arXiv subjects

Shaojie Hu

Publications and source records attributed to Shaojie Hu.

13 recordsLinked to original sources

arXiv2026

Unveiling Orbital-mediated Ultrafast Demagnetization in Rare Earth-Transition-Metal Ferrimagnets

The ultimate speed limit of magnetic recording and spintronic devices is set by the efficiency of angular-momentum transfer during ultrafast demagnetization, yet its microscopic pathway in Rare-Earth-Transition-Metal (RE-TM) ferrimagnets remains debated. Here, we establish an orbital-mediated framework in which 3d spin-orbit coupling (SOC) governs angular momentum (AM) dissipation. Strong 3d-SOC in RE-Co enables sub-picosecond, single-step demagnetization via direct orbital-to-lattice transfer, whereas weak 3d-SOC in RE-Fe redirects AM into 4f orbitals, producing slower two-step dynamics. The second-stage rate scales with 4f-SOC strength, revealing a distinct orbital-mediated dissipation channel. Using time-resolved magneto-optical Kerr measurements, supported by an extended four-temperature model, corroborate this picture across diverse RE-TM systems (RE = Sm, Gd, Tb, Dy, Ho and TM = Fe, Co, CoNi). Our results identify the SOC-driven competition between 3d and 4f orbital channels as the universal mechanism governing ultrafast demagnetization in RE-TM ferrimagnets, enabling rational design of the switching speed for next-generation spintronic devices.

cond-mat.mtrl-sci↗

arXiv2026

Nonlinear spin-Wave Doppler effect for flexible tuning of magnonic frequencies

We theoretically propose a nonlinear spin-wave Doppler effect, in which the time-dependent motion of a magnetic energy boundary acts as an active frequency modulator, directly converting boundary-induced phase dynamics into instantaneous spectral synthesis for propagating spin-wave modes. In contrast to the conventional linear Doppler effect governed by constant relative velocity, this mechanism enables dynamic phase-to-frequency transduction, generating high-order harmonics, magnonic frequency combs, and coherent chirped sidebands, without requiring nonlinear magnon-magnon coupling or multi-magnon scattering. Micromagnetic simulations on voltage-controlled anisotropy boundaries in ferroelectric/ferromagnetic (FE/FM) heterostructures demonstrate that the comb spacing and spectral topology are determined solely by boundary kinematics, confirming direct Doppler phase coupling between boundary motion and spin-wave propagation. These results establish moving magnetic-energy boundaries as a new class of on-chip spectral synthesizers and define a coherent and energy-efficient framework for flexible tuning of magnonic frequencies, fundamentally distinct from traditional passive scattering or nonlinear multi-magnon mechanisms.

physics.app-ph↗

arXiv2025

Electrical manipulation of magnetic domain structure in van der Waals ferromagnetic Fe$_3$GaTe$_2$ using ferroelectric PMN-PT single crystal

2D van der Waals (vdW) ferromagnets have emerged as promising materials for spintronic applications due to their unique magnetic properties and tunability. Controlling ferromagnetism via external stimuli is critical for both fundamental research and device integration. In particular, modulation of magnetic anisotropy and exchange interactions through strain offers a viable pathway for functional control. Owing to their weak interlayer coupling, vdW ferromagnets exhibit pronounced sensitivity to strain, enabling effective tuning of their magnetic states. In this study, electric-field-induced magnetoelectric coupling is investigated in the above-room-temperature vdW ferromagnet Fe$_3$GaTe$_2$ integrated on a ferroelectric PMN-PT substrate. It is demonstrated that application of an electric field leads to a substantial reduction in coercive force along with dynamic reconfiguration of the magnetic domain structure. These effects are attributed to electric-field-induced modulation of the vdW interlayer gap and enhancement of the Dzyaloshinskii-Moriya interaction. These findings reveal a strong interplay between electric fields and magnetism in vdW systems, offering a viable route toward the development of low-power, multifunctional magnetic devices. This work establishes a foundation for the electric-field control of magnetic properties in vdW ferromagnets and highlights their potential in next-generation spintronic technologies.

cond-mat.mtrl-sci↗

arXiv2025

Distinguishing Backward Volume Magnetostatic Spin Wave Vectors via the Spin Wave Doppler Effect

