arXiv subjects

S. H. Chun

Publications and source records attributed to S. H. Chun.

23 records · Page 2Linked to original sources

arXiv2000

Breakdown of the lattice polaron picture in La0.7Ca0.3MnO3 single crystals

When heated through the magnetic transition at Tc, La0.7Ca0.3MnO3 changes from a band metal to a polaronic insulator. The Hall constant R_H, through its activated behavior and sign anomaly, provides key evidence for polaronic behavior. We use R_H and the Hall mobility to demonstrate the breakdown of the polaron phase. Above 1.4Tc, the polaron picture holds in detail, while below, the activation energies of both R_H and the mobility deviate strongly from their polaronic values. These changes reflect the presence of metallic, ferromagnetic fluctuations, in the volume of which the Hall effect develops additional contributions tied to quantal phases.

cond-mat.str-el↗

arXiv1999

Magnetotransport in manganites and the role of quantal phases I: Theory

A microscopic picture of charge transport in manganites is developed, with particular attention being paid to the neighborhood of the ferromagnet-to- paramagnet phase transition. The basic transport mechanism invoked is inelastically-assisted carrier hopping between states localized by magnetic disorder. In the context of the anomalous Hall effect, central roles are played by the Pancharatnam and spin-orbit quantal phases.

cond-mat.str-el↗

arXiv1999

Magnetotransport in manganites and the role of quantal phases II: Experiment

As in conventional ferromagnets, the Hall resistivity rho_xy of a La_{2/3}(Ca,Pb)_{1/3}MnO_3 single crystal exhibits both ordinary and anomalous contributions at low temperature. However, these contributions, unexpectedly, have opposite signs. Near Tc, the ordinary contribution is no longer evident and rho_xy is solely determined by the sample magnetization, reaching an extremum at approximately 40% of the saturated magnetization. A new model for the anomalous Hall effect, incorporating the quantal phase accumulated by double-exchange, three-site hopping reproduces this result. Below Tc, rho_xy reflects the competition between normal and anomalous Hall effects.

cond-mat.str-el↗

arXiv1999

Coexistence of localized and itinerant carriers near Tc in calcium-doped manganites

We explore the possibility that polaronic distortions in the paramagnetic phase of La$_{0.67}$Ca$_{0.33}$MnO$_3$ manganites persist in the ferromagnetic phase by considering the observed electrical resistivity to arise from coexisting field- and temperature-dependent polaronic and band-electron fractions. We use an effective medium approach to compute the total resistivity of the two-component system, and find that a limit with low percolation threshold explains the data rather well. To test the validity of this model, we apply it to the thermoelectric coefficient. We propose a plausible mean-field model that reproduces the essential features of a microscopic model and provides a comparison with the experimental mixing fraction, as well as the magnetization and magnetic susceptibility.

cond-mat.str-el↗

arXiv1998

Hall Effect of La2/3(Ca,Pb)1/3MnO3 Single Crystals near the Critical Temperature

The Hall resistivity rho_{xy} of a La_{2/3}(Ca,Pb)_{1/3}MnO_3 single crystal has been measured as a function of temperature and field. The overall behavior is similar to that observed previously in thin-films. At 5 K, rho_{xy} is positive and linear in field, indicating that the anomalous contribution $R_S$ is negligible. However, the effective carrier density in a free electron model is n_{eff}=2.4 holes/Mn, even larger than the 0.85-1.9 holes/Mn reported for thin-films and far larger than the 0.33 holes/Mn expected from the doping level. As temperature increases, a strong, negative contribution to rho_{xy} appears, that we ascribe to R_S. Using detailed magnetization data, we separate the ordinary (\propto B) and anomalous (\propto M) contributions. Below T_C, R_S \propto rho_{xx}, indicating that magnetic skew scattering is the dominant mechanism in the metallic ferromagnetic regime. At and above the resistivity-peak temperature, we find that rho_{xy}/rho_{xx}M is a constant, independent of temperature and field. This implies that the anomalous Hall coefficient is proportional to the magnetoresistance. A different explanation based on two fluid model is also presented.

cond-mat.str-el↗