arXiv subjects

Romain Quidant

Publications and source records attributed to Romain Quidant.

At least 37 records · Page 2Linked to original sources

arXiv2022

Mechanical squeezing via unstable dynamics in a microcavity

We theoretically show that strong mechanical quantum squeezing in a linear optomechanical system can be rapidly generated through the dynamical instability reached in the far red-detuned and ultrastrong coupling regime. We show that this mechanism, which harnesses unstable multimode quantum dynamics, is particularly suited to levitated optomechanics, and we argue for its feasibility for the case of a levitated nanoparticle coupled to a microcavity via coherent scattering. We predict that for sub-millimeter-sized cavities the particle motion, initially thermal and well above its ground state, becomes mechanically squeezed by tens of decibels on a microsecond timescale. Our results bring forth optical microcavities in the unresolved sideband regime as powerful mechanical squeezers for levitated nanoparticles, and hence as key tools for quantum-enhanced inertial and force sensing.

quant-ph↗

arXiv2022

On-Demand Activation of Photochromic Nanoheaters for High Color Purity 3D Printing

The creation of white and multicoloured 3D-printed objects with high colour fidelity via powder sintering processes is currently limited by discolouration from thermal sensitizers used in the printing process. Here we circumvent this problem by using switchable, photochromic tungsten oxide nanoparticles, which are colourless even at high concentrations. Upon ultraviolet illumination, the tungsten oxide nanoparticles can be reversibly activated making them highly absorbing in the infrared. Their strong infrared absorption upon activation renders them efficient photothermal sensitizers that can act as fusing agents for polymer powders in sintering-based 3D printing. The WO3 nanoparticles show fast activation times, and when mixed with polyamide powders they exhibit a heating-to-colour-change ratio greatly exceeding other sensitizers in the literature. Upon mixing with coloured inks, powders containing WO3 display identical colouration to a pristine powder. This demonstrates the potential of WO3, and photochromic nanoparticles in general as a new class of material for advanced manufacturing.

physics.app-ph↗

arXiv2022

A chemical nano-reactor based on a levitated nanoparticle in vacuum

A single levitated nanoparticle is used as a nano-reactor for studying surface chemistry at the nanoscale. Optical levitation under controlled pressure, surrounding gas composition, and humidity provides extreme control over the nanoparticle, including dynamics, charge, and surface chemistry. Using a single nanoparticle avoids ensemble averages and allows to study how the presence of silanol groups at its surface affects the adsorption and desorption of water from the background gas with unprecedented real time, spatial, and temporal resolution. Here, we demonstrate the unique potential of this versatile platform by studying the Zhuravlev model in silica particles. In contrast to standard methods, our system allowed the first observation of an abrupt and irreversible change in scattering cross section, mass, and mechanical eigenfrequency during the dehydroxylation process, indicating changes in density, refractive index and volume.

physics.chem-ph↗

arXiv2021

Precision calibration of the Duffing oscillator with phase control

The Duffing oscillator is a nonlinear extension of the ubiquitous harmonic oscillator and as such plays an outstanding role in science and technology. Experimentally, the system parameters are determined by a measurement of its response to an external excitation. When changing the amplitude or frequency of the external excitation, a sudden jump in the response function reveals the nonlinear dynamics prominently. However, this bistability leaves part of the full response function unobserved, which limits the precise measurement of the system parameters. Here, we exploit the often unknown fact that the response of a Duffing oscillator with nonlinear damping is a unique function of its phase. By actively stabilizing the oscillator's phase we map out the full response function. This phase control allows us to precisely determine the system parameters. Our results are particularly important for characterizing nanoscale resonators, where nonlinear effects are observed readily and which hold great promise for next generation of ultrasensitive force and mass measurements. We demonstrate our approach experimentally with an optically levitated particle in high vacuum.

