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Sebastien Michelin

Publications and source records attributed to Sebastien Michelin.

At least 37 records · Page 2Linked to original sources

Phoretic and hydrodynamic interactions of weakly-confined autophoretic particles

Phoretic particles self-propel using self-generated physico-chemical gradients at their surface. Within a suspension, they interact hydrodynamically by setting the fluid around them into motion, and chemically by modifying the chemical background seen by their neighbours. While most phoretic systems evolve in confined environments due to buoyancy effects, most models focus on their interactions in unbounded flows. Here, we propose a first model for the interaction of phoretic particles in Hele-Shaw confinement and show that in this limit, hydrodynamic and phoretic interactions share not only the same scaling but also the same form, albeit in opposite directions. In essence, we show that phoretic interactions effectively reverse the sign of the interactions that would be obtained for swimmers interacting purely hydrodynamically. Yet, hydrodynamic interactions can not be neglected as they significantly impact the magnitude of the interactions. This model is then used to analyse the behaviour of a suspension. The suspension exhibits swirling and clustering collective modes dictated by the orientational interactions between particles, similar to hydrodynamic swimmers, but here governed by the surface properties of the phoretic particle; the reversal in the sign of the interaction tends to slow down the swimming motion of the particles.

physics.flu-dyn↗

Viscous growth and rebound of a bubble near a rigid surface

Motivated by the dynamics of microbubbles near catalytic surfaces in bubble-powered microrockets, we consider theoretically the growth of a free spherical bubble near a flat no-slip surface in a Stokes flow. The flow at the bubble surface is characterised by a constant slip length allowing to tune the hydrodynamic mobility of its surface and tackle in one formulation both clean and contaminated bubbles as well as rigid shells. Starting with a bubble of infinitesimal size, the fluid flow and hydrodynamic forces on the growing bubble are obtained analytically. We demonstrate that, depending on the value of the bubble slip length relative to the initial distance to the wall, the bubble will either monotonically drain the fluid separating it from the wall, which will exponentially thin, or it will bounce off the surface once before eventually draining the thin film. Clean bubbles are shown to be a singular limit who always monotonically get repelled from the surface. The bouncing events for bubbles with finite slip lengths are further analysed in detail in the lubrication limit. In particular, we identify the origin of the reversal of the hydrodynamic force direction as due to the change in the flow pattern in the film between the bubble and the surface and to the associated lubrication pressure. Finally, the final drainage dynamics of the film is observed to follow a universal algebraic scaling for all finite slip lengths.

physics.flu-dyn↗

Self-propulsion near the onset of Marangoni instability of deformable active droplets

Experimental observations indicate that chemically active droplets suspended in a surfactant-laden fluid can self-propel spontaneously. The onset of this motion is attributed to a symmetry-breaking Marangoni instability resulting from the nonlinear advective coupling of the distribution of surfactant to the hydrodynamic flow generated by Marangoni stresses at the droplet's surface. Here, we use weakly nonlinear analysis to characterize the self-propulsion near the instability threshold and the influence of the droplet's deformability. We report that in vicinity of the threshold, deformability enhances self-propulsion of viscous droplets, but hinders propulsion of drops that are roughly less viscous than the surrounding fluid. Our asymptotics further reveals that droplet deformability may alter the type of bifurcation leading to symmetry breaking: for moderately deformable droplets the onset of self-propulsion is transcritical and a regime of steady self-propulsion is stable; while in the case of highly deformable drops, no steady flows can be found within the asymptotic limit considered in this paper suggesting that the bifurcation is subcritical.

physics.flu-dyn↗

Clustering-induced self-propulsion of isotropic autophoretic particles

Self-diffusiophoretic particles exploit local concentration gradients of a solute species in order to self-propel at the micron scale. While an isolated chemically- and geometrically-isotropic particle cannot swim, we show that it can achieve self-propulsion through interactions with other individually-non-motile particles by forming geometrically-anisotropic clusters via phoretic and hydrodynamic interactions. This result identifies a new route to symmetry-breaking for the concentration field and to self-propulsion, that is not based on an anisotropic design, but on the collective dynamics of identical and homogeneous active particles. Using full numerical simulations as well as theoretical modelling of the clustering process, the statistics of the propulsion properties are obtained for arbitrary initial arrangement of the particles. The robustness of these results to thermal noise, and more generally the effect of Brownian motion of the particles, is also discussed.

