arXiv subjects

Serge Florens

Publications and source records attributed to Serge Florens.

At least 37 records · Page 2Linked to original sources

arXiv2017

Spontaneous emission of Schrödinger cats in a waveguide at ultrastrong coupling

Josephson circuits provide a realistic physical setup where the light-matter fine structure constant can become of order one, allowing to reach a regime dominated by non-perturbative effects beyond standard quantum optics. Simple processes, such as spontaneous emission, thus acquire a many-body character, that can be tackled using a new description of the time-dependent state vector in terms of quantum-superposed coherent states. We find that spontaneous atomic decay at ultrastrong coupling leads to the emission of spectrally broad Schrödinger cats rather than of monochromatic single photons. These cats states remain partially entangled with the emitter at intermediate stages of the dynamics, even after emission, due to a large separation in time scales between fast energy relaxation and exponentially slow decoherence. Once decoherence of the qubit is finally established, quantum information is completely transfered to the state of the emitted cat.

cond-mat.mes-hall↗

arXiv2017

Anatomy of quantum critical wave functions in dissipative impurity problems

Quantum phase transitions reflect singular changes taking place in a many-body ground state, however, computing and analyzing large-scale critical wave functions constitutes a formidable challenge. New physical insights into the sub-Ohmic spin-boson model are provided by the coherent state expansion (CSE), which represents the wave function by a linear combination of classically displaced configurations. We find that the distribution of low-energy displacements displays an emergent symmetry in the absence of spontaneous symmetry breaking, while experiencing strong fluctuations of the order parameter near the quantum critical point. Quantum criticality provides two strong fingerprints in critical low-energy modes: an algebraic decay of the average displacement and a constant universal average squeezing amplitude. These observations, confirmed by extensive variational matrix product states (VMPS) simulations and field theory arguments, offer precious clues into the microscopics of critical many-body states in quantum impurity models.

cond-mat.str-el↗

arXiv2016

Magneto-electric spectroscopy of Andreev bound states in Josephson quantum dots

We theoretically investigate the behavior of Andreev levels in a single-orbital interacting quantum dot in contact to superconducting leads, focusing on the effect of electrostatic gating and applied magnetic field, as relevant for recent experimental spectroscopic studies. In order to account reliably for spin-polarization effects in presence of correlations, we extend here two simple and complementary approaches that are tailored to capture effective Andreev levels: the static functional renormalization group (fRG) and the self-consistent Andreev bound states (SCABS) theory. We provide benchmarks against the exact large-gap solution as well as NRG calculations and find good quantitative agreement in the range of validity. The large flexibility of the implemented approaches then allows us to analyze a sizeable parameter space, allowing to get a deeper physical understanding into the Zeeman field, electrostatic gate, and flux dependence of Andreev levels in interacting nanostructures.

cond-mat.str-el↗

arXiv2016

Fate of spinons at the Mott point

Gapless spin liquids have recently been observed in several frustrated Mott insulators, with elementary spin excitations - "spinons" - reminiscent of degenerate Fermi systems. However, their precise role at the Mott point, where charge fluctuations begin to proliferate, remains controversial and ill-understood. Here we present the simplest theoretical framework that treats the dynamics of emergent spin and charge excitations on the same footing, providing a new physical picture of the Mott metal-insulator transition at half filing. We identify a generic orthogonality mechanism leading to strong damping of spinons, arising as soon as the Mott gap closes. Our results indicates that spinons should not play a significant role within the high-temperature quantum critical regime above the Mott point - in striking agreement with all available experiments.

cond-mat.str-el↗

arXiv2016

Dynamics of a Qubit in a High-Impedance Transmission Line from a Bath Perspective

We investigate quantum dynamics of a generic model of light-matter interaction in the context of high impedance waveguides, focusing on the behavior of the emitted photonic states, in the framework of the spin-boson model Quantum quenches as well as scattering of an incident coherent pulse are studied using two complementary methods. First, we develop an approximate ansatz for the electromagnetic waves based on a single multimode coherent state wavefunction; formally, this approach combines ideas from adiabatic renormalization, the Born-Markov approximation, and input-output theory. Second, we present numerically exact results for scattering of a weak intensity pulse by using NRG calculations. NRG provides a benchmark for any linear response property throughout the ultra-strong coupling regime. We find that in a sudden quantum quench, the coherent state approach produces physical artifacts, such as improper relaxation to the steady state. These previously unnoticed problems are related to the simplified form of the ansatz that generates spurious correlations within the bath. In the scattering problem, NRG is used to find the transmission and reflection of a single photon, as well as the inelastic scattering of that single photon. Simple analytical formulas are established and tested against the NRG data that predict quantitatively the transport coefficients for up to moderate environmental impedance. These formulas resolve pending issues regarding the presence of inelastic losses in the spin-boson model near absorption resonances, and could be used for comparison to experiments in Josephson waveguide QED. Finally, the scattering results using the coherent state wavefunction approach are compared favorably to the NRG results for very weak incident intensity. We end our study by presenting results at higher power where the response of the system is nonlinear.

