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S. Lee

Publications and source records attributed to S. Lee.

At least 199 records · Page 11Linked to original sources
arXiv2017

Putative spin liquid in the triangle-based iridate Ba$_3$IrTi$_2$O$_9$

We report on thermodynamic, magnetization, and muon spin relaxation measurements of the strong spin-orbit coupled iridate Ba$_3$IrTi$_2$O$_9$, which constitutes a new frustration motif made up a mixture of edge- and corner-sharing triangles. In spite of strong antiferromagnetic exchange interaction of the order of 100~K, we find no hint for long-range magnetic order down to 23 mK. The magnetic specific heat data unveil the $T$-linear and -squared dependences at low temperatures below 1~K. At the respective temperatures, the zero-field muon spin relaxation features a persistent spin dynamics, indicative of unconventional low-energy excitations. A comparison to the $4d$ isostructural compound Ba$_3$RuTi$_2$O$_9$ suggests that a concerted interplay of compass-like magnetic interactions and frustrated geometry promotes a dynamically fluctuating state in a triangle-based iridate.

cond-mat.str-el↗
arXiv2017

Quantum criticality in the coupled two-leg spin ladder Ba2CuTeO6

We report on zero-field muon spin rotation, electron spin resonance and polarized Raman scattering measurements of the coupled quantum spin ladder Ba2CuTeO6. Zero-field muon spin rotation and electron spin resonance probes disclose a successive crossover from a paramagnetic through a spin-liquid-like into a magnetically ordered state with decreasing temperature. More significantly, the two-magnon Raman response obeys a T-linear scaling relation in its peak energy, linewidth and intensity. This critical scaling behavior presents an experimental signature of proximity to a quantum critical point from an ordered side in Ba2CuTeO6.

cond-mat.str-el↗
arXiv2017

Femtosecond profiling of shaped X-ray pulses

Arbitrary manipulation of the temporal and spectral properties of X-ray pulses at free-electron lasers (FELs) would revolutionize many experimental applications. At the Linac Coherent Light Source at Stanford National Accelerator Laboratory, the momentum phase-space of the FEL driving electron bunch can be tuned to emit a pair of X-ray pulses with independently variable photon energy and femtosecond delay. However, while accelerator parameters can easily be adjusted to tune the electron bunch phase-space, the final impact of these actuators on the X-ray pulse cannot be predicted with sufficient precision. Furthermore, shot-to-shot instabilities that distort the pulse shape unpredictably cannot be fully suppressed. Therefore, the ability to directly characterize the X-rays is essential to ensure precise and consistent control. In this work, we have generated X-ray pulse pairs and characterized them on a single-shot basis with femtosecond resolution through time-resolved photoelectron streaking spectroscopy. This achievement completes an important step toward future X-ray pulse shaping techniques.

physics.acc-ph↗
arXiv2017

Hadron detection with a dual-readout fiber calorimeter

In this paper, we describe measurements of the response functions of a fiber-based dual- readout calorimeter for pions, protons and multiparticle "jets" with energies in the range from 10 to 180 GeV. The calorimeter uses lead as absorber material and has a total mass of 1350 kg. It is complemented by leakage counters made of scintillating plastic, with a total mass of 500 kg. The effects of these leakage counters on the calorimeter performance are studied as well. In a separate section, we investigate and compare different methods to measure the energy resolution of a calorimeter. Using only the signals provided by the calorimeter, we demonstrate that our dual-readout calorimeter, calibrated with electrons, is able to reconstruct the energy of proton and pion beam particles to within a few percent at all energies. The fractional widths of the signal distributions for these particles (sigma/E) scale with the beam energy as 30%/sqrt(E), without any additional contributing terms.

physics.ins-det↗
arXiv2017

Incomplete rotational cooling in a 22-pole ion trap

Cryogenic 22-pole ion traps have found many applications in ion-molecule reaction kinetics and in high resolution molecular spectroscopy. For most of these applications it is important to know the translational and internal temperatures of the trapped ions. Here, we present detailed rotational state thermometry measurements over an extended temperature range for the two ion/buffer gas systems OH-/He and OD-/HD with ion-to-neutral mass ratios of 4.25 and 6 respectively. The measured rotational temperatures show a termination of the thermalisation with the buffer gas around 25K, independent of mass ratio and confinement potential of the trap. Different possible explanations for this incomplete thermalisation have been investigated, among them the thermalisation of the buffer gas and the heating due to room temperature blackbody radiation and room temperature gas entering the trap.

physics.atom-ph↗
arXiv2016

Enhanced metallic properties of SrRuO3 thin films via kinetically controlled pulsed laser epitaxy