cond-mat.soft↗

Physics of Bubble-Propelled Microrockets

A popular method to induce synthetic propulsion at the microscale is to use the forces created by surface-produced gas bubbles inside the asymmetric body of a catalytic swimmer (referred to in the literature as microrocket). Gas bubbles nucleate and grow within the catalytic swimmer and migrate toward one of its opening under the effect of asymmetric geometric confinement, thus generating a net hydrodynamic force which propels the device. In this paper we use numerical simulations to develop a joint chemical (diffusive) and hydrodynamic (Stokes) analysis of the bubble growth within a conical catalytic microrocket and of the associated bubble and microrocket motion. Our computational model allows us to solve for the bubble dynamics over one full bubble cycle ranging from its nucleation to its exiting the conical rocket and therefore to identify the propulsion characteristics as function of all design parameters, including geometry and chemical activity of the motor, surface tension phenomena, and all physicochemical constants. Our results suggest that hydrodynamics and chemistry partially decouple in the motion of the bubbles, with hydrodynamics determining the distance travelled by the microrocket over each cycle while chemistry setting the bubble ejection frequency. Our numerical model finally allows us to identify an optimal microrocket shape and size for which the swimming velocity (distance travelled per cycle duration) is maximized.

physics.flu-dyn↗

Monitoring the orientation of rare-earth-doped nanorods for flow shear tomography

Rare-earth phosphors exhibit unique luminescence polarization features originating from the anisotropic symmetry of the emitter ion's chemical environment. However, to take advantage of this peculiar property, it is necessary to control and measure the ensemble orientation of the host particles with a high degree of precision. Here, we show a methodology to obtain the photoluminescence polarization of Eu-doped LaPO4 nano rods assembled in an electrically modulated liquid-crystalline phase. We measure Eu3+ emission spectra for the three main optimal configurations (σ, π and α, depending on the direction of observation and the polarization axes) and use them as a reference for the nano rod orientation analysis. Based on the fact that flowing nano rods tend to orient along the shear strain profile, we use this orientation analysis to measure the local shear rate in a flowing liquid. The potential of this approach is then demonstrated through tomographic imaging of the shear rate distribution in a microfluidic system.

physics.flu-dyn↗

Geometric tuning of self-propulsion for Janus catalytic particles

Catalytic swimmers have attracted much attention as alternatives to biological systems for examining collective microscopic dynamics and the response to physico-chemical signals. Yet, understanding and predicting even the most fundamental characteristics of their individual propulsion still raises important challenges. While chemical asymmetry is widely recognized as the cornerstone of catalytic propulsion, different experimental studies have reported that particles with identical chemical properties may propel in opposite directions. Here, we show that, beyond its chemical properties, the detailed shape of a catalytic swimmer plays an essential role in determining its direction of motion, demonstrating the compatibility of the classical theoretical framework with experimental observations.

cond-mat.soft↗

Synchronized flutter of two slender flags

The interactions and synchronization of two parallel and slender flags in a uniform axial flow are studied in the present paper by generalizing Lighthill's Elongated Body Theory (EBT) and Lighthill's Large Amplitude Elongated Body Theory (LAEBT) to account for the hydrodynamic coupling between flags. The proposed method consists in two successive steps, namely the reconstruction of the flow created by a flapping flag within the LAEBT framework and the computation of the fluid force generated by this nonuniform flow on the second flag. In the limit of slender flags in close proximity, we show that the effect of the wakes have little influence on the long time coupled-dynamics and can be neglected in the modeling. This provides a simplified framework extending LAEBT to the coupled dynamics of two flags. Using this simplified model, both linear and large amplitude results are reported to explore the selection of the flapping regime as well as the dynamical properties of two side-by-side slender flags. Hydrodynamic coupling of the two flags is observed to destabilize the flags for most parameters, and to induce a long-term synchronization of the flags, either in-phase or out-of-phase.

