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Sébastien Hentz

Publications and source records attributed to Sébastien Hentz.

12 recordsLinked to original sources

Origins of microwave losses in superconducting circuits made with silicon-on-insulator substrates

Silicon-on-insulator technology is widely used to fabricate silicon based devices, from advanced transistors to photonic circuits or nanomechanical systems. Integrating low loss superconducting quantum circuits with silicon-on-insulator substrates enables to couple the advantages offered by the mature silicon technology to the exquisite sensitivity of superconducting circuits. The natural approach, inherited from research in superconducting microwave devices, is to use a substrate made with highly resistive silicon, known for its low level of microwave losses. In this work, using superconducting microwave resonators, we show that counterintuitively, standard resistivity silicon-on-insulator substrates perform better than high resistivity silicon-on-insulator substrates at cryogenic temperatures. In the latter case, the presence of a parasitic sheet conduction at the interface between bulk silicon and silicon oxide acts as the dominant loss mechanism. This parasitic sheet can be suppressed using substrates with intentionally induced traps. In such substrates, losses are ultimately limited by the dielectric losses of the silicon oxide layer. These substrates offer interesting perspectives for the development of superconducting nanoelectromechanical systems. First, the release, i.e. the removal of the silicon oxide, could be limited to the moving parts, thereby maintaining the mechanical integrity of the rest of the device. Additionally, such structure would enhance heat evacuation into the bulk of the substrate which is an issue in current devices such as microwave-to-optics converters.

cond-mat.mes-hall↗

Multiphysics optomechanical sensing of a liquid on the micron scale

We present an optomechanical device platform for characterization of optical, thermal, and rheological properties of fluids on the micron scale. A suspended silicon microdisk resonator with a vibrating mass of 100 fg and an effective measurement volume of less than a pL is used to monitor properties of different fluids at rest. By employing analytical models for thermo-optical effects, thermal diffusion and fluid-structure interactions, our platform determines the refractive index, thermal conductivity, viscosity, density and compressibility of the fluid, in a compact measurement setup. A single measurement takes as short as 70 microseconds, and the employed power can be less than 100 microwatts, guaranteeing measurement at rest and in thermal equilibrium.

physics.app-ph↗

Amplitude stabilization in a synchronized nonlinear nanomechanical oscillator

In contrast to the well-known phenomenon of frequency stabilization in a synchronized noisy nonlinear oscillator, little is known about its amplitude stability. In this paper, we investigate experimentally and theoretically the amplitude evolution and stability of a nonlinear nanomechanical self-sustained oscillator that is synchronized with an external harmonic drive. We show that the phase difference between the tones plays a critical role on the amplitude level, and we demonstrate that in the strongly nonlinear regime, its amplitude fluctuations are reduced considerably. These findings bring to light a new facet of the synchronization phenomenon, extending its range of applications beyond the field of clock-references and suggesting a new means to enhance oscillator amplitude stability.

physics.app-ph↗

Optomechanical mass spectrometry

It has been demonstrated in the recent years that nanomechanical mass spectrometry was well suited for the analysis of specific high mass species such as viruses. Still, the exclusive use of one-dimensional devices such as vibrating beams forces a trade-off between analysis time (related to capture area) and mass resolution (inversely proportional to device mass). Such devices also require complex readout schemes to simultaneously monitor multiple resonance modes, in particular when stiffness or shape come into play, which degrades mass resolution. These issues restrict nanomechanical MS to the analysis of species with specific properties. We report here the first demonstration of single-particle mass spectrometry with nano-optomechanical resonators fabricated with a Very Large Scale Integration process. The unique motion sensitivity of optomechanical techniques allows the use of resonators with new topologies. The device introduced here is designed to be impervious to particle position, stiffness or shape, opening the way to the analysis of large aspect ratio biological objects of great significance such as viruses with a tail or fibrils. Compared to top-down beam resonators with electrical read-out and state-of-the-art mass resolution, we show a three-fold improvement in capture area with no resolution degradation, despite the use of a single resonance mode. Short analysis time is in reach thanks to the sensitivity and bandwidth of optomechanical read-out and its compliance with telecom multiplexing techniques.

