arXiv subjects

S. Okamoto

Publications and source records attributed to S. Okamoto.

At least 19 recordsLinked to original sources

arXiv2026

Disentangling multi-spin dynamic correlations in the Heisenberg spin-$\frac{1}{2}$ chain

Higher-order correlations are essential for understanding exotic phases and uncovering universal aspects of quantum dynamics. While inelastic neutron scattering provides well-established access to two-particle correlations, measuring correlations in solids involving more than two particles remains a major challenge. Focusing on magnetic excitations in the Heisenberg spin-$\frac{1}{2}$ chain, we demonstrate that resonant inelastic X-ray scattering (RIXS) can selectively probe multi-spin dynamical correlations by exciting distinct intermediate states through energy detuning. Through theoretical modeling, we isolate the two- and multi- spin responses, and establish that: (i) The resonant energies of the two- and multi- spin dynamical correlations are separated by $\approx \frac{3}{4}J$; implying that the multi-spin part of the cross-section comes from intermediate states that contain spin flips; (ii) The spectral weight of the two-spin channel exhibits a Lorentzian resonant energy profile consistent with a single dominant electronic configuration, whereas the multi-spin channel response shows a Gaussian-like profile, implying contributions from multiple intermediate spin configurations. These characteristics are reproduced by exact diagonalization of the $t-J$ Hamiltonian, which further reveals that the widths of Lorentzian and Gaussian resonant energy profiles depend primarily on core-hole lifetime ($\Gamma/2$) and $\frac{2J}{\Gamma}$, respectively. Controlled access to multi-spin dynamics, using RIXS energy detuning as a knob, can open new pathways to explore many-body dynamics in quantum materials.

cond-mat.str-el↗

arXiv2026

Magnetic Imaging of Macroscopic Spin Chirality Flipping

Chirality is a fundamental organizing principle of correlated and topological states. In quantum magnets, chirality arises from the geometric twisting of spins and serves as an emergent source of Berry curvature and quantum metrics. Although external fields can reversibly tune the spin chirality, understanding how spontaneous reversal occurs on macroscopic length scale remains an unresolved challenge. In this letter, we use resonant magnetic x-ray scattering with 2.5-micron spatial resolution to image intertwined spin, charge, and lattice orders of the correlated topological magnet EuAl4. We uncover a macroscopic chirality flipping transition and a remarkable chiral memory effect. The chiral magnetic domain tracks the landscape of the underlying charge density wave, implicating emergent chiral magnetic interactions arising from competing chiral and nematic lattice fields. Our results reveal the fundamental significance of magnetoelastic coupling in stabilizing homochiral and topological magnetic states.

cond-mat.str-el↗

arXiv2025

Isoscalar Giant Resonances in Highly-Deformed $^{172}$Yb

To study the isoscalar giant resonances in a deformed case, background-free $\alpha$-particle inelastic scattering measurements using a 386 MeV $\alpha$ beam were performed on the highly-deformed $^{172}$Yb nucleus using the Grand Raiden spectrometer at the Research Center for Nuclear Physics (RCNP) at very forward angles, including $0^\circ$. The strength distributions for the isoscalar giant resonances up to $L \leq 3$ were obtained using multipole decomposition analysis. The isoscalar giant monopole resonance (ISGMR) strength exhibits a splitting into two components, interpreted as the coupling of the ISGMR with the $K=0$ component of the isoscalar giant quadrupole resonance (ISGQR). A \textit{bimodal} structure is observed in the strength distribution of the isoscalar giant dipole resonance. The ISGQR strength shows an enhancement near 25 MeV, attributed to the excitation of an overtone mode, while the broadening of the main-tone peak is associated with nuclear deformation. The experimental results are well reproduced by theoretical strength distributions calculated using the quasiparticle finite amplitude method for $L \leq 3$.

nucl-ex↗

arXiv2025

Why the Northern Hemisphere Needs a 30-40 m Telescope and the Science at Stake: Resolved Stellar Populations Studies in M31 and its Satellites