physics.app-ph↗

arXiv2021

Strong Optomechanical Coupling at Room Temperature by Coherent Scattering

Quantum control of a system requires the manipulation of quantum states faster than any decoherence rate. For mesoscopic systems, this has so far only been reached by few cryogenic systems. An important milestone towards quantum control is the so-called strong coupling regime, which in cavity optomechanics corresponds to an optomechanical coupling strength larger than cavity decay rate and mechanical damping. Here, we demonstrate the strong coupling regime at room temperature between a levitated silica particle and a high finesse optical cavity. Normal mode splitting is achieved by employing coherent scattering, instead of directly driving the cavity. The coupling strength achieved here approaches three times the cavity linewidth, crossing deep into the strong coupling regime. Entering the strong coupling regime is an essential step towards quantum control with mesoscopic objects at room temperature.

quant-ph↗

arXiv2020

Slow thermo-optomechanical pulsations in suspended 1D photonic crystal nanocavities

We investigate the nonlinear optical response of suspended 1D photonic crystal nanocavities fabricated on a silicon nitride chip. Strong thermo-optical nonlinearities are demonstrated for input powers as low as $2\,μ\text{W}$ and a self-sustained pulsing regime is shown to emerge with periodicity of several seconds. As the input power and laser wavelength are varied the temporal patterns change in period, duty cycle and shape. This dynamics is attributed to the multiple timescale competition between thermo-optical and thermo-optomechanical effects and closely resembles the relaxation oscillations states found in mathematical models of neuronal activity. We introduce a simplified model that reproduces all the experimental observations and allows us to explain them in terms of the properties of a 1D critical manifold which governs the slow evolution of the system.

physics.optics↗

arXiv2020

Extending vacuum trapping to absorbing objects with hybrid Paul-optical traps

The levitation of condensed matter in vacuum allows the study of its physical properties under extreme isolation from the environment. It also offers a venue to investigate quantum mechanics with large systems, at the transition between the quantum and classical worlds. In this work, we study a novel hybrid levitation platform that combines a Paul trap with a weak but highly focused laser beam, a configuration that integrates a deep potential with excellent confinement and motion detection. We combine simulations and experiments to demonstrate the potential of this approach to extend vacuum trapping and interrogation to a broader range of nanomaterials, such as absorbing particles. We study the stability and dynamics of different specimens, like fluorescent dielectric crystals and gold nanorods, and demonstrate stable trapping down to pressures of 1 mbar.

physics.app-ph↗

arXiv2020

Simple experimental procedures to distinguish photothermal from hot-carrier processes in plasmonics

Light absorption and scattering of plasmonic metal nanoparticles can lead to non-equilibrium charge carriers, intense electromagnetic near-fields, and heat generation, with promising applications in a vast range of fields, from chemical and physical sensing, to nanomedicine, and photocatalysis for the sustainable production of fuels and chemicals. Disentangling the relative contribution of thermal and non-thermal contributions in plasmon driven processes is however difficult. Nanoscale temperature measurements are technically challenging and macroscale experiments are often characterized by collective heating effects, which tend to make the actual temperature increase unpredictable. This work is intended to help the reader experimentally detect and quantify photothermal effects in plasmon-driven chemical reactions, to discriminate their contribution from the one due to photochemical processes, and to cast a critical eye on the current literature. To this aim, we review, and in some cases propose, seven simple experimental procedures, which do not require the use of complex or expensive thermal microscopy techniques. These proposed procedures are adaptable to a wide range of experiments and fields of research where photothermal effects need to be assessed, such as plasmonic-assisted chemistry, heterogeneous catalysis, photovoltaics, biosensing and enhanced molecular spectroscopy.

physics.optics↗

arXiv2019

Electrically Driven Varifocal Silicon Metalens

Optical metasurfaces have shown to be a powerful approach to planar optical elements, enabling an unprecedented control over light phase and amplitude. At that stage, where wide variety of static functionalities have been accomplished, most efforts are being directed towards achieving reconfigurable optical elements. Here, we present our approach to an electrically controlled varifocal metalens operating in the visible frequency range. It relies on dynamically controlling the refractive index environment of a silicon metalens by means of an electric resistor embedded into a thermo-optical polymer. We demonstrate precise and continuous tuneability of the focal length and achieve focal length variation larger than the Rayleigh length for voltage as small as 12 volts. The system time-response is of the order of 100 ms, with the potential to be reduced with further integration. Finally, the imaging capability of our varifocal metalens is successfully validated in an optical microscopy setting. Compared to conventional bulky reconfigurable lenses, the presented technology is a lightweight and compact solution, offering new opportunities for miniaturized smart imaging devices.