Metal electrodes are a universal element of all electronic devices. Conducting SrRuO3 (SRO) epitaxial thin films have been extensively used as electrodes in complex-oxide heterostructures due to good lattice mismatches with perovskite substrates. However, when compared to SRO single crystals, SRO thin films have shown reduced conductivity and Curie temperatures (T_C), which can lead to higher Joule heating and energy loss in the devices. Here, we report that high-quality SRO thin films can be synthesized by controlling the plume dynamics and growth rate of pulsed laser epitaxy (PLE) with real-time optical spectroscopic monitoring. The SRO thin films grown under the kinetically controlled conditions, down to ca. 16 nm in thickness, exhibit both enhanced conductivity and T_C as compared to bulk values, due to their improved stoichiometry and a strain-mediated increase of the bandwidth of Ru 4d electrons. This result provides a direction for enhancing the physical properties of PLE-grown thin films and paves a way for improved device applications.

cond-mat.mtrl-sci↗
arXiv2015

Localized High Frequency Electrodynamic Behavior of Optimally-doped Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ Single Crystal films

Localized high frequency (several GHz) electrodynamic properties of a high quality epitaxial, single-crystal Iron-Pnicitde Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ thin film near optimal doping (x=0.08) are measured under a localized and strong RF magnetic field, created by a near-field microwave microscope. Two reflection electrodynamic measurements, including linear and the third harmonic responses, are performed to understand the electromagnetic properties of Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$. Our measurement results show that Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ has have a wide superconducting transition width and may have a multi-gap nature. In addition, based on the $1/T^2$ dependence of the third harmonics signal at lower temperature, Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ shows the possibility of nodal behavior.

cond-mat.supr-con↗
arXiv2015

A Storage Ring Experiment to Detect a Proton Electric Dipole Moment

A new experiment is described to detect a permanent electric dipole moment of the proton with a sensitivity of $10^{-29}e\cdot$cm by using polarized "magic" momentum $0.7$~GeV/c protons in an all-electric storage ring. Systematic errors relevant to the experiment are discussed and techniques to address them are presented. The measurement is sensitive to new physics beyond the Standard Model at the scale of 3000~TeV.

physics.acc-ph↗
arXiv2014

Development of very high Jc in Ba(Fe1-xCox)2As2 thin films grown on CaF2

Ba(Fe1-xCox)2As2 is the most tunable of the Fe-based superconductors (FBS) in terms of acceptance of high densities of self-assembled and artificially introduced pinning centres which are effective in significantly increasing the critical current density, Jc. Moreover, FBS are very sensitive to strain, which induces an important enhancement in critical temperature, Tc, of the material. In this paper we demonstrate that strain induced by the substrate can further improve Jc of both single and multilayer films by more than that expected simply due to the increase in Tc. The multilayer deposition of Ba(Fe1-xCox)2As2 on CaF2 increases the pinning force density Fp by more than 60% compared to a single layer film, reaching a maximum of 84 GN/m^3 at 22.5T and 4.2 K, the highest value ever reported in any 122 phase.

cond-mat.supr-con↗
arXiv2014

Enhancement of muonium emission rate from silica aerogel with a laser ablated surface

Emission of muonium ($μ^+e^-$) atoms from a laser-processed aerogel surface into vacuum was studied for the first time. Laser ablation was used to create hole-like regions with diameter of about 270$~μ$m in a triangular pattern with hole separation in the range of 300--500$~μ$m. The emission probability for the laser-processed aerogel sample is at least eight times higher than for a uniform one.

physics.ins-det↗
arXiv2014

Electrodynamics of superconducting pnictide superlattices

It has been recently reported (S. Lee et al., Nature Materials 12, 392, 2013) that superlattices where layers of the 8% Co-doped BaFe2As2 superconducting pnictide are intercalated with non superconducting ultrathin layers of either SrTiO3 or of oxygen-rich BaFe2As2, can be used to control flux pinning, thereby increasing critical fields and currents, without significantly affecting the critical temperature of the pristine superconducting material. However, little is known about the electron properties of these systems. Here we investigate the electrodynamics of these superconducting pnictide superlattices in the normal and superconducting state by using infrared reflectivity, from THz to visible range. We find that multi-gap structure of these superlattices is preserved, whereas some significant changes are observed in their electronic structure with respect to those of the original pnictide. Our results suggest that possible attempts to further increase the flux pinning may lead to a breakdown of the pnictide superconducting properties.