A 30 m class optical/near-IR telescope in the Northern Hemisphere, equipped for diffraction-limited imaging and high-resolution, multi-object spectroscopy of faint stars, would enable a transformational investigation of the formation and evolution of M31 and its satellite system - on par with what Gaia, the HST, and other major photometric and spectroscopic facilities have achieved for the Milky Way (MW) and its satellites. The unprecedented detail obtained for our home system has reshaped our understanding of the assembly of the MW disk, halo, and bulge, and that of its satellites, which now serve as a benchmark for galaxy formation and evolution models. Extending this level of insight to the M31 system - that of the nearest massive spiral and the only one for which such a comprehensive, resolved stellar population study is feasible - will allow us to address a fundamental question: how representative is the MW and its satellite system within the broader context of galaxy evolution?

astro-ph.IM↗

arXiv2025

Precise measurement of the $\gamma$-decay probability of the Hoyle state with a new triple coincidence-detection method

We measured the $\gamma$-decay probability of the Hoyle state with a new method of triple coincidence detection of a scattered $\alpha$ particle, a recoil $\rm ^{12}C$ nucleus, and a $\gamma$ ray in inelastic alpha scattering on $\rm ^{12}C$. This method successfully enabled a low-background measurement and a precise determination of the $\gamma$-decay probability of the Hoyle state as $\Gamma_\mathrm{\gamma}/\Gamma=[4.00 \pm 0.22 \mathrm{(sta.)} \pm 0.18 \mathrm{(sys.)}]\times10^{-4}$, which is consistent with the previous literature value. Therefore, we concluded that the literature value can be reliably used in the study of nucleosynthesis in the universe.

nucl-ex↗

arXiv2024

Effect of ground-state deformation on the Isoscalar Giant Monopole Resonance and the first observation of overtones of the Isoscalar Giant Quadrupole Resonance in rare-earth Nd isotopes

The strength distributions of the Isoscalar Giant Monopole Resonance (ISGMR) and Isoscalar Giant Quadrupole Resonance (ISGQR) in 142,146-150Nd have been determined via inelastic alpha-particle scattering with the Grand Raiden (GR) Spectrometer at the Research Center for Nuclear Physics (RCNP), Japan. In the deformed nuclei 146-150Nd, the ISGMR strength distributions exhibit a splitting into two components, while the nearly spherical nucleus 142Nd displays a single peak in the ISGMR strength distribution. A noteworthy achievement in this study is the first-time detection of overtones in the Isoscalar Giant Quadrupole Resonance (ISGQR) strength distributions within Nd isotopes at an excitation energy around 25 MeV obtained through Multipole Decomposition Analysis (MDA).

nucl-ex↗

arXiv2023

Search for the 6$α$ condensed state in $^{24}$Mg using the $^{12}\rm{C}+{}^{12}\rm{C}$ scattering

We searched for the 6$α$-condensed state in $^{24}$Mg by measuring the $^{12}\rm{C}+{}^{12}\rm{C}$ scattering with the SAKRA Si detector array at $E_\rm{cm}$ = 17.5-25.0 MeV. By using the invariant-mass method for the detected 3$α$ particles, the inclusive cross sections for the $^{12}\rm{C}+{}^{12}\rm{C}\to{}^{12}\rm{C}(0^+_2)+X$ and $^{12}\rm{C}(3^-_1)+X$ reactions were determined. In addition, the missing-mass spectroscopy was successfully utilized to determine the excitation energy of the residual $^{12}\rm{C}$ nucleus and the exclusive cross sections for the $^{12}\rm{C}+{}^{12}\rm{C}\to{}^{12}\rm{C}(0^+_2)+{}^{12}\rm{C}(0^+_1)$, $^{12}\rm{C}(0^+_2)+{}^{12}\rm{C}(2^+_1)$, and $^{12}\rm{C}(0^+_2)+{}^{12}\rm{C}(0^+_2)$ reactions. In both the inclusive $^{12}\rm{C}(0^+_2)+X$ channel and the exclusive $^{12}\rm{C}(0^+_2)+{}^{12}\rm{C}(0^+_1)$ channel, the cross section peaked at $E_rm{cm}$ = 19.4 MeV, which correspond to the excitation energy of $E_x$ = 33.3 MeV in $^{24}\rm{Mg}$. This 19.4-MeV state is a candidate for the 6$α$-condensed state because of the agreement of the excitation energy with the theoretical value and its decay property. In the exclusive $^{12}\rm{C}(0^+_2)+{}^{12}\rm{C}(0^+_2)$ channel, a broad state was observed at $E_\rm{cm}$ = 22.5 MeV, which correspond to the excitation energy of $E_x$ = 36.4 MeV in $^{24}\rm{Mg}$. From the angular distribution of the differential cross section, the spin and parity of this 22.5-MeV state was assigned to be $4^+$. In addition, a $2^+$ state was suggested at the low-energy side of the 22.5-MeV state. Because their excitation energies are higher than the theoretical value of the 6$α$-condensed state, these states might be excited states of the 6$α$-condensed state such as the $2^+_2$ and $4^+_1$ states in $^{12}\rm{C}$.

