arXiv subjects

S. -H. Lee

Publications and source records attributed to S. -H. Lee.

At least 19 recordsLinked to original sources

arXiv2025

Photocurrent detected 2D spectroscopy via pulse shaper: insights and strategies for optimally untangling the nonlinear response

Action-detected two-dimensional electronic spectroscopy (A-2DES) provides valuable insights into ultrafast dynamics within functional materials and devices by measuring incoherent signals like photocurrent. This work details the implementation and optimization of a pulse-shaper-based A-2DES setup, focusing on methodological strategies crucial for acquiring high-fidelity data. We present a comprehensive analysis of phase modulation routines, elucidating the critical interplay between pattern parameters (N, $\mathrm{n}_\mathrm{i}$), pattern repetitions ($\mathrm{N}_\mathrm{rep}$), laser repetition rate, and acousto-optic pulse shaper constraints (e.g., streaming rate, RF generator nonlinearities). Utilizing a perovskite solar cell as a model system, we systematically identify and characterize significant inaccuracies inherent to A-2DES measurements. These include distortions originating from Fourier transform processing of improperly trimmed time-domain data (phase leakage), signal accumulation effects due to insufficient sample response discharge between pulse sequences at high repetition rates, and shortcomings induced by pulse shaper operation at elevated streaming powers. Crucially, we demonstrate robust data post-processing strategies, including precise data point selection for Fourier analysis and phase correction routine, to effectively mitigate these imperfections and retrieve accurate 2D spectra. This rigorous methodological investigation and anomalous features characterization provides essential guidelines for optimizing pulse-shaper-based A-2DES experiments, ensuring data integrity and enabling reliable extraction of complex photophysical information in complex systems.

physics.chem-ph↗

arXiv2025

Tracing the ejecta structure of SN 1987A: Insights and diagnostics from 3D MHD simulations

Supernova (SN) 1987A provides a unique window into the aftermath of a massive stellar explosion, offering key insights into the ejecta's morphology, composition, explosion mechanism, progenitor system, and circumstellar medium (CSM) interaction. We investigate large-scale ejecta asymmetries in SN 1987A. By comparing the simulations with JWST observations and making predictions for XRISM, we aim to refine our understanding of the explosion mechanism and the remnant's evolution. We performed 3D MHD simulations that trace the evolution of SN 1987A from the SN to the SNR, extending our predictions up to 5000 years into the future and considering the Ni-bubble effects. The simulation results are compared with JWST observations and used to predict XRISM spectra, to evaluate the accuracy of the modeled ejecta structure. Our simulations reproduce the large-scale Fe-rich ejecta morphology seen by JWST, revealing two clumps suggestive of a bipolar explosion. Ni-bubble effects in the first year boost Fe-rich ejecta expansion and their interaction with the reverse shock. However, discrepancies with JWST observations in clump velocities and spatial distribution suggest stronger explosion asymmetries than modeled. Since 2021, our models predict that shocked ejecta have contributed increasingly to X-ray emission, now rivaling shocked CSM and soon dominating as the latter fades. Future XRISM observations will trace the evolution of these ejecta structures, refining constraints on explosion geometry. Early remnant asymmetries from CSM interaction may persist for at least 100 years. Our results underscore the role of asymmetric core-collapse mechanisms in shaping SN 1987A's ejecta and constraining its explosion geometry. Future studies should explore more extreme asymmetries, in neutrino-driven core collapse or magneto-rotational SN models, to identify the origin of its bipolar Fe-rich structure.

astro-ph.HE↗

arXiv2024

Unveiling the Physics of Core-Collapse Supernovae with the Line Emission Mapper: Observing Cassiopeia A