physics.flu-dyn↗

Electro-hydrodynamic synchronization of piezoelectric flags

Hydrodynamic coupling of flexible flags in axial flows may profoundly influence their flapping dynamics, in particular driving their synchronization. This work investigates the effect of such coupling on the harvesting efficiency of coupled piezoelectric flags, that convert their periodic deformation into an electrical current. Considering two flags connected to a single output circuit, we investigate using numerical simulations the relative importance of hydrodynamic coupling to electrodynamic coupling of the flags through the output circuit due to the inverse piezoelectric effect. It is shown that electrodynamic coupling is dominant beyond a critical distance, and induces a synchronization of the flags' motion resulting in enhanced energy harvesting performance. We further show that this electrodynamic coupling can be strengthened using resonant harvesting circuits.

physics.flu-dyn↗

Phoretic flow induced by asymmetric confinement

Internal phoretic flows due to the interactions of solid boundaries with local chemical gradients may be created using chemical patterning. Alternatively, we demonstrate here that internal flows might also be induced by geometric asymmetries of chemically-homogeneous surfaces. We characterise the circulatory flow created in a cavity enclosed between two eccentric cylindrical walls of uniform chemical activity. Local gradients of the diffusing solute induce a slip flow along the surface of the cylinders, leading to a circulatory bulk flow pattern which can be solved analytically in the diffusive limit. The flow strength can be controlled by adjusting the relative positions of the cylinders and an optimal configuration is identified. These results provide a model system for tunable phoretic pumps.

physics.flu-dyn↗

Synchronized switch harvesting applied to piezoelectric flags

In this article the energy transfer between a flow and a fluttering piezoelectric plate is investigated. In particular, the benefits of the use of a Synchronized Switch Harvesting on Inductor (SSHI) circuit are studied. Both wind tunnel experiments and numerical simulations are conducted in order to analyse the influence of the switching process on the dynamics and the efficiency of the system. Numerical simulations consist of a weakly non-linear model of a plate in axial flow equipped with a single pair of piezoelectric patches, discretized using a Galerkin method where basis functions are the modes of the plate in vacuum. The discretized model is then integrated in time. The results presented in this paper show that a significant improvement of the harvested energy can be obtained using SSHI circuits compared to basic resistive circuits. It is also shown that for strongly coupled systems, the switching process inherent to he SSHI circuit has a significant impact on the dynamics of the flag, which tends to decrease the relative efficiency gain.

physics.flu-dyn↗

Resonance-induced enhancement of the energy harvesting performance of piezoelectric flags

The spontaneous flapping of a flag can be used to produce electrical energy from a fluid flow when coupled to a generator. In this paper, the energy harvesting performance of a flag covered by a single pair of PVDF piezoelectric electrodes is studied both experimentally and numerically. The electrodes are connected to a resistive-inductive circuit that forms a resonant circuit with the piezoelectric's intrinsic capacitance. Compared with purely resistive circuits, the resonance between the circuit and the flag's flapping motion leads to a significant increase in the harvested energy. Our experimental study also validates our fluid-solid-electric nonlinear numerical model.

physics.flu-dyn↗

A regularised singularity approach to phoretic problems

An efficient, accurate, and flexible numerical method is proposed for the solution of the swimming problem of one or more autophoretic particles in the purely-diffusive limit. The method relies on successive boundary element solutions of the Laplacian and the Stokes flow equations using regularised Green's functions for swift, simple implementations, an extension of the well-known method of "regularised stokeslets" for Stokes flow problems. The boundary element method is particularly suitable for phoretic problems, since no quantities in the domain bulk are required to compute the swimming velocity. For time-dependent problems, the method requires no re-meshing and simple boundaries such as a plane wall may be added at no increase to the size of the linear system through the method of images. The method is validated against two classical examples for which an analytical or semi-analytical solution is known, a two-sphere system and a Janus particle, and provides a rigorous computational pipeline to address further problems with complex geometry and multiple bodies.