nucl-ex↗

arXiv2023

Spin wave Hamiltonian and anomalous scattering in NiPS$_3$

We report a comprehensive spin wave analysis of the semiconducting honeycomb van der Waal antiferromagnet NiPS$_3$. Using single crystal inelastic neutron scattering, we map out the full Brillouin zone and fit the observed modes to a spin wave model with rigorously defined uncertainty. We find that the third neighbor exchange $J_3$ dominates the Hamiltonian, a feature which we fully account for by ab-initio density functional theory calculations. We also quantify the degree to which the three-fold rotation symmetry is broken and account for the $Q=0$ excitations observed in other measurements, yielding a spin exchange model which is consistent across multiple experimental probes. We also identify a strongly reduced static ordered moment and reduced low-energy intensity relative to the linear spin wave calculations, signaling unexplained features in the magnetism which requires going beyond the linear spin wave approximation.

cond-mat.str-el↗

arXiv2022

Spin-phonon coupling driven Charge density wave in a Kagome Magnet

The intertwining between spin, charge, and lattice degrees of freedom can give rise to unusual macroscopic quantum states, including high-temperature superconductivity and quantum anomalous Hall effects. Recently, a charge density wave (CDW) is observed in the kagome antiferromagnet FeGe, indicative of possible intertwining physics. An outstanding question is that whether magnetic correlation is fundamental for the spontaneous spatial symmetry breaking orders. Here, utilizing elastic and high-resolution inelastic x-ray scattering, we discover a charge dimerization superlattice that coexists with the 2$\times$2$\times$1 CDW in the kagome sublattice. Most interestingly, between the magnetic and CDW transition temperature, the phonon dynamical structure factor shows a giant phonon-energy hardening and a substantial phonon linewidth broadening near the charge-dimerization wavevectors, both signaling the spin-phonon coupling. By first principles calculations, we show that both the static and dynamic spin excitations intertwine with the phonon to drive the spatial symmetry breaking.

cond-mat.str-el↗

arXiv2022

PANDORA project: photo-nuclear reactions below $A=60$

Photo-nuclear reactions of light nuclei below a mass of $A=60$ are studied experimentally and theoretically by the PANDORA (Photo-Absorption of Nuclei and Decay Observation for Reactions in Astrophysics) project. Two experimental methods, virtual-photon excitation by proton scattering and real-photo absorption by a high-brilliance gamma-ray beam produced by laser Compton scattering, will be applied to measure the photo-absorption cross sections and the decay branching ratio of each decay channel as a function of the photon energy. Several nuclear models, e.g. anti-symmetrized molecular dynamics, mean-field type models, a large-scale shell model, and ab initio models, will be employed to predict the photo-nuclear reactions. The uncertainty in the model predictions will be evaluated from the discrepancies between the model predictions and the experimental data. The data and the predictions will be implemented in a general reaction calculation code TALYS . The results will be applied to the simulation of the photo-disintegration process of ultra-high-energy cosmic rays in inter-galactic propagation.

nucl-ex↗

arXiv2022

Non-linear magnons and exchange Hamiltonians of delafossite proximate quantum spin liquids

