new capabilities for various disciplines, including biomedicine and biochemistry. Here we present an integrated optofluidic platform that seamlessly combines droplet microfluidics and advanced hyperspectral imaging. This enables high-resolution, label-free analysis of single picolitre-sized droplets, providing valuable insights into their content. As a proof-of-principle, we demonstrate the ability of our platform to study rapid dynamic changes in a heterogeneous population of plasmonic nanoparticles with millisecond-time resolution. Furthermore, we demonstrate the effectiveness of the platform in biosensing applied to short DNA strands, achieving a detection sensitivity in the range of 100 pM. Finally, we show that the platform provides the flexibility to monitor samples over extended periods of time (hours) in a multiplexed manner.

q-bio.QM

Vacuum levitation and motion control on chip

Levitation in vacuum has evolved into a versatile technique which has already benefited diverse scientific directions, from force sensing and thermodynamics to material science and chemistry. It also holds great promises of advancing the study of quantum mechanics in the unexplored macroscopic regime. While most current levitation platforms are complex and bulky, miniaturization is sought to gain robustness and facilitate their integration into confined settings, such as cryostats or portable devices. Integration on chip is also anticipated to enhance the control over the particle motion through a more precise engineering of optical and electric fields. As a substantial milestone towards this goal, we present here levitation and motion control in high vacuum of a silica nanoparticle at the surface of a hybrid optical-electrostatic chip. By combining fiber-based optical trapping and sensitive position detection with cold damping through planar electrodes, we cool the particle motion to a few hundred phonons. Our results pave the way to the next generation of integrated levitation platforms combining integrated photonics and nanophotonics with engineered electric potentials, towards complex state preparation and read out.

physics.optics

Molecular fingerprinting of biological nanoparticles with a label-free optofluidic platform

Label-free detecting multiple analytes in a high-throughput fashion has been one of the long-sought goals in biosensing applications. Yet, for all-optical approaches, interfacing state-of-the-art label-free techniques with microfluidics tools that can process small volumes of sample with high throughput, and with surface chemistry that grants analyte specificity, poses a critical challenge to date. Here, we introduce an optofluidic platform that brings together state-of-the-art digital holography with PDMS microfluidics by using supported lipid bilayers as a surface chemistry building block to integrate both technologies. Specifically, this platform fingerprints heterogeneous biological nanoparticle populations via a multiplexed label-free immunoaffinity assay with single particle sensitivity. Herein, we first thoroughly characterise the robustness and performance of the platform, and then apply it to profile four distinct ovarian cell-derived extracellular vesicle populations over a panel of surface protein biomarkers, thus developing a unique biomarker fingerprint for each cell line. We foresee that our approach will find many applications where routine and multiplexed characterisation of biological nanoparticles is required.

q-bio.QM

Non steady-state thermometry with optical diffraction tomography

Measurement of local temperature using label-free optical methods has gained importance as a pivotal tool in both fundamental and applied research. Yet, most of these approaches are limited to steady-state measurements of planar heat sources. However, the time taken to reach steady-state is a complex function of the volume of the heated system, the size of the heat source, and the thermal conductivity of the surroundings. As such, said time can be significantly longer than expected and many relevant systems involve 3D heat sources, thus compromising reliable temperature retrieval. Here, we systematically study the thermal landscape in a model system consisting of optically excited gold nanorods (AuNRs) in a microchamber using optical diffraction tomography (ODT) thermometry. We experimentally unravel the effect of thermal conductivity of the surroundings, microchamber height, and pump pulse duration on the thermodynamics of the microchamber. We benchmark our experimental observations against 2D numerical sumulations and quantitative phase imaging (QPI) thermometry. We also demonstrate the advantage of ODT thermometry by measuring thermal landscapes inaccessible by QPI thermometry in the form of non-planar heat sources embedded in complex environments such as biological cells. Finally, we apply ODT thermometry to a complex dynamic system consisting of colloidal AuNRs in a microchamber.

