arXiv subjects

Serge Florens

Publications and source records attributed to Serge Florens.

At least 55 records · Page 3Linked to original sources

arXiv2011

Dissipative spin dynamics near a quantum critical point: Numerical Renormalization Group and Majorana diagrammatics

We provide an extensive study of the sub-ohmic spin-boson model with power law density of states J(ω)=ω^s (with 0<s<1), focusing on the equilibrium dynamics of the three possible spin components, from very weak dissipation to the quantum critical regime. Two complementary methods, the bosonic Numerical Renormalization Group (NRG) and Majorana diagrammatics, are used to explore the physical properties in a wide range of parameters. We show that the bosonic self-energy is the crucial ingredient for the description of critical fluctuations, but that many-body vertex corrections need to be incorporated as well in order to obtain quantitative agreement of the diagrammatics with the numerical simulations. Our results suggest that the out-of-equilibrium dynamics in dissipative models beyond the Bloch-Redfield regime should be reconsidered in the long-time limit. Regarding also the spin-boson Hamiltonian as a toy model of quantum criticality, some of the insights gained here may be relevant for field theories of electrons coupled to bosons in higher dimensions.

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arXiv2011

First order $0/π$ quantum phase transition in the Kondo regime of a superconducting carbon nanotube quantum dot

We study a carbon nanotube quantum dot embedded into a SQUID loop in order to investigate the competition of strong electron correlations with proximity effect. Depending whether local pairing or local magnetism prevails, a superconducting quantum dot will respectively exhibit positive or negative supercurrent, referred to as a 0 or $π$ Josephson junction. In the regime of strong Coulomb blockade, the 0 to $π$ transition is typically controlled by a change in the discrete charge state of the dot, from even to odd. In contrast, at larger tunneling amplitude the Kondo effect develops for an odd charge (magnetic) dot in the normal state, and quenches magnetism. In this situation, we find that a first order 0 to $π$ quantum phase transition can be triggered at fixed valence when superconductivity is brought in, due to the competition of the superconducting gap and the Kondo temperature. The SQUID geometry together with the tunability of our device allows the exploration of the associated phase diagram predicted by recent theories. We also report on the observation of anharmonic behavior of the current-phase relation in the transition regime, that we associate with the two different accessible superconducting states. Our results ultimately reveal the spin singlet nature of the Kondo ground state, which is the key process in allowing the stability of the 0-phase far from the mixed valence regime.

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arXiv2011

Universal transport signatures in two-electron molecular quantum dots: gate-tunable Hund's rule, underscreened Kondo effect and quantum phase transitions

We review here some universal aspects of the physics of two-electron molecular transistors in the absence of strong spin-orbit effects. Several recent quantum dots experiments have shown that an electrostatic backgate could be used to control the energy dispersion of magnetic levels. We discuss how the generically asymmetric coupling of the metallic contacts to two different molecular orbitals can indeed lead to a gate-tunable Hund's rule in the presence of singlet and triplet states in the quantum dot. For gate voltages such that the singlet constitutes the (non-magnetic) ground state, one generally observes a suppression of low voltage transport, which can yet be restored in the form of enhanced cotunneling features at finite bias. More interestingly, when the gate voltage is controlled to obtain the triplet configuration, spin S=1 Kondo anomalies appear at zero-bias, with non-Fermi liquid features related to the underscreening of a spin larger than 1/2. Finally, the small bare singlet-triplet splitting in our device allows to fine-tune with the gate between these two magnetic configurations, leading to an unscreening quantum phase transition. This transition occurs between the non-magnetic singlet phase, where a two-stage Kondo effect occurs, and the triplet phase, where the partially compensated (underscreened) moment is akin to a magnetically "ordered" state. These observations are put theoretically into a consistent global picture by using new Numerical Renormalization Group simulations, taylored to capture sharp finie-voltage cotunneling features within the Coulomb diamonds, together with complementary out-of-equilibrium diagrammatic calculations on the two-orbital Anderson model. This work should shed further light on the complicated puzzle still raised by multi-orbital extensions of the classic Kondo problem.

