arXiv subjects

S. Uchida

Publications and source records attributed to S. Uchida.

At least 109 records · Page 6Linked to original sources

arXiv2006

Experimental evidence of paired hole states in model high-$T_c$ compounds

The distribution of holes in Sr$_{14-x}$Ca$_x$Cu$_{24}$O$_{41}$ (SCCO) is revisited with semi-emperical reanalysis of the x-ray absorption (XAS) data and exact-diagonalized cluster calculations. A new interpretation of the XAS data leads to much larger ladder hole densities than previously suggested. These new hole densities lead to a simple interpretation of the hole crystal (HC) recently reported with 1/3 and 1/5 wave vectors along the ladder. Our interpretation is consistent with paired holes in the rung of the ladders. Exact diagonalization results for a minimal model of the doped ladders suggest that the stabilization of spin structures consisting of 4 spins in a square plaquette as a result of resonance valence bond (RVB) physics suppresses the hole crystal with a 1/4 wave vector.

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arXiv2005

Quantum melting of the hole crystal in the spin ladder of Sr14-xCaxCu24O41

The "spin ladder" is a reduced-dimensional analogue of the high temperature superconductors that was predicted to exhibit both superconductivity and an electronic charge density wave or "hole crystal" (HC). Both phenomena have been observed in the doped spin ladder system Sr14-xCaxCu24O41 (SCCO), which at x=0 exhibits a HC which is commensurate at all temperatures. To investigate the effects of discommensuration we used resonant soft x-ray scattering (RSXS) to study SCCO as a function of doped hole density, d. The HC forms only with the commensurate wave vectors L_L = 1/5 and L_L = 1/3 and exhibits a simple temperature scaling T_(1/3) / T_(1/5) = 5/3. For irrational wave vectors the HC "melts", perhaps through the motion of topological defects carrying fractional charge.

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arXiv2005

Doping Evolution of the Underlying Fermi Surface in La2-xSrxCuO4

We have performed a systematic doping dependent study of La$_{2-x}$Sr$_x$CuO$_4$ (LSCO) (0.03$\leq x \leq$0.3) by angle-resolved photoemission spectroscopy. In the entire doping range, the underlying ``Fermi surface" determined from the low energy spectral weight approximately satisfies Luttinger's theorem, even down to the lightly-doped region. This is in strong contrast to the result on Ca$_{2-x}$Na$_x$CuO$_2$Cl$_2$ (Na-CCOC), which shows a strong deviation from Luttinger's theorem. The differences between LSCO and Na-CCOC are correlated with the different behaviors of the chemical potential shift and spectral weight transfer induced by hole doping.

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arXiv2005

Field-enhanced diamagnetism in intense magnetic field in the pseudogap state of the cuprate $\rm Bi_2Sr_2CaCu_2O_{8+δ}

In hole-doped cuprates, Nernst experiments imply that the superconducting state is destroyed by spontaneous creation of vortices which destroy phase coherence. Using torque magnetometry on $\rm Bi_2Sr_2CaCu_2O_{8+δ}$, we uncover a field-enhanced diamagnetic signal $M$ above the transition temperature $T_c$ that increases with applied field to 32 Tesla and scales just like the Nernst signal. The magnetization results above $T_c$ distinguish $M$ from conventional amplitude fluctuations, and strongly support the vortex scenario for the loss of phase coherence at $T_c$.

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arXiv2005

Muon Spin Relaxation Studies of Magnetic-Field-Induced Effects in High-$T_{c}$ Superconductors

Muon spin relaxation ($μ$SR) measurements in high transverse magnetic fields ($\parallel \hat c$) revealed strong field-induced quasi-static magnetism in the underdoped and Eu doped (La,Sr)$_{2}$CuO$_{4}$ and La$_{1.875}$Ba$_{0.125}$CuO$_{4}$, existing well above $T_{c}$ and $T_{N}$. The susceptibility-counterpart of Cu spin polarization, derived from the muon spin relaxation rate, exhibits a divergent behavior towards $T \sim 25$ K. No field-induced magnetism was detected in overdoped La$_{1.81}$Sr$_{0.19}$CuO$_{4}$, optimally doped Bi2212, and Zn-doped YBa$_{2}$Cu$_{3}$O$_{7}$.

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arXiv2005

Effect of disorder outside the CuO$_{2}$ planes on $T_{c}$ of copper oxide superconductors

The effect of disorder on the superconducting transition temperature $T_{c}$ of cuprate superconductors is examined. Disorder is introduced into the cation sites in the plane adjacent to the CuO$_{2}$ planes of two single-layer systems, Bi$_{2.0}$Sr$_{1.6}$Ln$_{0.4}$CuO$_{6+δ}$ and La$_{1.85-y}$Nd$_{y}$Sr$_{0.15}$CuO$_{4}$. Disorder is controlled by changing rare earth (Ln) ions with different ionic radius in the former, and by varying the Nd content in the latter with the doped carrier density kept constant. We show that this type of disorder works as weak scatterers in contrast to the in-plane disorder produced by Zn, but remarkably reduces $T_{c}$ suggesting novel effects of disorder on high-$T_{c}$ superconductivity.

