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S. L. Zhang

Publications and source records attributed to S. L. Zhang.

At least 19 recordsLinked to original sources

Quantum phase-field model: vortices and THz-induced gap dynamics in superconductors

The ability to simulate the spatial and temporal ordering dynamics of quantum phases in inhomogeneous systems, particularly in the low-temperature regime, is crucial for understanding condensate physics and for enabling emerging device technologies. However, fully microscopic kinetic approaches are often computationally prohibitive for macroscopic spatiotemporal simulations in realistic device geometries, while the widely used phenomenological Ginzburg-Landau formulation is, in principle, valid only near the critical transition temperature $T_c$ and becomes inaccurate in the technologically relevant low-temperature regime. To describe the dynamics of quantum phase ordering, we propose a phase-field formulation derived from a microscopic many-body description using the superconducting order as an example. It leads to a compact dynamical evolution equation for the superconducting order parameter, enabling real-space and real-time simulations of phase ordering dynamics. The simulations successfully capture key dynamical phenomena, including vortex nucleation and motion under static magnetic fields, as well as ultrafast gap oscillations driven by THz fields, over the full temperature range from 0 K up to the critical transition temperature. Beyond superconductivity, this method can be extended to a broad class of quantum condensates and ordered systems, providing a practical computational approach to studying low-temperature ordering dynamics, topological defect evolution, and ultrafast electromagnetic responses of quantum phases in realistic geometries.

cond-mat.supr-con

Revealing THz optical signatures of Shiba-state-induced gapped and gapless superconductivity

We report a fully self-consistent calculation of the complex renormalization by exchange interactions and hence the complete phase diagram of conventional $s$-wave superconductors with magnetic impurities as well as the related physical properties including the optical response. We show that a small amount of magnetic disorder can drive the system into a gapless superconducting state, where the single-particle excitation gap vanishes whereas the superconducting order parameter $Δ_0$ remains finite. In this phase, the linear optical conductivity exhibits a finite absorption over the low-frequency regime, particularly for photon energies below the conventional threshold $2|Δ_0|$, even at low temperatures, in sharp contrast to the gapped state. The nonlinear response, however, remains coherent and is dominated by the Higgs-mode dynamics rather than gapless quasiparticle background. These findings reveal a fundamental distinction between dissipative single-particle excitations and coherent collective dynamics of the condensate, a feature likely general to other gapless superconductors, and introduces a fundamentally different detection scheme, using THz spectroscopy to probe the signatures of Shiba states.

cond-mat.supr-con

Depth-dependent magnetic crossover in a room-temperature skyrmion-hosting multilayer

Skyrmion-hosting multilayer stacks are promising avenues for applications, although little is known about the depth dependence of the magnetism. We address this by reporting the results of circular dichroic resonant elastic x-ray scattering (CD-REXS), micromagnetic simulations, and low-energy muon-spin rotation (LE-$μ^+$SR) measurements on a stack comprising [Ta/CoFeB/MgO]$_{16}$/Ta on a Si substrate. Energy-dependent CD-REXS shows a continuous, monotonic evolution of the domain-wall helicity angle with incident energy, consistent with a three-dimensional hybrid domain-wall-like structure that changes from Néel-like near the surface to Bloch-like deeper within the sample. LE-$μ^+$SR reveals that the magnetic field distribution in the trilayers near the surface of the stack is distinct from that in trilayers deeper within the sample. Our micromagnetic simulations support a quantitative analysis of the $μ^+$SR results. By increasing the applied magnetic field, we find a reduction in the volume occupied by domain walls at all depths, consistent with a crossover into a region dominated by skyrmions above approximately 180 mT.

cond-mat.str-el

Spontaneous ferromagnetism induced topological phase transition in EuB6

The interplay between various symmetries and electronic bands topology is one of the core issues for topological quantum materials. Spontaneous magnetism, which leads to the breaking of time-reversal symmetry, has been proven to be a powerful approach to trigger various exotic topological phases. In this work, utilizing the combination of angle-resolved photoemission spectroscopy, magneto-optical Kerr effect microscopy and first-principles calculations, we present the direct evidence on the realization of the long-sought spontaneous time-reversal symmetry breaking induced topological phase transition in soft ferromagnetic EuB$_6$. We successfully disentangle the bulk band structure from complicated surface states, and reveal the hallmark band inversion occurring between two opposite-parity bulk bands below the phase transition temperature. Besides, our magneto-optical Kerr effect microscopy result confirms the simultaneous formation of magnetic domains in EuB$_6$, implying the intimate link between the topological phase transition and broken time-reversal symmetry therein. Our results demonstrate that EuB$_6$ provides a potential platform to study the interplay between the topological phases and tunable magnetic orders.

