arXiv subjects

Shinobu Onoda

Publications and source records attributed to Shinobu Onoda.

At least 19 recordsLinked to original sources

arXiv2026

Enhanced Emission and Two-Photon Interference of Lead-Vacancy Centers in Diamond Solid Immersion Lenses

A negatively charged lead-vacancy (PbV-) center in diamond is a novel quantum system which can be operated at a high temperature above 4 K owing to its large ground state splitting. To unlock the quantum properties of the PbV- center, the enhancement of the fluorescence intensity is a key issue. Here, we demonstrate enhanced emission from PbV- centers by a factor of approximately 10 using solid immersion lenses (SILs) fabricated on rough diamond surface caused by high-temperature anneal over 2000°C. Resonant excitation reveals the narrow emission close to the transform-limited linewidth. Furthermore, we demonstrate two-photon interference using one single PbV- center in an SIL. This enhanced emission and indistinguishability will lead to further development of the PbV- center towards quantum network node applications.

quant-ph↗

arXiv2026

A near-quantum-limited diamond maser amplifier operating at millikelvin temperatures

Current microwave quantum technologies require the amplification of weak signals with minimal added noise at millikelvin temperatures. To date, this stringent requirement has been met exclusively by superconducting technologies, such as Josephson or kinetic-inductance parametric amplifiers. A fundamentally distinct alternative approach could be offered by masers, the microwave counterpart of lasers, which were predicted as early as the 1950s to achieve quantum-limited noise performance under ideal conditions. However, their dependence on cryogenic operation historically limited further advancement. Here we demonstrate the first-ever non-superconducting, near-quantum-limited maser amplifier operating at millikelvin temperatures utilising nitrogen impurity spins (P1 centres) in diamond. Population inversion is achieved via microwave pumping, exploiting a four-spin cross-relaxation mechanism. We realise a maximum power gain exceeding 30 dB, an added noise of approximately 2.55 quanta above the standard quantum limit, and a maximum 1 dB output compression point of -63 dBm at 6.595 GHz. The ability to operate in strong static magnetic fields of arbitrary orientation may offer a complementary, non-superconducting route for applications such as semiconducting spin-qubit readout, magnetic-resonance spectroscopy, and dark-matter axion searches.

quant-ph↗

arXiv2026

Robust gigahertz-range ac magnetometry with an ensemble of NV centers in diamond using concatenated continuous dynamical decoupling

Sub-picotesla level magnetometry has been demonstrated using negatively-charged nitrogen-vacancy (NV) centers in diamond by increasing the number of spins simultaneously used for sensing in an NV ensemble. However, such scale-up often introduces spatial inhomogeneities in detuning and control field amplitudes, which degrade sensitivity. Although several techniques have been utilized to overcome these challenges, including pulsed dynamical decoupling or shaped pulses, these are not generally compatible with the current state-of-the-art techniques for GHz-range AC magnetometry with NV ensembles, which are typically based on Rabi oscillations. In this work we experimentally demonstrate GHz-range AC magnetometry using a large ensemble of NV centers under spatially inhomogeneous drive fields by employing concatenated continuous dynamical decoupling, which is designed for robustness against such imperfections. We compare its performance with the conventional direct Rabi method and show that the robust dressed states in our method extend significantly the measuring range to weaker signals in GHz-range AC magnetometry.

quant-ph↗

arXiv2026

Diamond quantum-sensing platform with integrated boron-doped diamond microwave antenna and thermometer

Wide-field nitrogen-vacancy (NV) magnetic imaging at cryogenic temperatures requires microwave excitation and reliable knowledge of the temperature near the sensing region. Here, we report an integrated diamond quantum-sensing platform combining an ensemble of NV centers with a boron-doped diamond (BDD) microwave antenna and thermometer formed on the same diamond substrate. The BDD antenna provides microwave excitation for optically detected magnetic resonance measurements, and the BDD thermometer monitors the thermal environment near the NV sensing region. The BDD thermometer detected laser-induced local heating that was not clearly resolved by a stage-mounted thermometer. Using this platform, we imaged the temperature-dependent Meissner response of multiple cuprate superconductors while recording the temperature. These results demonstrate that the integrated BDD--NV platform provides a practical approach for cryogenic wide-field magnetic imaging with integrated microwave delivery and local thermometry.

physics.app-ph↗

arXiv2026

Wide-field NV magnetometry under simultaneous high-pressure and high-temperature conditions

