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S. Seo

Publications and source records attributed to S. Seo.

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Quantum Critical Scaling in Quasi-One-Dimensional YbFe$_5$P$_3$

We report measurements of the low temperature magnetization $M$ and specific heat $C$ as a function of temperature and magnetic field of the quasi-one-dimensional spin chain, heavy fermion compound YbFe$_5$P$_3$, which resides close to a quantum critical point. The results are compared to the predictions of scaling laws obtained from a generalized free energy function expected near an antiferromagnetic quantum critical point (AFQCP). The scaling behavior depends on the dimensionality $d$ of the fluctuations, the coherence length exponent $\nu$, and the dynamic exponent $z$. The free energy treats the magnetic field as a relevant renormalization group variable, which leads to a new exponent $\phi=\nu z_h$, where $z_h$ is a dynamic exponent expected in the presence of a magnetic field. When $z_h=z$, $T/H$ scaling is expected, as observed in several compounds close to a QCP; whereas in YbFe$_5$P$_3$, a $T/H^{3/4}$ dependence of the scaling is observed. This dependence reflects the relationship $z_h=(4z/3)$ and a field exponent $\phi =4/3$. A feature of the scaling law is that it restricts the possible values of the exponents to two cases for YbFe$_5$P$_3$: $d$=1, $\nu$=1, $z$=1, and $d$=2, $\nu$=1/2, $z$=2.

cond-mat.str-el

Probing quantum criticality in ferromagnetic CeRh6Ge4

CeRh$_6$Ge$_4$ is unusual in that its ferromagnetic transition can be suppressed continuously to zero temperature, i.e., to a ferromagnetic quantum-critical point (QCP), through the application of modest hydrostatic pressure. This discovery has raised the possibility that the ferromagnetic QCP may be of the Kondo-breakdown type characterized by a jump in Fermi volume, to which thermopower S measurements should be sensitive. Though $S/T$ changes both sign and magnitude around the critical pressure P$_{c}\approx{}0.8$ GPa, these changes are not abrupt but extend over a pressure interval from within the ferromagnetic state up to P$_c$. Together with temperature and pressure variations in electrical resistivity and previously reported heat capacity, thermopower results point to the near coincidence of two sequential effects near P$_c$, delocalization of 4f degrees-of-freedom through orbital-selective hybridization followed by quantum criticality of itinerant ferromagnetism.

cond-mat.str-el

Improved Measurements of Muonic Helium Ground-State Hyperfine Structure at a Near-Zero Magnetic Field

Muonic helium atom hyperfine structure (HFS) measurements are a sensitive tool to test the three-body atomic system and bound-state quantum electrodynamics theory, and determine fundamental constants of the negative muon magnetic moment and mass. The world's most intense pulsed negative muon beam at the Muon Science Facility of the Japan Proton Accelerator Research Complex allows improvement of previous measurements and testing further $CPT$ invariance by comparing the magnetic moments and masses of positive and negative muons (second-generation leptons). We report new ground-state HFS measurements of muonic helium-4 atoms at a near-zero magnetic field, performed for the first time using a small admixture of CH$_{4}$ as an electron donor to form neutral muonic helium atoms efficiently. Our analysis gives $\Delta\nu$ = 4464.980(20) MHz (4.5 ppm), which is more precise than both previous measurements at weak and high fields. The muonium ground-state HFS was also measured under the same conditions to investigate the isotopic effect on the frequency shift due to the gas density dependence in He with CH$_{4}$ admixture and compared with previous studies. Muonium and muonic helium can be regarded as light and heavy hydrogen isotopes with an isotopic mass ratio of 36. No isotopic effect was observed within the current experimental precision.

physics.atom-ph

Development of microwave cavities for measurement of muonium hyperfine structure at J-PARC

The MuSEUM collaboration is planning measurements of the ground-state hyperfine structure (HFS) of muonium at the Japan Proton Accelerator Research Complex (J-PARC), Materials and Life Science Experimental Facility. The high-intensity beam that will soon be available at H-line allows for more precise measurements by one order of magnitude. We plan to conduct two staged measurements. First, we will measure the Mu-HFS in a near-zero magnetic field, and thereafter we will measure it in a strong magnetic field. We have developed two microwave cavities for this purpose. Furthermore, we evaluated systematic uncertainties from such a fluctuation of microwave fields and confirm the requirement of the microwave system, we use a microwave field distribution calculated from the finite element method.

