arXiv subjects

S. Lee

Publications and source records attributed to S. Lee.

At least 217 records · Page 12Linked to original sources

arXiv2012

High Contrast X-ray Speckle from Atomic-Scale Order in Liquids and Glasses

The availability of ultrafast pulses of coherent hard x-rays from the Linac Coherent Light Source opens new opportunities for studies of atomic-scale dynamics in amorphous materials. Here we show that single ultrafast coherent x-ray pulses can be used to observe the speckle contrast in the high-angle diffraction from liquid Ga and glassy Ni2Pd2P and B2O3. We determine the thresholds above which the x-ray pulses disturb the atomic arrangements. Furthermore, high contrast speckle is observed in scattering patterns from the glasses integrated over many pulses, demonstrating that the source and optics are sufficiently stable for x-ray photon correlation spectroscopy studies of dynamics over a wide range of time scales.

cond-mat.mtrl-sci↗

arXiv2012

Suppression of the near-infrared OH night sky lines with fibre Bragg gratings - first results

The background noise between 1 and 1.8 microns in ground-based instruments is dominated by atmospheric emission from hydroxyl molecules. We have built and commissioned a new instrument, GNOSIS, which suppresses 103 OH doublets between 1.47 - 1.7 microns by a factor of ~1000 with a resolving power of ~10,000. We present the first results from the commissioning of GNOSIS using the IRIS2 spectrograph at the AAT. The combined throughput of the GNOSIS fore-optics, grating unit and relay optics is ~36 per cent, but this could be improved to ~46 per cent with a more optimal design. We measure strong suppression of the OH lines, confirming that OH suppression with fibre Bragg gratings will be a powerful technology for low resolution spectroscopy. The integrated OH suppressed background between 1.5 and 1.7 microns is reduced by a factor of 9 compared to a control spectrum using the same system without suppression. The potential of low resolution OH suppressed spectroscopy is illustrated with example observations. The GNOSIS background is dominated by detector dark current below 1.67 microns and by thermal emission above 1.67 microns. After subtracting these we detect an unidentified residual interline component of ~ 860 +/ 210 ph/s/m^2/micron/arcsec^2. This component is equally bright in the suppressed and control spectra. We have investigated the possible source of the interline component, but were unable to discriminate between a possible instrumental artifact and intrinsic atmospheric emission. Resolving the source of this emission is crucial for the design of fully optimised OH suppression spectrographs. The next generation OH suppression spectrograph will be focussed on resolving the source of the interline component, taking advantage of better optimisation for a FBG feed. We quantify the necessary improvements for an optimal OH suppressing fibre spectrograph design.

astro-ph.IM↗

arXiv2012

Ultrafast carrier dynamics and radiative recombination in multiferroic BiFeO$_{3}$

We report a comprehensive study of ultrafast carrier dynamics in single crystals of multiferroic BiFeO$_{3}$. Using femtosecond optical pump-probe spectroscopy, we find that the photoexcited electrons relax to the conduction band minimum through electron-phonon coupling with a $\sim$1 picosecond time constant that does not significantly change across the antiferromagnetic transition. Photoexcited electrons subsequently leave the conduction band and primarily decay via radiative recombination, which is supported by photoluminescence measurements. We find that despite the coexisting ferroelectric and antiferromagnetic orders in BiFeO$_{3}$, the intrinsic nature of this charge-transfer insulator results in carrier relaxation similar to that observed in bulk semiconductors.

cond-mat.mtrl-sci↗

arXiv2011

New tools for the direct characterisation of FinFETs

This paper discusses how classical transport theories such as the thermionic emission, can be used as a powerful tool for the study and the understanding of the most complex mechanisms of transport in Fin Field Effect Transistors (FinFETs). By means of simple current and differential conductance measurements, taken at different temperatures and different gate voltages ($V_G$'s), it is possible to extrapolate the evolution of important parameters such as the spatial region of transport and the height of thermionic barrier at the centre of the channel. Furthermore, if the measurements are used in conjunction with simulated data, it becomes possible to also extract the interface trap density of these objects. These are important results, also because these parameters are extracted directly on state-of-the-art devices and not in specially-designed test structures. The possible characterisation of the different regimes of transport that can arise in these ultra-scaled devices having a doped or an undoped channel are also discussed. Examples of these regimes are, full body inversion and weak body inversion. Specific cases demonstrating the strength of the thermionic tool are discussed in sections \ref{sec:II}, \ref{sec:III} and \ref{sec:IV}. This text has been designed as a comprehensive overview of 4 related publications (see Ref. [2-5]) and has been submitted as a book chapter in Ref. [6]).

