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Sören Dörscher

Publications and source records attributed to Sören Dörscher.

16 recordsLinked to original sources

International Optical Clock Comparison Using the European Optical Fiber Network

Optical clocks have achieved remarkable estimated fractional frequency uncertainties reaching the $10^{-18}$ level and below, enabling applications in fundamental physics, general relativity, and geodesy. However, the challenge of verifying the international consistency of optical clocks remains critical as efforts intensify toward redefining the SI second based on an optical transition or transitions. We report on a two-month international clock comparison campaign involving seven optical clocks in four national metrology institutes (INRIM, LNE-OP, NPL, and PTB) connected via the optical fiber network established in Europe. The campaign resulted in optical frequency ratios with uncertainties ranging from $7.7\times10^{-18}$ to $6.1\times10^{-17}$. Among the results, the $^{171}$Yb$^+$(E3) clocks at NPL and PTB demonstrated agreement within an uncertainty of $7.7\times10^{-18}$, marking the first international verification of two independently developed optical clocks below one part in $10^{17}$. The operation of the $^{199}$Hg clock at LNE-OP (formerly LNE-SYRTE) resulted in frequency ratios with improved uncertainties with $^{171}$Yb$^+$(E3), $^{171}$Yb, and $^{87}$Sr optical clocks. These results provide input for the redefinition of the second and underscore how fiber-linked clock networks can advance metrology and scientific applications.

physics.atom-ph↗

Interspecies clock comparison below $5 \times 10^{-18}$ uncertainty with a transportable clock

We report a measurement of the optical frequency ratio between the $^2\mathrm{S}_{1/2}(F=0)$--${^2\mathrm{F}_{7/2}(F=3)}$ electric-octupole (E3) transition of $^{171}$Yb$^{+}$ and the $^1\mathrm{S}_0$--${^3\mathrm{P}_0}$ transition of $^{87}$Sr, $ν_{\mathrm{Yb}^{+}}/ν_\mathrm{Sr} = 1.495\,991\,618\,544\,900\,588\,1(65)$. Reaching a fractional uncertainty of $4.3 \times 10^{-18}$, this result improves upon the previous best by more than a factor of three and is among the few that meet the requirements for interspecies clock comparisons specified by the roadmap towards the redefinition of the SI second. The comparison is between a transportable optical lattice clock and a stationary single-ion clock. It spans a period of nearly two years, during which the transportable clock was intermittently operated off-campus. The ratio was reproducibly measured during four separate campaigns, which are consistent within their statistical uncertainties. The results demonstrate reproducible $10^{-18}$ level operation of the transportable clock and thus validate its application for chronometric geodesy and as a transfer standard for inter-institute clock comparisons, e.g., in the absence of optical fiber links.

physics.atom-ph↗

An Al$^+$ clock with $1.6\times10^{-18}$ systematic uncertainty and its frequency ratios

Advances in optical clocks motivate a redefinition of the second, requiring rigorous evaluations of systematic uncertainties and robust consistency among the clocks. Here, we report the full evaluation of the systematic frequency shifts of an $^{27}\mathrm{Al}^+$ single-ion clock, and the measurement of its absolute frequency and frequency ratio with a $^{87}$Sr optical lattice clock at PTB. The evaluated total systematic fractional frequency uncertainty is $1.6\times10^{-18}$, mainly limited by the accuracy of the relevant atomic coefficients and by background gas collisions. The absolute frequency of the clock has been measured to be $ν_{\mathrm{Al}^+}=1 121 015 393 207 859.19(24)\,$Hz, obtained by comparison with two primary caesium fountain clocks at PTB. The frequency ratio between the Al and Sr optical clocks has been determined to be $ν_{\mathrm{Al}^+}/ν_{^{87}\mathrm{Sr}}=2.611 701 431 781 462 668(36)$, limited by the accuracy of the Sr clock. This ratio differs by $8.6σ$ and $1.2σ$ from the 2021 and 2025 frequency ratio published by the BACON collaboration, respectively. These results represent an important contribution toward a future redefinition of the second using optical clocks, and underscore the importance of independent measurements of clock-candidate frequency ratios across different institutions.

physics.atom-ph↗

A high-stability optical clock based on a continuously ground-state cooled Al$^+$ ion without compromising its accuracy