cond-mat.mtrl-sci

Spectroscopic Signature for Local-moment Magnetism in van der Waals Ferromagnet Fe$_3$GeTe$_2$

The van der Waals ferromagnet Fe$_3$GeTe$_2$ has recently attracted extensive research attention due to its intertwined magnetic, electronic and topological properties. Here, using high-resolution angle-resolved photoemission spectroscopy, we systematically investigate the temperature evolution of the electronic structure of bulk Fe$_3$GeTe$_2$. We observe largely dispersive energy bands that are narrowed by a factor of 1.6 compared with ab-initio calculation. Upon heating towards the ferromagnetic transition near 225 K, we observe a massive reduction of quasiparticle coherence in a large energy range, which is attributed to the enhanced magnetic fluctuation in the system. Remarkably, the electron bands barely shift with increasing temperature, which deviates from the exchange splitting picture within the itinerant Stoner model. We argue that the local magnetic moments play a crucial role in the ferromagnetism of Fe$_3$GeTe$_2$, despite its strongly itinerant nature. Our results provide important insights into the electronic and magnetic properties of Fe$_3$GeTe$_2$ and shed light on the generic understanding of itinerant magnetism in correlated materials.

cond-mat.mtrl-sci

Observation of charge density wave transition in TaSe3 mesowires

The quasi-one-dimensional (quasi-1D) TaSe3 attracts considerable attention for its intriguing superconductivity and possible interplay with nontrivial topology and charge density wave (CDW) state. However, unlike the isostructural analogues, CDW has not been observed for TaSe3 despite its quasi-1D character that is supposed to promote Peierls instabilities and CDW. Here we synthesize TaSe3 mesowires (MWs) using a one-step approach. For the MW of ~300 nm thick, a distinct CDW transition occurs at 65 K in the resistivity measurement, which has not been reported before and is further evidenced by the Raman characterization and susceptibility measurement. For comparison, we have also prepared bulk single crystal TaSe3. Although no anomaly appears in the resistivity and magnetoresistance measurements, the carrier type detected by Hall effect varies from n-type to p-type below 50 K, suggesting a reconstruction of Fermi surface that could be associated with CDW. The enhancement of CDW in the MWs is attributed to the reduced dimensionality. TaSe3 is demonstrated to be a promising platform to study the correlation and competition of CDW and superconductivity in the quasi-1D systems.

cond-mat.mes-hall

Topological semimetal state and field-induced Fermi surface reconstruction in antiferromagnetic monopnictide NdSb

We report the experimental realization of Dirac semimetal state in NdSb, a material with antiferromagnetic ground state. The occurrence of topological semimetal state has been well supported by our band structure calculations and the experimental observation of chiral anomaly induced negative magnetoresistance. A field-induced Fermi surface reconstruction is observed, in response to the change of spin polarization. The observation of topological semimetal state in a magnetic material provides an opportunity to investigate the magneto-topological phenomena.

cond-mat.mtrl-sci

Magnetoelectric and Raman spectroscopic studies of single-crystalline MnCr2O4

MnCr2O4 that exhibits spin frustration and complex spiral spin order is of great interest from both fundamental as well as application-oriented perspectives. Unlike CoCr2O4 whose ground state presents the coexistence of commensurate spiral spin order (CSSO) and ferroelectric order, MnCr2O4 shows no multiferroicity. One reason is that the spiral spin order is highly sensitive to the oxygen concentration in MnCr2O4. Here, we have successfully grown high-quality single-crystalline MnCr2O4 by the chemical vapor transport method. We observe a new first-order magnetic transition from the incommensurate spiral spin order (ICSSO) at 19.4 K to the CSSO at 17.4 K. This magnetic transition is verified by magnetization, specific heat, and magnetoelectric measurements, which also confirm that the ground state exhibits the coexistence of the CSSO and magnetoelectricity below 17.4 K. Interestingly, the temperature evolution of Raman spectra between 5.4 and 300 K suggests that the structure remains the same. We also find that the phase-transition temperature of the CSSO decreases as applied magnetic field increases up to 45 kOe.

cond-mat.mtrl-sci

Reciprocal space mapping of magnetic order in thick epitaxial MnSi films

We report grazing incidence small angle neutron scattering (GISANS) and complementary off-specular neutron reflectometry (OSR) of the magnetic order in a single-crystalline epitaxial MnSi film on Si(111) in the thick film limit. Providing a means of direct reciprocal space mapping, GISANS and OSR reveal a magnetic modulation perpendicular to the films under magnetic fields parallel and perpendicular to the film, where additional polarized neutron reflectometry (PNR) and magnetization measurements are in excellent agreement with the literature. Regardless of field orientation, our data does not suggest the presence of more complex spin textures, notably the formation of skyrmions. This observation establishes a distinct difference with bulk samples of MnSi of similar thickness under perpendicular field, in which a skyrmion lattice dominates the phase diagram. Extended x-ray absorption fine structure measurements suggest that small shifts of the Si positions within the unstrained unit cell control the magnetic state, representing the main difference between the films and thin bulk samples.

