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S. Santucci

Publications and source records attributed to S. Santucci.

10 recordsLinked to original sources

Exponential Stress Relaxation Driven by Elementary Plastic Events in Non-Ageing Liquid Foams

Liquid foams are archetypal athermal amorphous solids whose elasticity arises from the jamming of densely packed bubbles. We investigate the stress relaxation of non-ageing liquid foams following flow cessation, using fast X-ray tomo-rheoscopy. Thanks to in situ, time-resolved measurements, we uncover robust linear affine relationships between shear stress, plastic activity, and coordination number throughout the relaxation toward a residual stress state below the yield value. In contrast to previous studies on amorphous solids, we observe an exponential relaxation governed by the duration of individual plastic events, rather than by cascades of correlated ones associated with much longer, shear-rate-dependent timescales or power-law relaxations. Our results are consistent with a recent theoretical framework proposed by Cuny et al., suggesting that residual stress originates from the orientation of the stress tensor.

cond-mat.soft

Bending to kinetic energy transfer in adhesive peel front micro-instability

We report an extensive experimental study of a detachment front dynamics instability, appearing at microscopic scales during the peeling of adhesive tapes. The amplitude of this instability scales with its period as $A_{\text{mss}} \propto T_{\text{mss}}^{1/3}$, with a pre-factor evolving slightly with the peel angle $θ$, and increasing systematically with the bending modulus $B$ of the tape backing. Establishing a local energy budget of the detachment process during one period of this micro-instability, our theoretical model shows that the elastic bending energy stored in the portion of tape to be peeled is converted into kinetic energy, providing a quantitative description of the experimental scaling law.

cond-mat.soft

Sound and light from fractures in scintillators

Prompted by intriguing events observed in certain particle-physics searches for rare events, we study light and acoustic emission simultaneously in some inorganic scintillators subject to mechanical stress. We observe mechanoluminescence in ${Bi}_4{Ge}_{3}{O}_{12}$, ${CdWO}_{4}$ and ${ZnWO}_{4}$, in various mechanical configurations at room temperature and ambient pressure. We analyze how the light emission is correlated to acoustic emission during fracture. For ${Bi}_4{Ge}_{3}{O}_{12}$, we set a lower bound on the energy of the emitted light, and deduce that the fraction of elastic energy converted to light is at least $3 \times 10^{-5}$.

cond-mat.mtrl-sci

Field emission from single and few-layer graphene flakes

We report the observation and characterization of field emission current from individual single- and few-layer graphene flakes laid on a flat SiO2/Si substrate. Measurements were performed in a scanning electron microscope chamber equipped with nanoprobes, used as electrodes to realize local measurements of the field emission current. We achieved field emission currents up to 1 μA from the flat part of graphene flakes at applied fields of few hundred V/μm. We found that emission process is stable over a period of several hours and that it is well described by a Fowler-Nordheim model for currents over 5 orders of magnitude.

cond-mat.mes-hall

Field emission from single multi-wall carbon nanotubes

Electron field emission characteristics of individual multiwalled carbon nanotubes have been investigated by a piezoelectric nanomanipulation system operating inside a scanning electron microscopy chamber. The experimental setup ensures a high control capability on the geometric parameters of the field emission system (CNT length, diameter and anode-cathode distance). For several multiwalled carbon nanotubes, reproducible and quite stable emission current behaviour has been obtained with a dependence on the applied voltage well described by a series resistance modified Fowler-Nordheim model. A turn-on field of about 30 V/um and a field enhancement factor of around 100 at a cathode-anode distance of the order of 1 um have been evaluated. Finally, the effect of selective electron beam irradiation on the nanotube field emission capabilities has been extensively investigated.

cond-mat.mtrl-sci

Local probing of the field emission stability of vertically aligned multiwalled carbon nanotubes

Metallic cantilever in high vacuum atomic force microscope has been used as anode for field emission experiments from densely packed vertically aligned multi-walled carbon nanotubes. The high spatial resolution provided by the scanning probe technique allowed precise setting of the tip-sample distance in the submicron region. The dimension of the probe (curvature radius below 50nm) allowed to measure current contribution from sample areas smaller than 1um^2. The study of long-term stability evidenced that on these small areas the field emission current remains stable (within 10% fluctuations) several hours (at least up to 72 hours) at current intensities between 10-5A and 10-8A. Improvement of the current stability has been observed after performing long-time Joule heating conditioning to completely remove possible adsorbates on the nanotubes.

cond-mat.mtrl-sci

A local field emission study of partially aligned carbon-nanotubes by AFM probe

We report on the application of Atomic Force Microscopy (AFM) for studying the Field Emission (FE) properties of a dense array of long and vertically quasi-aligned multi-walled carbon nanotubes grown by catalytic Chemical Vapor Deposition on a silicon substrate. The use of nanometric probes enables local field emission measurements allowing investigation of effects non detectable with a conventional parallel plate setup, where the emission current is averaged on a large sample area. The micrometric inter-electrode distance let achieve high electric fields with a modest voltage source. Those features allowed us to characterize field emission for macroscopic electric fields up to 250 V/$μ$m and attain current densities larger than 10$^5$ A/cm$^2$. FE behaviour is analyzed in the framework of the Fowler-Nordheim theory. A field enhancement factor $γ\approx$ 40-50 and a turn-on field $E_{turn-on} \sim$15 V/$μ$m at an inter-electrode distance of 1 $μ$m are estimated. Current saturation observed at high voltages in the I-V characteristics is explained in terms of a series resistance of the order of M$Ω$. Additional effects as electrical conditioning, CNT degradation, response to laser irradiation and time stability are investigated and discussed.

cond-mat.mtrl-sci

Discrepancy between sub-critical and fast rupture roughness: a cumulant analysis

We study the roughness of a crack interface in a sheet of paper. We distinguish between slow (sub-critical) and fast crack growth regimes. We show that the fracture roughness is different in the two regimes using a new method based on a multifractal formalism recently developed in the turbulence literature. Deviations from monofractality also appear to be different in both regimes.

cond-mat.stat-mech

Thermal activation of rupture and slow crack growth in a model of homogenous brittle materials

Slow crack growth in a model of homogenous brittle elastic material is described as a thermal activation process where stress fluctuations allow to overcome a breaking threshold through a series of irreversible steps. We study the case of a single crack in a flat sheet for which analytical predictions can be made, and compare them with results from the equivalent problem of a 2D spring network. Good statistical agreement is obtained for the crack growth profile and final rupture time. The specific scaling of the energy barrier with stress intensity factor appears as a consequence of irreversibility. In addition, the model brings out a characteristic growth length whose physical meaning could be tested experimentally.

cond-mat.stat-mech

Mechanism of formation of a 2D binary alloy

Direct comparison of scanning tunneling microscopy and high resolution core level photo-emission experiments provides a rationale for the mechanism of formation of a two dimensional (2D) binary alloy (1/3 mono-layer (ML) Sn(1- x)Six/Si(111)-\sqrt3X\sqrt3R30). In contrast with recent theoretical predictions, the pure metal surface (x=0) results partitioned into two classes (2/9 ML and 1/9 ML) of ad-atoms occupying non-equivalent T4 sites. During the formation of the alloy, Si ad-atoms preferably occupy the majority type adsorption site. This peculiar substitution mechanism leads to a mutual arrangement of ad-atoms which is not random even at room temperature, but shows the typical short range order universally observed in 2D and quasi 2D binary alloys

cond-mat.mtrl-sci