arXiv subjects

S. J. J. M. F. Kokkelmans

Publications and source records attributed to S. J. J. M. F. Kokkelmans.

At least 37 records · Page 2Linked to original sources

arXiv2021

Cumulant theory of the unitary Bose gas: Prethermal and Efimovian dynamics

We study the quench of a degenerate ultracold Bose gas to the unitary regime, where interactions are as strong as allowed by quantum mechanics. We lay the foundations of a cumulant theory able to capture simultaneously the three-body Efimov effect and ergodic evolution. After an initial period of rapid quantum depletion, a universal prethermal stage is established characterized by a kinetic temperature and an emergent Bogoliubov dispersion law while the microscopic degrees of freedom remain far-from-equilibrium. Integrability is then broken by higher-order interaction terms in the many-body Hamiltonian, leading to a momentum-dependent departure from power law to decaying exponential behavior of the occupation numbers at large momentum. We find also signatures of the Efimov effect in the many-body dynamics and make a precise identification between the observed beating phenomenon and the binding energy of an Efimov trimer. Throughout the work, our predictions for a uniform gas are quantitatively compared with experimental results for quenched unitary Bose gases in uniform potentials.

cond-mat.quant-gas↗

arXiv2020

Multichannel effects in the Efimov regime from broad to narrow Feshbach resonances

We study Efimov physics of three identical bosons with pairwise multichannel interactions for Feshbach resonances of adjustable width. We find that the two-body multichannel nature of the interaction can affect the universal three-body spectrum, especially for resonances of intermediate width. The shifts in this universal spectrum are caused by trimer states in the closed interaction channels that couple to the universal Efimov states. However, in the narrow resonance limit we find that the Efimov spectrum is set by the resonance width parameter $r^*$ only independent of the interaction potential considered. In the broad resonance limit all excited Efimov trimer energies approach the ones from the corresponding single-channel system for the scenarios investigated.

cond-mat.quant-gas↗

arXiv2020

The multichannel nature of three-body recombination for ultracold $^{39}$K

We develop a full multichannel spin model in momentum space to investigate three-body recombination of identical alkali-metal atoms colliding in a magnetic field. The model combines the exact three-atom spin structure and realistic pairwise atom-atom interactions. By neglecting the interaction between two particles when the spectating particle is not in its initial spin state we arrive at an approximate model. With this approximate model we achieve excellent agreement with the recent precise measurement of the ground Efimov resonance position in potassium-39 close to 33.58 G [Chapurin $et$ $al$., Phys. Rev. Lett. 123, 233402 (2019)]. We analyze the limitations of our approximation by comparing to the numerical results for the full system and find that it breaks down for Feshbach resonances at larger magnetic fields in the same spin channel. There the relevant three-body closed channel thresholds are much closer to the open channel threshold, which enhances the corresponding multichannel couplings. Therefore the neglected components of the interaction should be included for those Feshbach resonances.

cond-mat.quant-gas↗

arXiv2020

Efficient three-body calculations with a two-body mapped grid method

We investigate the prospects of combining a standard momentum space approach for ultracold three-body scattering with efficient coordinate space schemes to solve the underlying two-body problem. In many of those schemes the two-body problem is numerically restricted up to a finite interparticle distance $r_\mathrm{b}$. We analyze effects of this two-body restriction on the two- and three-body level using pairwise square-well potentials that allow for analytic two-body solutions and more realistic Lennard-Jones van der Waals potentials to model atomic interactions. We find that the two-body $t$-operator converges exponentially in $r_\mathrm{b}$ for the square-well interaction. Setting $r_\mathrm{b}$ to 2000 times the range of the interaction, the three-body recombination rate can be determined accurately up to a few percent when the magnitude of the scattering length is small compared to $r_\mathrm{b}$, while the position of the lowest Efimov features is accurate up to the percent level. In addition we find that with the introduction of a momentum cut-off, it is possible to determine the three-body parameter in good approximation even for deep van der Waals potentials.

cond-mat.quant-gas↗

arXiv2020

Phonon-mediated spin-spin interactions between trapped Rydberg atoms

We theoretically investigate the possibility of creating phonon-mediated spin-spin interactions between neutral atoms trapped in optical tweezers. By laser coupling the atoms to Rydberg states, collective modes of motion appear. We show that these can be used to mediate effective spin-spin interactions or quantum logic gates between the atoms in analogy to schemes employed in trapped ions. In particular, we employ Rydberg dressing in a novel scheme to induce the needed interaction, and we show that it is possible to replicate the working of the Mølmer-Sørensen entanglement scheme. The Mølmer-Sørensen gate is widely used in emerging quantum computers using trapped ion qubits and currently features some of the highest fidelities of any quantum gate under consideration. We find arbitrarily high fidelity for the coherent time evolution of the two-atom state even at non-zero temperature.