Quantum spin liquids (QSL) are theoretical states of matter with long-range entanglement and exotic quasiparticles. However, they generally elude quantitative theory, rendering their underlying phases mysterious and hampering efforts to identify experimental QSL states. Here we study triangular lattice resonating valence bond QSL candidate materials KYbSe$_2$ and NaYbSe$_2$. We measure the magnon modes in their 1/3 plateau phase, where quantitative theory is tractable, using inelastic neutron scattering and fit them using nonlinear spin wave theory. We also fit the KYbSe$_2$ heat capacity using high temperature series expansion. Both KYbSe$_2$ fits yield the same magnetic Hamiltonian to within uncertainty, confirming previous estimates and showing the Heisenberg $J_2/J_1$ to be an accurate model for these materials. Most importantly, comparing KYbSe$_2$ and NaYbSe$_2$ shows that smaller $A$-site Na$^+$ ion has a larger $J_2/J_1$ ratio. However, hydrostatic pressure applied to KYbSe$_2$ increases the ordering temperature (a result consistent with density functional theory calculations), indicating that pressure decreases $J_2/J_1$. These results show how periodic table and hydrostatic pressure can tune the $A$YbSe$_2$ materials in a controlled way.

cond-mat.str-el↗

arXiv2022

Spin sensitive transport in RuCl_3/Pt heterostructures: revealing a field-transverse spin anisotropy in a spin liquid candidate

Alpha-phase (a-) RuCl_3 has emerged as a possible candidate for a quantum spin liquid (QSL) that promises exotic quasi-particles relevant for fault-tolerant quantum computation. Here, we report spin-sensitive transport measurements using a proximal spin Hall metal -- platinum (Pt) -- to probe magnetic moments in the insulator a-RuCl_3. We observe a spin Hall magnetoresistance (SMR) where both the transverse and longitudinal resistivities of a-RuCl_3/Pt exhibit oscillations as functions of the angle between the in-plane magnetic field and the current, arising from the interplay between the spin Hall effect in Pt and local magnetic moments in a-RuCl3. The oscillations are observed from 1.5 T to 18 T, spanning the range of magnetic fields where zig-zag antiferromagnetic phase, the putative QSL phase, and the partially field-polarized states are reported in a-RuCl_3. The phase of the SMR oscillations suggest that the local moments, regardless of static or fluctuating, in a-RuCl_3 develop an anisotropy with an in-plane quantization axis that aligns largely transverse to the magnetic field for all fields above 1.5 T. Temperature dependance of the SMR revealed that the spin anisotropy has a similar energy scale to reported QSL signatures in a-RuCl_3. The coupling between the spin states within a-RuCl_3 and Pt demonstrated in our experiment opens a transport route to exploring exotic spin phases and device functionalities of QSL materials.

cond-mat.str-el↗

arXiv2021

Divergence of Majorana-Phonon Scattering in Kitaev Quantum Spin Liquid

Magnetoelastic interaction couples spin and lattice degrees of freedom and plays a key role in thermal transport properties of magnetic insulators. In the Kitaev quantum spin liquid, the low energy excitations are charge neutral Majorana fermions, which transform the magnetoelasctic interaction into Majorana-phonon scattering. Motivated by anomalous thermal properties of the Kitaev quantum spin liquid candidate RuCl$_3$, in this letter, we combine meV resolution inelastic x-ray scattering and theoretical calculation to examine the Majorana-phonon scattering. We analytically derive the velocity-dependent Majorana-phonon scattering and find a divergence when the acoustic phonons and the itinerant Majorana fermions have the same velocity. Based on the experimentally determined acoustic phonon velocity in RuCl$_3$, we estimate the range in the Kitaev interaction for which divergent Majorana-phonon scattering can happen. Our result opens a new avenue to uncover fractionalized quasiparticles in the Kitaev quantum spin liquid and emphasizes the critical role of lattice excitations in RuCl$_3$.