cond-mat.mes-hall↗

arXiv2015

Universal spatial correlations in the anisotropic Kondo screening cloud: analytical insights and numerically exact results from a coherent state expansion

We analyze the spatial correlations in the spin density of an electron gas in the vicinity of a Kondo impurity. Our analysis extends to the spin-anisotropic regime, which was not investigated in the literature. We use an original and numerically exact method, based on a systematic coherent-state expansion of the ground state of the underlying spin-boson Hamiltonian, which we apply to the computation of observables that are specific to the fermionic Kondo model. We also present an important technical improvement to the method, that obviates the need to discretize modes of the Fermi sea, and allows one to tackle the problem in the thermodynamic limit. One can thus obtain excellent spatial resolution over arbitrary length scales, for a relatively low computational cost, a feature that gives the method an advantage over popular techniques such as NRG and DMRG. We find that the anisotropic Kondo model shows rich universal scaling behavior in the spatial structure of the entanglement cloud. First, SU(2) spin-symmetry is dynamically restored in a finite domain in parameter space in vicinity of the isotropic line, as expected from poor man's scaling. We are also able to obtain in closed analytical form a set of different, yet universal, scaling curves for strong exchange asymmetry, which are parametrized by the longitudinal exchange coupling. Deep inside the cloud, i.e. for distances smaller than the Kondo length, the correlation between the electron spin density and the impurity spin oscillates between ferromagnetic and antiferromagnetic values at the scale of the Fermi wavelength, an effect that is drastically enhanced at strongly anisotropic couplings. Our results also provide further numerical checks and alternative analytical approximations for the recently computed Kondo overlaps [PRL 114, 080601 (2015)].

cond-mat.str-el↗

arXiv2015

Josephson-Kondo screening cloud in circuit quantum electrodynamics

We show that the non-local polarization response in a multimode circuit-QED setup, devised from a Cooper pair box coupled to a long chain of Josephson junctions, provides an alternative route to access the elusive Kondo screening cloud. For moderate circuit impedance, we compute analytically the universal lineshape for the decay of the charge susceptibility along the circuit, that relates to spatial entanglement between the qubit and its electromagnetic environment. At large circuit impedance, we numerically find further spatial correlations that are specific to a true many-body state.

cond-mat.mes-hall↗

arXiv2014

Impact of quantized vibrations on the efficiency of interfacial charge separation in photovoltaic devices

We demonstrate that charge separation at donor-acceptor interfaces is a complex process that is controlled by the combined action of Coulomb binding for electron-hole pairs and partial relaxation due to quantized phonons. A joint electron-vibration quantum dynamical study reveals that high energy vibrations sensitively tune the charge transfer probability as a function of time and injection energy, due to polaron formation. These results have bearings for the optimization of energy transfer both in organic and quantum dot photovoltaics, as well as in biological light harvesting complexes.

cond-mat.mtrl-sci↗

arXiv2014

A generalized multi-polaron expansion for the spin-boson model: Environmental entanglement and the biased two-state system

We develop a systematic variational coherent state expansion for the many-body ground state of the spin-boson model, in which a quantum two-level system is coupled to a continuum of harmonic oscillators. Energetic constraints at the heart of this technique are rationalized in terms of polarons (displacements of the bath states in agreement with classical expectations) and antipolarons (counter-displacements due to quantum tunneling effects). We present a comprehensive study of the ground state two-level system population and coherence as a function of tunneling amplitude, dissipation strength, and bias (akin to asymmetry of the double well potential defining the two-state system). The entanglement among the different environmental modes is investigated by looking at spectroscopic signatures of the bipartite entanglement entropy between a given environmental mode and all the other modes. We observe a drastic change in behavior of this entropy for increasing dissipation, indicative of the entangled nature of the environmental states. In addition, the entropy spreads over a large energy range at strong dissipation, a testimony to the wide entanglement window characterizing the underlying Kondo state. Finally, comparisons to accurate numerical renormalization group calculations and to the exact Bethe Ansatz solution of the model demonstrate the rapid convergence of our variationally-optimized multi-polaron expansion, suggesting that it should also be a useful tool for dissipative models of greater complexity, as relevant for numerous systems of interest in quantum physics and chemistry.