cond-mat.mes-hall↗

arXiv2011

Superfluid density measurements of Ba(CoxFe1-x)2As2 films near optimal doping

We report the first direct measurements of superfluid density, ns(T) \propto λ-2(T), in films of Fe-pnictide superconductors. The magnetic penetration depth, λ(0), in our epitaxial, single-crystal Ba(CoxFe1-x)2As2 films near optimal doping (x=0.08) is 350 nm to 430 nm, comparable to bulk single crystals. The T-dependence of λ-2 indicates a small s-wave gap, 2Δ(0)/kBTc = 2.2 \pm 0.1. In detail, λ has power-law behavior at low T: λ(T)/λ(0) - 1 \approx 0.60*(T/Tc)2.5\pm0.1. The small gap, together with power-law behavior at low T, suggests strong intraband scattering on the larger-gap Fermi surface and significant interband scattering between large-gap and small-gap Fermi surfaces.

cond-mat.supr-con↗

arXiv2010

Multi-gap superconductivity in a BaFe1.84Co0.16As2 film from optical measurements at terahertz frequencies

We measured the THz reflectance properties of a high quality epitaxial thin film of the Fe-based superconductor BaFe$_{1.84}$Co$_{0.16}$As$_2$ with T$_c$=22.5 K. The film was grown by pulsed laser deposition on a DyScO$_3$ substrate with an epitaxial SrTiO$_3$ intermediate layer. The measured $R_S/R_N$ spectrum, i.e. the reflectivity ratio between the superconducting and normal state reflectance, provides clear evidence of a superconducting gap $Δ_A$ close to 15 cm$^{-1}$. A detailed data analysis shows that a two-band, two-gap model is absolutely necessary to obtain a good description of the measured $R_S/R_N$ spectrum. The low-energy $Δ_A$ gap results to be well determined ($Δ_A$=15.5$\pm$0.5 cm$^{-1}$), while the value of the high-energy gap $Δ_B$ is more uncertain ($Δ_B$=55$\pm$7 cm$^{-1}$). Our results provide evidence of a nodeless isotropic double-gap scenario, with the presence of two optical gaps corresponding to 2$Δ/kT_c$ values close to 2 and 7.

cond-mat.supr-con↗

arXiv2010

Observation of a coherence peak and pair-breaking effects in THz conductivity of BaFe$_{2-2x}$Co$_{2x}$As$_2$

We report a study of high quality pnictide superconductor BaFe$_{1.84}$Co$_{0.16}$As$_2$ thin films using time-domain THz spectroscopy. Near T$_c$ we find evidence for a coherence peak and qualitative agreement with the weak-coupling Mattis-Bardeen form of the conductivity. At low temperature, we find that the real part of the THz conductivity is not fully suppressed and $σ_2$ is significantly smaller than the Matthis-Bardeen expectation. The temperature dependence of the penetration depth $λ$ follows a power law with an unusually high exponent of 3.1. We interpret these results as consistent with impurity scattering induced pair-breaking. Taken together our results are strong evidence for an extended s$\pm$ symmetry order parameter.

cond-mat.supr-con↗

arXiv2010

Conductance asymmetry in point-contacts on epitaxial thin films of Ba(Fe$_{0.92}$Co$_{0.08}$)$_2$As$_2$

Point-contact spectroscopy is a powerful tool for probing superconductors. One of the most common observations in the point-contact spectra on the recently discovered ferropnictide superconductors is a large conductance asymmetry with respect to voltage across the point-contact. In this paper we show that the antisymmetric part of the point-contact spectrum between a silver tip and an epitaxial thin film of Ba(Fe$_{0.92}$Co$_{0.08}$)$_2$As$_2$ shows certain unique features. These features have an interesting evolution with increasing temperature up to a temperature that is 30% larger than the critical temperature $T_c$ of the superconductor. We argue that this evolution can be associated with the rich normal state properties of these materials.

cond-mat.supr-con↗

arXiv2010

Auger decay of 1σg and 1σu hole states of N2 molecule: disentangling decay routes from coincidence measurements