physics.flu-dyn↗

A reciprocal theorem for boundary-driven channel flows

In a variety of physical situations, a bulk viscous flow is induced by a distribution of surface velocities, for example in diffusiophoresis (as a result of chemical gradients) and above carpets of cilia (as a result of biological activity). When such boundary-driven flows are used to pump fluids, the primary quantity of interest is the induced flow rate. In this letter we propose a method, based on the reciprocal theorem of Stokes flows, to compute the net flow rate for arbitrary flow distribution and periodic pump geometry using solely stress information from a dual Poiseuille-like problem. After deriving the general result we apply it to straight channels of triangular, elliptic and rectangular geometries and quantify the relationship between bulk motion and surface forcing.

physics.flu-dyn↗

Geometric pumping in autophoretic channels

Many microfluidic devices use macroscopic pressure differentials to overcome viscous friction and generate flows in microchannels. In this work, we investigate how the chemical and geometric properties of the channel walls can drive a net flow by exploiting the autophoretic slip flows induced along active walls by local concentration gradients of a solute species. We show that chemical patterning of the wall is not required to generate and control a net flux within the channel, rather channel geometry alone is sufficient. Using numerical simulations, we determine how geometric characteristics of the wall influence channel flow rate, and confirm our results analytically in the asymptotic limit of lubrication theory.

physics.flu-dyn↗

Phoretic self-propulsion at large Peclet numbers

We analyse the self-diffusiophoresis of a spherical particle animated by a nonuniform chemical reaction at its boundary. We consider two models of solute absorption, one with a specified distribution of interfacial solute flux, and one where this flux is governed by first-order kinetics with a specified distribution of rate constant. We employ a macroscale model where the short-range interaction of the solute with the particle boundary is represented by an effective slip condition. The solute transport is governed by an advection-diffusion equation. We focus upon the singular limit of large Péclet numbers, $Pe\gg 1$. In the fixed-flux model, the excess-solute concentration is confined to a narrow boundary layer. The scaling pertinent to that limit allows to decouple the problem governing the solute concentration from the flow field. The resulting nonlinear boundary-layer problem is handled using a transformation to stream-function coordinates and a subsequent application of Fourier transforms, and is thereby reduced to a nonlinear integral equation governing the interfacial concentration. Its solution provides the requisite approximation for the particle velocity, which scales as $Pe^{-1/3}$. In the fixed-rate model, large Péclet numbers may be realized in different limit processes. We consider the case of large swimmers or strong reaction, where the Damköhler number $Da$ is large as well, scaling as $Pe$. In that double limit, where no boundary layer is formed, we obtain a closed-form approximation for the particle velocity, expressed as a nonlinear functional of the rate-constant distribution; this velocity scales as $Pe^{-2}$. Both the fixed-flux and fixed-rate asymptotic predictions agree with the numerical values provided by computational solutions of the nonlinear transport problem.

physics.flu-dyn↗

Autophoretic locomotion from geometric asymmetry

Among the few methods which have been proposed to create small-scale swimmers, those relying on self-phoretic mechanisms present an interesting design challenge in that chemical gradients are required to generate net propulsion. Building on recent work, we propose that asymmetries in geometry are sufficient to induce chemical gradients and swimming. We illustrate this idea using two different calculations. We first calculate exactly the self-propulsion speed of a system composed of two spheres of unequal sizes but identically chemically homogeneous. We then consider arbitrary, small-amplitude, shape deformations of a chemically-homogeneous sphere, and calculate asymptotically the self-propulsion velocity induced by the shape asymmetries. Our results demonstrate how geometric asymmetries can be tuned to induce large locomotion speeds without the need of chemical patterning.

physics.flu-dyn↗

Fluid-solid-electric lock-in of energy-harvesting piezoelectric flags

The spontaneous flapping of a flag in a steady flow can be used to power an output circuit using piezoelectric elements positioned at its surface. Here, we study numerically the effect of inductive circuits on the dynamics of this fluid-solid-electric system and on its energy harvesting efficiency. In particular, a destabilization of the system is identified leading to energy harvesting at lower flow velocities. Also, a frequency lock-in between the flag and the circuit is shown to significantly enhance the system's harvesting efficiency. These results suggest promising efficiency enhancements of such flow energy harvesters through the output circuit optimization.

physics.flu-dyn↗