cond-mat.supr-con↗
arXiv2013

Dual-readout Calorimetry

The RD52 Project at CERN is a pure instrumentation experiment whose goal is to understand the fundamental limitations to hadronic energy resolution, and other aspects of energy measurement, in high energy calorimeters. We have found that dual-readout calorimetry provides heretofore unprecedented information event-by-event for energy resolution, linearity of response, ease and robustness of calibration, fidelity of data, and particle identification, including energy lost to binding energy in nuclear break-up. We believe that hadronic energy resolutions of σ/E $\approx$ 1 - 2% are within reach for dual-readout calorimeters, enabling for the first time comparable measurement preci- sions on electrons, photons, muons, and quarks (jets). We briefly describe our current progress and near-term future plans. Complete information on all aspects of our work is available at the RD52 website http://highenergy.phys.ttu.edu/dream/.

physics.ins-det↗
arXiv2013

Artificially engineered superlattices of pnictide superconductor

Significant progress has been achieved in fabricating high quality bulk and thinfilm iron-based superconductors. In particular, artificial layered pnictide superlattices offer the possibility of tailoring the superconducting properties and understanding the mechanism of the superconductivity itself. For high field applications, large critical current densities (Jc) and irreversibility fields (Hirr) are indispensable along all crystal directions. On the other hand, the development of superconducting devices such as tunnel junctions requires multilayered heterostructures. Here we show that artificially engineered undoped Ba-122 / Co doped Ba-122 compositionally modulated superlattices produce ab-aligned nanoparticle arrays. These layer and self-assemble along c-axis aligned defects, and combine to produce very large Jc and Hirr enhancements over a wide angular range. We also demonstrate a structurally modulated SrTiO3 (STO) / Co doped Ba-122 superlattice with sharp interfaces. Success in superlattice fabrication involving pnictides will aid the progress of heterostructured systems exhibiting novel interfacial phenomena and device applications.

cond-mat.supr-con↗
arXiv2013

Simultaneous Electrical and Optical Readout of Graphene-Coated High Q Silicon Nitride Resonators

We have fabricated and tested mechanical resonators consisting of a single-atomic-layer of graphene deposited on suspended silicon nitride membranes. With the addition of the graphene layer we retain the desirable mechanical properties of silicon nitride but utilize the electrical and optical properties of graphene to transduce resonant motion by both optical and electrical means. By positioning the graphene-on-silicon-nitride drums in a tunable optical cavity we observe position dependent damping and resonant frequency control of the devices due to optical absorption by graphene.

cond-mat.mes-hall↗
arXiv2013

Spin-valley lifetimes in a silicon quantum dot with tunable valley splitting

Although silicon is a promising material for quantum computation, the degeneracy of the conduction band minima (valleys) must be lifted with a splitting sufficient to ensure formation of well-defined and long-lived spin qubits. Here we demonstrate that valley separation can be accurately tuned via electrostatic gate control in a metal-oxide-semiconductor quantum dot, providing splittings spanning 0.3 - 0.8 meV. The splitting varies linearly with applied electric field, with a ratio in agreement with atomistic tight-binding predictions. We demonstrate single-shot spin readout and measure the spin relaxation for different valley configurations and dot occupancies, finding one-electron lifetimes exceeding 2 seconds. Spin relaxation occurs via phonon emission due to spin-orbit coupling between the valley states, a process not previously anticipated for silicon quantum dots. An analytical theory describes the magnetic field dependence of the relaxation rate, including the presence of a dramatic rate enhancement (or hot-spot) when Zeeman and valley splittings coincide.

cond-mat.mes-hall↗
arXiv2012

Artificial and self-assembled pinning centers in Ba(Fe1-xCox)2As2 thin films as a route to very high current density

We report on the superior vortex pinning of single and multilayer Ba(Fe1-xCox)2As2 thin films with self-assembled c-axis and artificially introduced ab-plane pins. Ba(Fe1-xCox)2As2 can accept a very high density of pins (15-20 vol%) without Tc suppression. The matching field is greater than 12 T, producing a significant enhancement of the critical current density Jc, an almost isotropic Jc (Theta,20T) > 10^5 A/cm2, and global pinning force density Fp of about 50 GN/m^3. This scenario strongly differs from the high temperature cuprates where the addition of pins without Tc suppression is limited to 2-4 vol%, leading to small HIrr enhancements and improved Jc only below 3-5 Tesla.

cond-mat.supr-con↗
arXiv2012

Bi-disperse particle-laden flows in the Stokes regime

This arXiv article describes the fluid dynamics video on `Bi-disperse particle-laden flows in the Stokes regime', presented at the 65th Annual Meeting of the APS Division of Fluid Dynamics in San Diego, CA in November 2012. The video shows three different experiments which aim to investigate the dynamics of a thin film of silicone oil, laden with glass beads and the effects of adding a second species of particles to the slurry. The mixture of oil and particles is allowed to flow down an incline under the action of gravity. The videos were recorded at the UCLA Applied Math Laboratory.

physics.flu-dyn↗