Results of the most sophisticated measurements in coincidence of the angular resolved K-shell photo- and Auger-electrons, and of two atomic ions produced by dissociation of N2 molecule, are analyzed. Detection of photoelectrons at certain angles allows separating the Auger decay processes of the 1σg and 1σu core hole states. The Auger electron angular distributions for each of these hole states are measured as a function of the kinetic energy release of two atomic ions and are compared with the corresponding theoretical angular distributions. From that comparison one can disentangle the contributions of different repulsive doubly charged molecular ion states to the Auger decay. Different kinetic energy release values are directly related to the different internuclear distances. In this way one can trace experimentally the behavior of the potential energy curves of dicationic final states inside the Frank-Condon region. Presentation of the Auger electron angular distributions as a function of kinetic energy release of two atomic ions opens a new dimension in the study of Auger decay.

physics.atom-ph↗

arXiv2010

Phase-incoherent superconducting pairs in the normal state of Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$

The normal state properties of the recently discovered ferropnictide superconductors might hold the key to understanding their exotic superconductivity. Using point-contact spectroscopy we show that Andreev reflection between an epitaxial thin film of Ba(Fe$_{0.92}$Co$_{0.08}$)$_2$As$_2$ and a silver tip can be seen in the normal state of the film up to temperature $T\sim1.3T_c$, where $T_c$ is the critical temperature of the superconductor. Andreev reflection far above $T_c$ can be understood only when superconducting pairs arising from strong fluctuation of the phase of the complex superconducting order parameter exist in the normal state. Our results provide spectroscopic evidence of phase-incoherent superconducting pairs in the normal state of the ferropnictide superconductors.

cond-mat.supr-con↗

arXiv2010

Electrical transport properties of high quality Bi-2223 crystal

We have studied electrical transport properties of a high quality Bi2Sr2Ca2Cu3O10+x crystal below a superconducting critical temperature, Tc. In magnetic fields B parallel to the c-axis just above a voltage response onset resistance vs temperature data are well fitted to the vortex-glass model. Obtained from the vortex-glass analysis a melting transition boundary for Bi-2223 crystal shifted towards lower temperatures compared to previously reported data for a (Bi,Pb)-2223 single crystal. The critical current density, Jc, of Bi-2223 crystals is close to presented elsewhere Jc values for Bi-2223 tapes suggesting a principal role of weak intrinsic pinning properties of Bi-2223 as a main limiting factor of Jc of Bi-2223 conductors.

cond-mat.supr-con↗

arXiv2010

Strong vortex pinning in Co-doped BaFe2As2 single crystal thin films

We report measurements of the field and angular dependences of Jc of truly epitaxial Co-doped BaFe2As2 thin films grown on SrTiO3/(La,Sr)(Al,Ta)O3 with different SrTiO3 template thicknesses. The films show Jc comparable to Jc of single crystals and a maximum pinning force Fp(0.6Tc) > 5 GN/m3 at H/Hirr ~ 0.5 indicative of strong vortex pinning effective up to high fields. Due to the strong correlated c-axis pinning, Jc for field along the c-axis exceeds Jc for H//ab plane, inverting the expectation of the Hc2 anisotropy. HRTEM reveals that the strong vortex pinning is due to a high density of nanosize columnar defects.

cond-mat.supr-con↗

arXiv2009

Weak-link behavior of grain boundaries in superconducting Ba(Fe1-xCox)2As2 bicrystals

We show that despite the low anisotropy, strong vortex pinning and high irreversibility field Hirr close to the upper critical field Hc2 of Ba(Fe1-xCox)2As2, the critical current density Jgb across [001] tilt grain boundaries (GBs) of thin film Ba(Fe1-xCox)2As2 bicrystals is strongly depressed, similar to high-Tc cuprates. Our results suggest that weak-linked GBs are characteristic of both cuprates and pnictides because of competing orders, low carrier density, and unconventional pairing symmetry.