We demonstrate wide-field optically detected magnetic resonance (ODMR) under simultaneous high-pressure and high-temperature conditions using nitrogen-vacancy (NV) centers. Although NV-center magnetometry has been widely used for spatially resolved magnetic-field imaging, its application to extreme environments combining pressure and temperature remains challenging. In this work, we show that ODMR can be observed at 5 GPa and 500 K, demonstrating the feasibility of NV spin readout under such combined extreme conditions. We further perform wide-field ODMR of iron at 7 GPa and 500 K, where the stray magnetic field from the sample is spatially visualized through the pressure cell. These results establish NV-center magnetometry as a promising platform for imaging magnetic phenomena in materials under high-pressure and high-temperature environments.

physics.app-ph↗

arXiv2026

Coherent Dark State Formation of a Lead-Vacancy Spin Qubit in Diamond

A lead-vacancy (PbV) center in diamond exhibits coherent emission above the liquid helium temperature, making it highly attractive for quantum network applications. Here, we report the magneto-optical and spin properties of PbV centers in diamond. We record a spin lifetime of 12 ms at 7.5 K under large off-axis magnetic field. Furthermore, we observe formation of the coherent dark state by coherent population trapping and estimate a spin dephasing time of 177 ns at 6.5 K. This work demonstrates the outstanding thermal robustness of the PbV spin compared to other group-IV centers above 4 K.

quant-ph↗

arXiv2026

Ten-Second Electron-Spin Coherence in Isotopically Engineered Diamond

Solid-state spin defects are a promising platform for quantum networks. A key requirement is to combine long ground-state spin-coherence times with a coherent optical transition for spin-photon entanglement. Here, we investigate the spin and optical coherence of single nitrogen-vacancy (NV) centres in (111)-grown isotopically engineered diamond. Our diamond-growth process yields a precisely controlled $^{13}\mathrm{C}$ concentration and low-ppb nitrogen concentrations. Combined with the mitigation of 50 Hz noise using a real-time feedforward scheme and tailored decoupling sequences, this enables record defect-electron-spin coherence times of $T_2 = 6.8(1)$ ms for a Hahn echo and of $T_2^{DD} = 11.2(8)$ s under dynamical decoupling. In addition, we observe coherent optical transitions with a near-lifetime-limited homogeneous linewidth of 16.9(4) MHz and characterize the spectral diffusion dynamics. These results provide new avenues to investigate the incorporation of impurities in diamond and new opportunities for improved spin-qubit control for quantum networks and other quantum technologies.

quant-ph↗

arXiv2026

Probing the Meissner effect in single crystals of $\mathbf{Bi_2Sr_2Ca_2Cu_3O_{10+δ}}$ via wide-field quantum microscopy under high pressure

We investigated the pressure dependence of the superconducting transition temperature ($T_{\rm c}$) in optimally doped Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+δ}$ (Bi-2223) single crystals using different pressure-transmitting media. Previous high-pressure studies have reported conflicting behaviors, ranging from a resurgence of $T_{\rm c}$ of optimally doped Bi-2223 in fluid media to an insulating-like transition in solid media. However, a direct comparison of the effects of different pressure-transmitting media is lacking. Here, we employed wide-field quantum microscopy based on nitrogen-vacancy centers to probe the magnetic response under high pressure, utilizing cBN and KBr as media. We observed that a diamagnetic response near 70 K, indicative of the superconducting transition, persisted up to 23 GPa in KBr, whereas it disappeared above 11 GPa and 70 K in cBN. These results demonstrate the high sensitivity of Bi-2223 to the pressure environment and highlight the critical role of hydrostatic pressure in cuprate superconductors.

cond-mat.supr-con↗

arXiv2026

A Highly Sensitive Diamond NV Magnetometer Using Ramsey Interferometry with a Short Sensor-to-Sample Distance

In this study, we developed a diamond quantum magnetometer based on Ramsey interferometry with a short sensor-to-sample distance. Conventional biomagnetic sensors with ensemble nitrogen-vacancy centers using continuous-wave optically detected magnetic resonance and Ramsey methods typically rely on watt-level lasers to achieve high sensitivity, resulting in thermal issues. In contrast, by employing the light-trapping diamond waveguide technique in a high-pressure and high-temperature diamond sample treated with electron beam irradiation, we obtained a high photon conversion efficiency of 9.5%, enabling us to simultaneously achieve a high sensitivity of 2.93(7) pT/Hz^1/2 in the 100-400 Hz frequency range and a minimal temperature increase of only approximately 13 K at a low laser power of 210 mW. Using a dry phantom designed to mimic magnetoencephalography signals, we measured a weak magnetic field of 77.7(2) pT without signal averaging at a sensor-to-sample distance of 2.5 mm. This short-distance measurement prevents severe spatial signal attenuation, yielding a high signal-to-noise ratio. The development here is crucial for practical biomagnetic applications based on Ramsey interferometry.