physics.app-ph↗

Optomechanical Resonating Probe for Very High Speed Sensing of Atomic Forces

Atomic force spectroscopy and microscopy (AFM) are invaluable tools to characterize nanostructures and biological systems. Most experiments, including state-of-the-art images of molecular bonds, are achieved by driving probes at their mechanical resonance. This resonance reaches the MHz for the fastest AFM micro-cantilevers, with typical motion amplitude of a few nanometres. Next-generation investigations of molecular scale dynamics, including faster force imaging and higher-resolution spectroscopy of dissipative interactions, require more bandwidth and vibration amplitudes below interatomic distance, for non-perturbative short-range tip-matter interactions. Probe frequency is a key parameter to improve bandwidth while reducing Brownian motion, allowing large signal-to-noise for exquisite resolution. Optomechanical resonators reach motion detection at 10^(-18) m.(Hz)^(-1/2), while coupling light to bulk vibration modes whose frequencies largely surpass those of cantilevers. Here we introduce an optically operated resonating optomechanical atomic force probe of frequency 2 decades above the fastest functional AFM cantilevers while Brownian motion is 4 orders below. Based on a Silicon-On-Insulator technology, the probe demonstrates high-speed sensing of contact and non-contact interactions with sub-picometre driven motion, breaking open current locks for faster and finer atomic force spectroscopy.

physics.ins-det↗

Charge-independent mass spectrometry of single virus capsids above 100MDa with nanomechanical resonators

Most technologies, including conventional mass spectrometry, struggle to measure the mass of particles in the MDa to GDa range. Although this mass range appears optimal for nanomechanical resonators, early nanomechanical-MS systems suffered from prohibitive sample loss, extended analysis time or inadequate resolution. Here, we report on a novel system architecture combining nebulization of the analytes from solution, their efficient transfer and focusing without relying on electromagnetic fields, and the mass measurements of individual particles using nanomechanical resonator arrays. This system determined the mass distribution of ~30 MDa polystyrene nanoparticles with a detection efficiency 6 orders of magnitude higher than previous nanomechanical-MS systems with ion guides, and successfully performed the highest molecular mass measurement to date with less than 1 picomole of bacteriophage T5 105 MDa viral capsids.

physics.app-ph↗

Single-particle Mass Spectrometry with arrays of frequency-addressed nanomechanical resonators

One of the main challenges to overcome to perform nanomechanical Mass Spectrometry (NEMS-MS) analysis in a practical time frame stems from the size mismatch between the analyte beam and the extremely small nanomechanical detector area. We report here the demonstration of NEMS-MS with arrays of 20 individually addressed nanomechanical resonators where the number of inputs-outputs for the whole array is the same as that of a single resonator. While all resonators within an array are interconnected via two metal levels, each resonator is designed with a distinct resonance frequency which becomes its individual address. In order to perform single-particle Mass Spectrometry, the resonance frequencies of the two first modes of each NEMS within an array are monitored simultaneously. Using such an array, mass spectra of metallic aggregates in the MDa range are acquired with more than one order of magnitude improvement in analysis time due to the increase in capture cross section compared to individual resonators. A 20 NEMS array is probed in 150ms with the same mass limit of detection as a single resonator. Spectra acquired with a conventional Time- of-Flight (TOF) mass spectrometer in the same system show excellent agreement. As individual information for each resonator within the array is retained, the array becomes a particle imager, each resonator acting as a pixel. With this technique, we demonstrate how Mass Spectrometry Imaging (MSI) at the single particle level becomes possible by mapping a 4cm-particle beam in the MDa range and above.