(Abridged) Core-collapse supernova remnants (SNRs) display complex morphologies and asymmetries, reflecting anisotropies from the explosion and early interactions with the circumstellar medium (CSM). Spectral analysis of these remnants can provide critical insights into supernova (SN) engine dynamics, the nature of progenitor stars, and the final stages of stellar evolution, including mass-loss mechanisms in the millennia leading up to the SN. This white paper evaluates the potential of the Line Emission Mapper (LEM), an advanced X-ray probe concept proposed in response to NASA 2023 APEX call, to deliver high-resolution spectra of SNRs. Such capabilities would allow detailed analysis of parent SNe and progenitor stars, currently beyond our possibilities. We employed a hydrodynamic model that simulates the evolution of a neutrino-driven SN from core-collapse to a 2000-year-old mature remnant. This model successfully replicates the large-scale properties of Cassiopeia A at an age of about 350 years. Using this model, we synthesized mock LEM spectra from different regions of the SNR, considering factors like line shifts and broadening due to plasma bulk motion and thermal ion motion, deviations from ionization and temperature equilibrium, and interstellar medium absorption. Analyzing these mock spectra with standard tools revealed LEM impressive capabilities. We demonstrated that fitting these spectra with plasma models accurately recovers the line-of-sight velocity of the ejecta, enabling 3D structure exploration of shocked ejecta, similar to optical methods. LEM also distinguishes between Doppler and thermal broadening of ion lines and measures ion temperatures near the limb of SNRs, providing insights into ion heating at shock fronts and cooling in post-shock flows. This study highlights LEM potential to advance our understanding of core-collapse SN dynamics and related processes.

astro-ph.HE↗

arXiv2023

Photo-excited charge carrier lifetime enhanced by slow cation molecular dynamics in lead iodide perovskite FAPbI$_3$

Using muon spin relaxation ($μ$SR) measurements on formamidinium lead iodide [FAPbI$_3$, where FA denotes HC(NH$_2)_2$] we show that, among the five structurally distinct phases of FAPbI$_3$ exhibited through two different temperature hysteresis, the reorientation motion of FA molecules is quasi-static below $\approx50$ K over the time scale of 10$^{-6}$ s in the low-temperature (LT) hexagonal (Hex-LT, $<160$ K) phase which has relatively longer photo-excited charge carrier lifetime ($τ_{\rm c}\sim$10$^{-6}$ s). In contrast, a sharp increase in the FA molecular motion was found above $\approx50$ K in the Hex-LT phase, LT-tetragonal phase (Tet-LT, $<140$ K), the high-temperature (HT) hexagonal phase (Hex-HT, 160-380 K), and the HT-tetragonal phase (Tet-HT, 140-280 K) where $τ_{\rm c}$ decreases with increasing temperature. More interestingly, the reorientation motion is further promoted in the cubic phase at higher temperatures ($>380/280$ K), while $τ_{\rm c}$ is recovered to comparable or larger than that of the LT phases. These results indicate that there are two factors that determine $τ_{\rm c}$, one related to the local reorientation of cationic molecules that is not unencumbered by phonons, and the other to the high symmetry of the bulk crystal structure.

cond-mat.mtrl-sci↗

arXiv2022

Organic Molecular Dynamics and Charge-carrier Lifetime in Lead Iodide Perovskite MAPbI$_3$

The long charge carrier lifetime of the hybrid organic-inorganic perovskites (HOIPs) is the key for their remarkable performance as a solar cell material. The microscopic mechanism for the long lifetime is still in debate. Here, by using muon spin relaxation technique that probes the fluctuation of local magnetic fields, we show that the muon depolarization rate ($Δ$) of a prototype HOIP methylammonium lead iodide (MAPbI$_3$) shows a sharp decrease with increasing temperature in two steps above 120 K and 190 K across the structural transition from orthorhombic to tetragonal structure at 162 K. Our analysis shows that the reduction of $Δ$ is quantitatively in agreement with the expected behavior due to the rapid development of MA jumping rotation around the $C_3$ and $C_4$ symmetry axes. Our results provide direct evidence for the intimate relation between the rotation of the electric dipoles of MA molecules and the charge carrier lifetime in HOIPs.

cond-mat.mtrl-sci↗

arXiv2019

Spin gap and L modulated intensity at the low-energy incommensurate magnetic fluctuations in the superconducting state of Sr2RuO4

