arXiv subjects

Sergey I. Bozhevolnyi

Publications and source records attributed to Sergey I. Bozhevolnyi.

At least 37 records · Page 2Linked to original sources

arXiv2023

Nonlocal Electro-Optic Metasurfaces for Free-Space Light Modulation

Dynamic optical metasurfaces with ultrafast temporal response, i.e., spatiotemporal optical metasurfaces, provide attractive solutions and open fascinating perspectives for modern highly integrated optics and photonics. In this work, electro-optically controlled optical metasurfaces operating in reflection and utilizing resonant waveguide mode excitation are demonstrated from the viewpoint of free-space propagating light modulation. The modulation of reflected light power with superior characteristics in comparison with prior research is achieved by identifying a suitable low-loss waveguide mode and exploiting its resonant excitation. The electro-optic Pockels effect in a 300-nm-thick lithium niobate (LN) film sandwiched between a continuous thick gold film and an array of gold nanostripes, serving also as control electrodes, is exploited to realize fast and efficient light modulation. The fabricated compact (active area <1000 $μ$m) modulators operate in the wavelength range of 850-950 nm, featuring a maximum intensity modulation depth of $\sim\!$ 42 % at the driving voltage of $\pm$10 V within the bandwidth of 13.5 MHz (with the potential bandwidth of 6.5 GHz). The introduced nonlocal electro-optic metasurface configuration opens new avenues towards the realization of ultrafast, efficient and robust free-space light modulators based on an LN flat optics approach.

physics.optics↗

arXiv2022

60-nm-span wavelength-tunable vortex fiber laser with intracavity plasmon metasurfaces

Wavelength-tunable vortex fiber lasers that could generate beams carrying orbital angular momentum (OAM) hold great interest in large-capacity optical communications. The wavelength tunability of conventional vortex fiber lasers is however limited by the range of 35 nm due to narrow bandwidth and/or insertion loss of mode conversion components. Optical metasurfaces apart from being compact planar components can flexibly manipulate light with high efficiency in a broad wavelength range. Here, we propose and demonstrate for the first time, to the best of our knowledge, a metasurface-assisted vortex fiber laser that can directly generate OAM beams with changeable topological charges. Due to the designed broadband gap-surface plasmon metasurface, combined with an intracavity tunable filter, the laser enables OAM beam with center wavelength continuously tunable from 1015 nm to 1075 nm, nearly twice of other vortex fiber lasers ever reported. The metasurface can be designed at will to satisfy requirements for either low pump threshold or high slope efficiency of the laser. Furthermore, the cavity-metasurface configuration can be extended to generate higher-order OAM beams or more complex structured beams in different wavelength regions, which greatly broadens the possibilities for developing low-cost and high-quality structured-beam laser sources.

physics.optics↗

arXiv2022

Ultimate limit for optical losses in gold, revealed by quantitative near-field microscopy

We report thorough measurements of surface plasmon polaritons (SPPs) running along nearly perfect air-gold interfaces formed by atomically flat surfaces of chemically synthesized gold monocrystals. By means of amplitude- and phase-resolved near-field microscopy, we obtain their propagation length and effective mode index at visible wavelengths (532, 594, 632.8, 729, and 800 nm). The measured values are compared with the values obtained from the dielectric functions of gold that are reported in literature. Importantly, a reported dielectric function of monocrystalline gold implies $\sim 1.5$ times shorter propagation lengths than those observed in our experiments, whereas a dielectric function reported for properly fabricated polycrystalline gold leads to SPP propagation lengths matching our results. We argue that the SPP propagation lengths measured in our experiments signify the ultimate limit of optical losses in gold, encouraging further comprehensive characterization of optical material properties of pure gold as well as other plasmonic materials.