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arXiv2005

Multiple Bosonic Mode Coupling in Electron Self-Energy of (La_2-xSr_x)CuO_4

High resolution angle-resolved photoemission spectroscopy data along the (0,0)-($π$,$π$) nodal direction with significantly improved statistics reveal fine structure in the electron self-energy of the underdoped (La$_{2-x}$Sr$_x$)CuO$_4$ samples in the normal state. Fine structure at energies of (40$\sim$46) meV and (58$\sim$63)meV, and possible fine structure at energies of (23$\sim$29)meV and (75$\sim$85)meV, have been identified. These observations indicate that, in LSCO, more than one bosonic modes are involved in the coupling with electrons.

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arXiv2005

Polaronic behavior of undoped high-Tc cuprates

We present angle-resolved photoemission spectroscopy (ARPES) data on undoped La2CuO4, indicating polaronic coupling between bosons and charge carriers. Using a shell model, we calculate the electron-phonon coupling and find that it is strong enough to give polarons. We develop an efficient method for calculating ARPES spectra in undoped systems. Using the calculated couplings, we find the width of the phonon side band in good agreement with experiment. We analyze reasons for the observed dependence of the width on the binding energy.

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arXiv2004

High Pressure Study of Structural Phase Transitions and Superconductivity in La1.48Nd0.4Sr0.12CuO4

We have determined the crystal structures and superconducting transition temperatures of La1.48Nd0.4Sr0.12CuO4 under nearly hydrostatic pressures in diamond anvil cells to 5.0 GPa and 19.0 GPa, respectively. Synchrotron x-ray powder diffraction measurements were used to establish the pressure-temperature structural phase diagram. Under pressure the superconducting transition temperature increases rapidly from Tc = 3 K to a maximum value of 22 K at 5 GPa, a pressure slightly greater than that required to stabilize the undistorted I4/mmm structure in the superconducting state. Increasing the pressure further to 19 GPa leads to a decrease in Tc to ~12 K. These results are discussed in relation to earlier high pressure measurements for similar materials.

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arXiv2004

Molecular orbital excitations in cuprates

We report resonant inelastic x-ray scattering studies of electronic excitations in a wide variety of cuprate compounds. Specifically, we focus on the charge-transfer type excitation of an electron from a bonding molecular orbital to an antibonding molecular orbital in a copper oxygen plaquette. Both the excitation energy and the amount of dispersion are found to increase significantly as the copper oxygen bond-length is reduced. We also find that the estimated bond-length dependence of the hopping integral t_pd is much stronger than that expected from tight-binding theory.

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arXiv2004

Asymmetries in the electron-hole pair dynamics and strong Mott pseudogap effect in the phase diagram of cuprates

Electron behavior in doped Mott systems continues to be a major unsolved problem in quantum many-electron physics. A central issue in understanding the universal Mott behavior in a variety of complex systems is to understand the nature of their electron-hole pair excitation modes. Using high resolution resonant inelastic x-ray scattering (RIXS) we resolve the momentum dependence of electron-hole pair excitations in two major classes of doped copper oxides which reveals a Mott pseudogap over the full Brillouin zone and over the entire phase diagram. The pair bandwidth and zone-boundary pair velocity renormalize on either sides of the phase diagram at very different rates indicating strong particle-hole doping asymmetries observed for the first time.

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arXiv2004

Destruction of antinodal state coherence via `checkerboard' charge ordering in strongly underdoped superconducting BSCCO-2212

Microscopy (STM). At all dopings, the low energy density-of-states modulations are analyzed according to a simple model of quasiparticle interference and found to be consistent with Fermi-arc superconductivity. The superconducting coherence-peaks, ubiquitous in near-optimal tunneling spectra, are destroyed with strong underdoping and a new spectral type appears. Exclusively in regions exhibiting this new spectrum, we find local `checkerboard' charge-order with wavevector Q=(2pi/4.5a,0);(0,2pi/4.5a)+15%. Surprisingly, this order coexists harmoniously with the the low energy

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arXiv2004

Homogenous nodal superconductivity coexisting with inhomogeneous charge order in strongly underdoped Bi-2212

We use novel STM techniques in concert to study the doping dependence of electronic structure in Bi-2212. At all dopings, the low energy states are relatively homogenous except for dispersive density-of-states modulations whose properties are used to elucidate the momentum-space characteristics of quasi-particles. The superconductive coherence-peaks, ubiquitous in near-optimal tunneling spectra, are destroyed with strong underdoping. A new spectral type, likely characteristic of the zero temperature pseudogap regime, appears in these samples. Exclusively in regions exhibiting this new spectrum, we find a quasi periodic modulations in dI/dV as well as in topograph with Q(2pi/4.5a,0) and (0,2pi/4.5a)+-15%. This is consistent with the existence of a local charge density modulation at these wave vectors. Surprisingly, this state coexists harmoniously with the low energy nodal quasi-particles. We discuss the relevance of these findings to the cuprate phase diagram and to the relationship between the pseudogap and superconductivity.