physics.ins-det

Rabi-Oscillation Spectroscopy of the Hyperfine Structure of Muonium Atoms

As a new method to determine the resonance frequency, Rabi-oscillation spectroscopy has been developed. In contrast to the conventional spectroscopy which draws the resonance curve, Rabi-oscillation spectroscopy fits the time evolution of the Rabi oscillation. By selecting the optimized frequency, it is shown that the precision is twice as good as the conventional spectroscopy with a frequency sweep. Furthermore, the data under different conditions can be treated in a unified manner, allowing more efficient measurements for systems consisting of a limited number of short-lived particles produced by accelerators such as muons. We have developed a fitting function that takes into account the spatial distribution of muonium and the spatial distribution of the microwave intensity to apply the new method to ground-state muonium hyperfine structure measurements at zero field. This was applied to the actual measurement data and the resonance frequencies were determined under various conditions. The result of our analysis gives $\nu_{\rm HFS}=4\ 463\ 301.61 \pm 0.71\ {\rm kHz}$, which is the world's highest precision under zero field conditions.

hep-ex

New precise spectroscopy of the hyperfine structure in muonium with a high-intensity pulsed muon beam

A hydrogen-like atom consisting of a positive muon and an electron is known as muonium. It is a near-ideal two-body system for a precision test of bound-state theory and fundamental symmetries. The MuSEUM collaboration performed a new precision measurement of the muonium ground-state hyperfine structure at J-PARC using a high-intensity pulsed muon beam and a high-rate capable positron counter. The resonance of hyperfine transition was successfully observed at a near-zero magnetic field, and the muonium hyperfine structure interval of ${\nu}_{\text{HFS}}$ = 4.463302(4) GHz was obtained with a relative precision of 0.9 ppm. The result was consistent with the previous ones obtained at Los Alamos National Laboratory and the current theoretical calculation. We present a demonstration of the microwave spectroscopy of muonium for future experiments to achieve the highest precision.

hep-ex

Nematic state in CeAuSb$_{2}$

At ambient pressure and zero field, tetragonal CeAuSb$_{2}$ hosts stripe antiferromagnetic order at $T_{N} = 6.3$ K. Here we first show via bulk thermodynamic probes and x-ray diffraction measurements that this magnetic order is connected with a structural phase transition to a superstructure which likely breaks $C_{4}$ symmetry, thus signaling nematic order. The temperature-field-pressure phase diagram of CeAuSb$_{2}$ subsequently reveals the emergence of additional ordered states under applied pressure at a multicritical point. Our phenomenological model supports the presence of a vestigial nematic phase in CeAuSb$_{2}$ akin to iron-based high-temperature superconductors; however, superconductivity, if present, remains to be discovered.

cond-mat.str-el

Disorder in a Quantum Critical Superconductor

In four classes of materials, the layered copper-oxides, organics, iron-pnictides and heavy-fermion compounds, an unconventional superconducting state emerges as a magnetic transition is tuned toward absolute zero temperature, that is, toward a magnetic quantum-critical point (QCP). In most materials, the QCP is accessed by chemical substitutions or applied pressure. CeCoIn5 is one of the few materials that are born as a quantum-critical superconductor and, therefore, offers the opportunity to explore the consequences of chemical disorder. Cadmium-doped crystals of CeCoIn5 are a particularly interesting case where Cd substitution induces long-range magnetic order, as in Zn-doped copper-oxides. Applied pressure globally supresses the Cd-induced magnetic order and restores bulk superconductivity. Here we show, however, that local magnetic correlations, whose spatial extent decreases with applied pressure, persist at the extrapolated QCP. The residual droplets of impurity-induced magnetic moments prevent the reappearance of conventional signatures of quantum criticality, but induce a heterogeneous electronic state. These discoveries show that spin droplets can be a source of electronic heterogeneity in classes of strongly correlated electron systems and emphasize the need for caution when interpreting the effects of tuning a correlated system by chemical substitution.

cond-mat.supr-con

Nanoscale Topographical Replication of Graphene Architecture by Artificial DNA nanostructures

Despite many studies on how geometry can be used to control the electronic properties of graphene, certain limitations to fabrication of designed graphene nanostructures exist. Here, we demonstrate controlled topographical replication of graphene by artificial deoxyribonucleic acid (DNA) nanostructures. Owing to the high degree of geometrical freedom of DNA nanostructures, we controlled the nanoscale topography of graphene. The topography of graphene replicated from DNA nanostructures showed enhanced thermal stability and revealed an interesting negative temperature coefficient of sheet resistivity when underlying DNA nanostructures were denatured at high temperatures.

cond-mat.mes-hall

Effects of pressure on the ferromagnetic state of the CDW compound SmNiC2

We report the pressure response of charge-density-wave (CDW) and ferromagnetic (FM) phases of the rare-earth intermetallic SmNiC2 up to 5.5 GPa. The CDW transition temperature (T_{CDW}), which is reflected as a sharp inflection in the electrical resistivity, is almost independent of pressure up to 2.18 GPa but is strongly enhanced at higher pressures, increasing from 155.7 K at 2.2 GPa to 279.3 K at 5.5 GPa. Commensurate with the sharp increase in T_{CDW}, the first-order FM phase transition, which decreases with applied pressure, bifurcates into the upper (T_{M1}) and lower (T_c) phase transitions and the lower transition changes its nature to second order above 2.18 GPa. Enhancement both in the residual resistivity and the Fermi-liquid T^2 coefficient A near 3.8 GPa suggests abundant magnetic quantum fluctuations that arise from the possible presence of a FM quantum critical point.