quant-ph↗

arXiv2025

Multichannel highly sensitive diamond quantum magnetometer

We demonstrate a highly sensitive real-time magnetometry method at two measurement points. This magnetometry method is based on the frequency-division multiplexing of continuous-wave optically detected magnetic resonance. We use two ensembles of nitrogen-vacancy (NV) centers separated by 3.6 mm to measure a magnetic field. A different bias field is applied to the two NV ensembles to resolve the resonance peak for each ensemble in the frequency space and enables the multiplexed magnetometry at the two points. The sensitivities achieved at the measurement points are $21~\mathrm{pT/\sqrt{Hz}}$ and $22~\mathrm{pT/\sqrt{Hz}}$. The proposed magnetometry method can be expanded to include more measurement points and shorter spacing. The capability of real-time measurement at numerous points with short spacing and high sensitivity is beneficial for various applications, including biomagnetic sensing, geophysical research, and material science.

quant-ph↗

arXiv2025

Optical charge state manipulation of lead-vacancy centers in diamond

Group-IV vacancy centers in diamond exhibit excellent optical and spin coherence properties, making them highly promising and scalable spin qubit candidates. Since only specific charge states are magneto-optically active, control over the charge state is fundamental for quantum applications. Here, we realize the charge state control of lead-vacancy centers (PbV) through multi-color laser irradiation. We achieve tunable population manipulation of the negatively charged state from 0 to 89%, paving the way for spin control of the negatively charged PbV center. Furthermore, through analysis of charge state dynamics, we propose a charge cycle between the neutral and negatively charged states, indicating a possible pathway to the neutral PbV center with a spin-1 system.

quant-ph↗

arXiv2025

Current comparator for both AC and DC ratio measurements with 10-8-level accuracy

Accurate measurements of alternating current (AC) and direct current(DC) ratios are fundamental to electric power metrology. However, conventional current comparators for AC and DC typically rely on distinct technologies-electromagnetic induction for AC and superconducting quantum interference devices for DC. This technological divide leads to a fragmented and complex traceability system. Bridging this gap is critical for developing unified current standards that meet the demands of emerging power technologies. In this work, we present a compact, room-temperature AC/DC current comparator that integrates a diamond-based magnetometer using nitrogen-vacancy centers. The device achieves an accuracy of 10-8 for both AC and DC signals and supports a system bandwidth up to 300 Hz, without the need for cryogenics. It surpasses the performance of typical AC comparators, offering ten-fold higher accuracy, and matches that of state-of-the-art DC comparators. This unified, cryogenics-free solution not only enhances precision and versatility but also expands the applicability of the system to DC resistance bridges in quantum electrical standards.

quant-ph↗

arXiv2025

Efficient Detection of Statistical RF Fields at High Magnetic Field with a Quantum Sensor

Nuclear magnetic resonance (NMR) spectroscopy is widely used in fields ranging from chemistry, material science to neuroscience. Nanoscale NMR spectroscopy using Nitrogen-vacancy (NV) centers in diamond has emerged as a promising platform due to an unprecedented sensitivity down to the single spin level. At the nanoscale, high nuclear spin polarization through spin fluctuations (statistical polarization) far outweighs thermal polarization. However, until now efficient NMR detection using coherent averaging techniques could not be applied to the detection of statistical polarization, leading to long measurement times. Here we present two protocols to enable coherent averaging of statistical oscillating signals through rectification. We demonstrate these protocols on an artificial radiofrequency signal detected with a single NV center at 2.7 T. Through this, the signal-to-noise scaling with number of measurements $N$ is improved from $N^{0.5}$ to $N^1$, improving the measurement time significantly. The relevance of rectification for the detection of statistical polarization using NV ensembles is outlined, paving the way for efficient nanoscale NMR spectroscopy.