physics.optics↗

arXiv2021

Molding Photon Emission with Hybrid Plasmon-Emitter Coupled Metasurfaces

Directional emission of photons with designed polarizations and orbital angular momenta is crucial for exploiting full potential of quantum emitters (QEs) within quantum information technologies. Capitalizing on the concept of hybrid plasmon-QE coupled metasurfaces, we develop a holography-based design approach allowing one to construct surface nanostructures for outcoupling QE-excited circularly diverging surface plasmon polaritons (SPPs) into well-collimated beams of photons with desirable polarization characteristics propagating along given directions. Using the well-established simulation framework, we demonstrate the efficiency and versatility of the developed approach by analyzing different hybrid SPP-QE coupled metasurfaces designed for generation of linearly, radially and circularly polarized photons propagating in various off-axis directions. Our work enables the design of single-photon sources with radiation channels that have distinct directional and polarization characteristics, extending thereby possibilities for designing complex photonic systems for quantum information processing. Moreover, we believe that the developed scattering holography approach is generally useful when employing surface electromagnetic excitations, including SPP modes, as reference waves for signal wave reconstruction.

physics.optics↗

arXiv2021

Extremely confined gap plasmon modes: when nonlocality matters

Historically, the field of plasmonics has been relying on the framework of classical electrodynamics, with the local-response approximation of material response being applied even when dealing with nanoscale metallic structures. However, when approaching the atomic-scale confinement of the electromagnetic radiation, mesoscopic effects are anticipated to become observable, e.g., those associated with the nonlocal electrodynamic surface response of the electron gas. We investigate nonlocal effects in propagating gap surface plasmon modes in ultrathin metal--dielectric--metal planar waveguides, exploiting monocrystalline gold flakes separated by atomic-layer-deposited aluminum oxide. We use scanning near-field optical microscopy to directly access the near-field of such confined gap plasmon modes and measure their dispersion relation (via their complex-valued propagation constants). We compare our experimental findings with the predictions of the generalized nonlocal optical response theory to unveil signatures of nonlocal damping, which becomes appreciable for smaller dielectric gaps.

cond-mat.mes-hall↗

arXiv2021

Electrical Tuning of Fresnel Lens in Reflection

Optical metasurfaces have been extensively investigated, demonstrating diverse and multiple functionalities with complete control over the transmitted and reflected fields. Most optical metasurfaces are however static, with only a few configurations offering (rather limited) electrical control, thereby jeopardizing their application prospects in emerging flat optics technologies. Here, we suggest an approach to realize electrically tunable optical metasurfaces, demonstrating dynamic Fresnel lens focusing. The active Fresnel lens (AFL) exploits the electro-optic Pockels effect in a 300-nm-thick lithium niobate layer sandwiched between a continuous thick and nanostructured gold film serving as electrodes. We fabricate and characterize the AFL, focusing 800-900 nm radiation at the distance of 40 $\mathrmμ$m with the focusing efficiency of 15 % and demonstrating the modulation depth of 1.5 % with the driving voltage of $\pm 10$ V within the bandwidth of $\sim\! 4$ MHz. We believe that the electro-optic metasurface concept introduced is useful for designing dynamic flat optics components.

physics.optics↗

arXiv2021

Room-temperature on-chip orbital angular momentum single-photon sources

On-chip photon sources carrying orbital angular momentum (OAM) are in demand for high-capacity optical information processing in both classical and quantum regimes. However, currently-exploited integrated OAM sources have been primarily limited to the classical regime. Herein, we demonstrate a room-temperature on-chip integrated OAM source that emits well-collimated single photons, with a single-photon purity of g(2)(0) = 0.22, carrying entangled spin and orbital angular momentum states and forming two spatially separated entangled radiation channels with different polarization properties. The OAM-encoded single photons are generated by efficiently outcoupling diverging surface plasmon polaritons excited with a deterministically positioned quantum emitter via Archimedean spiral gratings. Our OAM single-photon sources bridge the gap between conventional OAM manipulation and nonclassical light sources, enabling high-dimensional and large-scale photonic quantum systems for information processing.