physics.ins-det↗

Frequency fluctuations in silicon nanoresonators

Frequency stability is key to performance of nanoresonators. This stability is thought to reach a limit with the resonator's ability to resolve thermally-induced vibrations. Although measurements and predictions of resonator stability usually disregard fluctuations in the mechanical frequency response, these fluctuations have recently attracted considerable theoretical interest. However, their existence is very difficult to demonstrate experimentally. Here, through a literature review, we show that all studies of frequency stability report values several orders of magnitude larger than the limit imposed by thermomechanical noise. We studied a monocrystalline silicon nanoresonator at room temperature, and found a similar discrepancy. We propose a new method to show this was due to the presence of frequency fluctuations, of unexpected level. The fluctuations were not due to the instrumentation system, or to any other of the known sources investigated. These results challenge our current understanding of frequency fluctuations and call for a change in practices.

cond-mat.mes-hall↗

Overcoming limitations of nanomechanical resonators with simultaneous resonances

Dynamic stabilization by simultaneous primary and superharmonic resonances for high order nonlinearity cancellation is demonstrated with an electrostatically-actuated, piezoresistively-transduced nanomechanical resonator. We prove experimentally how the combination of both the third-order nonlinearity cancellation and simultaneous resonances can be used to linearly drive a nanocantilever up to very large amplitudes compared to fundamental limits like pull-in occurrence, opening the way towards resonators with high frequency stability for high-performance sensing or time reference.

cond-mat.mes-hall↗

Neutral particle Mass Spectrometry with Nanomechanical Systems

Current approaches to Mass Spectrometry (MS) require ionization of the analytes of interest. For high-mass species, the resulting charge state distribution can be complex and difficult to interpret correctly. In this article, using a setup comprising both conventional time-of-flight MS (TOF-MS) and Nano-Electro-Mechanical-Systems-based MS (NEMS-MS) in situ, we show directly that NEMS-MS analysis is insensitive to charge state: the spectrum consists of a single peak whatever the species charge state, making it significantly clearer than existing MS analysis. In subsequent tests, all charged particles are electrostatically removed from the beam, and unlike TOF-MS, NEMS-MS can still measure masses. This demonstrates the possibility to measure mass spectra for neutral particles. Thus, it is possible to envisage MS-based studies of analytes that are incompatible with current ionization techniques and the way is now open for the development of cutting edge system architectures with unique analytical capability.

physics.ins-det↗

High Frequency top-down Junction-less Silicon Nanowire Resonators

We report here the first realization of top-down silicon nanowires (SiNW) transduced by both junction-less field effect transistor (FET) and the piezoresistive (PZR) effect. The suspended SiNWs are among the smallest top-down SiNWs reported to date, featuring widths down to ~20nm. This has been achieved thanks to a 200mm-wafer-scale, VLSI process fully amenable to monolithic CMOS co-integration. Thanks to the very small dimensions, the conductance of the silicon nanowire can be controlled by a nearby electrostatic gate. Both the junction-less FET and the previously demonstrated PZR transduction have been performed with the same SiNW. These self-transducing schemes have shown similar signal-to-background ratios, and the PZR transduction has exhibited a relatively higher output signal. Allan deviation AD of the same SiNW has been measured with both schemes, and we obtain AD~20ppm for the FET detection and AD~3ppm for the PZR detection at room temperature and low pressure. Orders of magnitude improvements are expected from tighter electrostatic control via changes in geometry and doping level, as well as from CMOS integration. The compact, simple topology of these elementary SiNW resonators opens up new paths towards ultra-dense arrays for gas and mass sensing, time keeping or logic switching systems in SiNW-CMOS platform.

cond-mat.mes-hall↗

Comparison of capacitive and frequential readout when scaling accelerometers down from Micro- to Nano- Electro Mechanical Systems

This paper shows the effect of scaling silicon accelerometers down from MEMS to NEMS. It models both electronics and Brownian noise sources for both capacitive and resonant devices, and computes the minimum detectable signal attainable. Computed results are remarkably close to published experimental results. It shows the relatively low influence of the quality factor and of the beam width in the resonant case. Different scaling rules are investigated, and it appears that resonant sensing may satisfy some new application requirements, in particular for critical dimensions below a few hundreds of nm, when it is better resolved than capacitive sensing.

physics.ins-det↗