Single ion optical clocks have shown systematic frequency uncertainties below $10^{-18}$, but typically require more than one week of averaging to achieve a corresponding statistical uncertainty. This time can be reduced with longer probe times, but comes at the cost of a higher time-dilation shift due to motional heating of the ions in the trap. We show that sympathetic ground-state cooling using electromagnetically-induced transparency (EIT) of an \Al clock ion via a co-trapped \Ca ion during clock interrogation suppresses the heating of the ions. \Al can be kept close to the motional ground state, independent from the chosen interrogation time, at a relative time dilation shift of $(-1.69\pm0.20)\times10^{-18}$. The \Ca cooling light introduces an additional light shift on the \Al clock transition of $(-9.27\pm 1.03)\times10^{-18}$. We project that the uncertainty of this light shift can be further reduced by nearly an order of magnitude. This sympathetic cooling enables seconds of interrogation time with $10^{-19}$ motional and cooling laser-induced uncertainties for \Al and can be employed in other ion clocks as well.

physics.atom-ph↗

Entanglement-enhanced optical ion clock

Entangled states hold the promise of improving the precision and accuracy of quantum sensors. We experimentally demonstrate that spectroscopy of an optical clock transition using entangled states can outperform its classical counterpart. Two ^{40}\text{Ca}^{+} ions are entangled in a quantum state with vanishing first-order magnetic field sensitivity, extending the coherence time of the atoms and enabling near lifetime-limited probe times of up to 550 ms. In our protocol, entangled ions reach the same instability as uncorrelated ions, but at half the probe time, enabling faster cycle times of the clock. We run two entangled ^{40}\text{Ca}^{+} ions as an optical clock and compare its frequency instability with a ^{87}\text{Sr} lattice clock. The instability of the entangled ion clock is below a clock operated with classically correlated states for all probe times. We observe instabilities below the theoretically expected quantum projection noise limit of two uncorrelated ions for interrogation times below 100 ms. The lowest fractional frequency instability of 7e-16 / sqrt(tau / 1 s) is reached for 250 ms probe time, limited by residual phase noise of the probe laser. This represents the lowest instability reported to date for a ^{40}\text{Ca}^{+} ion clock.

physics.atom-ph↗

Coordinated international comparisons between optical clocks connected via fiber and satellite links

Optical clocks provide ultra-precise frequency references that are vital for international metrology as well as for tests of fundamental physics. To investigate the level of agreement between different clocks, we simultaneously measured the frequency ratios between ten optical clocks in six different countries, using fiber and satellite links. This is the largest coordinated comparison to date, from which we present a subset of 38 optical frequency ratios and an evaluation of the correlations between them. Four ratios were measured directly for the first time, while others had significantly lower uncertainties than previously achieved, supporting the advance towards a redefinition of the second and the use of optical standards for international time scales.

physics.atom-ph↗

International comparison of optical frequencies with transportable optical lattice clocks

Optical clocks have improved their frequency stability and estimated accuracy by more than two orders of magnitude over the best caesium microwave clocks that realise the SI second. Accordingly, an optical redefinition of the second has been widely discussed, prompting a need for the consistency of optical clocks to be verified worldwide. While satellite frequency links are sufficient to compare microwave clocks, a suitable method for comparing high-performance optical clocks over intercontinental distances is missing. Furthermore, remote comparisons over frequency links face fractional uncertainties of a few $10^{-18}$ due to imprecise knowledge of each clock's relativistic redshift, which stems from uncertainty in the geopotential determined at each distant location. Here, we report a landmark campaign towards the era of optical clocks, where, for the first time, state-of-the-art transportable optical clocks from Japan and Europe are brought together to demonstrate international comparisons that require neither a high-performance frequency link nor information on the geopotential difference between remote sites. Conversely, the reproducibility of the clocks after being transported between countries was sufficient to determine geopotential height offsets at the level of 4 cm. Our campaign paves the way for redefining the SI second and has a significant impact on various applications, including tests of general relativity, geodetic sensing for geosciences, precise navigation, and future timing networks.

physics.atom-ph↗

Experimental determination of the E2-M1 polarizability of the strontium clock transition