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arXiv2011

Numerical Renormalization Group at marginal spectral density: application to quantum tunneling in Luttinger liquids

Many quantum mechanical problems (such as dissipative phase fluctuations in metallic and superconducting nanocircuits, or impurity scattering in Luttinger liquids) involve a continuum of bosonic modes with a marginal spectral density diverging as the inverse of energy. We construct a Numerical Renormalization Group in this singular case, with a manageable violation of scale separation at high energy, capturing reliably the low energy physics. The method is demonstrated by a non-perturbative solution over several energy decades for the dynamical conductance of a Luttinger liquid with a single static defect.

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arXiv2010

Transmission coefficient through a saddle-point electrostatic potential for graphene in the quantum Hall regime

From the scattering of semicoherent-state wavepackets at high magnetic field, we derive analytically the transmission coefficient of electrons in graphene in the quantum Hall regime through a smooth constriction described by a quadratic saddle-point electrostatic potential. We find anomalous half-quantized conductance steps that are rounded by a backscattering amplitude related to the curvature of the potential. Furthermore, the conductance in graphene breaks particle-hole symmetry in cases where the saddle-point potential is itself asymmetric in space. These results have implications both for the interpretation of split-gate transport experiments, and for the derivation of quantum percolation models for graphene.

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arXiv2010

High magnetic field theory for the local density of states in graphene with smooth arbitrary potential landscapes

We study theoretically the energy and spatially resolved local density of states (LDoS) in graphene at high perpendicular magnetic field. For this purpose, we extend from the Schrödinger to the Dirac case a semicoherent-state Green's-function formalism, devised to obtain in a quantitative way the lifting of the Landau-level degeneracy in the presence of smooth confinement and smooth disordered potentials. Our general technique, which rigorously describes quantum-mechanical motion in a magnetic field beyond the semi-classical guiding center picture of vanishing magnetic length (both for the ordinary two-dimensional electron gas and graphene), is connected to the deformation (Weyl) quantization theory in phase space developed in mathematical physics. For generic quadratic potentials of either scalar (i.e., electrostatic) or mass (i.e., associated with coupling to the substrate) types, we exactly solve the regime of large magnetic field (yet at finite magnetic length - formally, this amounts to considering an infinite Fermi velocity) where Landau-level mixing becomes negligible. Hence, we obtain a closed-form expression for the graphene Green's function in this regime, providing analytically the discrete energy spectra for both cases of scalar and mass parabolic confinement. Furthermore, the coherent-state representation is shown to display a hierarchy of local energy scales ordered by powers of the magnetic length and successive spatial derivatives of the local potential, which allows one to devise controlled approximation schemes at finite temperature for arbitrary and possibly disordered potential landscapes. As an application, we derive general analytical non-perturbative expressions for the LDoS, which may serve as a good starting point for interpreting experimental studies.

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arXiv2009

Observation of the underscreened Kondo effect in a molecular transistor

We present the first quantitative experimental evidence for the underscreened Kondo effect, an uncomplete compensation of a quantized magnetic moment by conduction electrons, as originally proposed by Nozieres and Blandin. The device consists of an even charge spin S = 1 molecular quantum dot, obtained by electromigration of C60 molecules into gold nanogaps and operated in a dilution fridge. The persistence of logarithmic singularities in the low temperature conductance is demonstrated by a comparison to the fully screened configuration obtained in odd charge spin S = 1/2 Coulomb diamonds. We also discover an extreme sensitivity of the underscreened Kondo resonance to magnetic field, that we confirm on the basis of numerical renormalization group calculations.

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arXiv2009

Local density of states in disordered two-dimensional electron gases at high magnetic field

Motivated by high-accuracy scanning tunneling spectroscopy measurements on disordered two-dimensional electron gases in strong magnetic field, we present an exact solution for the local density of states (LDoS) of electrons moving in an arbitrary potential smooth on the scale of the magnetic length, that can be locally described up to its second derivatives. We use a technique based on coherent state Green's functions, allowing us to treat on an equal footing confining and open quantum systems. The energy-dependence of the LDoS is found to be universal in terms of local geometric properties, such as drift velocity and potential curvature. We also show that thermal effects are quite important close to saddle points, leading to an overbroadening of the tunneling trajectories.