cond-mat.mes-hall↗

arXiv2014

Signatures of Rashba Spin-Orbit Interaction in Charge and Spin Properties of Quantum Hall Systems

We study the local equilibrium properties of two-dimensional electron gases at high magnetic fields in the presence of random smooth electrostatic disorder, Rashba spin-orbit coupling, and the Zeeman interaction. Using a systematic magnetic length ($l_B$) expansion within a Green's function framework we derive quantum functionals for the local spin-resolved particle and current densities which can be useful for future studies combining disorder and mean-field electron-electron interaction in the quantum Hall regime. We point out that the spin polarization presents a peculiar spatial dependence which can be used to determine the strength of the Rashba coupling by local probes. The spatial structure of the current density, consisting of both compressible and incompressible contributions, also essentially reflects the effects of Rashba spin-orbit interaction on the energy spectrum. We show that in the semiclassical limit $l_B \rightarrow 0$ the local Hall conductivity remains, however, still quantized in units of $e^2/h$ for any finite strength of the spin-orbit interaction. In contrast, it becomes half-integer quantized when the latter is infinite, a situation which corresponds to a disordered topological insulator surface consisting of a single Dirac cone. Finally, we argue how to define at high magnetic fields a spin Hall conductivity related to a dissipationless angular momentum flow, which is characterized by a sequence of plateaus as a function of the inverse magnetic field (thus free of resonances).

cond-mat.mes-hall↗

arXiv2014

Stabilizing Spin Coherence Through Environmental Entanglement in Strongly Dissipative Quantum Systems

The key feature of a quantum spin coupled to a harmonic bath---a model dissipative quantum system---is competition between oscillator potential energy and spin tunneling rate. We show that these opposing tendencies cause environmental entanglement through superpositions of adiabatic and antiadiabatic oscillator states, which then stabilizes the spin coherence against strong dissipation. This insight motivates a fast-converging variational coherent-state expansion for the many-body ground state of the spin-boson model, which we substantiate via numerical quantum tomography.

quant-ph↗

arXiv2014

Transport Signatures of Majorana Quantum Criticality Realized by Dissipative Resonant Tunneling

We consider theoretically the transport properties of a spinless resonant electronic level coupled to strongly dissipative leads, in the regime of circuit impedance near the resistance quantum. Using the Luttinger liquid analogy, one obtains an effective Hamiltonian expressed in terms of interacting Majorana fermions, in which all environmental degrees of freedom (leads and electromagnetic modes) are encapsulated in a single fermionic bath. General transport equations for this system are then derived in terms of the Majorana T-matrix. Perturbative treatment of the Majorana interaction term yields the appearance of a marginal, linear dependence of the conductance on temperature when the system is tuned to its quantum critical point, in agreement with recent experimental observations. We investigate in detail the different crossovers involved in the problem, and analyze the role of the interaction terms in the transport scaling functions. In particular, we show that single barrier scaling applies when the system is slightly tuned away from its Majorana critical point, strengthening the general picture of dynamical Coulomb blockade.

cond-mat.mes-hall↗

arXiv2013

Spectral Properties and Local Density of States of Disordered Quantum Hall Systems with Rashba Spin-Orbit Coupling

We theoretically investigate the spectral properties and the spatial dependence of the local density of states (LDoS) in disordered two-dimensional electron gases (2DEG) in the quantum Hall regime, taking into account the combined presence of electrostatic disorder, random Rashba spin-orbit in- teraction, and finite Zeeman coupling. To this purpose, we extend a coherent-state Green's function formalism previously proposed for spinless 2DEG in the presence of smooth arbitrary disorder, that here incorporates the nontrivial coupling between the orbital and spin degrees of freedom into the electronic drift states. The formalism allows us to obtain analytical and controlled nonperturbative expressions of the energy spectrum in arbitrary locally flat disorder potentials with both random electric fields and Rashba coupling. As an illustration of this theory, we derive analytical microscopic expressions for the LDoS in different temperature regimes which can be used as a starting point to interpret scanning tunneling spectroscopy data at high magnetic fields. In this context, we study the spatial dependence and linewidth of the LDoS peaks and explain an experimentally-noticed correlation between the spatial dispersion of the spin-orbit splitting and the local extrema of the potential landscape.