physics.optics↗

arXiv2021

High-speed plasmonic electro-optic beam deflectors

Highly integrated active nanophotonics addressing both device footprint and operation speed demands is a key enabling technology for the next generation optical networks. Plasmonic systems have proven to be a serious contender to alleviate current performance limitations in electro-optic devices. Here, we demonstrate a plasmonic optical phased array (OPA) consisting of two 10-$μ$m-long plasmonic phase shifters, utilized to control the far-field radiation pattern of two subwavelength-separated emitters for aliasing-free beam steering with an angular range of $\pm5^\circ$ and flat frequency response up to 18 GHz (with the potential bandwidth of 1.2 THz). Extreme optical and electrostatic field confinement with great spatial overlap results in high phase modulation efficiency ($V_πL=0.24\: \text{Vcm}$). The demonstrated approach of using plasmonic lithium niobate technology for optical beam manipulation offers inertia-free, robust, ultra-compact and high-speed beam steering.

physics.optics↗

arXiv2021

Dynamic MEMS-based optical metasurfaces

Optical metasurfaces (OMSs) have shown unprecedented capabilities for versatile wavefront manipulations at the subwavelength scale, thus opening fascinating perspectives for next generation ultracompact optical devices and systems. However, to date, most well-established OMSs are static, featuring well-defined optical responses determined by OMS configurations set during their fabrication. Dynamic OMS configurations investigated so far by using controlled constituent materials or geometrical parameters often exhibit specific limitations and reduced reconfigurability. Here, by combining a thin-film piezoelectric micro-electro-mechanical system (MEMS) with a gap-surface plasmon based OMS, we develop an electrically driven dynamic MEMS-OMS platform that offers controllable phase and amplitude modulation of the reflected light by finely actuating the MEMS mirror. Using this platform, we demonstrate MEMS-OMS components for polarization-independent beam steering and two-dimensional focusing with high modulation efficiencies (~ 50%), broadband operation (~ 20% near the operating wavelength of 800 nm) and fast responses (< 0.4 ms). The developed MEMS-OMS platform offers flexible solutions for realizing complex dynamic 2D wavefront manipulations that could be used in reconfigurable and adaptive optical networks and systems.

physics.optics↗

arXiv2020

Anisotropic Second Harmonic Generation From Monocrystalline Gold Flakes

Noble metals with well-defined crystallographic orientation constitute an appealing class of materials for controlling light-matter interactions on the nanoscale. Nonlinear optical processes, being particularly sensitive to anisotropy, are a natural and versatile probe of crystallinity in nano-optical devices. Here we study the nonlinear optical response of monocrystalline gold flakes, revealing a polarization dependence in second-harmonic generation from the {111} surface that is markedly absent in polycrystalline films. Apart from suggesting an approach for directional enhancement of nonlinear response in plasmonic systems, we anticipate that our findings can be used as a rapid and non-destructive method for characterization of crystal quality and orientation that may be of significant importance in future applications.

physics.optics↗

arXiv2020

On-Chip Spin-Orbit Controlled Excitation of Quantum Emitters Coupled to Hybrid Plasmonic Nanocircuits

On-chip realization of complex photonic functionalities is essential for further progress in planar integrated nanophotonics, especially when involving nonclassical light sources such as quantum emitters (QEs). Hybrid plasmonic nanocircuits integrated with QEs have been attracting considerable attention due to the prospects of significantly enhancing QE emission rates and miniaturizing quantum nanophotonic components. Spin-orbit interactions on subwavelength scales have been increasingly explored in both conventional and quantum nanophotonics for realization and utilization of the spin-dependent flow of light. Here, we propose and realize a dielectric-loaded plasmonic nanocircuit consisting of an achiral spin-orbit coupler for unidirectional routing of pump radiation into branched QE-integrated waveguides. We demonstrate experimentally the circular-polarization controlled coupling of 532-nm pump laser light into polymer-loaded branched waveguides followed by the excitation of spatially separated (by a distance of ~ 10 μm) QEs, nanodiamonds, with multiple nitrogen vacancy centres, that are embedded in and efficiently coupled to the corresponding waveguides. The realization of on-chip spin-orbit controlled excitation of different QEs coupled to branched waveguides opens new avenues for designing complex quantum plasmonic nanocircuits exploiting the spin degree of freedom within chiral quantum nanophotonics.

