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Sang-Yun Lee

Publications and source records attributed to Sang-Yun Lee.

27 records · Page 2Linked to original sources

Robustness of reference-frame-independent quantum key distribution against the relative motion of the reference frames

Reference-Frame-Independent quantum key distribution (RFI-QKD) is known to be robust against slowly varying reference frames. However, other QKD protocols such as BB84 can also provide secrete keys if the speed of the relative motion of the reference frames is slow enough. While there has been a few studies to quantify the speed of the relative motion of the reference frames in RFI- QKD, it is not yet clear if RFI-QKD provides better performance than other QKD protocols under this condition. Here, we analyze and compare the security of RFI-QKD and BB84 protocol in the presence of the relative motion of the reference frames. In order to compare their security in real world implementation, we also consider the QKD protocols with decoy state method. Our analysis shows that RFI-QKD provides more robustness than BB84 protocol against the relative motion of the reference frames.

quant-ph↗

Vector magnetometry using silicon vacancies in 4H-SiC at ambient conditions

Point defects in solids promise precise measurements of various quantities. Especially magnetic field sensing using the spin of point defects has been of great interest recently. When optical readout of spin states is used, point defects achieve optical magnetic imaging with high spatial resolution at ambient conditions. Here, we demonstrate that genuine optical vector magnetometry can be realized using the silicon vacancy in SiC, which has an uncommon S=3/2 spin. To this end, we develop and experimentally test sensing protocols based on a reference field approach combined with multi frequency spin excitation. Our works suggest that the silicon vacancy in an industry-friendly platform, SiC, has potential for various magnetometry applications at ambient conditions.

cond-mat.mes-hall↗

Vector magnetometry based on S=3/2 electronic spins

Electronic spin systems with S>1/2 provide an efficient method for DC vector magnetometry, since the conventional electron spin resonance spectra at a given magnetic field reflect not only the field strength but also orientation in the presence of strong spin-spin interactions. S=1 spins, e.g. the nitrogen-vacancy centers in diamond, have been intensively investigated for such a purpose. In this report, we compare S=1 and S=3/2 spins, and discuss how one can apply general principles for the use of high spin systems as a vector magnetometer to the S=3/2 spin systems. We find analytical solutions which allow a reconstruction of the magnetic field strength and polar angle using the observed resonance transitions if an uniaxial symmetry exists for the spin-spin interaction as in S=1 systems. We also find that an ambiguity of determining the field parameters may arise due to the unique properties of S=3/2 systems, and present solutions for it utilizing additional transitions in the low-field region. The electronic spins of the silicon vacancy in silicon carbide will be introduced as a model for the S=3/2 DC vector magnetometer and the practical usage of it, including the magic-angle spinning type method, will be presented too.

cond-mat.mes-hall↗

Faraday Filtering on the Cs-D$_1$-Line for Quantum Hybrid Systems

Narrow-band filtering of light is widely used in optical spectroscopy. Atomic filters, which rely on the Faraday effect, allow for GHz-wide transmission spectra, which are intrinsically matched to an atomic transition. We present an experimental realization and a theoretical study of a Faraday anomalous dispersion optical filter (FADOF) based on cesium and its D$_1$-line-transition ($6^2S_{1/2}\rightarrow6^2P_{1/2}$) around 894nm. We also present the prospects and visions for combining this filter with the single photon emission of a single quantum dot (QD), which matches with the atomic transition.

physics.atom-ph↗

Single Molecule DNA Detection with an Atomic Vapor Notch Filter

The detection of single molecules has facilitated many advances in life- and material-sciences. Commonly, it founds on the fluorescence detection of single molecules, which are for example attached to the structures under study. For fluorescence microscopy and sensing the crucial parameters are the collection and detection efficiency, such that photons can be discriminated with low background from a labeled sample. Here we show a scheme for filtering the excitation light in the optical detection of single stranded labeled DNA molecules. We use the narrow-band filtering properties of a hot atomic vapor to filter the excitation light from the emitted fluorescence of a single emitter. The choice of atomic sodium allows for the use of fluorescent dyes, which are common in life-science. This scheme enables efficient photon detection, and a statistical analysis proves an enhancement of the optical signal of more than 15% in a confocal and in a wide-field configuration.