cond-mat.mes-hall↗

arXiv2013

Magnetotransport in the Kondo model with ferromagnetic exchange interaction

We consider the transport properties in an applied magnetic field of the spin S=1/2 Kondo model with ferromagnetic exchange coupling to electronic reservoirs, a description relevant for the strong coupling limit of underscreened spin S=1 Kondo impurities. Because the ferromagnetic Kondo interaction is marginally irrelevant, perturbative methods should prove accurate down to low energies. For the purpose of this study, we use a combination of Majorana diagrammatic theory with Density Matrix Numerical Renormalization Group simulations. In the standard case of antiferromagnetic Kondo exchange, we first show that our technique recovers previously obtained results for the T-matrix and spin relaxation at weak coupling (above the Kondo temperature). Considering then the ferromagnetic case, we demonstrate how the low-energy Kondo anomaly splits for arbitrary small values of the Zeeman energy, in contrast to fully screened Kondo impurities near the strong coupling Fermi liquid fixed point, and in agreement with recent experimental findings for spin S=1 molecular quantum dots.

cond-mat.mes-hall↗

arXiv2013

Influence of spin fluctuations near the Mott transition: a DMFT study

Dynamics of magnetic moments near the Mott metal-insulator transition is investigated by a combined slave-rotor and Dynamical Mean-Field Theory solution of the Hubbard model with additional fully-frustrated random Heisenberg couplings. In the paramagnetic Mott state, the spinon decomposition allows to generate a Sachdev-Ye spin liquid in place of the collection of independent local moments that typically occurs in the absence of magnetic correlations. Cooling down into the spin-liquid phase, the onset of deviations from pure Curie behavior in the spin susceptibility is found to be correlated to the temperature scale at which the Mott transition lines experience a marked bending. We also demonstrate a weakening of the effective exchange energy upon approaching the Mott boundary from the Heisenberg limit, due to quantum fluctuations associated to zero and doubly occupied sites.

cond-mat.str-el↗

arXiv2013

Unveiling environmental entanglement in strongly dissipative qubits

The coupling of a qubit to a macroscopic reservoir plays a fundamental role in understanding the complex transition from the quantum to the classical world. Considering a harmonic environment, we use both intuitive arguments and numerical many-body quantum tomography to study the structure of the complete wavefunction arising in the strong-coupling regime, reached for intense qubit-environment interaction. The resulting strongly-correlated many-body ground state is built from quantum superpositions of adiabatic (polaron-like) and non-adiabatic (antipolaron-like) contributions from the bath of quantum oscillators. The emerging Schrödinger cat environmental wavefunctions can be described quantitatively via simple variational coherent states. In contrast to qubit-environment entanglement, we show that non-classicality and entanglement among the modes in the reservoir are crucial for the stabilization of qubit superpositions in regimes where standard theories predict an effectively classical spin.

cond-mat.mes-hall↗

arXiv2012

Transport via classical percolation at quantum Hall plateau transitions

We consider transport properties of disordered two-dimensional electron gases under high perpendicular magnetic field, focusing in particular on the peak longitudinal conductivity $σ_{xx}^\mathrm{peak}$ at the quantum Hall plateau transition. We use a local conductivity model, valid at temperatures high enough such that quantum tunneling is suppressed, taking into account the random drift motion of the electrons in the disordered potential landscape and inelastic processes provided by electron-phonon scattering. A diagrammatic solution of this problem is proposed, which leads to a rich interplay of conduction mechanisms, where classical percolation effects play a prominent role. The scaling function for $σ_{xx}^\mathrm{peak}$ is derived in the high temperature limit, which can be used to extract universal critical exponents of classical percolation from experimental data.

cond-mat.mes-hall↗

arXiv2011

Diagrammatic Approach for the High-Temperature Regime of Quantum Hall Transitions

We use a general diagrammatic formalism based on a local conductivity approach to compute electronic transport in continuous media with long-range disorder, in the absence of quantum interference effects. The method allows us then to investigate the interplay of dissipative processes and random drifting of electronic trajectories in the high-temperature regime of quantum Hall transitions. We obtain that the longitudinal conductance σ_{xx} scales with an exponent κ=0.767\pm0.002 in agreement with the value κ=10/13 conjectured from analogies to classical percolation. We also derive a microscopic expression for the temperature-dependent peak value of σ_{xx}, useful to extract κ from experiments.

cond-mat.mes-hall↗