arXiv subjects

S. W. Finch

Publications and source records attributed to S. W. Finch.

10 recordsLinked to original sources

arXiv2026

A detailed view at magnetic dipole strengths: The case of semi-magic $^{50}$Ti

Magnetic dipole, $M1$, strengths were studied in semi-magic $^{50}$Ti up to the neutron-separation threshold by combining data from $(d,p)$ one-neutron transfer, $(γ,γ')$ real-photon scattering, $(e,e')$ inelastic scattering at extreme backward angles, and $(p,p')$ at $E_p = 210$ MeV and extreme forward angles. The combination of all probes provided unique access to the neutron spin-flip contribution and the possibility to evaluate its role in generating the spin-flip $M1$ strengths. The small contribution of the neutron $(1f_{7/2})^{-1}(1f_{5/2})^{+1}$ spin-flip transitions, which were probed with the $(d,p)$ reaction, to the overall strength in $^{50}$Ti questions the standard picture for the microscopic origin of spin-flip strength in the $fp$ shell. For $^{50}$Ti, this letter shows that $J^π = 1^+$ states with larger neutron $(1f_{7/2})^{-1}(1f_{5/2})^{+1}$ spectroscopic factors do not correspond to the ones with the largest $B(M1;0^+_1 \rightarrow 1^+_i)$ strengths.

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arXiv2026

Photonuclear Cross Sections for the $^{197}$Au($γ$,pn)$^{195m}$Pt Reaction Near Threshold

Platinum radioisotopes are of growing interest for targeted cancer therapy and diagnostic imaging because their decay delivers highly localized radiation doses in tissue, herewith enabling precise DNA damage through Auger-electron emission. Developing production technologies that provide platinum isotopes with high specific activity is therefore essential, and photonuclear reactions on stable nuclei offer a viable accelerator-based route when supported by reliable cross-section data. We report photonuclear cross-section measurements for the $^{197}$Au($γ$,pn)$^{195m}$Pt reaction at incident $γ$-ray energies of 27, 29, and 31 MeV using the activation method. The measurements were performed by irradiating a stack of concentric-ring gold targets with a quasi-monoenergetic $γ$-ray beam provided by the High Intensity Gamma-ray Source (HI$γ$S). The induced $^{195m}$Pt activity was quantified using off-line $γ$-ray spectroscopy. These data provide the first experimental constraints on the $^{197}$Au($γ$,pn)$^{195m}$Pt cross section in the near-threshold region. The measured excitation function is compared with PHITS and TALYS calculations and indicates that the reaction becomes measurable only near 30 MeV, with substantially higher bremsstrahlung end-point energies required for practically meaningful production.

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arXiv2026

Core Breaking at Low Spin in $^{68}$Zn from Nuclear Resonance Fluorescence

Low-spin excited states in $^{68}$Zn have been studied at the High Intensity Gamma-Ray Source (HI$γ$S) from the ground state up to the particle emission threshold using the nuclear resonance fluorescence technique (NRF) and the newly developed Clover Array. Low-spin levels were excited by linearly-polarized, $2.90 - 9.79$ MeV photon beams. Spin-parity quantum numbers as well as associated $M1$ and $E1$ decay strengths were determined for a large fraction of the 158 states observed. In addition, long-duration coincidence measurements at 9.46 and 9.79 MeV enabled the investigation of the level scheme near the ground state. The results have been interpreted with shell-model calculations using two different model spaces and several effective interactions often used to describe nuclei in this mass region. While the structure near the ground state can be understood in terms of excitations involving solely valence nucleons, core breaking is required to account for the evolution of the total $M1$ strength at excitation energies above $\sim5$ MeV.

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arXiv2026

Enhanced sensitivity to trace $^{238}$U impurity of sapphire via coincidence neutron activation analysis

Sapphire has mechanical and electrical properties that are advantageous for the construction of internal components of radiation detectors such as time projection chambers and bolometers. However, it has proved difficult to assess its $\rm ^{232}Th$ and $\rm ^{238}U$ content down to the picogram per gram level. This work reports an experimental verification of a computational study that demonstrates $γγ$ coincidence counting, coupled with neutron activation analysis (NAA), can reach ppt sensitivities. Combining results from $γγ$ coincidence counting with those of earlier single-$γ$ counting based NAA shows that a sample of Saint Gobain sapphire has $\rm ^{232}Th$ and $\rm ^{238}U$ concentrations of $<0.26$ ppt and $<2.3$ ppt, respectively; the best constraints on the radiopurity of sapphire.

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arXiv2025

Deviations from the Porter-Thomas Distribution due to Nonstatistical $γ$ Decay below the $^{150}$Nd Neutron Separation Threshold

We introduce a new method for the study of fluctuations of partial transition widths based on nuclear resonance fluorescence experiments with quasimonochromatic linearly polarized photon beams below particle separation thresholds. It is based on the average branching of decays of $J=1$ states of an even-even nucleus to the $2^+_1$ state in comparison to the ground state. Between 5 and 7 MeV, a constant average branching ratio for $γ$ decays from $1^-$ states of 0.490(16) is observed for the nuclide $^{150}$Nd. Assuming $χ^2$-distributed partial transition widths, this average branching ratio is related to a degree of freedom of $ν= 1.93(12)$, rejecting the validity of the Porter-Thomas distribution, requiring $ν=1$. The observed deviation can be explained by nonstatistical effects in the $γ$-decay behavior with contributions in the range of 9.4(10)% up to 94(10)%.

