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Satoru Emori

Publications and source records attributed to Satoru Emori.

31 records · Page 2Linked to original sources

Spin-orbit torque and spin pumping in YIG/Pt with interfacial insertion layers

We experimentally investigate spin-orbit torque and spin pumping in Y$_3$Fe$_5$O$_{12}$(YIG)/Pt bilayers with ultrathin insertion layers at the interface. An insertion layer of Cu suppresses both spin-orbit torque and spin pumping, whereas an insertion layer of Ni$_{80}$Fe$_{20}$ (permalloy, Py) enhances them, in a quantitatively consistent manner with the reciprocity of the two spin transmission processes. However, we observe a large enhancement of Gilbert damping with the insertion of Py that cannot be accounted for solely by spin pumping, suggesting significant spin-memory loss due to the interfacial magnetic layer. Our findings indicate that the magnetization at the YIG-metal interface strongly influences the transmission and depolarization of pure spin current.

cond-mat.mtrl-sci↗

Spin transport and dynamics in all-oxide perovskite La$_{2/3}$Sr$_{1/3}$MnO$_3$/SrRuO$_3$ bilayers probed by ferromagnetic resonance

Thin films of perovskite oxides offer the possibility of combining emerging concepts of strongly correlated electron phenomena and spin current in magnetic devices. However, spin transport and magnetization dynamics in these complex oxide materials are not well understood. Here, we experimentally quantify spin transport parameters and magnetization damping in epitaxial perovskite ferromagnet/paramagnet bilayers of La$_{2/3}$Sr$_{1/3}$MnO$_3$/SrRuO$_3$ (LSMO/SRO) by broadband ferromagnetic resonance spectroscopy. From the SRO thickness dependence of Gilbert damping, we estimate a short spin diffusion length of $\lesssim$1 nm in SRO and an interfacial spin-mixing conductance comparable to other ferromagnet/paramagnetic-metal bilayers. Moreover, we find that anisotropic non-Gilbert damping due to two-magnon scattering also increases with the addition of SRO. Our results demonstrate LSMO/SRO as a spin-source/spin-sink system that may be a foundation for examining spin-current transport in various perovskite heterostructures.

cond-mat.mtrl-sci↗

Comparison of spin-orbit torques and spin pumping across NiFe/Pt and NiFe/Cu/Pt interfaces

We experimentally investigate spin-orbit torques and spin pumping in NiFe/Pt bilayers with direct and interrupted interfaces. The damping-like and field-like torques are simultaneously measured with spin-torque ferromagnetic resonance tuned by a dc bias current, whereas spin pumping is measured electrically through the inverse spin Hall effect using a microwave cavity. Insertion of an atomically thin Cu dusting layer at the interface reduces the damping-like torque, field-like torque, and spin pumping by nearly the same factor of ~1.4. This finding confirms that the observed spin-orbit torques predominantly arise from diffusive transport of spin current generated by the spin Hall effect. We also find that spin-current scattering at the NiFe/Pt interface contributes to additional enhancement in magnetization damping that is distinct from spin pumping.

cond-mat.mes-hall↗

Interfacial spin-orbit torque without bulk spin-orbit coupling

An electric current in the presence of spin-orbit coupling can generate a spin accumulation that exerts torques on a nearby magnetization. We demonstrate that, even in the absence of materials with strong bulk spin-orbit coupling, a torque can arise solely due to interfacial spin-orbit coupling, namely Rashba-Eldestein effects at metal/insulator interfaces. In magnetically soft NiFe sandwiched between a weak spin-orbit metal (Ti) and insulator (Al$_2$O$_3$), this torque appears as an effective field, which is significantly larger than the Oersted field and sensitive to insertion of an additional layer between NiFe and Al$_2$O$_3$. Our findings point to new routes for tuning spin-orbit torques by engineering interfacial electric dipoles.

cond-mat.mtrl-sci↗

Control of magnetic relaxation by electric-field-induced ferroelectric phase transition and inhomogeneous domain switching

Electric-field modulation of magnetism in strain-mediated multiferroic heterostructures is considered a promising scheme for enabling memory and magnetic microwave devices with ultralow power consumption. However, it is not well understood how electric-field-induced strain influences magnetic relaxation, an important physical process for device applications. Here we investigate resonant magnetization dynamics in ferromagnet/ferrolectric multiferroic heterostructures, FeGaB/PMN-PT and NiFe/PMN-PT, in two distinct strain states provided by electric-field-induced ferroelectric phase transition. The strain not only modifies magnetic anisotropy but also magnetic relaxation. In FeGaB/PMN-PT, we observe a nearly two-fold change in intrinsic Gilbert damping by electric field, which is attributed to strain-induced tuning of spin-orbit coupling. By contrast, a small but measurable change in extrinsic linewidth broadening is attributed to inhomogeneous ferroelastic domain switching during the phase transition of the PMN-PT substrate.

cond-mat.mtrl-sci↗

Large voltage-induced modification of spin-orbit torques in Pt/Co/GdOx

We report on large modifications of current-induced spin-orbit torques in a gated Pt/Co/Gd-oxide microstrip due to voltage-driven O$^{2-}$ migration. The Slonczewski-like and field-like torques are quantified using a low-frequency harmonic technique based on the polar magneto-optical Kerr effect. Voltage-induced oxidation of Co enhances the Slonczewski-like torque by as much as an order of magnitude, and simultaneously reduces the anisotropy energy barrier by a factor of ~5. Such magneto-ionic tuning of interfacial spin-orbit effects may significantly enhance the efficiency of magnetization switching and provide additional degrees of freedom in spintronic devices.

cond-mat.mtrl-sci↗

Quantification of the spin-Hall anti-damping torque with a resonance spectrometer