Spin waves (SWs) and their quanta, magnons, are essential to achieving low-power information transmission in future spintronic devices. Backward volume magnetostatic spin waves (BVMSWs) exhibit a unique dispersion relationship: one frequency corresponding to two distinct wave vectors. At low wave numbers, dipole-dipole interactions dominate, resulting in negative group velocities, whereas at high wave numbers, exchange interactions prevail, producing positive group velocities. This dual behavior complicates wave vector identification and obscures intrinsic spin-wave interactions. In this study, we propose an approach based on the spin wave Doppler effect to effectively distinguish different wave vectors. At low wave numbers, the inverse Doppler effect occurs due to antiparallel phase and group velocities, while at high wave numbers, a normal Doppler effect emerges from parallel velocities. This method not only clarifies the underlying spin-wave interactions but also help mitigate serious interference issues in the design of spin logic circuits.

physics.app-ph↗

arXiv2025

Thermal noise induced probability switching in magnetic tunnel junction based on spin-circuit simulation

The probability switching characteristics in spin transfer torque magnetic tunnel junctions (STT-MTJs) are simulated by considering thermal noise using a spin-circuit module. Thermal noise significantly affects the probability switching for pulse durations exceeding 10 ns, while no probability switching properties are observed for pulses shorter than 1 ns due to the precessional switching. For pulse durations between 1 ns and 10 ns, the occurrence of mixed probability and abrupt switching suggests that thermal noise partially influences the switching properties. These results demonstrate the effectiveness of our simulation model in capturing the MTJ properties under the influence of thermal noise. The spin-circuit module used in this study lays the groundwork for future circuit system designs utilizing MTJ devices, such as true random number generators and neural network computing.

physics.app-ph↗

arXiv2024

Magnetic vortex polarity reversal induced gyrotropic motion spectrum splitting in a ferromagnetic disk

We investigate the gyrotropic motion of the magnetic vortex core in a chain of a few micron-sized Permalloy disks by electrical resistance measurement with amplitude-modulated magnetic field. We observe a distinctive splitting of the resistance peak due to the resonant vortex-core motion under heightened radio frequency (RF) magnetic field excitation. Our micromagnetic simulation identifies the splitting of the resonant peak as an outcome of vortex polarity reversal under substantial RF amplitudes. This study enhances our understanding of nonlinear magnetic vortex dynamics amidst large RF amplitudes and proposes a potential pathway for spintronic neural computing thanks to their unique and controllable magnetization dynamics.

physics.app-ph↗

arXiv2024

Exchange bias induced by spin-glass-like state in Te-rich FeGeTe van der Waals ferromagnet

We have experimentally investigated the mechanism of the exchange bias in the 2D van der Waals (vdW) ferromagnets by means of the anomalous Hall effect (AHE) together with the dynamical magnetization property. The temperature dependence of the AC susceptibility with its frequency response indicates a glassy transition of the magnetic property for the Te-rich FeGeTe vdW ferromagnet. We also found that the irreversible temperature dependence in the anomalous Hall voltage follows the Almeida-Thouless line. Moreover, the freezing temperature of the spin-glass-like phase is found to correlate with the disappearance temperature of the exchange bias. These important signatures suggest that the emergence of magnetic exchange bias in the 2D van der Waals ferromagnets is induced by the presence of the spin-glass-like state in FeGeTe. The unprecedented insights gained from these findings shed light on the underlying principles governing exchange bias in vdW ferromagnets, contributing to the advancement of our understanding in this field.

cond-mat.mtrl-sci↗

arXiv2024

Optimization of thermo-spin voltage in vertical nanostructures by geometrical means

The thermo-spin conversion provides new concepts for further developing the green energy-harvesting technology because spin can be controlled with minimal energy in nanostructures. Through theoretical analysis of thermo-spin generation, transportation and conversion in ferromagnet/non-ferromagnet/heavy metal (FM/NM/HM) vertical structures, we found that the output transverse thermo-spin voltage is independent of the structure's width, but varies in a linear function with the structure's length. To validate our predictions, we fabricated the thermo-spin devices with a CoFeAl/Cu/Pt structure. Our results indicate that FM/NM/HM structures can be utilized to design flexible thermo-spin conversion devices.