quant-ph↗

arXiv2025

High-Fidelity Electron Spin Gates for Scaling Diamond Quantum Register

Diamond is a promising platform for quantum information processing as it can host highly coherent qubits that could allow for the construction of large quantum registers. A prerequisite for such devices is a coherent interaction between nitrogen vacancy (NV) electron spins. Entanglement between dipolar-coupled NV spin pairs has been demonstrated, but with a limited entanglement fidelity and its error sources have not been characterized. Here, we design and implement a robust, easy to implement entangling gate between NV spins in diamond and quantify the influence of multiple error sources on the gate performance. Experimentally, we demonstrate a record gate fidelity of $F=(96.0 \pm 2.5)$ % under ambient conditions. Our identification of the dominant errors paves the way towards NV-NV gates beyond the error correction threshold.

quant-ph↗

arXiv2025

Narrow Inhomogeneous Distribution and Charge State Stabilization of Lead-Vacancy Centers in Diamond

Lead-vacancy (PbV) centers in diamond with a large ground state splitting are expected to be a building block of quantum network nodes. Due to the heaviness of the Pb atom, it is challenging to fabricate high-quality PbV centers with a narrow inhomogeneous distribution and stable charge state. In this study, for the formation of the PbV centers, high temperature anneal up to 2300°C is performed after Pb ion implantation. At a lower temperature of 1800°C, the PbV centers show a large inhomogeneous distribution and spectral diffusion, while higher temperatures of 2200-2300°C leads to narrow inhomogeneous distributions with standard deviations of ~5 GHz. The charge state transition of the PbV centers formed at 2200°C occurs by capturing photo-carriers generated from surrounding defects under 532 nm laser irradiation. Finally, multiple stable PbV centers with nearly identical photon frequencies are obtained, which is essential for applications in quantum information processing.

quant-ph↗

arXiv2025

Blueprint for Diamond Magnetometry: Unraveling Quantum Dephasing of Nitrogen-Vacancy Center Ensembles in Diamond

Diamonds with nitrogen-vacancy (NV) center ensembles are one of the most promising solid-state quantum platforms for various sensing applications. The combination of a long spin dephasing time ($T_2^*$) and a high NV center concentration is crucial for pushing the sensitivity limits. In this work, we propose a systematic measurement approach to quantify the electron spin dephasing in NV center ensembles and analyze the contributions of various sources to the dephasing time, including NV-NV interactions, strain and electric field distributions, $^{13}$C nuclear spins, and P1 electron spins. Our method is validated using a series of high-performance diamond samples, providing a comprehensive understanding of dephasing mechanisms and revealing correlations between NV concentration and different dephasing sources. Based on these insights, we further evaluate and propose strategies to improve the achievable sensitivity limits for DC magnetic field measurements.

quant-ph↗

arXiv2024

Performance Evaluation of a Diamond Quantum Magnetometer for Biomagnetic Sensing: A Phantom Study

We employ a dry-type phantom to evaluate the performance of a diamond quantum magnetometer with a high sensitivity of about $6~\mathrm{pT/\sqrt{Hz}}$ from the viewpoint of practical measurement in biomagnetic sensing. The dry phantom is supposed to represent an equivalent current dipole (ECD) generated by brain activity, emulating an encephalomagnetic field. The spatial resolution of the magnetometer is evaluated to be sufficiently higher than the length of the variation in the encephalomagnetic field distribution. The minimum detectable ECD moment is evaluated to be 0.2 nA m by averaging about 8000 measurements for a standoff distance of 2.4 mm from the ECD. We also discuss the feasibility of detecting an ECD in the measurement of an encephalomagnetic field in humans. We conclude that it is feasible to detect an encephalomagnetic field from a shallow cortex area such as the primary somatosensory cortex.

physics.ins-det↗

arXiv2024

Charge state transition of spectrally stabilized tin-vacancy centers in diamond

Solid-state quantum emitters are an important platform for quantum information processing. The fabrication of the emitters with stable photon frequency and narrow linewidth is a fundamental issue, and it is essential to understand optical conditions under which the emitter keeps a bright charge state or transitions to a dark state. For these purposes, in this study, we investigate the spectral stability and charge state transition of tin-vacancy (SnV) centers in diamond. The photoluminescence excitation spectra of multiple SnV centers are basically stable over time with nearly transform-limited linewidths under resonant excitation, while simultaneous irradiation of resonant and non-resonant lasers makes spectra from the SnV centers unstable. We find that the instability occurs due to the charge state transition to a dark state. The charge state transition rates are quantitatively investigated depending on the laser powers. Lastly, with first-principle calculations, we model the charge state transition of the SnV center under the laser irradiation.

quant-ph↗