cond-mat.str-el

First-principles Study on Structural, Thermal, Mechanical and Dynamic Stability of T'-MoS$_2$

Using first-principles density functional theory calculations, we investigate the structure, stability, optical modes and electronic band gap of a distorted tetragonal MoS$_2$ monolayer (T'-MoS$_2$). Our simulated scanning tunnel microscopy (STM) images of T'-MoS$_2$ are dramatically similar with those STM images which were identified as K$_{x}$(H$_{2}$O)$_{y}$MoS$_{2}$ from a previous experimental study. This similarity suggests that T'-MoS$_2$ might have already been observed in experiment but was unexpectedly misidentified. Furthermore, we verify the stability of T'-MoS$_2$ from thermal, mechanical and dynamic aspects, by \emph{ab initio} molecular dynamics simulation, elastic constants evaluation and phonon band structure calculation based on density functional perturbation theory, respectively. In addition, we calculate the eigenfrequencies and eigenvectors of the optical modes of T'-MoS$_2$ at $Γ$ point and distinguish their Raman and infrared activity by pointing out their irreducible representations using group theory; at the same time, we compare the Raman modes of T'-MoS$_2$ with those of H-MoS$_2$ and T-MoS$_2$. Our results provide a useful guidance for further experimental identification and characterization of T'-MoS$_2$.

cond-mat.mes-hall

Imaging and manipulation of skyrmion lattice domains in Cu2OSeO3

Nanoscale chiral skyrmions in noncentrosymmetric helimagnets are promising binary state variables in high-density, low-energy nonvolatile memory. Skyrmions are ubiquitous as an ordered, single-domain lattice phase, which makes it difficult to write information unless they are spatially broken up into smaller units, each representing a bit. Thus, the formation and manipulation of skyrmion lattice domains is a prerequisite for memory applications. Here, using an imaging technique based on resonant magnetic x-ray diffraction, we demonstrate the mapping and manipulation of skyrmion lattice domains in Cu2OSeO3. The material is particularly interesting for applications owing to its insulating nature, allowing for electric field-driven domain manipulation.

cond-mat.mes-hall

Strain in epitaxial MnSi films on Si(111) in the thick film limit studied by polarization-dependent extended x-ray absorption fine structure

We report a study of the strain state of epitaxial MnSi films on Si(111) substrates in the thick film limit (100-500~Å) as a function of film thickness using polarization-dependent extended x-ray absorption fine structure (EXAFS). All films investigated are phase-pure and of high quality with a sharp interface between MnSi and Si. The investigated MnSi films are in a thickness regime where the magnetic transition temperature $T_\mathrm{c}$ assumes a thickness-independent enhanced value of $\geq$43~K as compared with that of bulk MnSi, where $T_\mathrm{c} \approx 29~{\rm K}$. A detailed refinement of the EXAFS data reveals that the Mn positions are unchanged, whereas the Si positions vary along the out-of-plane [111]-direction, alternating in orientation from unit cell to unit cell. Thus, for thick MnSi films, the unit cell volume is essentially that of bulk MnSi --- except in the vicinity of the interface with the Si substrate (thin film limit). In view of the enhanced magnetic transition temperature we conclude that the mere presence of the interface, and its specific characteristics, strongly affects the magnetic properties of the entire MnSi film, even far from the interface. Our analysis provides invaluable information about the local strain at the MnSi/Si(111) interface. The presented methodology of polarization dependent EXAFS can also be employed to investigate the local structure of other interesting interfaces.

cond-mat.mtrl-sci

Multidomain Skyrmion Lattice State in Cu$_2$OSeO$_3$

Magnetic skyrmions in chiral magnets are nanoscale, topologically-protected magnetization swirls that are promising candidates for spintronics memory carriers. Therefore, observing and manipulating the skyrmion state on the surface level of the materials are of great importance for future applications. Here, we report a controlled way of creating a multidomain skyrmion state near the surface of a Cu$_{2}$OSeO$_{3}$ single crystal, observed by soft resonant elastic x-ray scattering. This technique is an ideal tool to probe the magnetic order at the $L_{3}$ edge of $3d$ metal compounds giving a depth sensitivity of ${\sim}50$ nm. The single-domain sixfold-symmetric skyrmion lattice can be broken up into domains overcoming the propagation directions imposed by the cubic anisotropy by applying the magnetic field in directions deviating from the major cubic axes. Our findings open the door to a new way to manipulate and engineer the skyrmion state locally on the surface, or on the level of individual skyrmions, which will enable applications in the future.