physics.optics↗

arXiv2019

Resolved Sideband Cooling of a Levitated Nanoparticle in the Presence of Laser Phase Noise

We investigate the influence of laser phase noise heating on resolved sideband cooling in the context of cooling the center-of-mass motion of a levitated nanoparticle in a high-finesse cavity. Although phase noise heating is not a fundamental physical constraint, the regime where it becomes the main limitation in Levitodynamics has so far been unexplored and hence embodies from this point forward the main obstacle in reaching the motional ground state of levitated mesoscopic objects with resolved sideband cooling. We reach minimal center-of-mass temperatures comparable to $T_{min}=10$mK at a pressure of $p = 3\times 10^{-7}$mbar, solely limited by phase noise. Finally we present possible strategies towards motional ground state cooling in the presence of phase noise.

quant-ph↗

arXiv2019

Optimal Feedback Cooling of a Charged Levitated Nanoparticle with Adaptive Control

We use an optimal control protocol to cool one mode of the center of mass motion of an optically levitated nanoparticle. The feedback technique relies on exerting a Coulomb force on a charged particle with a pair of electrodes and follows the control law of a linear quadratic regulator, whose gains are optimized by a machine learning algorithm in under 5 s. With a simpler and more robust setup than optical feedback schemes, we achieve a minimum center of mass temperature of 5 mK at $3\times 10^{-7}$ mbar and transients 10 to 600 times faster than cold damping. This cooling technique can be easily extended to 3D cooling and is particularly relevant for studies demanding high repetition rates and force sensing experiments with levitated objects.

physics.ins-det↗

arXiv2019

Accurate mass measurement of a levitated nanomechanical resonator for precision force sensing

Nanomechanical resonators are widely operated as force and mass sensors with sensitivities in the zepto-Newton and yocto-gram regime, respectively. Their accuracy, however, is usually undermined by high uncertainties in the effective mass of the system, whose estimation is a non-trivial task. This critical issue can be addressed in levitodynamics, where the nanoresonator typically consists of a single silica nanoparticle of well-defined mass. Yet, current methods assess the mass of the levitated nanoparticles with uncertainties up to a few tens of percent, therefore preventing to achieve unprecedented sensing performances. Here, we present a novel measurement protocol that uses the electrical field from a surrounding plate capacitor to directly drive a charged optically levitated particle in moderate vacuum. The developed technique estimates the mass within a statistical error below 1% and a systematic error of 2%, and paves the way toward more reliable sensing and metrology applications of levitodynamics systems.

physics.ins-det↗

arXiv2018

Plasmonic waveguide-integrated nanowire laser

Next-generation optoelectronic devices and photonic circuitry will have to incorporate on-chip compatible nanolaser sources. Semiconductor nanowire lasers have emerged as strong candidates for integrated systems with applications ranging from ultrasensitive sensing, to data communication technologies. Despite significant advances in their fundamental aspects, the integration within scalable photonic circuitry remains challenging. Here we report on the realization of hybrid photonic devices consisting of nanowire lasers integrated with wafer-scale lithographically designed V-groove plasmonic waveguides. We present experimental evidence of the lasing emission and coupling into the propagating modes of the V-grooves, enabling on-chip routing of coherent and sub-diffraction confined light with room temperature operation. Theoretical considerations suggest that the observed lasing is enabled by a waveguide hybrid photonic-plasmonic mode. This work represents a major advance towards the realization of application-oriented photonic circuits with integrated nanolaser sources.

physics.optics↗

arXiv2018

Quantum Emitters in Hexagonal Boron Nitride Have Spectrally Tunable Quantum Efficiency