physics.atom-ph↗

arXiv2020

Van der Waals universality near a quantum tricritical point

We study the three-body scattering hypervolume $D$ of atoms whose scattering length $a$ is on the order of or smaller than the typical range $r_{\mathrm{vdW}}$ of the van der Waals attraction. We find that the real part of $D$ behaves universally in this weakly interacting regime ($|a|/r_{\mathrm{vdW}}\lesssim 1$) in the absence of trimer resonances. This universality originates from hard-spherelike collisions that dominate elastic three-body scattering. We use this result to make quantitative predictions for the thermodynamics and elementary excitations of an atomic Bose-Einstein condensate in the vicinity of a quantum tricritical point, including quantum droplets stabilized by effective three-body interactions.

physics.atom-ph↗

arXiv2020

Three-level rate equations in cold, disordered Rydberg gases

We have investigated formation of structures of Rydberg atoms excited from a disordered gas of ultracold atoms, using rate equations for two-photon Rydberg excitation in a single atom without eliminating the intermediate state. We have explored the validity range of these rate equations and defined a simple measure to determine, whether our model is applicable for a given set of laser parameters. We have applied these rate equations in Monte Carlo simulations of ultracold gases, for different laser beam profiles, and compared these simulations to experimental observations and find a general agreement.

physics.atom-ph↗

arXiv2019

Scattering hypervolume for ultracold bosons from weak to strong interactions

The elastic scattering properties of three bosons at low energy enter the many-body description of ultracold Bose gases via the three-body scattering hypervolume $D$. We study this quantity for identical bosons that interact via a pairwise finite-range potential. Our calculations cover the regime from strongly repulsive potentials towards attractive potentials supporting multiple two-body bound states and are consistent with the few existing predictions for $D$. We present the first numerical confirmation of the universal predictions for $D$ in the strongly interacting regime, where Efimov physics dominates, for a local nonzero-range potential. Our findings highlight how $D$ is influenced by three-body quasibound states with strong $d$-wave or $g$-wave characteristics in the weakly interacting regime.

physics.atom-ph↗

arXiv2019

Pair formation in quenched unitary Bose gases

We study a degenerate Bose gas quenched to unitarity by solving a many-body model including three-body losses and correlations up to second order. As the gas evolves in this strongly-interacting regime, the buildup of correlations leads to the formation of extended pairs bound purely by many-body effects, analogous to the phenomenon of Cooper pairing in the BCS regime of the Fermi gas. Through fast sweeps away from unitarity, we detail how the correlation growth and formation of bound pairs emerge in the fraction of unbound atoms remaining post sweep, finding quantitative agreement with experiment. We comment on the possible role of higher-order effects in explaining the deviation of our theoretical results from experiment for slower sweeps and longer times spent in the unitary regime.

cond-mat.quant-gas↗

arXiv2019

Bunching, clustering, and the buildup of few-body correlations in a quenched unitary Bose gas

We study the growth of two- and three-body correlations in an ultracold Bose gas quenched to unitarity. This is encoded in the dynamics of the two- and three-body contacts analyzed in this work. Via a set of relations connecting many-body correlations dynamics with few-body models, signatures of the Efimov effect are mapped out as a function of evolution time at unitarity over a range of atomic densities $n$. For the thermal resonantly interacting Bose gas, we find that atom-bunching leads to an enhanced growth of few-body correlations. These atom-bunching effects also highlight the interplay between few-body correlations that occurs before genuine many-body effects enter on Fermi timescales.

cond-mat.quant-gas↗

arXiv2019

From coherent collective excitation to Rydberg blockade on an atom chip

Using time-resolved measurements, we demonstrate coherent collective Rydberg excitation crossing over into Rydberg blockade in a dense and ultracold gas trapped at a distance of 100 $μ$m from a room-temperature atom chip. We perform Ramsey-type measurements to characterize the coherence. The experimental data are in good agreement with numerical results from a master equation using a mean-field approximation, and with results from a super-atom-based Hamiltonian. These results represent significant progress in exploring a strongly interacting driven Rydberg gas on an atom chip.