Low-energy incommensurate (IC) magnetic fluctuations in the multiband superconductor Sr$_2$RuO$_4$ is investigated by high-resolution inelastic neutron scattering measurements and random phase approximation (RPA) calculations. Below $T_\text{c}$, the substantial spin gap is observed at $\mathbf{Q}_\text{IC}=(0.3, 0.3, L)$ where the quasi-one-dimensional $α$ and $β$ sheets consisting of the Fermi surfaces are in good nesting conditions. $L$ modulated intensity of the low-energy IC magnetic fluctuations and our RPA calculations indicate that the superconducting gaps regarding the $α$ and $β$ sheets have the horizontal line nodes.

cond-mat.supr-con↗

arXiv2018

3D MHD modeling of the expanding remnant of SN 1987A. Role of magnetic field and non-thermal radio emission

Aims. We investigate the role played by a pre-supernova (SN) ambient magnetic field on the dynamics of the expanding remnant of SN 1987A and the origin and evolution of the radio emission from the remnant, in particular, during the interaction of the blast wave with the nebula surrounding the SN. Methods. We model the evolution of SN 1987A from the breakout of the shock wave at the stellar surface to the expansion of its remnant through the surrounding nebula by 3D MHD simulations. The model considers the radiative cooling, the deviations from equilibrium of ionization, the deviation from temperature-equilibration between electrons and ions, and a plausible configuration of the pre-SN ambient magnetic field. From the simulations, we synthesize both thermal X-ray and non-thermal radio emission and compare the model results with observations. Results. The presence of an ambient magnetic field reduces the erosion and fragmentation of the dense equatorial ring after the impact of the SN blast wave. As a result, the ring survives the passage of the blast, at least, during the time covered by the simulations (40 years). Our model is able to reproduce the morphology and lightcurves of SN 1987A in both X-ray and radio bands. The model reproduces the observed radio emission if the flux originating from the reverse shock is heavily suppressed. In this case, the radio emission originates mostly from the forward shock traveling through the H II region. Possible mechanisms for the suppression of emission from the reverse shock are investigated. We find that synchrotron self-absorption and free-free absorption have negligible effects on the emission during the interaction with the nebula. We suggest that the emission from the reverse shock at radio frequencies might be limited by highly magnetized ejecta.

astro-ph.HE↗

arXiv2018

Whispering gallery effect in relativistic optics

A relativistic laser pulse, confined in a cylindrical target, performs multiple scattering along the target surface. The confinement property of the target results in a very effcient interaction. This proccess, which is just yet another example of the "whispering gallery" effect, may pronounce itself in plenty of physical phenomena, including surface grazing electron acceleration and generation of relativistic magnetized plasma structures.

physics.plasm-ph↗

arXiv2017

Laser electron acceleration on curved surfaces

Electron acceleration by relativistically intense laser beam propagating along a curved surface allows to split softly the accelerated electron bunch and the laser beam. The presence of a curved surface allows to switch an adiabatic invariant of electrons in the wave instantly leaving the gained energy to the particles. The efficient acceleration is provided by the presence of strong transient quasistationary fields in the interaction region and a long efficient acceleration length. The curvature of the surface allows to select the accelerated particles and provides their narrow angular distribution. The mechanism at work is explicitly demonstrated in theoretical models and experiments.

physics.plasm-ph↗

arXiv2017

Scaling of Memories and Crossover in Glassy Magnets

Glassiness is ubiquitous and diverse in characteristics in nature. Understanding their differences and classification remains a major scientific challenge. Here, we show that scaling of magnetic memories with time can be used to classify magnetic glassy materials into two distinct classes. The systems studied are high-temperature superconductor-related materials, spin-orbit Mott insulators, frustrated magnets, and dilute magnetic alloys. Our bulk magnetization measurements reveal that most densely populated magnets exhibit similar memory behavior characterized by a relaxation exponent of 1-n ~ 0.6(1). This exponent is different from 1-n ~ 1/3 of dilute magnetic alloys that was ascribed to their hierarchical and fractal energy landscape and is also different from 1-n=1 of the conventional Debye relaxation expected for a spin solid, a state with long range order. Furthermore, our systematic study on dilute magnetic alloys with varying magnetic concentration exhibits crossovers among the two glassy states and spin solid.