cond-mat.supr-con↗

arXiv2009

Study of D^{+} and D_{s}^{+} Decay Properties at Belle

We report the first observation of the doubly Cabibbo-suppressed decay, $D^{+}_{s} \to K^{+}K^{+}π^{-}$ and the significantly improved measurement of the doubly Cabibbo-suppressed decay, $D^{+} \to K^{+}π^{+}π^{-}$ using $\textrm{605 fb}^{-1}$ of data collected with the Belle detector at the KEKB asymmetric-energy $e^{+}e^{-}$ collider. The branching ratio with respect to its Cabibbo-favored counterpart are $\mathcal{B}(D^{+}_{s} \to K^{+}K^{+}π^{-})/\mathcal{B}(D^{+}_{s} \to K^{+}K^{-}π^{+}) = 0.229\pm0.028\pm0.012)%$ and $\mathcal{B}(D^{+} \to K^{+}π^{+}π^{-})/\mathcal{B}(D^{+} \to K^{-}π^{+}π^{+}) = (0.569\pm0.018\pm0.014)%$, where the first uncertainties are statistical and the second is systematic. We also report the improved measurement of $D^{+} \to K^{0}_{S}K^{+}$ and $D^{+}_{s} \to K^{0}_{S}π^{+}$ branching ratios using the same amount of data samples. The measured branching ratios with respect to the Cabibbo-favored modes are $\mathcal{B}(D^{+} \to K^{0}_{S}K^{+})/\mathcal{B}(D^{+} \to K^{0}_{S}π^{+}) = (0.1899\pm0.0011\pm0.0018)$ and $\mathcal{B}(D^{+}_{s} \to K^{0}_{S}π^{+})/\mathcal{B}(D^{+}_{s} \to K^{0}_{S}K^{+}) = (0.0803\pm0.0024\pm0.0012)$.

hep-ex↗

arXiv2009

Template engineering of Co-doped BaFe2As2 single-crystal thin films

Understanding new superconductors requires high-quality epitaxial thin films to explore intrinsic electromagnetic properties, control grain boundaries and strain effects, and evaluate device applications. So far superconducting properties of ferropnictide thin films appear compromised by imperfect epitaxial growth and poor connectivity of the superconducting phase. Here we report novel template engineering using single-crystal intermediate layers of (001) SrTiO3 and BaTiO3 grown on various perovskite substrates that enables genuine epitaxial films of Co-doped BaFe2As2 with high transition temperature (zero resistivity Tc of 21.5K), small transition widths (delta Tc = 1.3K), superior Jc of 4.5 MA/cm2 (4.2K, self field) and strong c-axis flux pinning. Implementing SrTiO3 or BaTiO3 templates to match the alkaline earth layer in the Ba-122 with the alkaline earth-oxygen layer in the templates opens new avenues for epitaxial growth of ferropnictides on multi-functional single crystal substrates. Beyond superconductors, it provides a framework for growing heteroepitaxial intermetallic compounds on various substrates by matching interfacial layers between templates and thin film overlayers.

cond-mat.supr-con↗

arXiv2009

Anomalous Corrections to Hall Resistivity of Spin-Polarized Two-Dimensional Holes in a GaAs/AlGaAs Heterostructure

Hall effect of two-dimensional holes that are spin-polarized by a strong parallel magnetic field was explored with a small tilt angle. The Hall resistivity increases nonlinearly with the magnetic field and exhibits negative corrections. The anomalous negative corrections increase with the perpendicular magnetization of the two-dimensional hole system. We attribute this to the anomalous Hall effect of spin-polarized carriers in a nonmagnetic system. The anomalous corrections to the conductivity exhibit non-monotonic dependence on the magnetic field.

cond-mat.mes-hall↗

arXiv2009

Vortex glass scaling in Pb-doped Bi2223 single crystal

We report on study of the vortex liquid in Pb-doped Bi-2223 single crystal using the in-plane resistivity measurements as a function of temperature and magnetic field up to 6T applied perpendicular to CuO planes. Below Tc at the upper part of superconducting transition we found Arrhenius-like resistivity behavior. With further temperature decrease close to resistivity onset resistivity shows power law dependence on temperature signaling approaching vortex-glass transition. The critical exponents nu(z-1)=4.6 plus-minus 0.5 are found to be field independent within experimental errors. We also present magnetic phase diagram defining region of nonzero critical current for Pb-doped Bi-2223 single crystal.

cond-mat.supr-con↗

arXiv2009

Spin-Charge-Lattice Coupling through Resonant Multi-Magnon Excitations in Multiferroic BiFeO3

Spin-charge-lattice coupling mediated by multi-magnon processes is demonstrated in multiferroic BiFeO3. Experimental evidence of two and three magnons excitations as well as multimagnon coupling at electronic energy scales and high temperatures are reported. Temperature dependent Raman experiments show up to five resonant enhancements of the 2-magnon excitation below the Neel temperature. These are shown to be collective interactions between on-site Fe d-d electronic resonance, phonons and multimagnons

cond-mat.other↗