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arXiv2009

Optimal broadening of finite energy spectra in the numerical renormalization group: application to dissipative dynamics in two-level systems

Numerical renormalization group (NRG) calculations of quantum impurity models, based on a logarithmic discretization in energy of electronic or bosonic Hamiltonians, provide a powerful tool to describe physics involving widely separated energy scales, as typically encountered in nanostructures and strongly correlated materials. This main advantage of the NRG was however considered a drawback for resolving sharp spectral features at finite energy, such as dissipative atomic peaks. Surprisingly, we find a bunching of many-body levels in NRG spectra near dissipative resonances, and exploit this by combining the widely-used Oliveira's $z$-trick, using an averaging over {\it few} discrete NRG spectra, with an optimized {\it frequency-dependent} broadening parameter $b(\w)$. This strategy offers a tremendous gain in computational power and extracts all the needed information from the raw NRG data without {\it a priori} knowledge of the various energy scales at play. As an application we investigate with high precision the crossover from coherent to incoherent dynamics in the spin boson model.

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arXiv2009

Self-consistent description of Andreev bound states in Josephson quantum dot devices

We develop a general perturbative framework based on a superconducting atomic limit for the description of Andreev bound states (ABS) in interacting quantum dots connected to superconducting leads. A local effective Hamiltonian for dressed ABS, including both the atomic (or molecular) levels and the induced proximity effect on the dot is argued to be a natural starting point. A self-consistent expansion in single-particle tunneling events is shown to provide accurate results even in regimes where the superconducting gap is smaller than the atomic energies, as demonstrated by a comparison to recent Numerical Renormalization Group calculations. This simple formulation may have bearings for interpreting Andreev spectroscopic experiments in superconducting devices, such as STM measurements on carbon nanotubes, or radiative emission in optical quantum dots.

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arXiv2008

Supplementary Information: Quantum phase transition in a single-molecule quantum dot

Quantum criticality is the intriguing possibility offered by the laws of quantum mechanics when the wave function of a many-particle physical system is forced to evolve continuously between two distinct, competing ground states. This phenomenon, often related to a zero-temperature magnetic phase transition, can be observed in several strongly correlated materials such as heavy fermion compounds or possibly high-temperature superconductors, and is believed to govern many of their fascinating, yet still unexplained properties. In contrast to these bulk materials with very complex electronic structure, artificial nanoscale devices could offer a new and simpler vista to the comprehension of quantum phase transitions. This long-sought possibility is demonstrated by our work in a fullerene molecular junction, where gate voltage induces a crossing of singlet and triplet spin states at zero magnetic field. Electronic tunneling from metallic contacts into the $\rm{C_{60}}$ quantum dot provides here the necessary many-body correlations to observe a true quantum critical behavior.

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arXiv2008

Quantum phase transition in a single-molecule quantum dot

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arXiv2008

Out-of-equilibrium singlet-triplet Kondo effect in a single C_60 quantum dot

We have used an electromigration technique to fabricate a $\rm{C_{60}}$ single-molecule transistor (SMT). Besides describing our electromigration procedure, we focus and present an experimental study of a single molecule quantum dot containing an even number of electrons, revealing, for two different samples, a clear out-of-equilibrium Kondo effect. Low temperature magneto-transport studies are provided, which demonstrates a Zeeman splitting of the finite bias anomaly.

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arXiv2008

Microscopics of disordered two-dimensional electron gases under high magnetic fields: Equilibrium properties and dissipation in the hydrodynamic regime

We develop in detail a new formalism [as a sequel to the work of T. Champel and S. Florens, Phys. Rev. B 75, 245326 (2007)] that is well-suited for treating quantum problems involving slowly-varying potentials at high magnetic fields in two-dimensional electron gases. For an arbitrary smooth potential we show that electronic Green's function is fully determined by closed recursive expressions that take the form of a high magnetic field expansion in powers of the magnetic length l_B. For illustration we determine entirely Green's function at order l_B^3, which is then used to obtain quantum expressions for the local charge and current electronic densities at equilibrium. Such results are valid at high but finite magnetic fields and for arbitrary temperatures, as they take into account Landau level mixing processes and wave function broadening. We also check the accuracy of our general functionals against the exact solution of a one-dimensional parabolic confining potential, demonstrating the controlled character of the theory to get equilibrium properties. Finally, we show that transport in high magnetic fields can be described hydrodynamically by a local equilibrium regime and that dissipation mechanisms and quantum tunneling processes are intrinsically included at the microscopic level in our high magnetic field theory. We calculate microscopic expressions for the local conductivity tensor, which possesses both transverse and longitudinal components, providing a microscopic basis for the understanding of dissipative features in quantum Hall systems.