physics.optics↗

arXiv2020

Engineering nanoparticles with pure high-order multipole scattering

The ability to control scattering directionality of nanoparticles is in high demand for many nanophotonic applications. One of the challenges is to design nanoparticles producing pure high-order multipole scattering (e.g., octopole, hexadecapole), whose contribution is usually negligible compared to strong low-order multipole scattering (i.e., dipole or quadrupole). Here we present an intuitive way to design such nanoparticles by introducing a void inside them. We show that both shell and ring nanostructures allow regimes with nearly pure high-order multipole scattering. Experimentally measured scattering diagrams from properly designed silicon rings at near-infrared wavelengths (~ 800 nm) reproduce well scattering patterns of an electric octopole and magnetic hexadecapole. Our findings advance significantly inverse engineering of nanoparticles from given complex scattering characteristics, with possible applications in biosensing, optical metasurfaces, and quantum communications.

physics.optics↗

arXiv2019

Spinning single photons

Single photons carrying spin angular momentum (SAM), i.e., circularly polarized single photons generated typically by subjecting a quantum emitter (QE) to a strong magnetic field at low temperatures are at the core of chiral quantum optics enabling non-reciprocal single-photon configurations and deterministic spin-photon interfaces. Here we propose a conceptually new approach to the room-temperature generation of SAM-coded single photons (SSPs) entailing QE non-radiative coupling to surface plasmons that are transformed, by interacting with an optical metasurface, into a collimated stream of SSPs with the designed handedness. We report on the design, fabrication and characterization of SSP sources consisting of dielectric circular nanoridges with azimuthally varying widths deterministically fabricated on a dielectric-protected silver film around a nanodiamond containing a nitrogen-vacancy centre. With properly engineered phases of QE-originated fields scattered by nanoridges, the out-coupled photons feature a well-defined SAM (with the chirality > 0.8) and high directionality (collection efficiency up to 92%).

cond-mat.mes-hall↗

arXiv2019

Efficient broadband infrared absorbers based on core-shell nanostructures

We suggest to exploit dielectric-metal core-shell nanostructures for efficient resonant and yet broadband absorption of infrared radiation with deeply subwavelength configurations. Realizing that nanostructures would efficiently absorb radiation only when their dielectric properties match those of the environment and making use of the effective medium approach, we develop the design strategy using core-shell nanostructures with very thin shells made of poor metals, i.e., metals having real and imaginary parts of their dielectric permittivities of the same order of magnitude. Analyzing in detail spherical and cylindrical core-shell nanostructures, we demonstrate that the resonant infrared absorption can be not only very efficient, i.e., with the absorption cross sections exceeding geometrical ones, but also broadband with the spectral width being of the order of the resonant wavelength. We obtain simple analytical expressions for the absorption resonances in spherical and cylindrical configurations that allow one to quickly identify the configuration parameters ensuring strong infrared absorption in a given spectral range. Relations to effective medium parameters obtained by the internal homogenization are established and discussed. We believe that our results can be used as practical guidelines for realization of efficient broadband infrared absorbers of subwavelength sizes desirable in diverse applications.