cond-mat.mtrl-sci

Resonant Elastic X-ray Scattering from the Skyrmion Lattice in Cu$_{2}$OSeO$_{3}$

We report the study of the skyrmion state near the surface of Cu$_2$OSeO$_3$ using soft resonant elastic x-ray scattering (REXS) at the Cu $L_3$ edge. Within the lateral sampling area of $200 \times 200$ $μ$m$^2$, we found a long-range-ordered skyrmion lattice phase as well as the formation of skyrmion domains via the multiple splitting of the diffraction spots. In a recent REXS study of the skyrmion phase of Cu$_2$OSeO$_3$ [Phys. Rev. Lett. 112, 167202 (2014)], Langner et al. reported the observation of the unexpected existence of two distinct skyrmion sublattices that arise from inequivalent Cu sites, and that the rotation and superposition of the two periodic structures leads to a moiré pattern. However, we find no energy splitting of the Cu peak in x-ray absorption measurements and, instead, discuss alternative origins of the peak splitting. In particular, we find that for magnetic field directions deviating from the major cubic axes, a multidomain skyrmion lattice state is obtained, which consistently explains the splitting of the magnetic spots into two - and more - peaks.

cond-mat.mtrl-sci

Transverse field muon-spin rotation measurement of the topological anomaly in a thin film of MnSi

We present the results of transverse-field muon-spin rotation measurements on an epitaxially grown 40 nm-thick film of MnSi on Si(111) in the region of the field-temperature phase diagram where a skyrmion phase has been observed in the bulk. We identify changes in the quasistatic magnetic field distribution sampled by the muon, along with evidence for magnetic transitions around $T\approx 40$ K and 30 K. Our results suggest that the cone phase is not the only magnetic texture realized in film samples for out-of-plane fields.

cond-mat.str-el

The effect of inserted NiO layer on spin-Hall magnetoresistance in Pt/NiO/YIG heterostructures

We investigate the spin-current transport through antiferromagnetic insulator (AFMI) by means of the spin-Hall magnetoressitance (SMR) over a wide temperature range in Pt/NiO/Y$_3$Fe$_5$O$_{12}$ (Pt/NiO/YIG) heterostructures. By inserting the AFMI NiO layer, the SMR dramatically decreases by decreasing the temperature down to the antiferromagnetically ordered state of NiO, which implies that the AFM order prevents rather than promotes the spin-current transport. On the other hand, the magnetic proximity effect (MPE) on induced Pt moments by YIG, which entangles with the spin-Hall effect (SHE) in Pt, can be efficiently screened, and pure SMR can be derived by insertion of NiO. The dual roles of the NiO insertion including efficiently blocking the MPE and transporting the spin current from Pt to YIG are outstanding compared with other antiferromagnetic (AFM) metal or nonmagnetic metal (NM).

cond-mat.mtrl-sci

Investigation of anomalous-Hall and spin-Hall effects of antiferromagnetic IrMn sandwiched by Pt and YIG layers

We report an investigation of temperature and IrMn layered thickness dependence of anomalous-Hall resistance (AHR), anisotropic magnetoresistance (AMR), and magnetization on Pt/Ir20Mn80/Y3Fe5O12 (Pt/IrMn/YIG) heterostructures. The magnitude of AHR is dramatically enhanced compared with Pt/YIG bilayers. The enhancement is much more profound at higher temperatures and peaks at the IrMn thickness of 3 nm. The observed spin-Hall magnetoresistance (SMR) in the temperature range of 10-300 K indicates that the spin current generated in the Pt layer can penetrate the entire thickness of the IrMn layer to interact with the YIG layer. The lack of conventional anisotropic magnetoresistance (CAMR) implies that the insertion of the IrMn layer between Pt and YIG efficiently suppresses the magnetic proximity effect (MPE) on induced Pt moments by YIG. Our results suggest that the dual roles of the InMn insertion in Pt/IrMn/YIG heterostructures are to block the MPE and to transport the spin current between Pt and YIG layers. We discuss possible mechanisms for the enhanced AHR.

cond-mat.str-el

Study of negative thermal expansion in the frustrated spinel ZnCr2Se4

The origin of negative thermal expansion (NTE) in the bond frustrated ZnCr2Se4 has been explored. ESR and FTIR document an ideal paramagnetic state above 100 K, below which ferromagnetic clusters coexist with the paramagnetic state down to TN. By fitting the inverse susceptibility above 100 K using a modified paramagnetic Curie-Weiss law, an exponentially changeable exchange integral J is deduced. In the case of the variable J, magnetic exchange and lattice elastic energy couple with each other effectively via magnetoelastic interaction in the ferromagnetic clusters, where NTE occurs at a loss of exchange energy while a gain of lattice elastic one.

cond-mat.str-el