physics.atom-ph↗

arXiv2018

Dynamical formation of the unitary Bose gas

We study the structure of a Bose-condensed gas after quenching interactions to unitarity. Using the method of cumulants, we decompose the evolving gas in terms of clusters. Within the quantum depletion we observe the emergence of two-body clusters bound purely by many-body effects, scaling continuously with the atomic density. As the unitary Bose gas forms, three-body Efimov clusters are first localized and then sequentially absorbed into the embedded atom-molecule scattering continuum of the surrounding depletion. These results motivate future experimental probes of a quenched Bose-condensate during evolution at unitarity.

cond-mat.quant-gas↗

arXiv2018

Trapping of Rydberg Atoms in Tight Magnetic Microtraps

We explore the possibility to trap Rydberg atoms in tightly confining magnetic microtraps. The trapping frequencies for Rydberg atoms are expected to be influenced strongly by magnetic field gradients. We show that there are regimes where Rydberg atoms can be trapped. Moreover, we show that so-called magic trapping conditions can be found for certain states of rubidium, where both Rydberg atoms and ground state atoms have the same trapping frequencies. Magic trapping is highly beneficial for implementing quantum gate operations that require long operation times.

physics.atom-ph↗

arXiv2016

Stability of rubidium molecules in the lowest triplet state

Experiments involving ultracold molecules require sufficiently long lifetimes, which can be very short for excited rovibrational states in the molecular potentials. For alkali atoms such as rubidium, a lowest rovibrational molecular state can both be found in the electronic singlet and triplet configurations. The molecular singlet ground state is absolutely stable. However, the lowest triplet state can decay to a deeper bound singlet molecule due to a radiative decay mechanism that involves the interatomic spin-orbit interaction. We investigate this mechanism, and find the lifetime of rubidium molecules in the lowest triplet rovibrational state to be about 21 minutes.

cond-mat.quant-gas↗

arXiv2014

Patterned Rydberg excitation and ionisation with a spatial light modulator

We demonstrate the ability to excite atoms at well-defined, programmable locations in a magneto-optical trap, either to the continuum (ionisation), or to a Rydberg state. To this end, excitation laser light is shaped into arbitrary intensity patterns with a spatial light modulator. These optical patterns are sensitive to aberrations of the phase of the light field, occuring while traversing the optical beamline. These aberrations are characterised and corrected without observing the actual light field in the vacuum chamber.

physics.atom-ph↗

arXiv2014

Feshbach resonances in ultracold gases

In this chapter, we describe scattering resonance phenomena in general, and focus on the mechanism of Feshbach resonances, for which a multi-channel treatment is required. We derive the dependence of the scattering phase shift on magnetic field and collision energy. From this, the scattering length and effective range coefficient can be extracted, expressions which are particularly useful for ultracold gases.

cond-mat.quant-gas↗

arXiv2012

Universal three-body parameter in ultracold 4He*

We have analyzed our recently-measured three-body loss rate coefficient for a Bose-Einstein condensate of spin-polarized metastable triplet 4He atoms in terms of Efimov physics. The large value of the scattering length for these atoms, which provides access to the Efimov regime, arises from a nearby potential resonance. We find the loss coefficient to be consistent with the three-body parameter (3BP) found in alkali-metal experiments, where Feshbach resonances are used to tune the interaction. This provides new evidence for a universal 3BP, the first outside the group of alkali-metal elements. In addition, we give examples of other atomic systems without Feshbach resonances but with a large scattering length that would be interesting to analyze once precise measurements of three-body loss are available.

cond-mat.quant-gas↗

arXiv2012

Feshbach spectroscopy and scattering properties of ultracold Li+Na mixtures

We have observed 26 interspecies Feshbach resonances at fields up to 2050 G in ultracold $^6$Li+$^{23}$Na mixtures for different spin-state combinations. Applying the asymptotic bound-state model to assign the resonances, we have found that most resonances have d-wave character. This analysis serves as guidance for a coupled-channel calculation, which uses modified interaction potentials to describe the positions of the Feshbach resonances well within the experimental uncertainty and to calculate their widths. The scattering length derived from the improved interaction potentials is experimentally confirmed and deviates from previously reported values in sign and magnitude. We give prospects for $^7$Li+$^{23}$Na and predict broad Feshbach resonances suitable for tuning.

cond-mat.quant-gas↗