cond-mat.dis-nn↗

arXiv2017

Comprehensive study of the dynamics of a classical Kitaev spin liquid

We study the spin-$S$ Kitaev model in the classical ($S \to \infty$) limit using Monte Carlo simulations combined with semi-classical spin dynamics. We discuss differences and similarities in the dynamical structure factors of the spin-$1/2$ and the classical Kitaev liquids. Interestingly, the low-temperature and low-energy spectrum of the classical model exhibits a finite energy peak, which is the precursor of the one produced by the Majorana modes of the $S=1/2$ model. The classical peak is spectrally narrowed compared to the quantum result and can be explained by magnon excitations within fluctuating one-dimensional manifolds (loops). Hence the difference from the classical limit to the quantum limit can be understood by the fractionalization of magnons propagating in one-dimensional manifolds. Moreover, we show that the momentum space distribution of the low-energy spectral weight of the $S=1/2$ model follows the momentum space distribution of zero modes of the classical model.

cond-mat.str-el↗

arXiv2017

Search for heavy neutrinos at Belle

We report on a search for heavy neutrinos in B-meson decays. The results are obtained using a data sample that contains 772x10^6 BB-bar pairs collected at the Upsilon(4S) resonance with the Belle detector at the KEKB asymmetric-energy e+e- collider. No signal is observed and upper limits are set on mixing of heavy neutrinos with left-handed neutrinos of the Standard Model in the mass range 0.5 - 5.0 GeV/c^2.

hep-ex↗

arXiv2016

Measurement of the Lepton Forward-Backward Asymmetry in $B \rightarrow X_s \ell^+ \ell^-$ Decays with a Sum of Exclusive Modes

We report the first measurement of the lepton forward-backward asymmetry ${\cal A}_{\rm FB}$ as a function of the squared four-momentum of the dilepton system, $q^2$, for the electroweak penguin process $B \rightarrow X_s \ell^+ \ell^-$ with a sum of exclusive final states, where $\ell$ is an electron or a muon and $X_s$ is a hadronic recoil system with an $s$ quark. The results are based on a data sample containing $772\times10^6$ $B\bar{B}$ pairs recorded at the $Υ(4S)$ resonance with the Belle detector at the KEKB $e^+ e^-$ collider. ${\cal A}_{\rm FB}$ for the inclusive $B \rightarrow X_s \ell^+ \ell^-$ is extrapolated from the sum of 10 exclusive $X_s$ states whose invariant mass is less than 2 GeV/$c^2$. For $q^2 > 10.2$ GeV$^2$/$c^2$, ${\cal A}_{\rm FB} < 0$ is excluded at the 2.3$σ$ level, where $σ$ is the standard deviation. For $q^2 < 4.3$ GeV$^2$/$c^2$, the result is within 1.8$σ$ of the Standard Model theoretical expectation.

hep-ex↗

arXiv2015

Rotational Dynamics of Organic Cations in CH3NH3PbI3 Perovskite

Methylammonium lead iodide (CH3NH3PbI3) based solar cells have shown impressive power conversion efficiencies of above 20%. However, the microscopic mechanism of the high photovoltaic performance is yet to be fully understood. Particularly, the dynamics of CH3NH3+ cations and their impact on relevant processes such as charge recombination and exciton dissociation are still poorly understood. Here, using elastic and quasi-elastic neutron scattering techniques and group theoretical analysis, we studied rotational modes of the CH3NH3+ cation in CH3NH3PbI3. Our results show that, in the cubic (T > 327K) and tetragonal (165K < T < 327K) phases, the CH3NH3+ ions exhibit four-fold rotational symmetry of the C-N axis (C4) along with three-fold rotation around the C-N axis (C3), while in orthorhombic phase (T < 165K) only C3 rotation is present. Around room temperature, the characteristic relaxation times for the C4 rotation is found to be ps while for the C3 rotation ps. The -dependent rotational relaxation times were fitted with Arrhenius equations to obtain activation energies. Our data show a close correlation between the C4 rotational mode and the temperature dependent dielectric permittivity. Our findings on the rotational dynamics of CH3NH3+ and the associated dipole have important implications on understanding the low exciton binding energy and slow charge recombination rate in CH3NH3PbI3 which are directly relevant for the high solar cell performance.