physics.optics↗

Coherent control of single spins in silicon carbide at room temperature

Spins in solids are cornerstone elements of quantum spintronics. Leading contenders such as defects in diamond, or individual phosphorous dopants in silicon have shown spectacular progress but either miss established nanotechnology or an efficient spin-photon interface. Silicon carbide (SiC) combines the strength of both systems: It has a large bandgap with deep defects and benefits from mature fabrication techniques. Here we report the characterization of photoluminescence and optical spin polarization from single silicon vacancies in SiC, and demonstrate that single spins can be addressed at room temperature. We show coherent control of a single defect spin and find long spin coherence time under ambient conditions. Our study provides evidence that SiC is a promising system for atomic-scale spintronics and quantum technology.

cond-mat.mes-hall↗

Electron Spin Decoherence in Silicon Carbide Nuclear Spin Bath

In this paper, we study the electron spin decoherence of single defects in silicon carbide (SiC) nuclear spin bath. We find that, although the natural abundance of $^{29}\rm{Si}$ ($p_{\rm{Si}}=4.7\%$) is about 4 times larger than that of $^{13}{\rm C}$ ($p_{\rm{C}}=1.1\%$), the electron spin coherence time of defect centers in SiC nuclear spin bath in strong magnetic field ($B>300~\rm{Gauss}$) is longer than that of nitrogen-vacancy (NV) centers in $^{13}{\rm C}$ nuclear spin bath in diamond. The reason for this counter-intuitive result is the suppression of heteronuclear-spin flip-flop process in finite magnetic field. Our results show that electron spin of defect centers in SiC are excellent candidates for solid state spin qubit in quantum information processing.

cond-mat.mes-hall↗

Readout and control of a single nuclear spin with a meta-stable electron spin ancilla

Electron and nuclear spins associated with point defects in insulators are promising systems for solid state quantum technology. While the electron spin usually is used for readout and addressing, nuclear spins are exquisite quantum bits and memory systems. With these systems single-shot readout of nearby nuclear spins as well as entanglement aided by the electron spin has been shown. While the electron spin in this example is essential for readout it usually limits nuclear spin coherence. This has set of the quest for defects with spin-free ground states. Here, we isolate a hitherto unidentified defect in diamond and use it at room temperature to demonstrate optical spin polarization and readout with exceptionally high contrast (up to 45%), coherent manipulation of an individual excited triplet state spin, and coherent nuclear spin manipulation using the triplet electron spin as a meta-stable ancilla. By this we demonstrate nuclear magnetic resonance and Rabi oscillations of the uncoupled nuclear spin in the spin-free electronic ground state. Our study demonstrates that nuclei coupled to single metastable electron spins are useful quantum systems with long memory times despite electronic relaxation processes.

quant-ph↗

Modulation frequency dependence of continuous-wave optically/electrically detected magnetic resonance

Continuous wave optically and electrically detected magnetic resonance spectroscopy (cwODMR/cwEDMR) allow the investigation of paramagnetic states involved in spin-dependent transitions, like recombination and transport. Although experimentally similar to conventional electron spin resonance (ESR), there exist limitations when applying models originally developed for ESR to observables (luminescence and electric current) of cwODMR and cwEDMR. Here we present closed-form solutions for the modulation frequency dependence of cwODMR and cwEDMR based on an intermediate pair recombination model and discuss ambiguities which arise when attempting to distinguish the dominant spin-dependent processes underlying experimental data. These include: 1) a large number of quantitatively different models cannot be differentiated, 2) signs of signals are determined not only by recombination, but also by other processes like dissociation, intersystem-crossing, pair generation, and even experimental parameter such as, modulation frequency, microwave power, and temperature, 3) radiative and non-radiative recombination cannot be distinguished due to the observed signs of cwODMR and cwEDMR experiments.

cond-mat.mtrl-sci↗