To operate an optical lattice clock at a fractional uncertainty below $10^{-17}$, one must typically consider not only electric-dipole (E1) interaction between an atom and the lattice light field when characterizing the resulting lattice light shift of the clock transition but also higher-order multipole contributions, such as electric-quadrupole (E2) and magnetic-dipole (M1) interactions. However, strongly incompatible values have been reported for the E2-M1 polarizability difference of the clock states $(5s5p)\,{}^{3}\mathrm{P}_{0}$ and $(5s^2)\,{}^{1}\mathrm{S}_{0}$ of strontium [Ushijima et al., Phys. Rev. Lett. 121 263202 (2018); Porsev et al., Phys. Rev. Lett. 120, 063204 (2018)]. This largely precludes operating strontium clocks with uncertainties of few $10^{-18}$, as the resulting lattice light shift corrections deviate by up to $1 \times 10^{-17}$ from each other at typical trap depths. We have measured the E2-M1 polarizability difference using our ${}^{87}\mathrm{Sr}$ lattice clock and find a value of $Δα_{\mathrm{qm}} = -987^{+174}_{-223} \; \mathrm{μHz}$. This result is in very good agreement with the value reported by Ushijima et al.

physics.atom-ph↗

A transportable clock laser system with an instability of $1.6 \times 10^{-16}$

We present a transportable ultra-stable clock laser system based on a Fabry-Pérot cavity with crystalline Al$_{0.92}$Ga$_{0.08}$As/GaAs mirror coatings, fused silica (FS) mirror substrates and a 20~cm-long ultra-low expansion (ULE\textsuperscript{\textregistered}) glass spacer with a predicted thermal noise floor of $\mathrm{mod}\,σ_\mathrm{y} = 7 \times 10^{-17}$ in modified Allan deviation at one second averaging time. The cavity has a cylindrical shape and is mounted at ten points. Its measured sensitivity of the fractional frequency to acceleration for the three Cartesian directions are $2(1) \times 10^{-12}$/(ms$^{-2}$), $3(3) \times 10^{-12}$/(ms$^{-2}$) and $3(1) \times 10^{-12}$/(ms$^{-2}$), which belong to the lowest acceleration sensitivities published for transportable systems. The laser system's instability reaches down to $\mathrm{mod}\,σ_\mathrm{y} = 1.6 \times 10^{-16}$

physics.optics↗

Optical frequency ratio of a ${}^{171}\mathrm{Yb}^+$ single-ion clock and a ${}^{87}\mathrm{Sr}$ lattice clock

We report direct measurements of the frequency ratio of the 642 THz ${}^2S_{1/2} (F=0)$--${}^2F_{7/2} (F=3)$ electric octupole transition in ${}^{171}\mathrm{Yb}^+$ and the 429 THz ${}^1S_0$--${}^3P_0$ transition in ${}^{87}\mathrm{Sr}$. A series of 107 measurements has been performed at the Physikalisch-Technische Bundesanstalt between December 2012 and October 2019. Long-term variations of the ratio are larger than expected from the individual measurement uncertainties of few $10^{-17}$. The cause of these variations remains unknown. Even taking these into account, we find a fractional uncertainty of the frequency ratio of $2.5 \times 10^{-17}$, which improves upon previous knowledge by one order of magnitude. The average frequency ratio is $ν_{\mathrm{Yb}^+} / ν_{\mathrm{Sr}} = 1.495\,991\,618\,544\,900\,537(38)$. This represents one of the most accurate measurements between two different atomic species to date.

physics.atom-ph↗

Dynamic decoupling of laser phase noise in compound atomic clocks

The frequency stability achieved by an optical atomic clock ultimately depends on the coherence of its local oscillator. Even the best ultrastable lasers only allow interrogation times of a few seconds, at present. Here we present a universal measurement protocol that overcomes this limitation. Engineered dynamic decoupling of laser phase noise allows any optical atomic clock with high signal-to-noise ratio in a single interrogation to reconstruct the laser's phase well beyond its coherence limit. A compound clock is then formed in combination with another optical clock of any type, allowing the latter to achieve significantly higher frequency stability than on its own. We demonstrate implementation of the protocol in a realistic proof-of-principle experiment with a phase reconstruction fidelity of 99 %. The protocol enables minute-long interrogation for the best ultrastable laser systems. Likewise, it can improve clock performance where less stable local oscillators are used, such as in transortable systems.

physics.atom-ph↗

Guidelines for developing optical clocks with $10^{-18}$ fractional frequency uncertainty