physics.app-ph↗

arXiv2023

Electric Field Switching of Magnon Spin Current in a Compensated Ferrimagnet

Manipulation of directional magnon propagation, known as magnon spin current, is essential for developing magnonic memory and logic devices featuring nonvolatile functionalities and ultralow power consumption. Magnon spin current can usually be modulated by magnetic field or current-induced spin torques. However, these approaches may lead to energy dissipation caused by Joule heating. Electric-field switching of magnon spin current without charge current is highly desired but very challenging to realize. By integrating magnonic and piezoelectric materials, we demonstrate manipulation of the magnon spin current generated by the spin Seebeck effect in the ferrimagnetic insulator Gd3Fe5O12 (GdIG) film on a piezoelectric substrate. We observe reversible electric-field switching of magnon polarization without applied charge current. Through strain-mediated magnetoelectric coupling, the electric field induces the magnetic compensation transition between two magnetic states of the GdIG, resulting in its magnetization reversal and the simultaneous switching of magnon spin current. Our work establishes a prototype material platform that pave the way for developing magnon logic devices characterized by all electric field reading and writing and reveals the underlying physics principles of their functions.

cond-mat.mes-hall↗

arXiv2023

Voltage-controlled significant spin wave Doppler shift in FM/FE heterojunction

Efficient manipulation of spin waves (SWs) is considered as one of the promising means for encoding information with low power consumption in next generation spintronic devices. The SW Doppler shift is one important phenomenon by manipulating SWs propagation. Here, we predict an efficient way to control the SW Doppler shift by voltage control magnetic anisotropy boundary (MAB) movement in FM/FE heterojunction. From the micromagnetic simulation, we verified that the SW Doppler shift aligns well with our theoretical predictions in Fe/$\rm BaTiO_3$ heterostructure. The SW Doppler shift also shows ultra wide-band shift (over 5 GHz) property with voltage. Such efficient SW Doppler shift may provide one possible way to measure the Hawking radiation of an analogue black hole in the SW systems.

physics.app-ph↗

arXiv2023

Efficient thermo-spin conversion in van der Waals ferromagnet FeGaTe

Recent discovery of 2D van der Waals (vdW) magnetic materials has spurred progress in developing advanced spintronic devices. A central challenge lies in enhancing the spin-conversion efficiency for building spin-logic or spin-memory devices. We systematically investigated the anomalous Hall effect and anomalous Nernst effect in above-room-temperature van der Waals ferromagnet FeGaTe with perpendicular anisotropy, uncovering significant spin-conversion effects. The anomalous Hall effect demonstrated an efficient electric spin-charge conversion, with a notable spin Hall angle of 6 $\%$ - 10.38 $\%$. The temperature-dependent behavior of the anomalous Nernst voltage primarily results from the thermo-spin conversion. Uniquely, we have experimentally achieved thermo-spin polarization values of over 690 $\%$ at room temperature and extremely large of 4690 $\%$ at about 93 K. This study illuminates the potential of vdW ferromagnets in advancing efficient spin conversion devices.

cond-mat.mtrl-sci↗

arXiv2022

Dual function spin-wave logic gates based on electric field control magnetic anisotropy boundary

Spin waves (SWs) have been considered a promising candidate for encoding information with lower power consumption. Here, we propose the dual function SW logic gates based on the electric field controlling the SW propagation in the Fe film of Fe/BaTiO3 heterostructure with the motion of magnetic anisotropy boundary (MAB). We show micromagnetic simulations to validate the AND-OR and NAND-NOR logic gates. Our research may find a path for simplifying integrated logic circuits using such dual function SW logic gates.

physics.app-ph↗

arXiv2015

Spin Currents injected electrically and thermally from highly spin polarized Co$_2$MnSi

We demonstrate the injection and detection of electrically and thermally generated spin currents probed in Co$_2$MnSi/Cu lateral spin valves. Devices with different electrode separations are patterned to measure the non-local signal as a function of the electrode spacing and we determine a relatively high effective spin polarization $α$ of Co$_2$MnSi to be 0.63 and the spin diffusion length of Cu to be 500 nm at room temperature. The electrically generated non-local signal is measured as a function of temperature and a maximum signal is observed for a temperature of 80 K. The thermally generated non-local signal is measured as a function of current density and temperature in a second harmonic measurement detection scheme. We find different temperature dependences for the electrically and thermally generated non-local signals, which allows us to conclude that the temperature dependence of the signals is not just dominated by the transport in the Cu wire, but that there is a crucial contribution from the different generation mechanisms, which has been largely disregarded to date.

cond-mat.mes-hall↗