Understanding the properties of novel solid-state quantum emitters is pivotal for a variety of applications in field ranging from quantum optics to biology. Recently discovered defects in hexagonal boron nitride are especially interesting, as they offer much desired characteristics such as narrow emission lines and photostability. Here, we study the dependence of the emission on the excitation wavelength. We find that, in order to achieve bright single photon emission with high quantum efficiency, the excitation wavelength has to be matched to the emitter. This is a strong indication that the emitters possess a complex level scheme and cannot be described by a simple two or three level system. Using this excitation dependence of the emission, we thus gain further insight to the internal level scheme and demonstrate how to distinguish different emitters both spatially as well as in terms of their photon correlations.

cond-mat.mes-hall↗

arXiv2017

Optically levitated nanoparticle as a model system for stochastic bistable dynamics

Nano-mechanical resonators have gained an increasing importance in nanotechnology owing to their contributions to both fundamental and applied science. Yet, their small dimensions and mass raises some challenges as their dynamics gets dominated by nonlinearities that degrade their performance, for instance in sensing applications. Here, we report on the precise control of the nonlinear and stochastic bistable dynamics of a levitated nanoparticle in high vacuum. We demonstrate how it can lead to efficient signal amplification schemes, including stochastic resonance. This work paves the way for the use of levitated nanoparticles as a model system for stochastic bistable dynamics, with applications to a wide variety of fields.

physics.optics↗

arXiv2017

On-a-chip biosensing based on all-dielectric nanoresonators

Nanophotonics has become a key enabling technology in biomedicine with great promises in early diagnosis and less invasive therapies. In this context, the unique capability of plasmonic noble metal nanoparticles to concentrate light on the nanometer scale has widely contributed to biosensing and enhanced spectroscopy. Recently, high-refractive index dielectric nanostructures featuring low loss resonances have been proposed as a promising alternative to nanoplasmonics, potentially offering better sensing performances along with full compatibility with the microelectronics industry. In this letter we report the first demonstration of biosensing with silicon nanoresonators integrated in state-of-the-art microfluidics. Our lab-on-a-chip platform enables detecting Prostate Specific Antigen (PSA) cancer marker in human serum with a sensitivity that meets clinical needs. These performances are directly compared with its plasmonic counterpart based on gold nanorods. Our work opens new opportunities in the development of future point-of-care devices towards a more personalized healthcare.

physics.app-ph↗

arXiv2016

Trapping and manipulation of individual nanoparticles in a planar Paul trap

Visualization and manipulation of nanoscale matter is one of the main and current challenges in nanosciences. To this aim, different techniques have been recently developed to non-invasively trap and manipulate nano-specimens, like nanoparticles or molecules. However, operating in air or vacuum still remains very challenging since most approaches are limited to a liquid environment. In this letter, we design and characterize a planar Paul trap optimized to trap and manipulate individual charged nanoparticles. This configuration offers competitive capabilities to manipulate nano-specimens in air or vacuum including in-plane integration, high trap confinement along with dynamical trap reconfiguration.

cond-mat.mes-hall↗

arXiv2016

Direct Measurement of Photon Recoil from a Levitated Nanoparticle

The momentum transfer between a photon and an object defines a fundamental limit for the precision with which the object can be measured. If the object oscillates at a frequency $Ω_0$, this measurement back-action adds quanta $\hbarΩ_0$ to the oscillator's energy at a rate $Γ_{\rm recoil}$, a process called photon recoil heating, and sets bounds to quantum coherence times in cavity optomechanical systems. Here, we use an optically levitated nanoparticle in ultrahigh vacuum to directly measure $Γ_{\rm recoil}$. By means of a phase-sensitive feedback scheme, we cool the harmonic motion of the nanoparticle from ambient to micro-Kelvin temperatures and measure its reheating rate under the influence of the radiation field. The recoil heating rate is measured for different particle sizes and for different excitation powers, without the need for cavity optics or cryogenic environments. The measurements are in quantitative agreement with theoretical predictions and provide valuable guidance for the realization of quantum ground-state cooling protocols and the measurement of ultrasmall forces

physics.optics↗