physics.optics↗

arXiv2019

Plasmonic monolithic lithium niobate directional coupler switches

From the onset of high-speed optical communications, lithium niobite (LN) has been the material of choice for electro-optic modulators owing to its large electro-optic response, wide transparent window, excellent thermal stability and long-term material reliability. Conventional LN electro-optic modulators while continue to be the workhorse of the optoelectronic industry become progressively too bulky, expensive and power hungry to fully serve the needs of this industry rapidly progressing towards highly integrated, cost-effective and energy efficient components and circuits. Recently developed monolithic LN nanophotonic platform enables the realization of electro-optic modulators that are significantly improved in terms of compactness, bandwidth and energy efficiency, while still demanding relatively long, on the mm-scale, interaction lengths. Here we successfully deal with this challenge and demonstrate plasmonic electro-optic directional coupler switches consisting of two closely spaced nm-thin gold nanostripes monolithically fabricated on LN substrates that guide both coupled electromagnetic modes and electrical signals influencing their coupling and thereby enabling ultra-compact switching and modulatiofunctionalities. The extreme confinement of both slow-plasmon modes and electrostatic fields created by two nanostripes along with their nearly perfect spatial overlap allowed us to achieve a 90% modulation depth with 20-$μ$m-long switches characterized by a electro-optic modulation efficiency of 0.3 Vcm. Our monolithic LN plasmonic platform enables ultra-dense integration of high-performance active photonic components, enabling a wide range of cost-effective optical communication applications demanding $μ$m-scale footprints, ultrafast operation, robust design and high environmental stability.

physics.app-ph↗

arXiv2019

Multifunctional Metamirrors Involving Simultaneous Linear-polarization Conversion and Focusing

Reducing a set of diverse bulk-optic-based optical components to a single ultrathin and compact element that enables the same complex functionality has become an emerging research area, propelling further integration and miniaturization in photonics. In this work, we establish a versatile metasurface platform based on gap-surface plasmon meta-atoms enabling efficient linear-polarization conversion along with the complete phase control over reflected fields. Capitalizing on the meta-atom design, multifunctional metamirrors involving linear-polarization conversion and focusing are experimentally demonstrated to generate various kinds of focused beams with distinct phase distributions and wavefronts, reproducing thereby the combined functionalities of conventional half-wave plates, lenses, and even spatial light modulators. The proof-of-concept fabricated metamirrors exhibit excellent capability of linear-polarization conversion and focusing within the wavelength range from 800 to 950 nm under linearly-polarized excitation. The multifunctional metamirrors design developed in this study opens new avenues in the advanced research and applications targeting photonics integration of diversified functionalities.

physics.optics↗

arXiv2019

Unidirectional single-photon emission from germanium-vacancy zero-phonon lines: Deterministic emitter-waveguide interfacing at plasmonic hot spots

Striving for nanometer-sized solid-state single-photon sources, we investigate atom-like quantum emitters based on single germanium vacancy (GeV) centers isolated in crystalline nanodiamonds (NDs). Cryogenic characterization indicated symmetry-protected and bright (> 10^6 counts/s with off-resonance excitation) zero-phonon optical transitions with up to 6-fold enhancement in energy splitting of their ground states as compared to that found for GeV centers in bulk diamonds (i.e., up to 870 GHz in highly strained NDs vs 150 GHz in bulk). Utilizing lithographic alignment techniques, we demonstrate an integrated nanophotonic platform for deterministic interfacing plasmonic waveguides with isolated GeV centers in NDs that enables 10-fold enhancement of single-photon decay rates along with the emission direction control by judiciously designing and positioning a Bragg reflector. This approach allows one to realize the unidirectional emission from single-photon dipolar sources introducing a novel method that is alternative to the propagation-direction-dependent techniques based on chiral interactions or topological protection. The developed plasmon-based nanophotonic platform opens thereby new perspectives for quantum nanophotonics in general and for realizing entanglement between single photons and spin qubits, in particular.

physics.app-ph↗

arXiv2018

Ultra-thin titanium nitride films for refractory spectral selectivity

We demonstrate a selectively emitting optical Fabry-Pérot resonator based on a few-nm-thin continuous metallic titanium nitride film, separated by a dielectric spacer from an optically thick titanium nitride back-reflector, which exhibits excellent stability at 1070 K against chemical degradation, thin-film instabilities and melting point depression. The structure paves the way to the design and fabrication of refractory thermal emitters using the well-established processes known from the field of multilayer and rugate optical filters. We demonstrate that a few-nanometer thick films of titanium nitride can be stable under operation at temperatures exceeding 1070 K. This type of selective emitter provides a means towards near-infrared thermal emission that could potentially be tailored to the accuracy level known from rugate optical filters.

physics.app-ph↗