cond-mat.mtrl-sci↗

arXiv2015

Simulating Cherenkov Telescope Array observation of RX J1713.7-3946

We perform simulations of Cherenkov Telescope Array (CTA) observations of a young supernova remnant RX J1713.7-3946. This target is not only one of the brightest sources ever discovered in very high-energy gamma rays but also well observed in other wavebands. In X-rays, the emission is dominated by synchrotron radiation, which links directly to the existence of high-energy electrons. Radio observations of CO and HI gas have revealed a highly inhomogeneous medium surrounding the SNR, such as clumpy molecular clouds. Therefore gamma rays from hadronic interactions are naturally expected. However, the spectrum in GeV energy range measured by Fermi/LAT indicates more typical of leptonic emission from accelerated electrons. Despite lots of multi-wavelength information, the competing interpretations have led to much uncertainty in the quest of unraveling the true origin of the gamma-ray emission from RX~J1713.7--3946. CTA will achieve highest performance ever in sensitivity, angular resolution, and energy resolution. We estimate CTA capability to examine the emission mechanisms of the gamma rays through simulated spatial distribution, spectra, and their time variation.

astro-ph.HE↗

arXiv2015

Matter Mixing in Core-collapse Supernova Ejecta: Large Density Perturbations in the Progenitor Star?

Matter mixing is one important topic in the study of core-collapse supernova (CCSN) explosions. In this paper, we perform two-dimensional hydrodynamic simulations to reproduce the high velocity $^{56}$Ni clumps observed in SN 1987A. This is the first time that large density perturbation is proposed in the CCSN progenitor to generate Rayleigh-Taylor (RT) instability and make the effective matter mixing. In the case of a spherical explosion, RT instability is efficient at both C+O/He and He/H interfaces of the SN progenitor. Radial coherent structures shown in perturbation patterns are important for obtaining high velocity $^{56}$Ni clumps. We can also obtain matter mixing features and high velocity $^{56}$Ni clumps in some cases of aspherical explosion. We find that one of the most favorable models in our work has a combination of bipolar and equatorially asymmetric explosions in which at least 25\% of density perturbation is introduced at different composition interfaces of the CCSN progenitor. These simulation results are comparable to the observational findings of SN 1987A.

astro-ph.HE↗

arXiv2015

An orbital glass state of a nearly metallic spinel, CoV$_2$O$_4$

Strain, magnetization, and unpolarized and polarized neutron diffraction measurements were performed to study the magnetic and structural properties of spinel CoV$_{2}$O$_{4}$. Magnetostriction measurements indicate that a subtle distortion of the crystal along the direction of magnetization, $ΔL/L \sim 10^{-4}$, exists and varies from elongation to contraction in a second order fashion upon cooling. Unpolarized and polarized single-crystal neutron experiments indicate that upon cooling the ferrimagnetic structure changes from collinear to noncollinear at $T \sim 90$ K, where the elongation of the crystal is maximized. These results imply the existence of an orbital glassy state in the nearly metallic frustrated magnet CoV$_{2}$O$_{4}$.

cond-mat.str-el↗

arXiv2014

Coexistence of ferromagnetism and superconductivity in CeO$_{0.3}$F$_{0.7}$BiS$_{2}$

Bulk magnetization, transport and neutron scattering measurements were performed to investigate the electronic and magnetic properties of a polycrystalline sample of the newly discovered ferromagnetic superconductor, CeO$_{0.3}$F$_{0.7}$BiS$_{2}$. Ferromagnetism develops below T$_{FM}$ = 6.54(8) K and superconductivity is found to coexist with the ferromagnetic state below T$_{SC}$ ~ 4.5 K. Inelastic neutron scattering measurements reveal a very weakly dispersive magnetic excitation at 1.8 meV that can be explained by an Ising-like spin Hamiltonian. Under application of an external magnetic field, the direction of the magnetic moment changes from the c-axis to the ab-plane and the 1.8 meV excitation splits into two modes. A possible mechanism for the unusual magnetism and its relation to superconductivity is discussed.

cond-mat.supr-con↗