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arXiv2007

Spin-orbital Kondo decoherence by environmental effects in capacitively coupled quantum dot devices

Strong correlation effects in a capacitively coupled double quantum-dot setup were previously shown to provide the possibility of both entangling spin-charge degrees of freedom and realizing efficient spin-filtering operations by static gate-voltage manipulations. Motivated by the use of such a device for quantum computing, we study the influence of electromagnetic noise on a general spin-orbital Kondo model, and investigate the conditions for observing coherent, unitary transport, crucial to warrant efficient spin manipulations. We find a rich phase diagram, where low-energy properties sensitively depend on the impedance of the external environment and geometric parameters of the system. Relevant energy scales related to the Kondo temperature are also computed in a renormalization-group treatment, allowing to assess the robustness of the device against environmental effects.

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arXiv2007

Nanoscale Dynamical Mean-Field Theory for Molecules and Mesoscopic Devices in the Strong-Correlation Regime

We develop a nanoscale dynamical mean-field theory (nano-DMFT) to deal with strong Coulomb interaction effects in physical systems that are intermediate in size between atoms and bulk materials, taking into account the tunneling into nearby electrodes. Focusing on a simplified treelike geometry, the usual DMFT loop simply stops when the finite lattice is fully covered, starting with an initial seed provided by the electronic environment at the boundary. To illustrate this nano-DMFT, we investigate the disappearance of the quasiparticle weight in a correlated nano object near the Mott transition. In contrast to thermally driven classical phase transitions, quantum effects lead to unexpected oscillations of the order parameter, related to the interference of coherent renormalized quasiparticles. This behavior also implies a spatially inhomogeneous Mott localization process at the nanoscale.

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arXiv2007

Quantum transport properties of two-dimensional electron gases under high magnetic fields

We study quantum transport properties of two-dimensional electron gases under high perpendicular magnetic fields. For this purpose, we reformulate the high-field expansion, usually done in the operatorial language of the guiding-center coordinates, in terms of vortex states within the framework of real-time Green functions. These vortex states arise naturally from the consideration that the Landau levels quantization can follow directly from the existence of a topological winding number. The microscopic computation of the current can then be performed within the Keldysh formalism in a systematic way at finite magnetic fields $B$ (i.e. beyond the semi-classical limit $B = \infty$). The formalism allows us to define a general vortex current density as long as the gradient expansion theory is applicable. As a result, the total current is expressed in terms of edge contributions only. We obtain the first and third lowest order contributions to the current due to Landau-levels mixing processes, and derive in a transparent way the quantization of the Hall conductance. Finally, we point out qualitatively the importance of inhomogeneities of the vortex density to capture the dissipative longitudinal transport.

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arXiv2007

Interplay of electromagnetic noise and Kondo effect in quantum dots

We investigate the influence of an electromagnetic environment, characterized by a finite impedance $Z(ω)$, on the Kondo effect in quantum dots. The circuit voltage fluctuations couple to charge fluctuations in the dot and influence the spin exchange processes transferring charge between the electrodes. We discuss how the low-energy properties of a Kondo quantum dot subject to dynamical Coulomb blockade resemble those of Kondo impurities in Luttinger liquids. Using previous knowledge based on the bosonization of quantum impurity models, we show that low-voltage conductance anomalies appear at zero temperature. The conductance can vanish at low temperatures even in presence of a screened impurity spin. Moreover, the quantitative determination of the corresponding Kondo temperature depends on the full frequency-dependent impedance of the circuit. This is demonstrated by a weak-coupling calculation in the Kondo interaction, taking into account the full distribution $P(E)$ of excited environmental modes.

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