physics.optics

Levitated Optomechanics with Meta-Atoms

We propose to introduce additional control in levitated optomechanics by trapping a meta-atom, i.e. a subwavelength and high-permittivity dielectric particle supporting Mie resonances. In particular, we theoretically demonstrate that optical levitation and center-of-mass ground-state cooling of silicon nanoparticles in vacuum is not only experimentally feasible but it offers enhanced performance over widely used silica particles, in terms of both trap frequency and trap depth. Moreover, we show that, by adjusting the detuning of the trapping laser with respect to the particle's resonance, the sign of the polarizability becomes negative, enabling levitation in the minimum of laser intensity e.g. at the nodes of a standing wave. The latter opens the door to trapping nanoparticles in the optical near-field combining red and blue-detuned frequencies, in analogy to two-level atoms, which is of interest for generating strong coupling to photonic nanostructures and short-distance force sensing.

physics.optics

Ultra-thin Tunable Optomechanical Metalens

Reconfigurable metasurfaces offer great promises to enhance photonics technology by combining integration with improved functionalities. Recently, reconfigurability in otherwise static metasurfaces has been achieved by modifying the electric permittivity of the meta-atoms themselves or their immediate surrounding. Yet, it remains challenging to achieve significant and fast tunability without increasing bulkiness. Here, we demonstrate an ultra-thin tunable metalens whose focal distance can be changed through optomechanical control with moderate continuous wave intensities. We achieve fast focal length changes of more than 5% with response time of the order of 10$μ$s

physics.optics

Simultaneous ground-state cooling of two mechanical modes of a levitated nanoparticle

The quantum ground state of a massive mechanical system is a steppingstone for investigating macroscopic quantum states and building high fidelity sensors. With the recent achievement of ground-state cooling of a single motional mode, levitated nanoparticles have entered the quantum domain. To overcome detrimental cross-coupling and decoherence effects, quantum control needs to be expanded to more system dimensions, but the effect of a decoupled dark mode has thus far hindered cavity-based ground state cooling of multiple mechanical modes. Here, we demonstrate two-dimensional (2D) ground-state cooling of an optically levitated nanoparticle. Utilising coherent scattering into an optical cavity mode, we reduce the occupation numbers of two separate centre-of-mass modes to 0.83 and 0.81, respectively. By controlling the frequency separation and the cavity coupling strengths of the nanoparticle's mechanical modes, we show the transition from 1D to 2D ground-state cooling while avoiding the effect of dark modes. Our results lay the foundations for generating quantum-limited high orbital angular momentum states with applications in rotation sensing. The demonstrated 2D control, combined with already shown capabilities of ground-state cooling along the third motional axis, opens the door for full 3D ground-state cooling of a massive object.

quant-ph

Roadmap for Optical Tweezers

Optical tweezers are tools made of light that enable contactless pushing, trapping, and manipulation of objects ranging from atoms to space light sails. Since the pioneering work by Arthur Ashkin in the 1970s, optical tweezers have evolved into sophisticated instruments and have been employed in a broad range of applications in life sciences, physics, and engineering. These include accurate force and torque measurement at the femtonewton level, microrheology of complex fluids, single micro- and nanoparticle spectroscopy, single-cell analysis, and statistical-physics experiments. This roadmap provides insights into current investigations involving optical forces and optical tweezers from their theoretical foundations to designs and setups. It also offers perspectives for applications to a wide range of research fields, from biophysics to space exploration.

physics.optics

Mechanical squeezing via unstable dynamics in a microcavity

We theoretically show that strong mechanical quantum squeezing in a linear optomechanical system can be rapidly generated through the dynamical instability reached in the far red-detuned and ultrastrong coupling regime. We show that this mechanism, which harnesses unstable multimode quantum dynamics, is particularly suited to levitated optomechanics, and we argue for its feasibility for the case of a levitated nanoparticle coupled to a microcavity via coherent scattering. We predict that for sub-millimeter-sized cavities the particle motion, initially thermal and well above its ground state, becomes mechanically squeezed by tens of decibels on a microsecond timescale. Our results bring forth optical microcavities in the unresolved sideband regime as powerful mechanical squeezers for levitated nanoparticles, and hence as key tools for quantum-enhanced inertial and force sensing.

quant-ph