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arXiv2004

Site-Dilution in quasi one-dimensional antiferromagnet Sr2(Cu1-xPdx)O3: reduction of Neel Temperature and spatial distribution of ordered moment sizes

We investigate the Neel temperature of Sr2CuO3 as a function of the site dilution at the Cu (S=1/2) sites with Pd (S=0), utilizing the muon spin relaxation (muSR) technique. The Neel temperature, which is Tn=5.4K for the undoped system, becomes significantly reduced for less than one percent of doping Pd, giving a support for the previous proposal for the good one-dimensionality. The Pd concentration dependence of the Neel temperature is compared with a recent theoretical study (S. Eggert, I. Affleck and M.D.P. Horton, Phys. Rev. Lett. 89, 47202 (2002)) of weakly coupled one-dimensional antiferromagnetic chains of S=1/2 spins, and a quantitative agreement is found. The inhomogeneity of the ordered moment sizes is characterized by the muSR time spectra. We propose a model that the ordered moment size recovers away from the dopant S=0 sites with a recovery length of ξ= 150-200 sites. The origin of the finite recovery length ξfor the gapless S=1/2 antiferromagnetic chain is compared to the estimate based on the effective staggered magnetic field from the neighboring chains.

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arXiv2004

The Dichotomy between Nodal and Antinodal Quasiparticles in Underdoped (La$_{2-x}$Sr$_x$)CuO$_4$ Superconductors

High resolution angle-resolved photoemission measurements on underdoped (La$_{2-x}$Sr$_x$)CuO$_4$ system show that, at energies below 70 meV, the quasiparticle peak is well defined around the ($π$/2,$π$/2) nodal region and disappears rather abruptly when the momentum is changed from the nodal point to the ($π$,0) antinodal point along the underlying ``Fermi surface''. It indicates that there is an extra low energy scattering mechanism acting upon the antinodal quasiparticles. We propose that this mechanism is the scattering of quasiparticles across the nearly parallel segments of the Fermi surface near the antinodes.

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arXiv2004

Expansion of Vortex Cores by Strong Electronic Correlation in La$_{2-x}$Sr$_x$CuO$_4$ at Low Magnetic Induction

The vortex core radius \rv, defined as the peak position of the supercurrent around the vortex, has been determined by muon spin rotation measurements in the mixed state of \lscox for $x=0.13$, 0.15, and 0.19. At lower doping (x=0.13 and 0.15), \rv(T) increases with decreasing temperature T, which is opposite to the behavior predicted by the conventional theory. Moreover, \rv(T\to0) is significantly larger than the Ginsburg-Landau coherence length determined by the upper critical field, and shows a clear tendency to decrease with increasing the doping x. These features can be qualitatively reproduced in a microscopic model involving antiferromagnetic electronic correlations.

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arXiv2004

Thermodynamic and transport properties of underdoped cuprates from ARPES data

he relationship between photoemission spectra of high-$T_{\textrm{c}}$ cuprates and their thermodynamic and transport properties are discussed. The doping dependence of the expected quasi-particle density at the Fermi level ($E_\mathrm{F}$) are compared with the electronic specific heat coefficient $γ$ and that of the spectral weight at $E_\mathrm{F}$ with the in-plane and out-of-plane superfluid density. We have estimated the electrical resistivity of underdoped cuprates from the momentum distribution curve (MDC) at $E_\mathrm{F}$ in the nodal direction. The temperature dependence of the MDC width is also consistent with that of the electrical resistivity.

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arXiv2004

In-plane optical conductivity of La$_{2-x}$Sr$_x$CuO$_4$: Reduced superconducting condensate and residual Drude-like response

Temperature dependences of the optical spectra of La$_{2-x}$Sr$_x$CuO$_4$ with $x$=0.12 and 0.15 were carefully examined for a polarization parallel to the CuO$_2$-plane over a wide frequency range down to 8 cm$^{-1}$. Selection of well-characterized crystals enabled us to measure purely in-plane polarized spectra without any additional peak. The weight of superconducting (SC) condensate estimated from the missing area in $σ_1(ω$) well agrees with the estimate from the slope of $σ_2(ω$) vs 1/$ω$ plot, showing no evidence that the Ferrell-Glover-Tinkham sum-rule is violated in the optical spectrum. We demonstrate that the optically estimated SC condensate is much smaller than the value obtained from the $μ$SR measurement of magnetic penetration depth. We also find an anomalous increase of conductivity in sub-millimeter region towards $ω$=0 below $T_c$, which suggests the microscopic inhomogeneity in the superconducting state. Both observations are discussed in relation with the inhomogeneous electronic state that might be inherent to high-$T_c$ cuprates.

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