cond-mat.str-el

Breakdown of the interlayer coherence in twisted bilayer graphene

Coherent motion of the electrons in the Bloch states is one of the fundamental concepts of the charge conduction in solid state physics. In layered materials, however, such a condition often breaks down for the interlayer conduction, when the interlayer coupling is significantly reduced by e.g. large interlayer separation. We report that complete suppression of coherent conduction is realized even in an atomic length scale of layer separation in twisted bilayer graphene. The interlayer resistivity of twisted bilayer graphene is much higher than the c-axis resistivity of Bernal-stacked graphite, and exhibits strong dependence on temperature as well as on external electric fields. These results suggest that the graphene layers are significantly decoupled by rotation and incoherent conduction is a main transport channel between the layers of twisted bilayer graphene.

cond-mat.mes-hall

Pressure effects on the heavy-fermion antiferromagnet CeAuSb2

The f-electron compound CeAuSb2, which crystallizes in the ZrCuSi2-type tetragonal structure, orders antiferromagnetically between 5 and 6.8 K, where the antiferromagnetic transition temperature T_N depends on the occupancy of the Au site. Here we report the electrical resistivity and heat capacity of a high-quality crystal CeAuSb2 with T_N of 6.8 K, the highest for this compound. The magnetic transition temperature is initially suppressed with pressure, but is intercepted by a new magnetic state above 2.1 GPa. The new phase shows a dome shape with pressure and coexists with another phase at pressures higher than 4.7 GPa. The electrical resistivity shows a T^2 Fermi liquids behavior in the complex magnetic state, and the residual resistivity and the T^2 resistivity coefficient increases with pressure, suggesting the possibility of a magnetic quantum critical point at a higher pressure.

cond-mat.str-el

Non-monotonic temperature dependent transport in graphene grown by Chemical Vapor Deposition

Temperature-dependent resistivity of graphene grown by chemical vapor deposition (CVD) is investigated. We observe in low mobility CVD graphene device a strong insulating behavior at low temperatures and a metallic behavior at high temperatures manifesting a non-monotonic in the temperature dependent resistivity.This feature is strongly affected by carrier density modulation. To understand this anomalous temperature dependence, we introduce thermal activation of charge carriers in electron-hole puddles induced by randomly distributed charged impurities. Observed temperature evolution of resistivity is then understood from the competition among thermal activation of charge carriers, temperature-dependent screening and phonon scattering effects. Our results imply that the transport property of transferred CVD-grown graphene is strongly influenced by the details of the environment

cond-mat.mes-hall

Scaling behaviors of RESET voltages and currents in unipolar resistance switching

Unipolar switching phenomena have attracted a great deal of recent attention, but the wide distributions of switching voltages still pose major obstacles for scientific advancement and practical applications. Using NiO capacitors, we investigated the distributions of the RESET voltage and current. We found that they scaled with the resistance value Ro in the low resistance state, and that the scaling exponents varied at Ro = 30 Ohm. We explain these intriguing scaling behaviors and their crossovers by analogy with percolation theory. We show that the connectivity of conducting filaments plays a crucial role in the RESET process.

cond-mat.mtrl-sci

Strong resistance nonlinearity and third harmonic generation in the unipolar resistance switching of NiO thin films

We investigated third harmonic generation in NiO thin films, which exhibit unipolar resistance switching behavior. We found that the low resistance states of the films were strongly nonlinear, with variations in the resistance R as large as 60%. This strong nonlinear behavior was most likely caused by Joule heating of conducting filaments inside the films. By carefully controlling the applied dc bias, we obtained several low resistance states, whose values of the third harmonic coefficient B3f were proportional to R2+w (with w = 2.07). This suggested that the resistance changes of the NiO films were accompanied by connectivity changes of the conducting filaments, as observed in classical percolating systems.

cond-mat.mtrl-sci

Abnormal Resistance Switching Behaviors of NiO Thin Films: Possible Occurrence of Simultaneous Formation and Rupture of Conducting Channels

We report the detailed current-voltage (I-V) characteristics of resistance switching in NiO thin films. In unipolar resistance switching, it is commonly believed that conducting filaments will rupture when NiO changes from a low resistance to a high resistance state. However, we found that this resistance switching can sometimes show abnormal behavior during voltage- and current-driven I-V measurements. We used the random circuit breaker network model to explain how abnormal switching behaviors could occur. We found that this resistance change can occur via a series of avalanche processes, where conducting filaments could be formed as well as ruptured.

cond-mat.mtrl-sci