We present a simple technique using a cavity-based resonance spectrometer to quantify the anti-damping torque due to the spin Hall effect. Modification of ferromagnetic resonance is observed as a function of small DC current in sub-mm-wide strips of bilayers, consisting of magnetically soft FeGaB and strong spin-Hall metal Ta. From the detected current-induced linewidth change, we obtain an effective spin Hall angle of 0.08-0.09 independent of the magnetic layer thickness. Our results demonstrate that a sensitive resonance spectrometer can be a general tool to investigate spin Hall effects in various material systems, even those with vanishingly low conductivity and magnetoresistance.

cond-mat.mtrl-sci↗

Spin Hall torque magnetometry of Dzyaloshinskii domain walls

Current-induced domain wall motion in the presence of the Dzyaloshinskii-Moriya interaction (DMI) is experimentally and theoretically investigated in heavy-metal/ferromagnet bilayers. The angular dependence of the current-induced torque and the magnetization structure of Dzyaloshinskii domain walls are described and quantified simultaneously in the presence of in-plane fields. We show that the DMI strength depends strongly on the heavy metal, varying by a factor of 20 between Ta and Pa, and that strong DMI leads to wall distortions not seen in conventional materials. These findings provide essential insights for understanding and exploiting chiral magnetism for emerging spintronics applications.

cond-mat.mtrl-sci↗

Generalized analysis of thermally activated domain-wall motion in Co/Pt multilayers

Thermally activated domain-wall (DW) motion driven by magnetic field and electric current is investigated experimentally in out-of-plane magnetized Pt(Co/Pt)$_3$ multilayers. We directly extract the thermal activation energy barrier for DW motion and observe the dynamic regimes of creep, depinning, and viscous flow. Further analysis reveals that the activation energy must be corrected with a factor dependent on the Curie temperature, and we derive a generalized Arrhenius-like equation governing thermally activated motion. By using this generalized equation, we quantify the efficiency of current-induced spin torque in assisting DW motion. Current produces no effect aside from Joule heating in the multilayer with 7-Å thick Co layers, whereas it generates a finite spin torque on DWs in the multilayer with atomically thin 3-Å Co layers. These findings suggest that conventional spin-transfer torques from in-plane spin-polarized current do not drive DWs in ultrathin Co/Pt multilayers.

cond-mat.mtrl-sci↗

Magneto-ionic Control of Interfacial Magnetism

In metal/oxide heterostructures, rich chemical, electronic, magnetic and mechanical properties can emerge from interfacial chemistry and structure. The possibility to dynamically control interface characteristics with an electric field paves the way towards voltage control of these properties in solid-state devices. Here we show that electrical switching of the interfacial oxidation state allows for voltage control of magnetic properties to an extent never before achieved through conventional magnetoelectric coupling mechanisms. We directly observe, for the first time, in situ voltage driven O$^{2-}$ migration in a Co/metal-oxide bilayer, which we use to toggle the interfacial magnetic anisotropy energy by >0.6 erg/cm$^2$. We exploit the thermally-activated nature of ion migration to dramatically increase the switching efficiency and to demonstrate reversible patterning of magnetic properties through local activation of ionic migration. These results suggest a path towards voltage-programmable materials based on solid-state switching of interface oxygen chemistry.

cond-mat.mtrl-sci↗

Current-driven dynamics of chiral ferromagnetic domain walls

In most ferromagnets the magnetization rotates from one domain to the next with no preferred handedness. However, broken inversion symmetry can lift the chiral degeneracy, leading to topologically-rich spin textures such as spin-spirals and skyrmions via the Dzyaloshinskii-Moriya interaction (DMI). Here we show that in ultrathin metallic ferromagnets sandwiched between a heavy metal and an oxide, the DMI stabilizes chiral domain walls (DWs) whose spin texture enables extremely efficient current-driven motion. We show that spin torque from the spin Hall effect drives DWs in opposite directions in Pt/CoFe/MgO and Ta/CoFe/MgO, which can be explained only if the DWs assume a Néel configuration with left-handed chirality. We directly confirm the DW chirality and rigidity by examining current-driven DW dynamics with magnetic fields applied perpendicular and parallel to the spin spiral. This work resolves the origin of controversial experimental results and highlights a new path towards interfacial design of spintronic devices.

cond-mat.mtrl-sci↗

Voltage-Gated Modulation of Domain Wall Velocity in an Ultrathin Metallic Ferromagnet

The influence of gate voltage, temperature and magnetic field on domain wall (DW) creep dynamics is investigated in Pt/Co/GdOx films with perpendicular magnetic anisotropy and imaged by a scanning magneto-optical Kerr effect technique. The DW creep velocity can be controlled by an electric field applied to the Co/GdOx interface via a linear modulation of the activation energy barrier with gate voltage. At low speeds, the DW velocity can be changed significantly by a gate voltage, but the effect is diminished as the DW velocity increases, which limits electric field control of fast DW motion.

cond-mat.mtrl-sci↗

Interfacial current-induced torques in Pt/Co/GdOx

Current-driven domain wall (DW) motion is investigated in Pt/Co/GdOx nanostrips with perpendicular magnetic anisotropy. Measurements of the propagation field and the energy barrier for thermally activated DW motion reveal a large current-induced torque equivalent to an out-of-plane magnetic field of ~60 Oe per 10^11 A/m^2. This same field-to-current scaling is shown to hold in both the slow thermally activated and fast near-flow regimes of DW motion. The current-induced torque decreases with 4 Å of Pt decorating the Co/GdOx interface and vanishes entirely with Pt replacing GdOx, suggesting that the Co/GdOx interface contributes directly to highly efficient current-driven DW motion.

cond-mat.mtrl-sci↗