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arXiv2025

Gamma decay of the $^{154}$Sm Isovector Giant Dipole Resonance: Smekal-Raman Scattering as a Novel Probe of Nuclear Ground-State Deformation

Gamma decays of the isovector giant dipole resonance (GDR) of the deformed nucleus $^{154}$Sm from $2^+_1$-Smekal-Raman and elastic scattering were measured using linearly polarized, quasimonochromatic photon beams. The two scattering processes were disentangled through their distinct angular distributions. Their branching ratio and cross sections were determined at six excitation energies covering the $^{154}$Sm GDR. Both agree with the predictions of the geometrical model for the GDR and establish $γ$ decay as an observable sensitive to the structure of the resonance. Consequently, the data place strong constraints on the nuclear shape, including the degree of triaxiality. The derived $^{154}$Sm shape parameters $β=0.2926(26)$ and $γ=5.0(14)$ agree well with other measurements and recent Monte Carlo Shell-Model calculations.

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arXiv2023

The earliest DT nuclear fusion discoveries

We describe the earliest measurements of the DT fusion cross section commissioned by the Manhattan Project, first at Purdue University in 1943 and then at Los Alamos 1945-6 and later, in 1951-2. The Los Alamos measurements led to the realization that a 3/2$^+$ resonance in the DT system enhances the fusion cross section by a factor of one hundred at energies relevant to applications. This was a transformational discovery, making the quest for terrestrial fusion energy possible. The earliest measurements were reasonably accurate given the technology of the time and the scarcity of tritium, and were quickly improved to provide cross section data accurate to just a few percent. We provide a previously-unappreciated insight: that DT fusion was first reported in Ruhlig's 1938 University of Michigan experiment and likely influenced Konopinski in 1942 to suggest its usefulness for thermonuclear technologies. We report on preliminary work to repeat the 1938 measurement, and our simulations of that experiment. We also present some work by Fermi, from his 1945 Los Alamos lectures, showing that he used the S-factor concept about a decade before it was introduced by nuclear astrophysicists.

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arXiv2022

Model-independent determination of the dipole response of $^{66}$Zn using quasi-monoenergetic and linearly-polarized photon beams

[Background] Photon strength functions are an important ingredient in calculations relevant for the nucleosynthesis of heavy elements. The relation to the photoabsorption cross section allows to experimentally constrain photon strength functions by investigating the photo-response of atomic nuclei. [Purpose] We determine the photoresponse of $^{66}$Zn in the energy region of 5.6 MeV to 9.9 MeV and analyze the contribution of the "elastic" decay channel back to the ground state. In addition, for the elastic channel electric and magnetic dipole transitions were separated. [Methods] Nuclear resonance fluorescence experiments were performed using a linearly-polarized quasi-monoenergetic photon beam at the High Intensity $γ$-ray Source. Photon beam energies from 5.6 to 9.9 MeV with an energy spread of about 3% were selected in steps of 200-300 keV. Two High Purity Germanium detectors were used for the subsequent $γ$-ray spectroscopy. [Results] Full photoabsorption cross sections are extracted from the data making use of the monoenergetic character of the photon beam. For the ground-state decay channel, the average contribution of electric and magnetic dipole strengths is disentangled. The average branching ratio back to the ground state is determined as well. [Conclusions] The new results indicate lower cross sections when compared to the values extracted from a former experiment using bremsstrahlung on $^{66}$Zn. In the latter, the average branching ratio to the ground state is estimated from statistical-model calculations in order to analyze the data. Corresponding estimates from statistical-model calculations underestimate this branching ratio compared to the values extracted from the present analysis, which would partly explain the high cross sections determined from the bremsstrahlung data.

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arXiv2022

Neutral-current neutrino cross section and expected supernova signals for $^{40}$Ar from a three-fold increase in the magnetic dipole strength

In view of the great interest in liquid argon neutrino detectors, the $^{40}$Ar($γ,γ'$)$^{40}$Ar$^{*}$ reaction was revisited to guide a calculation of the neutral current neutrino cross section at supernova energies. Using the nuclear resonance fluorescence technique with a monoenergetic, 99% linearly polarized photon beam, we report a three-fold increase in magnetic dipole strength at around 10 MeV in $^{40}$Ar. Based on shell-model calculations, and using the experimentally identified transitions, the neutral current neutrino cross sections for low-energy reactions on $^{40}$Ar are calculated.

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arXiv2020

Structure of high-lying levels populated in the $^{96}$Y $\rightarrow ^{96}$Zr $β$ decay

The nature of $J^π=1^-$ levels of $^{96}$Zr below the $β$-decay $Q_β$ value of $^{96}$Y has been investigated in high-resolution $γ$-ray spectroscopy following the $β$ decay as well as in a campaign of inelastic photon scattering experiments. Branching ratios extracted from $β$ decay allow the absolute $E1$ excitation strength to be determined for levels populated in both reactions. The combined data represents a comprehensive approach to the wavefunction of $1^-$ levels below the $Q_β$ value, which are investigated in the theoretical approach of the Quasiparticle Phonon Model. This study clarifies the nuclear structure properties associated with the enhanced population of high-lying levels in the $^{96}$Y$_{gs}$ $β$ decay, one of the three most important contributors to the high-energy reactor antineutrino spectrum.

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