cond-mat.str-el↗

arXiv2021

Giant Phonon Anomalies in the Proximate Kitaev Quantum Spin Liquid $α$-RuCl$_3$

The Kitaev quantum spin liquid epitomizes an entangled topological state, for which two flavors of fractionalized low-energy excitations are predicted: the itinerant Majorana fermion and the Z2 gauge flux. Detection of these excitations remains challenging, because of their fractional quantum numbers and non-locality. It was proposed recently that fingerprints of fractional excitations are encoded in the phonon spectra of Kitaev quantum spin liquids through a novel fractional-excitation-phonon coupling. Here, we uncover this effect in $α$-RuCl3 using inelastic X-ray scattering with meV resolution. At high temperature, we discover interlaced optical phonons intercepting a transverse acoustic phonon between 3 and 7 meV. Upon decreasing temperature, the optical phonons display a large intensity enhancement near the Kitaev energy, JK~8 meV, that coincides with a giant acoustic phonon softening near the Z2 gauge flux energy scale. This fractional excitation induced phonon anomalies uncover the key ingredient of the quantum thermal Hall effect in $α$-RuCl3 and demonstrates a proof-of-principle method to detect fractional excitations in topological quantum materials.

cond-mat.str-el↗

arXiv2021

Candidates for the 5$α$ condensed state in ${}^{20}$Ne

We conducted the coincidence measurement of $α$ particles inelastically scattered from ${}^{20}$Ne at $0^{\circ}$ and decay charged particles in order to search for the alpha-particle condensed state. We compared the measured excitation-energy spectrum and decay branching ratio with the statistical-decay-model calculations, and found that the newly observed states at $E_x$ = 23.6, 21.8, and 21.2 MeV in ${}^{20}$Ne are strongly coupled to a candidate for the 4$α$ condensed state in ${}^{16}$O. This result presents the first strong evidence that these states are the candidates for the 5$α$ condensed state.

nucl-ex↗

arXiv2021

Witnessing entanglement in quantum magnets using neutron scattering

We demonstrate how quantum entanglement can be directly witnessed in the quasi-1D Heisenberg antiferromagnet KCuF$_3$. We apply three entanglement witnesses --- one-tangle, two-tangle, and quantum Fisher information --- to its inelastic neutron spectrum, and compare with spectra simulated by finite-temperature density matrix renormalization group (DMRG) and classical Monte Carlo methods. We find that each witness provides direct access to entanglement. Of these, quantum Fisher information is the most robust experimentally, and indicates the presence of at least bipartite entanglement up to at least 50 K, corresponding to around 10% of the spinon zone-boundary energy. We apply quantum Fisher information to higher spin-S Heisenberg chains, and show theoretically that the witnessable entanglement gets suppressed to lower temperatures as the quantum number increases. Finally, we outline how these results can be applied to higher dimensional quantum materials to witness and quantify entanglement.

cond-mat.str-el↗

arXiv2020

A search for non-reciprocal magnons in MnPS$_3$

Recent articles have suggested that the quasi-two dimensional antiferromagnet MnPS$_3$ may have non-reciprocal magnons, whereby magnons in a Brillouin zone corner at +q have different energies than those at $-$q. The magnons along the Brillouin zone boundaries were measured using neutron three-axis spectrometry, paying careful attention to the resolution function, to determine whether such non-reciprocity was present. The data show that, within the resolution, there are no significant differences between the magnons in opposite Brillouin zone corners.

cond-mat.mtrl-sci↗

arXiv2020

Van Hove singularity in the magnon spectrum of the antiferromagnetic quantum honeycomb lattice

The magnetic excitation spectrum of the quantum magnet YbCl$_3$ is studied with inelastic neutron scattering. The spectrum exhibits an unusually sharp feature within a broad continuum, as well as conventional spin waves. By including both transverse and longitudinal channels of the neutron response, linear spin wave theory with a single Heisenberg interaction on the honeycomb lattice reproduces all of the key features in the spectrum. In particular, the broad continuum corresponds to a two-magnon contribution from the longitudinal channel, while the sharp feature within this continuum is identified as a Van Hove singularity in the joint density of states, which indicates the two-dimensional nature of the two-magnon continuum. We term these singularities magneto-caustic features in analogy with caustic features in ray optics where focused envelopes of light are generated when light passes through or reflects from curved or distorted surfaces. The experimental demonstration of a sharp Van Hove singularity in a two-magnon continuum is important because analogous features in potential two-spinon continua could distinguish quantum spin liquids from merely disordered systems. These results establish YbCl$_3$ as a nearly ideal two-dimensional honeycomb lattice material hosting strong quantum effects in the unfrustrated limit.

cond-mat.str-el↗