Seung-Cheol Lee — Page 4

arXiv2012

Monte Carlo simulations of the structure of Pt-based bimetallic nanoparticles

Pt-based bimetallic nanoparticles have attracted significant attention as a promising replacement for expensive Pt nanoparticles. In the systematic design of bimetallic nanoparticles, it is important to understand their preferred atomic structures. However, compared with unary systems, alloy nanoparticles present more structural complexity with various compositional configurations, such as mixed-alloy, core-shell, and multishell structures. In this paper, we developed a unified empirical potential model for various Pt-based binary alloys, such as Pd-Pt, Cu-Pt, Au-Pt, and Ag-Pt. Within this framework, we performed a series of Monte Carlo (MC) simulations that quantify the energetically favorable atomic arrangements of Pt-based alloy nanoparticles: an intermetallic compound structure for the Pd-Pt alloy, an onion-like multi-shell structure for the Cu-Pt alloy, and core-shell structures (Au@Pt and Ag@Pt) for the Au-Pt and Ag-Pt alloys. The equilibrium nanoparticle structures for the four alloy types were compared with each other, and the structural features can be interpreted by the interplay of their material properties, such as the surface energy and heat of formation.

cond-mat.mtrl-sci↗

arXiv2004

1D and 2D optical lattices on a chip for quantum computing

We propose a way to make arrays of optical frequency dipole-force microtraps for cold atoms above a dielectric substrate. Traps are nodes in the evanescent wave fields above an optical waveguide resulting from interference of different waveguide modes. The traps have features sought in developing neutral atom based architectures for quantum computing: ~ 1 mW of laser power yields very tight traps 150 nm above a waveguide with trap vibrational frequencies ~ 1 MHz and vibrational ground state sizes ~ 10 nm. The arrays are scalable and allow addressing of individual sites for quantum logic operations.

physics.atom-ph↗