There has been tremendous progress in the performance of optical frequency standards since the first proposals to carry out precision spectroscopy on trapped, single ions in the 1970s. The estimated fractional frequency uncertainty of today's leading optical standards is currently in the $10^{-18}$ range, approximately two orders of magnitude better than that of the best caesium primary frequency standards. This exceptional accuracy and stability is resulting in a growing number of research groups developing optical clocks. While good review papers covering the topic already exist, more practical guidelines are needed as a complement. The purpose of this document is therefore to provide technical guidance for researchers starting in the field of optical clocks. The target audience includes national metrology institutes (NMIs) wanting to set up optical clocks (or subsystems thereof) and PhD students and postdocs entering the field. Another potential audience is academic groups with experience in atomic physics and atom or ion trapping, but with less experience of time and frequency metrology and optical clock requirements. These guidelines have arisen from the scope of the EMPIR project "Optical clocks with $1 \times 10^{-18}$ uncertainty" (OC18). Therefore, the examples are from European laboratories even though similar work is carried out all over the world. The goal of OC18 was to push the development of optical clocks by improving each of the necessary subsystems: ultrastable lasers, neutral-atom and single-ion traps, and interrogation techniques. This document shares the knowledge acquired by the OC18 project consortium and gives practical guidance on each of these aspects.

physics.atom-ph↗

Lattice-induced photon scattering in an optical lattice clock

We investigate scattering of lattice laser radiation in a strontium optical lattice clock and its implications for operating clocks at interrogation times up to several tens of seconds. Rayleigh scattering does not cause significant decoherence of the atomic superposition state near a magic wavelength. Among the Raman scattering processes, lattice-induced decay of the excited state $(5s5p)\,{}^{3}\mathrm{P}_{0}$ to the ground state $(5s^2)\,{}^{1}\mathrm{S}_{0}$ via the state $(5s5p)\,{}^{3}\mathrm{P}_{1}$ is particularly relevant, as it reduces the effective lifetime of the excited state and gives rise to quantum projection noise in spectroscopy. We observe this process in our experiment and find a decay rate of $556(15)\times 10^{-6}\,\mathrm{s}^{-1}$ per photon recoil energy $E_\mathrm{r}$ of effective lattice depth, which agrees well with the rate we predict from atomic data. We also derive a natural lifetime $τ= 330(140)\,\mathrm{s}$ of the excited state ${}^{3}\mathrm{P}_{0}$ from our observations. Lattice-induced decay thus exceeds spontaneous decay at typical lattice depths used by present clocks. It eventually limits interrogation times in clocks restricted to high-intensity lattices, but can be largely avoided, e.g., by operating them with shallow lattice potentials.

physics.atom-ph↗

A high-performance optical lattice clock based on bosonic atoms

Optical lattice clocks with uncertainty and instability in the $10^{-17}$-range and below have so far been demonstrated exclusively using fermions. Here, we demonstrate a bosonic optical lattice clock with $3\times 10^{-18}$ instability and $2.0\times 10^{-17}$ accuracy, both values improving on previous work by a factor 30. This was enabled by probing the clock transition with an ultra-long interrogation time of 4 s, using the long coherence time provided by a cryogenic silicon resonator, by careful stabilization of relevant operating parameters, and by operating at low atom density. This work demonstrates that bosonic clocks, in combination with highly coherent interrogation lasers, are suitable for high-accuracy applications with particular requirements, such as high reliability, transportability, operation in space, or suitability for particular fundamental physics topics. As an example, we determine the $^{88}\textrm{Sr} - ^{87}$Sr isotope shift with 12 mHz uncertainty.

physics.atom-ph↗

Noise and instability of an optical lattice clock

We present an analysis of the different types of noise from the detection and interrogation laser in our strontium lattice clock. We develop a noise model showing that in our setup quantum projection noise--limited detection is possible if more than 130~atoms are interrogated. Adding information about the noise spectrum of our clock laser with sub-$10^{-16}$ fractional frequency instability allows to infer the clock stability for different modes of operation. Excellent agreement with experimental observations for the instability of the difference between two interleaved stabilizations is found. We infer a clock instability of $1.6 \times 10^{-16}/\sqrt{τ/ \mathrm{s}}$ as a function of averaging time $τ$ for normal clock operation.

physics.atom-ph↗

Creation of Quantum-Degenerate Gases of Ytterbium in a Compact 2D-/3D-MOT Setup

We report on the first experimental setup based on a 2D-/3D-MOT scheme to create both Bose-Einstein condensates and degenerate Fermi gases of several ytterbium isotopes. Our setup does not require a Zeeman slower and offers the flexibility to simultaneously produce ultracold samples of other atomic species. Furthermore, the extraordinary optical access favors future experiments in optical lattices. A 2D-MOT on the strong 1S0-1P1 transition captures ytterbium directly from a dispenser of atoms and loads a 3D-MOT on the narrow 1S0-3P1 intercombination transition. Subsequently, atoms are transferred to a crossed optical dipole trap and cooled evaporatively to quantum degeneracy.

cond-mat.quant-gas↗